35 results on '"Zimmerle D"'
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2. A Modeling Toolkit for Comparing Ac vs. Dc Electrical Distribution Efficiency in Buildings
- Author
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Othee, A., primary, Cale, James, additional, Santos, A., additional, Frank, S., additional, Zimmerle, D., additional, Ghatpande, O., additional, Duggan, G., additional, and Gerber, D., additional
- Published
- 2022
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3. A methane emissions reduction equivalence framework for alternative leak detection and repair programs
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Fox, T.A. (Thomas A.), Ravikumar, A.P. (Arvind P.), Hugenholtz, C.H. (Chris H.), Zimmerle, D. (Daniel), Barchyn, T.E. (Thomas E.), Johnson, M.R. (Matthew), Lyon, D. (David), Taylor, T. (Tim), Fox, T.A. (Thomas A.), Ravikumar, A.P. (Arvind P.), Hugenholtz, C.H. (Chris H.), Zimmerle, D. (Daniel), Barchyn, T.E. (Thomas E.), Johnson, M.R. (Matthew), Lyon, D. (David), and Taylor, T. (Tim)
- Abstract
Fugitive methane emissions from the oil and gas sector are typically addressed through periodic leak detection and repair surveys. These surveys, conducted manually using handheld leak detection technologies, are time-consuming. To improve the speed and cost-effectiveness of leak detection, technology developers are introducing innovative solutions using mobile platforms, close-range portable systems, and permanent installations. Many of these new approaches promise faster, cheaper, or more effective leak detection than conventional methods. However, ensuring mitigation targets are achieved requires demonstrating that alternative approaches are at least as effective in reducing emissions as current approaches – a concept known as emissions reduction equivalence. Here, we propose a five-stage framework for demonstrating equivalence that combines controlled testing, simulation modeling, and field trials. The framework was developed in consultation with operators, regulators, academics, solution providers, consultants, and non-profit groups from Canada and the U.S. We present the equivalence framework and discuss challenges to implementation.
- Published
- 2019
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4. Determinants of the marginal willingness to pay for improved domestic water and irrigation in partially electrified Rwandan villages
- Author
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Meunier, S., primary, Manning, D. T., additional, Quéval, L., additional, Cherni, J. A., additional, Dessante, P., additional, and Zimmerle, D., additional
- Published
- 2019
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5. Comparison of Load Models for Estimating Electrical Efficiency in DC Microgrids
- Author
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Santos, A., primary, Cale, J., additional, Singh, A., additional, Gerber, D., additional, Frank, S., additional, Duggan, G., additional, Zimmerle, D., additional, and Brown, R., additional
- Published
- 2019
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6. Electric Energy Management in the Smart Home: Perspectives on Enabling Technologies and Consumer Behavior
- Author
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Zipperer, A., primary, Aloise-Young, P. A., additional, Suryanarayanan, S., additional, Zimmerle, D., additional, Roche, R., additional, Earle, L., additional, Christensen, D., additional, and Bauleo, P., additional
- Published
- 2013
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7. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods
- Author
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Roscioli, J. R., primary, Yacovitch, T. I., additional, Floerchinger, C., additional, Mitchell, A. L., additional, Tkacik, D. S., additional, Subramanian, R., additional, Martinez, D. M., additional, Vaughn, T. L., additional, Williams, L., additional, Zimmerle, D., additional, Robinson, A. L., additional, Herndon, S. C., additional, and Marchese, A. J., additional
- Published
- 2015
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8. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods
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Roscioli, J. R., primary, Yacovitch, T. I., additional, Floerchinger, C., additional, Mitchell, A. L., additional, Tkacik, D. S., additional, Subramanian, R., additional, Martinez, D. M., additional, Vaughn, T. L., additional, Williams, L., additional, Zimmerle, D., additional, Robinson, A. L., additional, Herndon, S. C., additional, and Marchese, A. J., additional
- Published
- 2014
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9. Supplementary material to "Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods"
- Author
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Roscioli, J. R., primary, Yacovitch, T. I., additional, Floerchinger, C., additional, Mitchell, A. L., additional, Tkacik, D. S., additional, Subramanian, R., additional, Martinez, D. M., additional, Vaughn, T. L., additional, Williams, L., additional, Zimmerle, D., additional, Robinson, A. L., additional, Herndon, S. C., additional, and Marchese, A. J., additional
- Published
- 2014
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10. A Linear Programming Methodology to Quantify the Impact of PHEVs with V2G Capabilities on Distribution Systems
- Author
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Gireldez, J., primary, Roche, R., additional, Suryanarayanan, S., additional, and Zimmerle, D., additional
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- 2013
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11. A proposed framework for heuristic approaches to resource allocation in the emerging smart grid
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Hansen, T., primary, Roche, R., additional, Suryanarayanan, S., additional, Siegel, H. J., additional, Zimmerle, D., additional, Young, P. M., additional, and Maciejewski, A. A., additional
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- 2012
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12. A community-scale microgrid demonstration: FortZED/RDSI
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Zimmerle, D., primary
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- 2012
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13. A study of methods to predict and measure the transmission of sound through the walls of light aircraft. Integration of certain singular boundary element integrals for applications in linear acoustics
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Zimmerle, D and Bernhard, R. J
- Subjects
Acoustics - Abstract
An alternative method for performing singular boundary element integrals for applications in linear acoustics is discussed. The method separates the integral of the characteristic solution into a singular and nonsingular part. The singular portion is integrated with a combination of analytic and numerical techniques while the nonsingular portion is integrated with standard Gaussian quadrature. The method may be generalized to many types of subparametric elements. The integrals over elements containing the root node are considered, and the characteristic solution for linear acoustic problems are examined. The method may be generalized to most characteristic solutions.
- Published
- 1985
14. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement methods.
- Author
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Roscioli, J. R., Yacovitch, T. I., Floerchinger, C., Mitchell, A. L., Tkacik, D. S., Subramanian, R., Martinez, D. M., Vaughn, T. L., Williams, L., Zimmerle, D., Robinson, A. L., Herndon, S. C., and Marchese, A. J.
- Subjects
NATURAL gas production ,METHANE & the environment ,CARBON monoxide ,CARBON dioxide ,AIR quality - Abstract
Increased natural gas production in recent years has spurred intense interest in methane (CH
4 ) emissions associated with its production, gathering, processing, transmission and distribution. Gathering and processing facilities (G&P facilities) are unique in that the wide range of gas sources (shale, coal-bed, tight gas, conventional, etc.) results in a wide range of gas compositions, which in turn requires an array of technologies to prepare the gas for pipeline transmission and distribution. We present an overview and detailed description of the measurement method and analysis approach used during a 20-week field campaign studying CH4 emissions from the natural gas G&P facilities between October 2013 and April 2014. Dual tracer flux measurements and onsite observations were used to address the magnitude and origins of CH4 emissions from these facilities. The use of a second tracer as an internal standard revealed plume-specific uncertainties in the measured emission rates of 20-47 %, depending upon plume classification. Combining downwind methane, ethane (C2 H6 ), carbon monoxide (CO), carbon dioxide (CO2 ), and tracer gas measurements with onsite tracer gas release allows for quantification of facility emissions, and in some cases a more detailed picture of source locations. [ABSTRACT FROM AUTHOR]- Published
- 2014
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15. A Linear Programming Methodology to Quantify the Impact of PHEVs with V2G Capabilities on Distribution Systems.
- Author
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Giraldez, J., Roche, R., Suryanarayanan, S., and Zimmerle, D.
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- 2013
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16. Methane emissions from transmission & storage compressor stations
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Zimmerle, D. J., Williams, L. L., Vaughn, T. L., Casey Quinn, Subramanian, R., Duggan, G. P., Willson, B., Opsomer, J. D., Marchese, A. J., Martinez, D. M., and Robinson, A. L.
17. Assessing the Progress of the Performance of Continuous Monitoring Solutions under a Single-Blind Controlled Testing Protocol.
- Author
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Ilonze C, Emerson E, Duggan A, and Zimmerle D
- Subjects
- Single-Blind Method, Methane analysis, Air Pollutants analysis, Environmental Monitoring methods
- Abstract
The recent regulatory spotlight on continuous monitoring (CM) solutions and the rapid development of CM solutions have demanded the characterization of solution performance through regular, rigorous testing using consensus test protocols. This study is the second known implementation of such a protocol involving single-blind controlled testing of 9 CM solutions. Controlled releases of rates (6-7100 g) CH
4 /h over durations (0.4-10.2 h) under a wind speed range of (0.7-9.9 m/s) were conducted for 11 weeks. Results showed that 4 solutions achieved method detection limits (DL90s) within the tested emission rate range, with all 4 solutions having both the lowest DL90s (3.9 [3.0, 5.5] kg CH4 /h to 6.2 [3.7, 16.7] kg CH4 /h) and false positive rates (6.9-13.2%), indicating efforts at balancing low sensitivity with a low false positive rate. These results are likely best-case scenario estimates since the test center represents a near-ideal upstream field natural gas operation condition. Quantification results showed wide individual estimate uncertainties, with emissions underestimation and overestimation by factors up to >14 and 42, respectively. Three solutions had >80% of their estimates within a quantification factor of 3 for controlled releases in the ranges of [0.1-1] kg CH4 /h and > 1 kg CH4 /h. Relative to the study by Bell et al., current solutions performance, as a group, generally improved, primarily due to solutions from the study by Bell et al. that were retested. This result highlights the importance of regular quality testing to the advancement of CM solutions for effective emissions mitigation.- Published
- 2024
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18. Methane Quantification Performance of the Quantitative Optical Gas Imaging (QOGI) System Using Single-Blind Controlled Release Assessment.
- Author
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Ilonze C, Wang JL, Ravikumar AP, and Zimmerle D
- Abstract
Quantitative optical gas imaging (QOGI) system can rapidly quantify leaks detected by optical gas imaging (OGI) cameras across the oil and gas supply chain. A comprehensive evaluation of the QOGI system's quantification capability is needed for the successful adoption of the technology. This study conducted single-blind experiments to examine the quantification performance of the FLIR QL320 QOGI system under near-field conditions at a pseudo-realistic, outdoor, controlled testing facility that mimics upstream and midstream natural gas operations. The study completed 357 individual measurements across 26 controlled releases and 71 camera positions for release rates between 0.1 kg Ch4/h and 2.9 kg Ch4/h of compressed natural gas (which accounts for more than 90% of typical component-level leaks in several production facilities). The majority (75%) of measurements were within a quantification factor of 3 (quantification error of -67% to 200%) with individual errors between -90% and 831%, which reduced to -79% to +297% when the mean of estimates of the same controlled release from multiple camera positions was considered. Performance improved with increasing release rate, using clear sky as plume background, and at wind speeds ≤1 mph relative to other measurement conditions.
- Published
- 2024
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19. Impact of randomly assigned "pay-as-you-go" liquefied petroleum gas prices on energy use for cooking: Experimental pilot evidence from rural Rwanda.
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Witinok-Huber R, Keller KP, Abimana E, Ahishakiye C, Chang HH, L'Orange C, Manning DT, Mori R, Muhirwa EF, Muhongerwa L, Ntakirutimana T, Puzzolo E, Quinn C, Rosa G, Tanner K, Young BN, Zimmerle D, Kalisa E, Volckens J, and Clark ML
- Abstract
The disease burden related to air pollution from traditional solid-fuel cooking practices in low- and middle-income countries impacts millions of people globally. Although the use of liquefied petroleum gas (LPG) fuel for cooking can meaningfully reduce household air pollution concentrations, major barriers, including affordability and accessibility, have limited widespread adoption. Using a randomized controlled trial, our objective was to evaluate the association between the cost and use of LPG among 23 rural Rwandan households. We provided a 2-burner LPG stove with accessories and incorporated a "pay-as-you-go" (PAYG) LPG service model that included fuel delivery. PAYG services remove the large up-front cost of cylinder refills by integrating "smart meter" technology that allows participants to pay in incremental amounts, as needed. We assigned three randomized discounted prices for LPG to each household at ~4-week intervals over a 12-week period. We modeled the relationship between randomized PAYG LPG price and use (standardized to monthly periods), analyzing effect modification by relative household wealth. A 1000 Rwandan Franc (about 1 USD at the time of the study) increase in LPG price/kg was associated with a 4.1 kg/month decrease in use (95% confidence interval [CI]: -6.7, -1.6; n=69 observations). Wealth modified this association; we observed a 9.7 kg/month reduction (95% CI: -14.8, -4.5) among wealthier households and a 2.5 kg/month reduction (95% CI: -5.3, 0.3) among lower-wealth households (p-interaction=0.01). The difference in price sensitivity was driven by higher LPG use among wealthier households at more heavily discounted prices; from an 80% to 10% discount, wealthy households used 17.5 to 5.3 kg/month and less wealthy households used 6.2 to 3.1 kg/month. Our pilot-level experimental evidence of PAYG LPG in a rural low-resource setting suggests that further exploration of subsidized pricing varied by household wealth is needed to ensure future policy initiatives can achieve targets without exacerbating inequities., Competing Interests: Declaration of interests The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
- Published
- 2024
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20. Unaddressed Uncertainties When Scaling Regional Aircraft Emission Surveys to Basin Emission Estimates.
- Author
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Zimmerle D, Dileep S, and Quinn C
- Subjects
- Aircraft, Methane analysis, Natural Gas analysis, Air Pollutants analysis
- Abstract
Wide-area aerial methods provide comprehensive screening of methane emissions from oil and gas (O & G) facilities in production basins. Emission detections ("plumes") from these studies are also frequently scaled to the basin level, but little is known regarding the uncertainties during scaling. This study analyzed an aircraft field study in the Denver-Julesburg basin to quantify how often plumes identified maintenance events, using a geospatial inventory of 12,629 O & G facilities. Study partners (7 midstream and production operators) provided the timing and location of 5910 maintenance events during the 6 week study period. Results indicated three substantial uncertainties with potential bias that were unaddressed in prior studies. First, plumes often detect maintenance events, which are large, short-duration, and poorly estimated by aircraft methods: 9.2 to 46% (38 to 52%) of plumes on production were likely known maintenance events. Second, plumes on midstream facilities were both infrequent and unpredictable, calling into question whether these estimates were representative of midstream emissions. Finally, 4 plumes attributed to O & G (19% of emissions detected by aircraft) were not aligned with any O & G location, indicating that the emissions had drifted downwind of some source. It is unclear how accurately aircraft methods estimate this type of plume; in this study, it had material impact on emission estimates. While aircraft surveys remain a powerful tool for identifying methane emissions on O & G facilities, this study indicates that additional data inputs, e.g., detailed GIS data, a more nuanced analysis of emission persistence and frequency, and improved sampling strategies are required to accurately scale plume estimates to basin emissions.
- Published
- 2024
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21. Point Sensor Networks Struggle to Detect and Quantify Short Controlled Releases at Oil and Gas Sites.
- Author
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Day RE, Emerson E, Bell C, and Zimmerle D
- Abstract
This study evaluated multiple commercially available continuous monitoring (CM) point sensor network (PSN) solutions under single-blind controlled release testing conducted at operational upstream and midstream oil and natural gas (O&G) sites. During releases, PSNs reported site-level emission rate estimates of 0 kg/h between 38 and 86% of the time. When non-zero site-level emission rate estimates were provided, no linear correlation between the release rate and the reported emission rate estimate was observed. The average, aggregated across all PSN solutions during releases, shows 5% of the mixing ratio readings at downwind sensors were greater than the site's baseline plus two standard deviations. Four of seven total PSN solutions tested during this field campaign provided site-level emission rate estimates with the site average relative error ranging from -100% to 24% for solution D, -100% to -43% for solution E, -25% for solution F (solution F was only at one site), and -99% to 430% for solution G, with an overall average of -29% across all sites and solutions. Of all the individual site-level emission rate estimates, only 11% were within ±2.5 kg/h of the study team's best estimate of site-level emissions at the time of the releases.
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- 2024
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22. Informing Methane Emissions Inventories Using Facility Aerial Measurements at Midstream Natural Gas Facilities.
- Author
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Brown JA, Harrison MR, Rufael T, Roman-White SA, Ross GB, George FC, and Zimmerle D
- Abstract
Increased interest in greenhouse gas (GHG) emissions, including recent legislative action and voluntary programs, has increased attention on quantifying and ultimately reducing methane emissions from the natural gas supply chain. While inventories used for public or corporate GHG policies have traditionally utilized bottom-up (BU) methods to estimate emissions, the validity of such inventories has been questioned. Therefore, there is attention on utilizing full-facility measurements using airborne, satellite, or drone (top-down (TD)) techniques to inform, improve, or validate inventories. This study utilized full-facility estimates from two independent TD methods at 15 midstream natural gas facilities in the U.S.A., which were compared with a contemporaneous daily inventory assembled by the facility operator, employing comprehensive inventory methods. Estimates from the two TD methods statistically agreed in 2 of 28 paired measurements. Operator inventories, which included extensions to capture sources beyond regular inventory requirements and integration of local measurements, estimated significantly lower emissions than the TD estimates for 40 of 43 paired comparisons. Significant disagreement was observed at most facilities, both between the two TD methods and between the TD estimates and operator inventory. These findings have two implications. First, improving inventory estimates will require additional on-site or ground-based diagnostic screening and measurement of all sources. Second, the TD full-facility measurement methods need to undergo further testing, characterization, and potential improvement specifically tailored for complex midstream facilities.
- Published
- 2023
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23. Performance of Continuous Emission Monitoring Solutions under a Single-Blind Controlled Testing Protocol.
- Author
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Bell C, Ilonze C, Duggan A, and Zimmerle D
- Subjects
- Methane analysis, Natural Gas analysis, Single-Blind Method, Air Pollutants analysis, Environmental Monitoring methods
- Abstract
Continuous emission monitoring (CM) solutions promise to detect large fugitive methane emissions in natural gas infrastructure sooner than traditional leak surveys, and quantification by CM solutions has been proposed as the foundation of measurement-based inventories. This study performed single-blind testing at a controlled release facility (release from 0.4 to 6400 g CH
4 /h) replicating conditions that were challenging, but less complex than typical field conditions. Eleven solutions were tested, including point sensor networks and scanning/imaging solutions. Results indicated a 90% probability of detection (POD) of 3-30 kg CH4 /h; 6 of 11 solutions achieved a POD < 6 kg CH4 /h, although uncertainty was high. Four had true positive rates > 50%. False positive rates ranged from 0 to 79%. Six solutions estimated emission rates. For a release rate of 0.1-1 kg/h, the solutions' mean relative errors ranged from -44% to +586% with single estimates between -97% and +2077%, and 4 solutions' upper uncertainty exceeding +900%. Above 1 kg/h, mean relative error was -40% to +93%, with two solutions within ±20%, and single-estimate relative errors were from -82% to +448%. The large variability in performance between CM solutions, coupled with highly uncertain detection, detection limit, and quantification results, indicates that the performance of individual CM solutions should be well understood before relying on results for internal emissions mitigation programs or regulatory reporting.- Published
- 2023
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24. A Methane Emission Estimation Tool (MEET) for predictions of emissions from upstream oil and gas well sites with fine scale temporal and spatial resolution: Model structure and applications.
- Author
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Allen DT, Cardoso-Saldaña FJ, Kimura Y, Chen Q, Xiang Z, Zimmerle D, Bell C, Lute C, Duggan J, and Harrison M
- Subjects
- Methane analysis, Natural Gas analysis, Time Factors, Air Pollutants analysis, Oil and Gas Fields
- Abstract
In comparing observation based methane emission estimates for oil and gas well sites to routine emissions reported in inventories, the time scale of the measurement should match the time scale over which the inventoried emissions are estimated. Since many measurements are of relatively short duration (seconds to hours), a tool is needed to estimate emissions over these time scales rather than the annual totals reported in most emission inventories. This work presents a tool for estimating routine emissions from oil and gas well sites at multiple time scales; emissions at well sites vary over time due to changes in oil and gas production rates, operating practices and operational modes at the sites. Distributions of routine emissions (expected and inventoried) from well sites are generally skewed, and the nature and degree to which the distributions are skewed depends on the time scales over which emissions are aggregated. Abnormal emissions can create additional skew in these distributions. At very short time scales (emissions aggregated over 1 min) case study distributions presented in this work are both skewed and bimodal, with the modes depending on whether liquid storage tanks are flashing at the time of the measurement and whether abnormal emissions are occurring. At longer time scales (emissions aggregated over 1 day) distributions of routine emissions simulated in this work can have multiple modes if short duration, high emission rate events, such as liquid unloadings or large abnormal emissions, occur at the site. Multiple applications of the methane emission estimation tool (MEET), developed in this work, are presented. These results emphasize the importance of developing detailed emission inventories, which incorporate operational data, when comparing measurements to routine emissions. The model described in this work supports such comparisons and is freely available., Competing Interests: Declaration of competing interest The authors declare the following competing financial interest(s): This work was supported by the Collaboratory to Advance Methane Science (CAMS), a group of companies operating facilities in the natural gas supply chain., (Copyright © 2022 The Authors. Published by Elsevier B.V. All rights reserved.)
- Published
- 2022
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25. Modeling air emissions from complex facilities at detailed temporal and spatial resolution: The Methane Emission Estimation Tool (MEET).
- Author
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Zimmerle D, Duggan G, Vaughn T, Bell C, Lute C, Bennett K, Kimura Y, Cardoso-Saldaña FJ, and Allen DT
- Subjects
- Ethane analysis, Natural Gas analysis, Air Pollutants analysis, Methane analysis
- Abstract
Recent attention to methane emissions from oil and gas infrastructure has increased interest in comparing measurements with inventory emission estimates. While measurement methods typically estimate emissions over a few periods that are seconds to hours in length, current inventory methods typically produce long-term average emission estimates. This temporal mis-alignment complicates comparisons and leads to underestimates in the uncertainty of measurement methods. This study describes a new temporally and spatially resolved inventory emission model (MEET), and demonstrates the model by application to compressor station emissions - the key facility type in midstream natural gas operations The study looks at three common facility measurement methods: tracer flux methods for measuring station emissions, the use of ethane-methane ratios for source attribution of basin-scale estimates, and the behavior of continuous monitoring for leak detection at stations. Simulation results indicate that measurement methods likely underestimate uncertainties in emission estimates by failing to account for the variability in normal facility emissions and variations in ethane/methane ratios. A tracer-based measurement campaign could estimate emissions outside the 95% confidence interval of annual emissions 30% of the time, while ethane/methane ratios could be mis-estimated by as much as 50%. Use of MEET also highlights the need to improve data reporting from measurement campaigns to better capture the temporal and spatial variation in observed emissions., Competing Interests: Declaration of competing interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests: Daniel Zimmerle reports financial support was provided by Collaboratory to Advance Methane Science. David T Allen reports a relationship with Exxon Mobil Upstream Research Company that includes: funding grants. David T Allen reports a relationship with National Institute for Clean and low Carbon Energy (NICE) that includes: funding grants. Daniel Zimmerle reports a relationship with Chevron Inc. that includes: funding grants. Daniel Zimmerle reports a relationship with BP Plc that includes: funding grants. Daniel Zimmerle reports a relationship with The Environmental Partnership (API) that includes: funding grants. Daniel Zimmerle reports a relationship with Renewable Natural Gas Coalition that includes: funding grants. Daniel Zimmerle reports a relationship with Environmental Defense Fund that includes: funding grants. David T Allen reports a relationship with Eastern Research Group that includes: funding grants. Felipe Cardoza-Saldana reports a relationship with Exxon Mobil Upstream Research Company that includes: employment. Daniel Zimmerle reports a relationship with Colorado Air Quality Enterprise Board, as Colorado State Agency that includes: board membership. Over the past five years, multiple authors have also worked on methane emission measurement projects that have been supported by multiple natural gas producers, developers of leak detection solutions, and the Environmental Defense Fund. Multiple co-authors have been active the funded research projects declared by the Corresponding Author (Zimmerle) and co-Author (Allen)., (Copyright © 2022 The Authors. Published by Elsevier B.V. All rights reserved.)
- Published
- 2022
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26. Methane Exhaust Measurements at Gathering Compressor Stations in the United States.
- Author
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Vaughn TL, Luck B, Williams L, Marchese AJ, and Zimmerle D
- Subjects
- Methane analysis, Natural Gas analysis, United States, Vehicle Emissions, Air Pollutants analysis, Greenhouse Gases
- Abstract
Unburned methane entrained in exhaust from natural gas-fired compressor engines ("combustion slip") can account for a substantial portion of station-level methane emissions. A novel in-stack, tracer gas method was coupled with Fourier transform infrared (FTIR) species measurements to quantify combustion slip from natural gas compressor engines at 67 gathering and boosting stations owned or managed by nine "study partner" operators in 11 U.S. states. The mean methane emission rate from 63 four-stroke, lean-burn (4SLB) compressor engines was 5.62 kg/h (95% CI = 5.15-6.17 kg/h) and ranged from 0.3 to 12.6 kg/h. The mean methane emission rate from 39 four-stroke, rich-burn (4SRB) compressor engines was 0.40 kg/h (95% CI = 0.37-0.42 kg/h) and ranged from 0.01 to 4.5 kg/h. Study results for 4SLB engines were lower than both the U.S. EPA compilation of air pollutant emission factors (AP-42) and Inventory of U.S. Greenhouse Gas Emissions and Sinks (GHGI) by 8 and 9%, respectively. Study results for 4SRB engines were 43% of the AP-42 emission factor and 8% of the GHGI emission factor, the latter of which does not distinguish between engine types. Total annual combustion slip from the U.S. natural gas gathering and boosting sector was modeled using measured emission rates and compressor unit counts from the U.S. EPA Greenhouse Gas Reporting Program. Modeled results [328 Gg/y (95% CI = 235-436 Gg/y) of unburned methane] would account for 24% (95% CI = 17-31%) of the 1391 Gg of methane emissions for "Gathering and Boosting Stations", or 6% of the net emissions for "Natural Gas Systems" (5598 Gg) as reported in the 2020 U.S. EPA GHGI. Gathering and boosting combustion slip emissions reported in the 2020 GHGI (374 Gg) fall within the uncertainty of this model.
- Published
- 2021
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27. Detection Limits of Optical Gas Imaging for Natural Gas Leak Detection in Realistic Controlled Conditions.
- Author
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Zimmerle D, Vaughn T, Bell C, Bennett K, Deshmukh P, and Thoma E
- Subjects
- Limit of Detection, Oil and Gas Fields, Methane, Natural Gas
- Abstract
Optical gas imaging (OGI) is a commonly utilized leak detection method in the upstream and midstream sectors of the U.S. natural gas industry. This study characterized the detection efficacy of OGI surveyors, using their own cameras and protocols, with controlled releases in an 8-acre outdoor facility that closely resembles upstream natural gas field operations. Professional surveyors from 16 oil and gas companies and 8 regulatory agencies participated, completing 488 tests over a 10 month period. Detection rates were significantly lower than prior studies focused on camera performance. The leak size required to achieve a 90% probability-of-detection in this study is an order-of-magnitude larger than prior studies. Study results indicate that OGI survey experience significantly impacts leak detection rate: Surveyors from operators/contractors who had surveyed more than 551 sites prior to testing detected 1.7 (1.5-1.8) times more leaks than surveyors who had completed fewer surveys. Highly experienced surveyors adjust their survey speed, examine components from multiple viewpoints, and make other adjustments that improve their leak detection rate, indicating that modifications of survey protocols and targeted training could improve leak detection rates overall.
- Published
- 2020
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28. Methane Emissions from Gathering Compressor Stations in the U.S.
- Author
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Zimmerle D, Vaughn T, Luck B, Lauderdale T, Keen K, Harrison M, Marchese A, Williams L, and Allen D
- Subjects
- Industry, Methane analysis, Population Dynamics, Air Pollutants analysis, Greenhouse Gases
- Abstract
Using results from a nationally representative measurement campaign at 180 gathering compressor stations conducted with nine industry partners, this study estimated emissions for the U.S. gathering sector, where sector-specific emission factors have not been previously available. The study drew from a partner station population of 1705 stations-a significantly larger pool than was available for prior studies. Data indicated that whole gas emission rates from components on gathering stations were comparable to or higher than emission factors utilized by the EPA's greenhouse gas reporting program (GHGRP) but less than emission factors used for similar components on transmission compressor stations. Field data also indicated that the national population of stations likely has a higher fraction of smaller stations, operating at lower throughput per station, than the data used to develop the per-station emission factor used in EPA's greenhouse gas inventory (GHGI). This was the first national study to incorporate extensive activity data reported to the GHGRP, including 319 basin-level reports, covering 15,895 reported compressors. Combining study emission data with 2017 GHGRP activity data, the study indicated statistically lower national emissions of 1290 [1246-1342] Gg methane per year or 66% [64-69%] of current GHGI estimates, despite estimating 17% [12-22%] more stations than the 2017 GHGI (95% confidence interval). Finally, we propose a replicable method that uses GHGRP activity data to annually update GHGI gathering and boost sector emissions.
- Published
- 2020
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29. "Good versus Good Enough?" Empirical Tests of Methane Leak Detection Sensitivity of a Commercial Infrared Camera.
- Author
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Ravikumar AP, Wang J, McGuire M, Bell CS, Zimmerle D, and Brandt AR
- Subjects
- Environmental Monitoring, Natural Gas, Single-Blind Method, Greenhouse Gases, Methane
- Abstract
Methane, a key component of natural gas, is a potent greenhouse gas. A key feature of recent methane mitigation policies is the use of periodic leak detection surveys, typically done with optical gas imaging (OGI) technologies. The most common OGI technology is an infrared camera. In this work, we experimentally develop detection probability curves for OGI-based methane leak detection under different environmental and imaging conditions. Controlled single blind leak detection tests show that the median detection limit (50% detection likelihood) for FLIR-camera based OGI technology is about 20 g CH
4 /h at an imaging distance of 6 m, an order of magnitude higher than previously reported estimates of 1.4 g CH4 /h. Furthermore, we show that median and 90% detection likelihood limit follows a power-law relationship with imaging distance. Finally, we demonstrate that real-world marginal effectiveness of methane mitigation through periodic surveys approaches zero as leak detection sensitivity improves. For example, a median detection limit of 100 g CH4 /h is sufficient to detect the maximum amount of leakage that is possible through periodic surveys. Policy makers should take note of these limits while designing equivalence metrics for next-generation leak detection technologies that can trade sensitivity for cost without affecting mitigation priorities.- Published
- 2018
- Full Text
- View/download PDF
30. Variation in Methane Emission Rates from Well Pads in Four Oil and Gas Basins with Contrasting Production Volumes and Compositions.
- Author
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Robertson AM, Edie R, Snare D, Soltis J, Field RA, Burkhart MD, Bell CS, Zimmerle D, and Murphy SM
- Subjects
- Arkansas, Colorado, Environmental Monitoring, Natural Gas, Wyoming, Air Pollutants analysis, Methane analysis, Oil and Gas Fields
- Abstract
Atmospheric methane emissions from active natural gas production sites in normal operation were quantified using an inverse Gaussian method (EPA's OTM 33a) in four major U.S. basins/plays: Upper Green River (UGR, Wyoming), Denver-Julesburg (DJ, Colorado), Uintah (Utah), and Fayetteville (FV, Arkansas). In DJ, Uintah, and FV, 72-83% of total measured emissions were from 20% of the well pads, while in UGR the highest 20% of emitting well pads only contributed 54% of total emissions. The total mass of methane emitted as a percent of gross methane produced, termed throughput-normalized methane average (TNMA) and determined by bootstrapping measurements from each basin, varied widely between basins and was (95% CI): 0.09% (0.05-0.15%) in FV, 0.18% (0.12-0.29%) in UGR, 2.1% (1.1-3.9%) in DJ, and 2.8% (1.0-8.6%) in Uintah. Overall, wet-gas basins (UGR, DJ, Uintah) had higher TNMA emissions than the dry-gas FV at all ranges of production per well pad. Among wet basins, TNMA emissions had a strong negative correlation with average gas production per well pad, suggesting that consolidation of operations onto single pads may reduce normalized emissions (average number of wells per pad is 5.3 in UGR versus 1.3 in Uintah and 2.8 in DJ).
- Published
- 2017
- Full Text
- View/download PDF
31. Improved Mechanistic Understanding of Natural Gas Methane Emissions from Spatially Resolved Aircraft Measurements.
- Author
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Schwietzke S, Pétron G, Conley S, Pickering C, Mielke-Maday I, Dlugokencky EJ, Tans PP, Vaughn T, Bell C, Zimmerle D, Wolter S, King CW, White AB, Coleman T, Bianco L, and Schnell RC
- Subjects
- Aircraft, Natural Gas, Research Design, Air Pollutants analysis, Methane analysis
- Abstract
Divergence in recent oil and gas related methane emission estimates between aircraft studies (basin total for a midday window) and emissions inventories (annualized regional and national statistics) indicate the need for better understanding the experimental design, including temporal and spatial alignment and interpretation of results. Our aircraft-based methane emission estimates in a major U.S. shale gas basin resolved from west to east show (i) similar spatial distributions for 2 days, (ii) strong spatial correlations with reported NG production (R
2 = 0.75) and active gas well pad count (R2 = 0.81), and (iii) 2× higher emissions in the western half (normalized by gas production) despite relatively homogeneous dry gas and well characteristics. Operator reported hourly activity data show that midday episodic emissions from manual liquid unloadings (a routine operation in this basin and elsewhere) could explain ∼1/3 of the total emissions detected midday by the aircraft and ∼2/3 of the west-east difference in emissions. The 22% emission difference between both days further emphasizes that episodic sources can substantially impact midday methane emissions and that aircraft may detect daily peak emissions rather than daily averages that are generally employed in emissions inventories. While the aircraft approach is valid, quantitative, and independent, our study sheds new light on the interpretation of previous basin scale aircraft studies, and provides an improved mechanistic understanding of oil and gas related methane emissions.- Published
- 2017
- Full Text
- View/download PDF
32. Correction to Measurements of Methane Emissions from Natural Gas Gathering Facilities and Processing Plants: Measurement Results.
- Author
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Mitchell AL, Tkacik DS, Roscioli JR, Herndon SC, Yacovitch TI, Martinez DM, Vaughn TL, Williams L, Sullivan M, Floerchinger C, Omara M, Subramanian R, Zimmerle D, Marchese AJ, and Robinson AL
- Published
- 2015
- Full Text
- View/download PDF
33. Constructing a Spatially Resolved Methane Emission Inventory for the Barnett Shale Region.
- Author
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Lyon DR, Zavala-Araiza D, Alvarez RA, Harriss R, Palacios V, Lan X, Talbot R, Lavoie T, Shepson P, Yacovitch TI, Herndon SC, Marchese AJ, Zimmerle D, Robinson AL, and Hamburg SP
- Subjects
- Greenhouse Effect, Texas, United States, United States Environmental Protection Agency, Air Pollutants analysis, Geologic Sediments chemistry, Methane analysis
- Abstract
Methane emissions from the oil and gas industry (O&G) and other sources in the Barnett Shale region were estimated by constructing a spatially resolved emission inventory. Eighteen source categories were estimated using multiple data sets, including new empirical measurements at regional O&G sites and a national study of gathering and processing facilities. Spatially referenced activity data were compiled from federal and state databases and combined with O&G facility emission factors calculated using Monte Carlo simulations that account for high emission sites representing the very upper portion, or fat-tail, in the observed emissions distributions. Total methane emissions in the 25-county Barnett Shale region in October 2013 were estimated to be 72,300 (63,400-82,400) kg CH4 h(-1). O&G emissions were estimated to be 46,200 (40,000-54,100) kg CH4 h(-1) with 19% of emissions from fat-tail sites representing less than 2% of sites. Our estimate of O&G emissions in the Barnett Shale region was higher than alternative inventories based on the United States Environmental Protection Agency (EPA) Greenhouse Gas Inventory, EPA Greenhouse Gas Reporting Program, and Emissions Database for Global Atmospheric Research by factors of 1.5, 2.7, and 4.3, respectively. Gathering compressor stations, which accounted for 40% of O&G emissions in our inventory, had the largest difference from emission estimates based on EPA data sources. Our inventory's higher O&G emission estimate was due primarily to its more comprehensive activity factors and inclusion of emissions from fat-tail sites.
- Published
- 2015
- Full Text
- View/download PDF
34. Methane emissions from natural gas compressor stations in the transmission and storage sector: measurements and comparisons with the EPA greenhouse gas reporting program protocol.
- Author
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Subramanian R, Williams LL, Vaughn TL, Zimmerle D, Roscioli JR, Herndon SC, Yacovitch TI, Floerchinger C, Tkacik DS, Mitchell AL, Sullivan MR, Dallmann TR, and Robinson AL
- Subjects
- Air Pollutants standards, Environmental Monitoring legislation & jurisprudence, Environmental Monitoring standards, Extraction and Processing Industry standards, United States, Air Pollutants analysis, Environmental Monitoring methods, Extraction and Processing Industry instrumentation, Methane analysis, Natural Gas analysis, United States Environmental Protection Agency standards
- Abstract
Equipment- and site-level methane emissions from 45 compressor stations in the transmission and storage (T&S) sector of the US natural gas system were measured, including 25 sites required to report under the EPA greenhouse gas reporting program (GHGRP). Direct measurements of fugitive and vented sources were combined with AP-42-based exhaust emission factors (for operating reciprocating engines and turbines) to produce a study onsite estimate. Site-level methane emissions were also concurrently measured with downwind-tracer-flux techniques. At most sites, these two independent estimates agreed within experimental uncertainty. Site-level methane emissions varied from 2-880 SCFM. Compressor vents, leaky isolation valves, reciprocating engine exhaust, and equipment leaks were major sources, and substantial emissions were observed at both operating and standby compressor stations. The site-level methane emission rates were highly skewed; the highest emitting 10% of sites (including two superemitters) contributed 50% of the aggregate methane emissions, while the lowest emitting 50% of sites contributed less than 10% of the aggregate emissions. Excluding the two superemitters, study-average methane emissions from compressor housings and noncompressor sources are comparable to or lower than the corresponding effective emission factors used in the EPA greenhouse gas inventory. If the two superemitters are included in the analysis, then the average emission factors based on this study could exceed the EPA greenhouse gas inventory emission factors, which highlights the potentially important contribution of superemitters to national emissions. However, quantification of their influence requires knowledge of the magnitude and frequency of superemitters across the entire T&S sector. Only 38% of the methane emissions measured by the comprehensive onsite measurements were reportable under the new EPA GHGRP because of a combination of inaccurate emission factors for leakers and exhaust methane, and various exclusions. The bias is even larger if one accounts for the superemitters, which were not captured by the onsite measurements. The magnitude of the bias varied from site to site by site type and operating state. Therefore, while the GHGRP is a valuable new source of emissions information, care must be taken when incorporating these data into emission inventories. The value of the GHGRP can be increased by requiring more direct measurements of emissions (as opposed to using counts and emission factors), eliminating exclusions such as rod-packing vents on pressurized reciprocating compressors in standby mode under Subpart-W, and using more appropriate emission factors for exhaust methane from reciprocating engines under Subpart-C.
- Published
- 2015
- Full Text
- View/download PDF
35. Measurements of methane emissions from natural gas gathering facilities and processing plants: measurement results.
- Author
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Mitchell AL, Tkacik DS, Roscioli JR, Herndon SC, Yacovitch TI, Martinez DM, Vaughn TL, Williams LL, Sullivan MR, Floerchinger C, Omara M, Subramanian R, Zimmerle D, Marchese AJ, and Robinson AL
- Subjects
- United States, Air Pollutants analysis, Environmental Monitoring statistics & numerical data, Extraction and Processing Industry statistics & numerical data, Methane analysis, Natural Gas
- Abstract
Facility-level methane emissions were measured at 114 gathering facilities and 16 processing plants in the United States natural gas system. At gathering facilities, the measured methane emission rates ranged from 0.7 to 700 kg per hour (kg/h) (0.6 to 600 standard cubic feet per minute (scfm)). Normalized emissions (as a % of total methane throughput) were less than 1% for 85 gathering facilities and 19 had normalized emissions less than 0.1%. The range of methane emissions rates for processing plants was 3 to 600 kg/h (3 to 524 scfm), corresponding to normalized methane emissions rates <1% in all cases. The distributions of methane emissions, particularly for gathering facilities, are skewed. For example, 30% of gathering facilities contribute 80% of the total emissions. Normalized emissions rates are negatively correlated with facility throughput. The variation in methane emissions also appears driven by differences between inlet and outlet pressure, as well as venting and leaking equipment. Substantial venting from liquids storage tanks was observed at 20% of gathering facilities. Emissions rates at these facilities were, on average, around four times the rates observed at similar facilities without substantial venting.
- Published
- 2015
- Full Text
- View/download PDF
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