64 results on '"Alexander Tzalenchuk"'
Search Results
2. Low contact resistance in epitaxial graphene devices for quantum metrology
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Tom Yager, Arseniy Lartsev, Karin Cedergren, Rositsa Yakimova, Vishal Panchal, Olga Kazakova, Alexander Tzalenchuk, Kyung Ho Kim, Yung Woo Park, Samuel Lara-Avila, and Sergey Kubatkin
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Physics ,QC1-999 - Abstract
We investigate Ti/Au contacts to monolayer epitaxial graphene on SiC (0001) for applications in quantum resistance metrology. Using three-terminal measurements in the quantum Hall regime we observed variations in contact resistances ranging from a minimal value of 0.6 Ω up to 11 kΩ. We identify a major source of high-resistance contacts to be due bilayer graphene interruptions to the quantum Hall current, whilst discarding the effects of interface cleanliness and contact geometry for our fabricated devices. Moreover, we experimentally demonstrate methods to improve the reproducibility of low resistance contacts (
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- 2015
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3. The expanding role of National Metrology Institutes in the quantum era
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Alexander Tzalenchuk, Nicolas Spethmann, Tim Prior, Jay H. Hendricks, Yijie Pan, Vladimir Bubanja, Guilherme P. Temporão, Dai-Hyuk Yu, Damir Ilić, and Barbara L. Goldstein
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General Physics and Astronomy - Published
- 2022
4. Quasiadiabatic electron transport in room temperature nanoelectronic devices induced by hot-phonon bottleneck
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Pingping Chen, Le Yang, Susumu Komiyama, Qianchun Weng, Wei Lu, Zhenghua An, and Alexander Tzalenchuk
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Work (thermodynamics) ,Multidisciplinary ,Materials science ,Condensed matter physics ,business.industry ,Phonon ,Science ,General Physics and Astronomy ,Imaging techniques ,General Chemistry ,Electron ,Dissipation ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Electron transport chain ,Article ,General Biochemistry, Genetics and Molecular Biology ,Semiconductor ,Semiconductors ,Nanoelectronics ,Electronics ,business - Abstract
Since the invention of transistors, the flow of electrons has become controllable in solid-state electronics. The flow of energy, however, remains elusive, and energy is readily dissipated to lattice via electron-phonon interactions. Hence, minimizing the energy dissipation has long been sought by eliminating phonon-emission process. Here, we report a different scenario for facilitating energy transmission at room temperature that electrons exert diffusive but quasiadiabatic transport, free from substantial energy loss. Direct nanothermometric mapping of electrons and lattice in current-carrying GaAs/AlGaAs devices exhibit remarkable discrepancies, indicating unexpected thermal isolation between the two subsystems. This surprising effect arises from the overpopulated hot longitudinal-optical (LO) phonons generated through frequent emission by hot electrons, which induce equally frequent LO-phonon reabsorption (“hot-phonon bottleneck”) cancelling the net energy loss. Our work sheds light on energy manipulation in nanoelectronics and power-electronics and provides important hints to energy-harvesting in optoelectronics (such as hot-carrier solar-cells)., Minimizing the energy dissipation is usually sought by eliminating phonon-emission process. Here, the authors find a different approach for facilitating energy transmission at room temperature that electrons exert diffusive but quasiadiabatic transport, free from substantial energy loss.
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- 2021
5. A Highly Sensitive Detector for Radiation in the Terahertz Region.
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Peter Kleinschmidt, Stephen P. Giblin, Vladimir Antonov, Hideomi Hashiba, Leonid Kulik, Alexander Tzalenchuk, and Susumu Komiyama
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- 2007
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6. Strongly Absorbing Nanoscale Infrared Domains within Strained Bubbles at hBN–Graphene Interfaces
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Irina V. Grigorieva, Matthew J. Hamer, Olga Kazakova, Tom Vincent, Alexander Tzalenchuk, and Vladimir Antonov
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0303 health sciences ,Materials science ,Infrared ,Graphene ,Nanotechnology ,02 engineering and technology ,021001 nanoscience & nanotechnology ,law.invention ,03 medical and health sciences ,symbols.namesake ,law ,symbols ,General Materials Science ,Near-field scanning optical microscope ,0210 nano-technology ,Raman spectroscopy ,Absorption (electromagnetic radiation) ,Nanoscopic scale ,030304 developmental biology - Abstract
Graphene has great potential for use in infrared (IR) nanodevices. At these length scales, nanoscale features, and their interaction with light, can be expected to play a significant role in device performance. Bubbles in van der Waals heterostructures are one such feature, which have recently attracted considerable attention, thanks to their ability to modify the optoelectronic properties of two-dimensional (2D) materials through strain. Here, we use scattering-type scanning near-field optical microscopy (sSNOM) to measure the nanoscale IR response from a network of variously shaped bubbles in hexagonal boron nitride (hBN)-encapsulated graphene. We show that within individual bubbles there are distinct domains with strongly enhanced IR absorption. The IR domain boundaries coincide with ridges in the bubbles, which leads us to attribute them to nanoscale strain domains. We further validate the strain distribution in the graphene by means of confocal Raman microscopy and vector decomposition analysis. This shows intricate and varied strain configurations, in which bubbles of different shape induce more bi- or uniaxial strain configurations. This reveals pathways toward future strain-based graphene IR devices.
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- 2020
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7. Nanothermometry of electrons and phonons
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Le Yang, Craig Barton, Robb Puttock, Qianchun Weng, Susumu Komiyama, Wei Lu, Zhenghua An, Alexander Tzalenchuk, Yusuke Kajihara, and Vishal Panchal
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Microscope ,Materials science ,business.industry ,Infrared ,Terahertz radiation ,02 engineering and technology ,Electron ,Radiation ,021001 nanoscience & nanotechnology ,01 natural sciences ,law.invention ,Optics ,law ,0103 physical sciences ,Microscopy ,Electron temperature ,010306 general physics ,0210 nano-technology ,business ,Noise (radio) - Abstract
Infrared radiation thermometry, which derives temperature of an object from the intensity of emitted radiation, suffers from diffraction-limited insufficient spatial resolution. This limit is overcome by introducing a terahertz near-field technique to locally probe fluctuating electromagnetic (EM) evanescent fields. We report here nanoscale hot electron temperature distribution directly mapped with a newly developed near-field technique, called scanning noise microscope (SNoiM). Nanoscale lattice temperature distribution in the same sample was also mapped with a commercially available contact-type scanning thermal microscope (SThM). By comparison, subtle but essential difference has been found between the distributions of the lattice temperature and the electron temperature, leading to detailed understanding of the hot electron kinetics along with the phonon-relaxation process.
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- 2018
8. Observation of Coulomb blockade in nanostructured epitaxial bilayer graphene on SiC
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C. Chua, Charles G. Smith, Malcolm R. Connolly, Jinggao Sui, Alexander Tzalenchuk, R. K. Puddy, Vishal Panchal, Tjbm Janssen, Arseniy Lartsev, Rositsa Yakimova, C. L. Richardson, and Sergey Kubatkin
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Materials science ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Doping ,Conductance ,Coulomb blockade ,FOS: Physical sciences ,02 engineering and technology ,General Chemistry ,Electron ,021001 nanoscience & nanotechnology ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,01 natural sciences ,Magnetic field ,Condensed Matter::Materials Science ,0103 physical sciences ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,General Materials Science ,010306 general physics ,0210 nano-technology ,Bilayer graphene ,Graphene nanoribbons ,Quantum tunnelling - Abstract
We study electron transport in nanostructures patterned in bilayer graphene patches grown epitaxially on SiC as a function of doping, magnetic field, and temperature. Away from charge neutrality transport is only weakly modulated by changes in carrier concentration induced by a local side-gate. At low n-type doping close to charge neutrality, electron transport resembles that in exfoliated graphene nanoribbons and is well described by tunnelling of single electrons through a network of Coulomb-blockaded islands. Under the influence of an external magnetic field, Coulomb blockade resonances fluctuate around an average energy and the gap shrinks as a function of magnetic field. At charge neutrality, however, conduction is less insensitive to external magnetic fields. In this regime we also observe a stronger suppression of the conductance below $T^*$, which we interpret as a sign of broken interlayer symmetry or strong fluctuations in the edge/potential disorder.
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- 2017
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9. Polymer-encapsulated molecular doped epigraphene for quantum resistance metrology
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Rositsa Yakimova, Kyung Ho Kim, Alexander Tzalenchuk, Nick Fletcher, Yung Woo Park, S. Rozhko, Gunnar Eklund, Karin Cedergren, Sergey Kubatkin, Samuel Lara-Avila, Tobias Bergsten, and Hans He
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Materials science ,business.industry ,Graphene ,Pedagogy ,Doping ,Pedagogik ,General Engineering ,Quantum Hall effect ,01 natural sciences ,7. Clean energy ,Metrology ,law.invention ,010309 optics ,chemistry.chemical_compound ,Semiconductor ,chemistry ,law ,molecular doping ,graphene ,measurement standards ,quantum Hall effect ,0103 physical sciences ,Quantum metrology ,Silicon carbide ,Optoelectronics ,010306 general physics ,business ,Quantum - Abstract
One of the aspirations of quantum metrology is to deliver primary standards directly to end-users thereby significantly shortening the traceability chains and enabling more accurate products. Epitaxial graphene grown on silicon carbide (epigraphene) is known to be a viable candidate for a primary realisation of a quantum Hall resistance standard, surpassing conventional semiconductor two-dimensional electron gases, such as those based on GaAs, in terms of performance at higher temperatures and lower magnetic fields. The bottleneck in the realisation of a turn-key quantum resistance standard requiring minimum user intervention has so far been the need to fine-tune the carrier density in this material to fit the constraints imposed by a simple cryo-magnetic system. Previously demonstrated methods, such as via photo-chemistry or corona discharge, require application prior to every cool-down as well as specialist knowledge and equipment. To this end we perform metrological evaluation of epigraphene with carrier density tuned by a recently reported permanent molecular doping technique. Measurements at two National Metrology Institutes confirm accurate resistance quantisation below 5 n Omega Omega(-1). Furthermore, samples show no significant drift in carrier concentration and performance on multiple thermal cycles over three years. This development paves the way for dissemination of primary resistance standards based on epigraphene. Funding Agencies|Swedish-Korean Basic Research Cooperative Program of the NRF [NRF-2017R1A2A1A18070721]; Swedish Foundation for Strategic Research (SSF) [IS14-0053, GMT14-0077, RMA15-0024]; Swedish Research Council (VR); VINNOVA; Knut and Alice Wallenberg Foundation; Chalmers Area of Advance NANO; UK Department of Business, Energy and Industrial Strategy (BEIS); European Unions Horizon 2020 research and innovation programme [785219]
- Published
- 2019
10. Comparison of active and passive methods for the infrared scanning near-field microscopy
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Alexander Tzalenchuk, Yusuke Kajihara, Susumu Komiyama, Kuan-Ting Lin, Qianchun Weng, Vishal Panchal, and Liaoxin Sun
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010302 applied physics ,Thermal equilibrium ,Materials science ,Microscope ,Physics and Astronomy (miscellaneous) ,Infrared ,business.industry ,Physics::Optics ,02 engineering and technology ,Dielectric ,021001 nanoscience & nanotechnology ,Laser ,01 natural sciences ,law.invention ,Optics ,Optical microscope ,law ,0103 physical sciences ,Near-field scanning optical microscope ,0210 nano-technology ,business ,Noise (radio) - Abstract
We systematically compare the active and the passive methods for infrared scattering-type scanning near-field optical microscopy (s-SNOM). The active SNOM makes use of IR lasers or incoherent thermal emitters to illuminate a sample, whereas the passive method directly measures extremely weak fluctuating electromagnetic evanescent fields spontaneously generated at the sample surface without any external illumination. For this reason, our specific version of the passive SNOM is called a scanning noise microscope (SNoiM). In thermal equilibrium, the two methods are shown to be similar, both mapping the nanoscale variation of the complex dielectric constant of the sample. We demonstrate that a significant difference between the two methods emerges when the sample is driven out of thermal equilibrium, viz., the active SNOM is insensitive whereas the SNoiM is extremely sensitive to the electron temperature in locally heated nanoregions.
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- 2019
11. Practical and Fundamental Impact of Epitaxial Graphene on Quantum Metrology
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Theodoor Jan B. M. Janssen, Vladimir I. Fal'ko, Alexander Tzalenchuk, Samuel Lara-Avila, and Sergey Kubatkin
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Materials science ,Physics and Astronomy (miscellaneous) ,business.industry ,Graphene ,Nanotechnology ,Quantum Hall effect ,Gallium arsenide ,Metrology ,law.invention ,chemistry.chemical_compound ,Semiconductor ,chemistry ,law ,Quantum metrology ,Epitaxial graphene ,business ,Graphene nanoribbons - Abstract
The discovery 8 years ago of the quantum Hall effect (QHE) in graphene sparked an immediate interest in the metrological community. Here was a material which was completely different from commonly used semiconductor systems and which seemed to have some uniques properties which could make it ideally suited for high-precision resistance metrology. However, measuring the QHE in graphene turned out to be not so simple as first thought. In particular the small size of exfoliated graphene samples made precision measurements difficult. This dramatically changed with the development of large-area graphene grown on SiC and in this short review paper we discuss the journey from first observation to the highest-ever precision comparison of the QHE.
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- 2013
12. 3-D Mapping of Sensitivity of Graphene Hall Devices to Local Magnetic and Electrical Fields
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David Cox, S. R. P. Silva, Olga Kazakova, Alexander Tzalenchuk, Alessandra Manzin, and R. K. Rajkumar
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Materials science ,Condensed matter physics ,Graphene ,Thermal Hall effect ,Electronic, Optical and Magnetic Materials ,Magnetic field ,law.invention ,Hall effect ,law ,Electric field ,Electrical and Electronic Engineering ,Magnetic force microscope ,Graphene nanoribbons ,Voltage - Abstract
We report the response of sub-micron epitaxial graphene Hall devices to localized and inhomogeneous magnetic field produced by an MFM tip. We analyze the magneto-transport properties of epitaxial graphene and report the independent contribution of magnetic and electric fields in the measured transverse voltage maps with respect to the lateral and vertical position of the tip. A finite element model has also been developed to support the experimental results.
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- 2013
13. Single photon detection of the coherent THz radiation of HTS Josephson Junctions
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R. Shaikhaidarov, Vladimir Antonov, and Alexander Tzalenchuk
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010302 applied physics ,Josephson effect ,Physics ,Photon ,Electromagnetics ,Condensed matter physics ,business.industry ,Terahertz radiation ,Detector ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,Quantum dot ,Thermal radiation ,Condensed Matter::Superconductivity ,0103 physical sciences ,Optoelectronics ,Photonics ,0210 nano-technology ,business - Abstract
The voltage biased individual Josephson Junction made of high temperature superconductor (HTS JJ) can potentially serve as the tuneable spectral source of terahertz radiation. The power is however relatively small, and one needs a sensitive detector in order to study and to optimise such a source. We use a single photon semiconductor quantum dot detector to probe the radiation of the HTS JJ. The detector is a resonant device with a spectral resolution of 30% at resonance frequency. Despite a rather wide resonance line the detector allows to discriminate between the coherent and the thermal radiation of HTS JJ. We found that HTS JJ emits to vacuum only 10−18W in a form of the coherent radiation, which is only ∼ 4 × 10−10 part of the total dissipated power. Partially a small conversion factor can be attributed to the non optimal coupling of the HTS JJ to the planar metallic antenna. The experiments reveal also a specific of the operation of the quantum dot detector itself. We observe two resonances at 0.3 THz and 0.8 THz. They are likely related to excitation of the plasma mode in the patterned two dimensional electron gas.
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- 2016
14. Weak localization scattering lengths in epitaxial, and CVD graphene
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Alexander Tzalenchuk, Lain-Jong Li, Rositza Yakimova, Jack A. Alexander-Webber, Tjbm Janssen, Samuel Lara-Avila, Robin J. Nicholas, T. Altebaeumer, Sergey Kubatkin, Cheng-Te Lin, and A. M. R. Baker
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Materials science ,Magnetoresistance ,FOS: Physical sciences ,02 engineering and technology ,Conductivity ,Epitaxy ,01 natural sciences ,electronic-properties ,law.invention ,law ,Teknik och teknologier ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,0103 physical sciences ,bilayer graphene ,010306 general physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Graphene ,Scattering ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Electronic, Optical and Magnetic Materials ,Magnetic field ,Weak localization ,Physical Sciences ,Engineering and Technology ,0210 nano-technology ,Bilayer graphene - Abstract
Weak localization in graphene is studied as a function of carrier density in the range from 1 x 10(11) cm(-2) to 1.43 x 10(13) cm(-2) using devices produced by epitaxial growth onto SiC and CVD growth on thin metal film. The magnetic field dependent weak localization is found to be well fitted by theory, which is then used to analyze the dependence of the scattering lengths L-phi, L-i, and L-* on carrier density. We find no significant carrier dependence for L-phi, a weak decrease for L-i with increasing carrier density just beyond a large standard error, and a n(-1/4) dependence for L-*. We demonstrate that currents as low as 0.01 nA are required in smaller devices to avoid hot-electron artifacts in measurements of the quantum corrections to conductivity. DOI: 10.1103/PhysRevB.86.235441 Funding Agencies|UK EPSRC||Swedish Research Council||Foundation for Strategic Research||UK National Measurement Office||EU FP7 STREP ConceptGraphene
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- 2016
15. Fabrication of graphene quantum hall resistance standard in a cryogen-table-top system
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Tjbm Janssen, Sergey Kubatkin, Rositza Yakimova, Alexander Tzalenchuk, Samuel Lara-Avila, S. Rozhko, and Hans He
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Fabrication ,Materials science ,Physics::Instrumentation and Detectors ,Physics::Optics ,Nanotechnology ,02 engineering and technology ,Quantum Hall effect ,01 natural sciences ,law.invention ,Condensed Matter::Materials Science ,chemistry.chemical_compound ,law ,0103 physical sciences ,Silicon carbide ,010306 general physics ,business.industry ,Graphene ,Macroscopic quantum phenomena ,021001 nanoscience & nanotechnology ,Magnetic field ,Semiconductor ,chemistry ,Optoelectronics ,0210 nano-technology ,business ,Microfabrication - Abstract
We have demonstrated quantum Hall resistance measurements with metrological accuracy in a relatively easy to use and compact cryogen-free system operating at a temperature of around 3.8 K and magnetic field below 5 T. This advance in technology is due to the unique properties of epitaxial graphene on silicon carbide (SiC) which lifts the stringent requirements for quantum hall effect seen in conventional semiconductors. This paper presents the processes involved in fabrication and characterization of metrologically viable epitaxial graphene samples.
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- 2016
16. Towards a cryogen-free table-top primary resistance standard
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Jane Ireland, Sergey Kubatkin, Hans He, S. Rozhko, Jonathan M. Williams, Rositsa Yakimova, Alexander Tzalenchuk, Tjbm Janssen, Samuel Lara-Avila, and Stephen P. Giblin
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Materials science ,Physics::Instrumentation and Detectors ,business.industry ,Graphene ,Astrophysics::Instrumentation and Methods for Astrophysics ,Electrical engineering ,02 engineering and technology ,Quantum Hall effect ,021001 nanoscience & nanotechnology ,Table (information) ,01 natural sciences ,Cryogenic current comparator ,Magnetic field ,Metrology ,law.invention ,law ,0103 physical sciences ,Optoelectronics ,Current (fluid) ,010306 general physics ,0210 nano-technology ,business - Abstract
We demonstrate quantum Hall resistance measurements with metrological accuracy in a small cryogen-free system operating at a temperature of around 3.8 K and magnetic fields below 5 T. We use this system to investigate the optimisation of graphene/SiC devices for maximum breakdown current. In addition we report the first characterisation of a cryogen-free cryogenic current comparator which enables entirely cryogen-free primary resistance metrology.
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- 2016
17. Detection of Coherent Terahertz Radiation from a High-Temperature Superconductor Josephson Junction by a Semiconductor Quantum-Dot Detector
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Alexei Kalaboukhov, R. Shaikhaidarov, Vladimir Antonov, Koji Onomitsu, A. Sobolev, Andrew Casey, Sergey Kubatkin, Alexander Tzalenchuk, and Yuichi Harada
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Josephson effect ,Superconductivity ,Materials science ,Physics::Instrumentation and Detectors ,business.industry ,Terahertz radiation ,Detector ,Transistor ,General Physics and Astronomy ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,law.invention ,Pi Josephson junction ,law ,Condensed Matter::Superconductivity ,0103 physical sciences ,Physics::Accelerator Physics ,Optoelectronics ,Antenna (radio) ,010306 general physics ,0210 nano-technology ,business ,Common emitter - Abstract
We examine the application of Josephson radiation emitters to spectral calibration of single-photon-resolving detectors. Josephson junctions are patterned in a YBCO film on a bicrystal sapphire substrate and are voltage controlled to generate radiation in the frequency range of 0.05-1 THz. The detector used in this work consists of a gate-defined quantum-dot photon-to-charge transducer coupled to a single-electron transistor. Both the emitter and the detector are equipped with a matching on-chip wide-band antenna. The combination of a tuneable emitter and detector allows us to determine the efficacy of the YBCO emitter and also to analyze the elementary processes involved in the detection.
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- 2016
18. Engineering and metrology of epitaxial graphene
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Alexander Tzalenchuk, Mikael Syväjärvi, Sergey Kubatkin, Thomas Bjørnholm, Tjbm Janssen, Sergey Kopylov, Vladimir I. Fal'ko, Samuel Lara-Avila, Karin Cedergren, Olga Kazakova, Rositza Yakimova, and Kasper Moth-Poulsen
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Materials science ,Graphene ,Macroscopic quantum phenomena ,Nanotechnology ,General Chemistry ,Quantum Hall effect ,Condensed Matter Physics ,Metrology ,law.invention ,chemistry.chemical_compound ,chemistry ,law ,Materials Chemistry ,Silicon carbide ,Epitaxial graphene - Abstract
Here we review the concepts and technologies, in particular photochemical gating, which contributed to the recent progress in quantum Hall resistance metrology based on large scale epitaxial graphene on silicon carbide.
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- 2011
19. Non-Volatile Photochemical Gating of an Epitaxial Graphene/Polymer Heterostructure
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Rositza Yakimova, Vladimir I. Fal'ko, Thomas Bjørnholm, Alexander Tzalenchuk, Samuel Lara-Avila, Kasper Moth-Poulsen, and Sergey Kubatkin
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chemistry.chemical_classification ,Materials science ,Polymers ,Ultraviolet Rays ,Graphene ,Mechanical Engineering ,Heterojunction ,Nanotechnology ,Polymer ,Electron acceptor ,Photochemical Processes ,Nanomaterials ,law.invention ,chemistry.chemical_compound ,Photoactive layer ,chemistry ,Mechanics of Materials ,law ,Silicon carbide ,Graphite ,General Materials Science ,Volatilization ,Bilayer graphene - Abstract
A novel heterostructure based on epitaxial graphene grown on silicon carbide combined with two polymers is demonstrated, with a neutral spacer and a photoactive layer that provides potent electron acceptors under UV light exposure. UV exposure of this heterostructure enables control of the electrical parameters of graphene in a non-invasive, non-volatile, and reversible way.
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- 2011
20. Towards a quantum resistance standard based on epitaxial graphene
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Alexander Tzalenchuk, Samuel Lara-Avila, Alexei Kalaboukhov, Sara Paolillo, Mikael Syväjärvi, Rositza Yakimova, Olga Kazakova, T. J. B. M. Janssen, Vladimir Fal'ko, and Sergey Kubatkin
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Materials science ,Graphene ,Biomedical Engineering ,Bioengineering ,Nanotechnology ,Quantum Hall effect ,Condensed Matter Physics ,Engineering physics ,Atomic and Molecular Physics, and Optics ,law.invention ,Metrology ,chemistry.chemical_compound ,chemistry ,law ,Silicon carbide ,General Materials Science ,Wafer ,Electronics ,Electrical and Electronic Engineering ,Quantum ,Graphene nanoribbons - Abstract
The quantum Hall effect allows the international standard for resistance to be defined in terms of the electron charge and Planck's constant alone. The effect comprises the quantization of the Hall resistance in two-dimensional electron systems in rational fractions of R(K) = h/e(2) = 25,812.807557(18) Omega, the resistance quantum. Despite 30 years of research into the quantum Hall effect, the level of precision necessary for metrology--a few parts per billion--has been achieved only in silicon and iii-v heterostructure devices. Graphene should, in principle, be an ideal material for a quantum resistance standard, because it is inherently two-dimensional and its discrete electron energy levels in a magnetic field (the Landau levels) are widely spaced. However, the precisions demonstrated so far have been lower than one part per million. Here, we report a quantum Hall resistance quantization accuracy of three parts per billion in monolayer epitaxial graphene at 300 mK, four orders of magnitude better than previously reported. Moreover, by demonstrating the structural integrity and uniformity of graphene over hundreds of micrometres, as well as reproducible mobility and carrier concentrations across a half-centimetre wafer, these results boost the prospects of using epitaxial graphene in applications beyond quantum metrology.
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- 2010
21. A Highly Sensitive Detector for Radiation in the Terahertz Region
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L. Kulik, Alexander Tzalenchuk, Vladimir Antonov, Susumu Komiyama, H. Hashiba, P. Kleinschmidt, and Stephen P. Giblin
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Physics ,Lateral quantum dot ,Photon ,business.industry ,Terahertz radiation ,Detector ,Physics::Optics ,Particle detector ,Optics ,Quantum dot ,Optoelectronics ,Quantum efficiency ,Electrical and Electronic Engineering ,Photonics ,business ,Instrumentation - Abstract
In this paper, we report progress in the development of a detector for photons in the terahertz region consisting of a lateral quantum dot (QD), defined in a semiconductor heterostructure by mesa patterning and three negatively biased metallic gates, and a single-electron transistor (SET) on top of the mesa and, hence, capacitively coupled to the QD. We study the behavior of the QD as a function of the potential applied to the gates using the SET as a sensitive charge detector and identify the bias region of the device, where it is sensitive to incident terahertz radiation. The QD converts incident photons into charge excitations, which can be detected by the SET, resulting in a signal of the order 10 8 electrons for each absorbed photon. Based on the dark count rate and an estimate of the quantum efficiency, the detector should enable low-power measurements in the terahertz region with noise-equivalent power ~10-19 W/Hz1/2 exceeding the sensitivity of commercially available bolometers by two orders of magnitude
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- 2007
22. Influence of Impurity Spin Dynamics on Quantum Transport in Epitaxial Graphene
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Vladimir I. Fal'ko, Samuel Lara-Avila, Rositza Yakimova, Silvia Lüscher, Tjbm Janssen, Joshua Folk, Oleksiy Kashuba, Alexander Tzalenchuk, and Sergey Kubatkin
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Physics ,Quantum decoherence ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Magnetoresistance ,Graphene ,FOS: Physical sciences ,General Physics and Astronomy ,Kemi ,Materials Engineering ,Conductivity ,law.invention ,Nanomaterials ,Magnetic field ,Weak localization ,law ,Impurity ,Quantum mechanics ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Chemical Sciences ,Physical Sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
Experimental evidence from both spin-valve and quantum transport measurements points towards unexpectedly fast spin relaxation in graphene. We report magnetotransport studies of epitaxial graphene on SiC in a vector magnetic field showing that spin relaxation, detected using weak-localization analysis, is suppressed by an in-plane magnetic field B-parallel to, and thereby proving that it is caused at least in part by spinful scatterers. A nonmonotonic dependence of the effective decoherence rate on B-parallel to reveals the intricate role of the scatterers spin dynamics in forming the interference correction to the conductivity, an effect that has gone unnoticed in earlier weak localization studies. Funding Agencies|NSERC; CFI; Quantum Matter Institute (QMI); EC Graphene Flagship [CNECT-ICT-604391]; European Metrology Research Program (EMRP) project GraphOhm; ERC Synergy Grant Hetero2D; Deutsche Forschungsgemeinschaft [GRK 1621]; Linnaeus Centre for Quantum Engineering; Swedish Research Council; Knut and Alice Wallenberg Foundation; Swedish Foundation for Strategic Research (SSF); Chalmers Area of Advance NANO
- Published
- 2015
23. Operation of graphene quantum Hall resistance standard in a cryogen-free table-top system
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Rositsa Yakimova, Hans He, I. Antonov, Samuel Lara-Avila, Z. Melhem, Tjbm Janssen, Sergey Kubatkin, Alexander Tzalenchuk, Jonathan M. Williams, and S. Rozhko
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Materials science ,Condensed Matter - Mesoscale and Nanoscale Physics ,Graphene ,Mechanical Engineering ,FOS: Physical sciences ,Macroscopic quantum phenomena ,General Chemistry ,Kemi ,Quantum Hall effect ,Condensed Matter Physics ,Engineering physics ,Magnetic field ,Metrology ,law.invention ,graphene ,quantum Hall effect ,metrology ,Mechanics of Materials ,law ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Chemical Sciences ,Table (database) ,General Materials Science ,Epitaxial graphene ,Quantum - Abstract
We demonstrate quantum Hall resistance measurements with metrological accuracy in a small cryogen-free system operating at a temperature of around 3.8K and magnetic fields below 5T. Operating this system requires little experimental knowledge or laboratory infrastructure, thereby greatly advancing the proliferation of primary quantum standards for precision electrical metrology. This significant advance in technology has come about as a result of the unique properties of epitaxial graphene on SiC., 15 pages, 9 figures
- Published
- 2015
24. Physics of a disordered Dirac point in epitaxial graphene from temperature-dependent magnetotransport measurements
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Alexander Tzalenchuk, Rositsa Yakimova, Vladimir Antonov, Jack A. Alexander-Webber, Tjbm Janssen, Sergey Kubatkin, Samuel Lara-Avila, Jian Huang, A. M. R. Baker, Tom Yager, and Robin J. Nicholas
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media_common.quotation_subject ,02 engineering and technology ,Electron ,Conductivity ,7. Clean energy ,01 natural sciences ,Asymmetry ,law.invention ,law ,Hall effect ,Impurity ,0103 physical sciences ,010306 general physics ,media_common ,Physics ,Condensed matter physics ,Graphene ,Scattering ,scattering ,Kemi ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Electronic, Optical and Magnetic Materials ,boron-nitride ,Chemical Sciences ,transport ,0210 nano-technology ,Excitation - Abstract
We report a study of disorder effects on epitaxial graphene in the vicinity of the Dirac point by magnetotransport. Hall effect measurements show that the carrier density increases quadratically with temperature, in good agreement with theoretical predictions which take into account intrinsic thermal excitation combined with electron-hole puddles induced by charged impurities. We deduce disorder strengths in the range 10.2-31.2 meV, depending on the sample treatment. We investigate the scattering mechanisms and estimate the impurity density to be 3.0-9.1x10(10) cm(-2) for our samples. A scattering asymmetry for electrons and holes is observed and is consistent with theoretical calculations for graphene on SiC substrates. We also show that the minimum conductivity increases with increasing disorder strength, in good agreement with quantum-mechanical numerical calculations. Funding Agencies|U.K. EPSRC; NMS, E.U. Graphene Flagship [CNECT-ICT-604391]; EMRP Graph Ohm; Swedish Foundation for Strategic Research (SSF); Linnaeus Centre for Quantum Engineering; Knut and Alice Wallenberg Foundation; Chalmers AoA Nano; China Scholarship Council
- Published
- 2015
25. A prototype of R-K/200 quantum Hall array resistance standard on epitaxial graphene
- Author
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Alexander Tzalenchuk, Samuel Lara-Avila, Sergey Kubatkin, Arseniy Lartsev, Rositsa Yakimova, and Andrey Danilov
- Subjects
Materials science ,General Physics and Astronomy ,02 engineering and technology ,Quantum Hall effect ,Series and parallel circuits ,7. Clean energy ,01 natural sciences ,law.invention ,quantum Hall effect ,chemistry.chemical_compound ,resistance metrology ,law ,Electrical resistivity and conductivity ,0103 physical sciences ,Silicon carbide ,010306 general physics ,Condensed matter physics ,Graphene ,Kemi ,Orders of magnitude (numbers) ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Magnetic field ,chemistry ,Chemical Sciences ,0210 nano-technology ,Current density - Abstract
Epitaxial graphene on silicon carbide is a promising material for the next generation of quantum Hall resistance standards. Single Hall bars made of graphene have already surpassed their state-of-the-art GaAs based counterparts as an R-K/2 (RK = h/e(2)) standard, showing at least the same precision and higher breakdown current density. Compared to single devices, quantum Hall arrays using parallel or series connection of multiple Hall bars can offer resistance values spanning several orders of magnitude and (in case of parallel connection) significantly larger measurement currents, but impose strict requirements on uniformity of the material. To evaluate the quality of the available material, we have fabricated arrays of 100 Hall bars connected in parallel on epitaxial graphene. One out of four devices has shown quantized resistance that matched the correct value of R-K/200 within the measurement precision of 10(-4) at magnetic fields between 7 and 9 T. The defective behaviour of other arrays is attributed mainly to non-uniform doping. This result confirms the acceptable quality of epitaxial graphene, pointing towards the feasibility of well above 90% yield of working Hall bars. Funding Agencies|EU FP7 STREP ConceptGraphene; EMRP project GraphOhm; Graphene Flagship [CNECT-ICT-604391]; Swedish Foundation for Strategic Research (SSF); Linnaeus Centre for Quantum Engineering; Knut and Allice Wallenberg Foundation; Chalmers AoA Nano; EURAMET; European Union
- Published
- 2015
26. Measurement of the spatial sensitivity of miniature SQUIDs using magnetic-tipped STM
- Author
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J.C. Macfarlane, Julia A. Davies, L Brown, P.W Josephs-Franks, John Gallop, Olga Kazakova, Ling Hao, and Alexander Tzalenchuk
- Subjects
Physics ,Superconductivity ,Squid ,biology ,business.industry ,Physics::Medical Physics ,Metals and Alloys ,Nanotechnology ,Magnetic particle inspection ,Condensed Matter Physics ,Magnetic flux ,Magnetic field ,Scanning SQUID microscopy ,Condensed Matter::Superconductivity ,biology.animal ,Materials Chemistry ,Ceramics and Composites ,Magnetic nanoparticles ,Optoelectronics ,Sensitivity (control systems) ,Electrical and Electronic Engineering ,business - Abstract
Large area superconducting quantum interference devices (SQUIDs) are known to be ultimate sensors of magnetic flux. By diminishing the size of a SQUID loop, the energy sensitivity of the device can be increased to near quantum-limited operation whilst also making it less sensitive to external magnetic field noise and improving its coupling to any nano-scale magnetic particle within the loop. This makes it an ideal nano-sensor for magnetic particles including single molecules. It is, however, important to optimize the coupling between any magnetic nano-particle placed within the SQUID and the SQUID itself in order to achieve maximum sensitivity for the spin detection. We have made some preliminary calculations of the expected SQUID response to a magnetic particle placed at different locations within the SQUID device, and using a magnetic tip in a scanning tunnelling microscope (STM) we are able to produce a spatial map of the SQUID sensitivity. Initial results on a 3 µm diameter loop SQUID are presented to demonstrate this method.
- Published
- 2003
27. Sub-micron YBa2Cu3O7−δ step-edge Josephson junctions and micro-SQUIDs
- Author
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Peter Larsson, Alexander Tzalenchuk, Ke Chen, Per E. Magnelind, and Zdravko Ivanov
- Subjects
Physics ,Superconductivity ,Josephson effect ,Coupling ,business.industry ,Physics::Medical Physics ,Energy Engineering and Power Technology ,Condensed Matter Physics ,Electronic, Optical and Magnetic Materials ,law.invention ,Pi Josephson junction ,SQUID ,Modulation ,Scanning SQUID microscopy ,law ,Condensed Matter::Superconductivity ,Microscopy ,Optoelectronics ,Electrical and Electronic Engineering ,business - Abstract
We discuss the properties of sub-micron YBa2Cu3O7−δ step-edge Josephson junctions and their application in micro-SQUIDs. We suggest a design of a micro-SQUID sensor for the scanning SQUID microscopy. Two methods of coupling the modulation and feedback signals to the sensor are described. Influence of a superconducting sample on the sensor parameters is analyzed for the two configurations.
- Published
- 2002
28. Breakdown of the quantum Hall effect in epitaxial graphene
- Author
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Alexander Tzalenchuk, Robin J. Nicholas, Jack A. Alexander-Webber, Tjbm Janssen, and S. Rozhko
- Subjects
Materials science ,Condensed matter physics ,Orders of magnitude (temperature) ,Graphene ,law ,Hall effect ,Thermal Hall effect ,Quantum Hall effect ,Bilayer graphene ,Graphene nanoribbons ,Magnetic field ,law.invention - Abstract
© 2014 IEEE. We present the phase space defined by the quantum Hall effect breakdown in polymer gated epitaxial graphene on SiC (SiC/G) as a function of temperature, current, carrier density, and magnetic field. At 2 K, breakdown currents (Ic) almost 2 orders of magnitude greater than in GaAs devices are observed. We use this knowledge to explore the potential of using graphene as a high temperature (> 2 K) and low magnetic field (< 5 T) quantum resistance standard.
- Published
- 2014
29. The EMRP project GraphOhm - Towards quantum resistance metrology based on graphene
- Author
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A.F. Satrapinski, P. Vrabček, Rositza Yakimova, Blaise Jeanneret, W. Poirier, Alexander Tzalenchuk, C. Hwang, Franz J. Ahlers, Jan Kucera, Sergey Kubatkin, and Tobias Bergsten
- Subjects
Joint research ,Semiconductor ,business.industry ,Computer science ,Graphene ,law ,Electrical engineering ,Electrical measurements ,Quantum Hall effect ,business ,Quantum ,Metrology ,law.invention - Abstract
A new joint research project (JRP) integrating metrology institutes and universities from nine countries is aimed at realization of a new generation of standards for quantum resistance metrology. The project exploits graphene's properties to simplify operation of standards without compromising the unprecedented precision delivered by semiconductor quantum Hall devices. Higher operating temperatures (above 4.2 K, and up to 8 K) and together with lower magnetic fields (below 5 T, and potentially down to 2 T) will lead to a significantly improved and cost-saving dissemination of intrinsically referenced resistance standards to all end-users relying on electrical measurements.
- Published
- 2014
30. Visualisation of edge effects in side-gated graphene nanodevices
- Author
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Alessandra Manzin, Arseniy Lartsev, Alexander Tzalenchuk, Olga Kazakova, Vishal Panchal, and Rositza Yakimova
- Subjects
Conduction electron ,Multidisciplinary ,Materials science ,Condensed Matter - Mesoscale and Nanoscale Physics ,business.industry ,Graphene ,FOS: Physical sciences ,Kemi ,Physics - Applied Physics ,Applied Physics (physics.app-ph) ,Electron doped ,Edge (geometry) ,Thermal conduction ,Article ,law.invention ,Narrow band ,law ,Electric field ,Chemical Sciences ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Optoelectronics ,business ,Atmospheric contamination - Abstract
Using local scanning electrical techniques we study edge effects in side-gated Hall nanodevices made of epitaxial graphene. We demonstrate that lithographically defined edges of the graphene channel exhibit hole conduction within the narrow band of ~60-125 nm width, whereas the bulk of the material is electron doped. The effect is the most pronounced when the influence of atmospheric contamination is minimal. We also show that the electronic properties at the edges can be precisely tuned from hole to electron conduction by using moderate strength electrical fields created by side-gates. However, the central part of the channel remains relatively unaffected by the side-gates and retains the bulk properties of graphene., Comment: 4 Figures, 1 Table
- Published
- 2014
31. Tuning carrier density across Dirac point in epitaxial graphene on SiC by corona discharge
- Author
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Alexander Tzalenchuk, Sergey Kubatkin, Arseniy Lartsev, Tobias Bergsten, Samuel Lara-Avila, Rositza Yakimova, Tjbm Janssen, and Tom Yager
- Subjects
Materials science ,Physics and Astronomy (miscellaneous) ,business.industry ,Graphene ,Macroscopic quantum phenomena ,Nanotechnology ,Kemi ,Epitaxy ,7. Clean energy ,Ion ,law.invention ,Semiconductor ,law ,Topological insulator ,Physical Sciences ,Chemical Sciences ,Quantum metrology ,Optoelectronics ,business ,Corona discharge - Abstract
We demonstrate reversible carrier density control across the Dirac point (Delta n similar to 10(13) cm(-2)) in epitaxial graphene on SiC (SiC/G) via high electrostatic potential gating with ions produced by corona discharge. The method is attractive for applications where graphene with a fixed carrier density is needed, such as quantum metrology, and more generally as a simple method of gating 2DEGs formed at semiconductor interfaces and in topological insulators. Funding Agencies|Graphene Flagship [CNECT-ICT-604391]; Swedish Foundation for Strategic Research (SSF); Linnaeus Centre for Quantum Engineering; Knut and Allice Wallenberg Foundation; Chalmers AoA Nano; NMS (UK); EMRP project GraphOhm; EMRP within EURAMET; European Union
- Published
- 2014
32. Hot carrier relaxation of Dirac fermions in bilayer epitaxial graphene
- Author
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Samuel Lara-Avila, D. K. Gaskill, Jack A. Alexander-Webber, Jian Huang, Tjbm Janssen, Alexander Tzalenchuk, Sergey Kubatkin, Robin J. Nicholas, Tom Yager, Rachael L. Myers-Ward, and Virginia D. Wheeler
- Subjects
Physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Graphene ,Phonon ,Bilayer ,Relaxation (NMR) ,FOS: Physical sciences ,Condensed Matter Physics ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,law.invention ,Weak localization ,symbols.namesake ,Condensed Matter::Materials Science ,Dirac fermion ,law ,Monolayer ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,symbols ,General Materials Science ,Bilayer graphene - Abstract
Energy relaxation of hot Dirac fermions in bilayer epitaxial graphene is experimentally investigated by magnetotransport measurements on Shubnikov-de Haas oscillations and weak localization. The hot-electron energy loss rate is found to follow the predicted Bloch-Gr\"uneisen power-law behaviour of $T^4$ at carrier temperatures from 1.4 K up to $\sim$100 K, due to electron-acoustic phonon interactions with a deformation potential coupling constant of 22 eV. A carrier density dependence $n_e^{-1.5}$ in the scaling of the $T^4$ power law is observed in bilayer graphene, in contrast to the $n_e^{-0.5}$ dependence in monolayer graphene, leading to a crossover in the energy loss rate as a function of carrier density between these two systems. The electron-phonon relaxation time in bilayer graphene is also shown to be strongly carrier density dependent, while it remains constant for a wide range of carrier densities in monolayer graphene. Our results and comparisons between the bilayer and monolayer exhibit a more comprehensive picture of hot carrier dynamics in graphene systems., Comment: 9 pages, 8 figures
- Published
- 2014
- Full Text
- View/download PDF
33. Transport properties of submicron YBa2Cu3O7−δ step-edge Josephson junctions
- Author
-
Zdravko Ivanov, Peter Larsson, and Alexander Tzalenchuk
- Subjects
Josephson effect ,Materials science ,High-temperature superconductivity ,Condensed matter physics ,General Physics and Astronomy ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Microstructure ,law.invention ,SQUID ,Pi Josephson junction ,law ,Condensed Matter::Superconductivity ,Quasiparticle ,Superconducting tunnel junction ,Thin film - Abstract
Submicron step-edge Josephson junctions in YBa2Cu3O7−δ (YBCO) thin films were fabricated and studied. All measured junctions fall into three categories: low critical current resistively shunted Josephson junctions, intrinsic Josephson junctions, and quasiparticle tunnel junctions. The transport in the junctions is correlated with the microstructure of YBCO films grown on the step edge. We argue that the properties of conventional step-edge junctions can be understood as a superposition of those types.
- Published
- 2001
34. Tl/sub 2/Ba/sub 2/CaCu/sub 2/O/sub 8/ films: Growth and applications in dc SQUIDs and microwave devices
- Author
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I. M. Angelov, Y.F. Chen, Alexander L. Vasiliev, L.-G. Johansson, Evgeni Stepantsov, Alexander Tzalenchuk, Zdravko Ivanov, Tord Claeson, R. Kojouharov, V.A. Roddatis, and Eva Olsson
- Subjects
Josephson effect ,High-temperature superconductivity ,Materials science ,Condensed matter physics ,business.industry ,Yttrium barium copper oxide ,High-electron-mobility transistor ,Condensed Matter Physics ,Electronic, Optical and Magnetic Materials ,law.invention ,Resonator ,chemistry.chemical_compound ,chemistry ,law ,Phase noise ,Optoelectronics ,Electrical and Electronic Engineering ,Thin film ,business ,Microwave - Abstract
Tl-2212 thin films were grown ex situ in a two step process on a variety of substrates, including ones with artificially introduced high angle steps. Grain boundary weak links were formed on LaAlO/sub 3/ substrates with steps and on bicrystal substrates and were employed in dc SQUIDs. The white noise level of the SQUIDs was 50/spl mu//spl Phi//sub 0///spl radic/(Hz) at 77 K. A 12.5 GHz HEMT oscillator stabilized with a Tl-2212 resonator gave 8-10 dB lower phase noise than using a gold resonator.
- Published
- 1997
35. Quantum resistance metrology using graphene
- Author
-
Alexander Tzalenchuk, Samuel Lara-Avila, Sergey Kubatkin, Vladimir I. Fal'ko, and Tjbm Janssen
- Subjects
Physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Graphene ,General Physics and Astronomy ,FOS: Physical sciences ,Nanotechnology ,Material system ,02 engineering and technology ,Chemical vapor deposition ,021001 nanoscience & nanotechnology ,01 natural sciences ,Metrology ,law.invention ,Models, Chemical ,law ,Reference Values ,0103 physical sciences ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Electric Impedance ,Quantum Theory ,Computer Simulation ,Graphite ,010306 general physics ,0210 nano-technology ,Quantum - Abstract
In this paper we review the recent extraordinary progress in the development of a new quantum standard for resistance based on graphene. We discuss the unique properties of this material system relating to resistance metrology and discuss results of the recent highest-ever precision direct comparison of the Hall resistance between graphene and traditional GaAs. We mainly focus our review on graphene expitaxially grown on SiC, a system which so far resulted in the best results. We also brie y discuss progress in the two other graphene material systems, exfoliated graphene and chemical vapour deposition graphene, and make a critical comparison with SiC graphene. Finally we discuss other possible applications of graphene in metrology., arXiv admin note: substantial text overlap with arXiv:1202.2985
- Published
- 2013
- Full Text
- View/download PDF
36. Phase space for the breakdown of the quantum Hall effect in epitaxial graphene
- Author
-
Robin J. Nicholas, Rositsa Yakimova, Samuel Lara-Avila, A. M. R. Baker, Duncan K. Maude, Alexander Tzalenchuk, Jack A. Alexander-Webber, Benjamin A. Piot, Sergey Kubatkin, Tjbm Janssen, Department of Physics [Oxford], University of Oxford [Oxford], Department of Physics, Chemistry and Biology, Linköping University, Laboratoire national des champs magnétiques intenses - Grenoble (LNCMI-G), Centre National de la Recherche Scientifique (CNRS)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut National des Sciences Appliquées - Toulouse (INSA Toulouse), Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées, University of Oxford, Université Joseph Fourier - Grenoble 1 (UJF)-Institut National des Sciences Appliquées - Toulouse (INSA Toulouse), Institut National des Sciences Appliquées (INSA)-Université de Toulouse (UT)-Institut National des Sciences Appliquées (INSA)-Université de Toulouse (UT)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Centre National de la Recherche Scientifique (CNRS), Laboratoire national des champs magnétiques intenses - Toulouse (LNCMI-T), Institut National des Sciences Appliquées - Toulouse (INSA Toulouse), and Université de Toulouse (UT)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])
- Subjects
Phase boundary ,Materials science ,Magnetoresistance ,Orders of magnitude (temperature) ,FOS: Physical sciences ,General Physics and Astronomy ,02 engineering and technology ,Quantum Hall effect ,Plateau (mathematics) ,01 natural sciences ,7. Clean energy ,Condensed Matter::Materials Science ,Teknik och teknologier ,Condensed Matter::Superconductivity ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,0103 physical sciences ,010306 general physics ,ComputingMilieux_MISCELLANEOUS ,[PHYS.COND.CM-MSQHE]Physics [physics]/Condensed Matter [cond-mat]/Mesoscopic Systems and Quantum Hall Effect [cond-mat.mes-hall] ,Condensed matter physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Fermi energy ,021001 nanoscience & nanotechnology ,Magnetic field ,[PHYS.COND.CM-S]Physics [physics]/Condensed Matter [cond-mat]/Superconductivity [cond-mat.supr-con] ,Phase space ,Physical Sciences ,Engineering and Technology ,0210 nano-technology - Abstract
We report the phase space defined by the quantum Hall effect breakdown in polymer gated epitaxial graphene on SiC (SiC/G) as a function of temperature, current, carrier density, and magnetic fields up to 30 T. At 2 K, breakdown currents (Ic) almost 2 orders of magnitude greater than in GaAs devices are observed. The phase boundary of the dissipationless state (ρxx=0) shows a [1-(T/Tc)2] dependence and persists up to Tc>45 K at 29 T. With magnetic field Ic was found to increase ∝B3/2 and Tc∝B2. As the Fermi energy approaches the Dirac point, the ν=2 quantized Hall plateau appears continuously from fields as low as 1 T up to at least 19 T due to a strong magnetic field dependence of the carrier density. Funding Agencies|EuroMagNET II||EU|228043|U.K. EPSRC||EU Project ConceptGraphene||NPL Strategic Research Programme
- Published
- 2013
37. Energy loss rates of hot Dirac fermions in epitaxial, exfoliated, and CVD graphene
- Author
-
Tjbm Janssen, Jack A. Alexander-Webber, Alexander Tzalenchuk, Lain-Jong Li, S. D. McMullan, Robin J. Nicholas, Rositsa Yakimova, Samuel Lara-Avila, Cheng-Te Lin, T. Altebaeumer, Sergey Kubatkin, and A. M. R. Baker
- Subjects
electron ,Materials science ,Magnetoresistance ,02 engineering and technology ,Chemical vapor deposition ,Electron ,Epitaxy ,01 natural sciences ,7. Clean energy ,law.invention ,Condensed Matter::Materials Science ,symbols.namesake ,law ,Teknik och teknologier ,0103 physical sciences ,010306 general physics ,Condensed matter physics ,Graphene ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Exfoliation joint ,Electronic, Optical and Magnetic Materials ,Weak localization ,Dirac fermion ,Physical Sciences ,oscillations ,symbols ,Engineering and Technology ,0210 nano-technology - Abstract
Energy loss rates for hot carriers in graphene have been measured using graphene produced by epitaxial growth on SiC, exfoliation, and chemical vapor deposition (CVD). It is shown that the temperature dependence of the energy loss rates measured with high-field damped Shubnikov-de Haas oscillations and the temperature dependence of the weak localization peak close to zero field correlate well, with the high-field measurements understating the energy loss rates by similar to 40% compared to the low-field results. The energy loss rates for all graphene samples follow a universal scaling of T-e(4) at low temperatures and depend weakly on carrier density proportional to n(-1/2), evidence for enhancement of the energy loss rate due to disorder in CVD samples. Funding Agencies|UK EPSRC||Swedish Research Council||Foundation for Strategic Research||UK National Measurement Office||EU
- Published
- 2013
38. Standardization of surface potential measurements of graphene domains
- Author
-
Alexander Tzalenchuk, Ruth Pearce, Rositza Yakimova, Olga Kazakova, and Vishal Panchal
- Subjects
Materials science ,Surface Properties ,FOS: Physical sciences ,Scanning capacitance microscopy ,Microscopy, Scanning Probe ,Article ,Nanomaterials ,law.invention ,law ,Electrical resistivity and conductivity ,Teknik och teknologier ,Materials Testing ,Microscopy ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Work function ,Kelvin probe force microscope ,Multidisciplinary ,Condensed Matter - Mesoscale and Nanoscale Physics ,business.industry ,Graphene ,Contact resistance ,Nanoparticles ,Optoelectronics ,Engineering and Technology ,Graphite ,business - Abstract
We compare the three most commonly used scanning probe techniques to obtain a reliable value of the work function in graphene domains of different thickness. The surface potential (SP) of graphene is directly measured in Hall bar geometry via a combination of electrical functional microscopy and spectroscopy techniques, which enables calibrated work function measurements of graphene domains in ambient conditions with values Φ1LG ~4.55 ± 0.02 eV and Φ2LG ~ 4.44 ± 0.02 eV for single- and bi-layer, respectively. We demonstrate that frequency-modulated Kelvin probe force microscopy (FM-KPFM) provides more accurate measurement of the SP than amplitude-modulated (AM)-KPFM. The discrepancy between experimental results obtained by different techniques is discussed. In addition, we use FM-KPFM for contactless measurements of the specific components of the device resistance. We show a strong non-Ohmic behavior of the electrode-graphene contact resistance and extract the graphene channel resistivity. Funding Agencies|NMS under the IRD Graphene Project (NPL)||EU FP7 Project ConceptGraphene
- Published
- 2013
39. Small epitaxial graphene devices for magnetosensing applications
- Author
-
Alexander Tzalenchuk, Rositza Yakimova, Olga Kazakova, Vishal Panchal, Sergey Kubatkin, and Karin Cedergren
- Subjects
Electron mobility ,Research Groups and Centres\Physics\Low Temperature Physics ,Materials science ,Graphene ,business.industry ,Faculty of Science\Physics ,General Physics and Astronomy ,Nanotechnology ,Chemical vapor deposition ,Semiconductor device ,Epitaxy ,law.invention ,law ,Teknik och teknologier ,Monolayer ,Engineering and Technology ,Optoelectronics ,Hall effect sensor ,business ,Graphene nanoribbons - Abstract
Hall sensors with the width range from 0.5 to 20.0 mu m have been fabricated out of a monolayer graphene epitaxially grown on SiC. The sensors have been studied at room temperature using transport and noise spectrum measurements. The minimum detectable field of a typical 10-mu m graphene sensor is approximate to 2.5 mu T/root Hz, making them comparable with state of the art semiconductor devices of the same size and carrier concentration and superior to devices made of CVD graphene. Relatively high resistance significantly restricts performance of the smallest 500-nm devices. Carrier mobility is strongly size dependent, signifying importance of both intrinsic and extrinsic factors in the optimization of the device performance. Funding Agencies|EU|JRP IND 11
- Published
- 2012
- Full Text
- View/download PDF
40. Precision comparison of the quantum Hall effect in graphene and gallium arsenide
- Author
-
Nick Fletcher, R Goebel, Tjbm Janssen, Vladimir I. Fal'ko, Samuel Lara-Avila, Jonathan M. Williams, Sergey Kubatkin, Rositsa Yakimova, and Alexander Tzalenchuk
- Subjects
Physics ,Condensed matter physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Graphene ,General Engineering ,FOS: Physical sciences ,Heterojunction ,Quantum Hall effect ,Cryogenic current comparator ,Metrology ,law.invention ,Gallium arsenide ,chemistry.chemical_compound ,Quality (physics) ,Electrical resistance and conductance ,chemistry ,law ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) - Abstract
The half-integer quantum Hall effect in epitaxial graphene is compared with high precision to the well known integer effect in a GaAs/AlGaAs heterostructure. We find no difference between the quantised resistance values within the relative standard uncertainty of our measurement of $8.7\times 10^{-11}$. The result places new tighter limits on any possible correction terms to the simple relation $R_{\rm K}=h/e^2$, and also demonstrates that epitaxial graphene samples are suitable for application as electrical resistance standards of the highest metrological quality. We discuss the characterisation of the graphene sample used in this experiment and present the details of the cryogenic current comparator bridge and associated uncertainty budget.
- Published
- 2012
41. Breakdown of the quantum Hall effect in graphene
- Author
-
Sergey Kubatkin, Alexander Tzalenchuk, Robin J. Nicholas, Sergey Kopylov, Samuel Lara-Avila, Vladimir I. Fal'ko, A. M. R. Baker, Rositza Yakimova, Tjbm Janssen, and Jack A. Alexander-Webber
- Subjects
Materials science ,Condensed matter physics ,Graphene ,law ,Hall effect ,Wide-bandgap semiconductor ,Macroscopic quantum phenomena ,Quantum Hall effect ,Epitaxy ,Quantum ,Temperature measurement ,law.invention - Abstract
We present experimental details on the carrier density dependent breakdown current in epitaxial graphene grown on SiC. We show that in this system even at very low carrier densities and moderate temperatures it is still possible to have a breakdown current large enough for metrologically accurate quantum Hall resistance measurements. This work paves the way for a simple bench top/turnkey quantum resistance standard. © 2012 IEEE.
- Published
- 2012
42. Submicron YBa2Cu3Ox ramp Josephson junctions
- Author
-
Björn Högberg, Alexander Tzalenchuk, Philippe V. Komissinski, and Zdravko Ivanov
- Subjects
Josephson effect ,Crystal ,Materials science ,High-temperature superconductivity ,Physics and Astronomy (miscellaneous) ,Amorphous carbon ,Condensed matter physics ,law ,Electrode ,Ion milling machine ,Lithography ,Electron-beam lithography ,law.invention - Abstract
Submicron YBa2Cu3Ox/PrBa2Cu2.6Ga0.4Ox/YBa2Cu3Ox ramp-type Josephson junctions were fabricated and tested. The submicron bridges in the top electrode were patterned by e-beam lithography and Ar ion milling through an amorphous carbon (a-C) mask. Junctions with width ranging from 0.2 to 8 μm and oriented along different crystal directions of YBa2Cu3Ox have been produced. Current–voltage characteristics show a behavior consistent with the resistively shunted junction model with small excess current. Junction critical current densities of about 10 kA/cm2 and characteristic voltages up to 6 mV were measured at 4.2 K for the submicron junctions. Junctions along different crystal orientations showed different characteristics suggesting an influence from the d-wave order parameter.
- Published
- 2002
43. Disordered Fermi Liquid in Epitaxial Graphene from Quantum Transport Measurements
- Author
-
Tobias Bergsten, Rositza Yakimova, Samuel Lara-Avila, Sergey Kubatkin, Alexander Tzalenchuk, Karin Cedergren, Tjbm Janssen, and Vladimir I. Fal'ko
- Subjects
Length scale ,Physics ,Condensed matter physics ,General Physics and Astronomy ,Quantum oscillations ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,weak-localization ,Weak localization ,Condensed Matter::Materials Science ,Electrical resistivity and conductivity ,Teknik och teknologier ,0103 physical sciences ,Monolayer ,Physical Sciences ,Engineering and Technology ,Fermi liquid theory ,Quantum spin liquid ,010306 general physics ,0210 nano-technology ,Fermi gas - Abstract
We have performed magnetotransport measurements on monolayer epitaxial graphene and analyzed them in the framework of the disordered Fermi liquid theory. We have separated the electron-electron and weak-localization contributions to resistivity and demonstrated the phase coherence over a micrometer length scale, setting the limit of at least 50 ps on the spin relaxation time in this material. Funding Agencies|Swedish Research Council||Foundation for Strategic Research||UK National Measurement Office||EU
- Published
- 2011
44. Pound-locking for characterization of superconducting microresonators
- Author
-
Alexander Tzalenchuk, Mark Oxborrow, Jonathan Burnett, and Tobias Lindström
- Subjects
Superconductivity ,Physics ,Research Groups and Centres\Physics\Low Temperature Physics ,Physics - Instrumentation and Detectors ,business.industry ,Faculty of Science\Physics ,FOS: Physical sciences ,Instrumentation and Detectors (physics.ins-det) ,Noise (electronics) ,Characterization (materials science) ,Resonator ,Planar ,Superconducting resonators ,Optoelectronics ,Pound (networking) ,Allan variance ,business ,Superconducting device noise ,Instrumentation ,Throughput (business) - Abstract
We present a new application and implementation of the so-called Pound locking technique for the interrogation of superconducting microresonators. We discuss how by comparing against stable frequency sources this technique can be used to characterize properties of resonators that can not be accessed using traditional methods. Specifically, by analyzing the noise spectra and the Allan deviation we obtain valuable information about the nature of the noise in superconducting planar resonators. This technique also greatly improves the read-out accuracy and measurement throughput compared to conventional methods., 5 pages
- Published
- 2011
45. Anomalously strong pinning of the filling factor nu=2 in epitaxial graphene
- Author
-
Alexander Tzalenchuk, Sergey Kopylov, Tjbm Janssen, Samuel Lara-Avila, Vladimir I. Fal'ko, Sergey Kubatkin, and Rositsa Yakimova
- Subjects
Materials science ,FOS: Physical sciences ,TEKNIKVETENSKAP ,02 engineering and technology ,01 natural sciences ,law.invention ,Quantum capacitance ,Quantization (physics) ,law ,Hall effect ,gas ,0103 physical sciences ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,TECHNOLOGY ,010306 general physics ,quantum capacitance ,Condensed matter physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,Filling factor ,Graphene ,Macroscopic quantum phenomena ,Landau quantization ,resistance standard ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Electronic, Optical and Magnetic Materials ,Magnetic field ,Physical Sciences ,0210 nano-technology - Abstract
We explore the robust quantization of the Hall resistance in epitaxial graphene grown on Si-terminated SiC. Uniquely to this system, the dominance of quantum over classical capacitance in the charge transfer between the substrate and graphene is such that Landau levels (in particular, the one at exactly zero energy) remain completely filled over an extraordinarily broad range of magnetic fields. One important implication of this pinning of the filling factor is that the system can sustain a very high nondissipative current. This makes epitaxial graphene ideally suited for quantum resistance metrology, and we have achieved a precision of 3 parts in 1010 in the Hall resistance-quantization measurements. Original Publication:T J B M Janssen, A Tzalenchuk, Rositsa Yakimova, S Kubatkin, S Lara-Avila, S Kopylov and V I Falko, Anomalously strong pinning of the filling factor nu=2 in epitaxial graphene, 2011, PHYSICAL REVIEW B, (83), 23, 233402.http://dx.doi.org/10.1103/PhysRevB.83.233402Copyright: American Physical Societyhttp://www.aps.org/
- Published
- 2011
46. Quantum Hall resistance standard based on graphene
- Author
-
Alexander Tzalenchuk and Tjbm Janssen
- Subjects
Physics ,Quantization (physics) ,Condensed matter physics ,Quantum spin Hall effect ,Graphene ,law ,Hall effect ,Quantum mechanics ,Biasing ,Electron ,Quantum Hall effect ,Magnetic field ,law.invention - Abstract
We present a detailed study of ρ xx and ρ xy measured on a large high-quality epitaxially grown graphene sample. We have investigated the bias current, temperature, and magnetic field dependence and demonstrate quantization better than 1 part in 108. This level of accuracy easily satisfies all the usual criteria for reliable traceability based on the quantum Hall effect.
- Published
- 2010
47. Sensing individual terahertz photons
- Author
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Leonid Kulik, Alexander Tzalenchuk, Hideomi Hashiba, Vladimir Antonov, and Susumu Komiyama
- Subjects
Photon ,Electromagnetics ,Transistors, Electronic ,Terahertz radiation ,Bioengineering ,02 engineering and technology ,Electron ,Radiation Dosage ,7. Clean energy ,01 natural sciences ,law.invention ,Photometry ,law ,0103 physical sciences ,Quantum Dots ,Nanotechnology ,General Materials Science ,Electrical and Electronic Engineering ,010306 general physics ,Radiometry ,Physics ,Photons ,business.industry ,Waves in plasmas ,Mechanical Engineering ,Transistor ,General Chemistry ,Equipment Design ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,021001 nanoscience & nanotechnology ,Equipment Failure Analysis ,Mechanics of Materials ,Quantum dot ,Excited state ,Optoelectronics ,0210 nano-technology ,business ,Terahertz Radiation - Abstract
One of the promising ways to perform single-photon counting of terahertz radiation consists in sensitive probing of plasma excitation in the electron gas upon photon absorption. We demonstrate the ultimate sensor operating on this principle. It is assembled from a GaAs/AlGaAs quantum dot, electron reservoir and superconducting single-electron transistor. The quantum dot is isolated from the surrounding electron reservoir in such a way that when the excited plasma wave decays, an electron could tunnel off the dot to the reservoir. The resulting charge polarization of the dot is detected with the single-electron transistor. Such a system forms an easy-to-use sensor enabling single-photon counting in a very obscure wavelength region.
- Published
- 2010
48. Towards passive terahertz imaging using a semiconductor quantum dot sensor
- Author
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Alexander Tzalenchuk, S. Giblin, P. Kleinschmidt, L. Kulik, and Vladimir Antonov
- Subjects
Physics ,Photon ,business.industry ,Terahertz radiation ,Quantum sensor ,Macroscopic quantum phenomena ,Near and far field ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Optics ,Spectral sensitivity ,Quantum dot laser ,Quantum dot ,Optoelectronics ,business - Abstract
Passive terahertz imaging of high spectral sensitivity can be performed using a low temperature sensor coupled to an optical system delivering radiation from room temperature. We study this system in application to security screening and material analysis. Different types of low temperature sensors based on GaAs/AlGaAs quantum dots have been designed and characterised. The most sensitive sensor, which is able to detect individual terahertz photons, consists of a quantum dot coupled to a metallic single electron transistor. This sensor requires state of the art nanofabrication. A more robust but less sensitive sensor with relaxed nanofabrication demands, the point contact, is also being developed. The spectral sensitivity of the system is determined by the excitation spectrum of the quantum dot and spectral characteristics of the antenna. We designed a sensor to make an assessment of the combination of traditional log-periodic and near field antennae coupled to the quantum dot, and to compare performance of the sensors with single electron transistor and point contact.
- Published
- 2007
49. Low contact resistance in epitaxial graphene devices for quantum metrology
- Author
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Yung Woo Park, Rositsa Yakimova, Sergey Kubatkin, Alexander Tzalenchuk, Olga Kazakova, Karin Cedergren, Samuel Lara-Avila, Vishal Panchal, Arseniy Lartsev, Kyung Ho Kim, and Tom Yager
- Subjects
Materials science ,General Physics and Astronomy ,Nanotechnology ,02 engineering and technology ,Quantum Hall effect ,01 natural sciences ,law.invention ,law ,Hall effect ,0103 physical sciences ,Monolayer ,Quantum metrology ,010306 general physics ,Graphene ,business.industry ,Contact resistance ,Kemi ,Materials Engineering ,021001 nanoscience & nanotechnology ,lcsh:QC1-999 ,Metrology ,Chemical Sciences ,Optoelectronics ,Nano Technology ,0210 nano-technology ,business ,Bilayer graphene ,lcsh:Physics - Abstract
We investigate Ti/Au contacts to monolayer epitaxial graphene on SiC (0001) for applications in quantum resistance metrology. Using three-terminal measurements in the quantum Hall regime we observed variations in contact resistances ranging from a minimal value of 0.6 Omega up to 11 k Omega. We identify a major source of high-resistance contacts to be due bilayer graphene interruptions to the quantum Hall current, whilst discarding the effects of interface cleanliness and contact geometry for our fabricated devices. Moreover, we experimentally demonstrate methods to improve the reproducibility of low resistance contacts (less than 10 Omega) suitable for high precision quantum resistance metrology. Funding Agencies|Graphene Flagship [CNECT-ICT-604391]; Swedish Foundation for Strategic Research (SSF); Linnaeus Centre for Quantum Engineering; Knut and Alice Wallenberg Foundation; Chalmers AoA Nano; Swedish-Korean Basic Research Cooperative Program of the NRF [2014R1A2A1A1 2067266]; EMRP project GraphOhm; EMRP within EURAMET; EMRP within European Union
- Published
- 2015
50. Isolated quantum dot in application to terahertz photon counting
- Author
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H. Hashiba, Susumu Komiyama, Vladimir Antonov, L. Kulik, P. Kleinschmid, Alexander Tzalenchuk, and S. Giblin
- Subjects
Physics ,Research Groups and Centres\Physics\Low Temperature Physics ,Photon ,Terahertz radiation ,Faculty of Science\Physics ,Coulomb blockade ,Electrometer ,Condensed Matter Physics ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Photon counting ,Electronic, Optical and Magnetic Materials ,Terahertz spectroscopy and technology ,Quantum dot ,Black-body radiation ,Atomic physics - Abstract
We present an experimental study of a large quantum dot (QD) capacitively coupled to an aluminum single electron transistor (SET) and irradiated with terahertz radiation from a blackbody source. The SET is used as a noninvasive electrometer sensitive to a single-charge fluctuation on the QD. Qualitatively different regimes of QD confinement have been identified from the SET response. We demonstrate that the state of a nearly isolated QD can potentially be used for counting individual terahertz photons. © 2006 The American Physical Society.
- Published
- 2006
- Full Text
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