162 results on '"Transfer reaction"'
Search Results
2. Single-particle structure of ²⁹Mg on the approach to the N=20 island of inversion
- Author
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Macgregor, Patrick, Freeman, Sean, and Sharp, David
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transfer reaction ,spectroscopic factor ,solenoidal spectrometer ,single particle ,shell closure ,physics ,shell model ,magnesium ,nuclear ,HELIOS ,CERN ,ISOLDE ,island of inversion - Abstract
The nuclear structure of ²⁹Mg was probed using the d(²⁸Mg,p)²⁹Mg transfer reaction to populate its single-particle states. The ISOLDE facility at CERN provided a 9.473·A beam of ²⁸Mg which was directed at a deuterated target within the ISOLDE solenoidal spectrometer. Exploiting the kinematic advantages of this technique allowed most states up to 5 MeV to be resolved, and angular distributions of the reaction cross section to be obtained. The DWBA code DWUCK5 was used to obtain spectroscopic factors for these states. Additionally, some higher-lying excited states were identified, and their possible properties were proposed. Theoretical calculations in this region broadly reproduced the observed behaviour in ²⁹Mg, as well as matching trends from other nuclides in the N=17 isotones. These calculations indicate that the nucleon-nucleon interaction between protons and neutrons, with the tensor interaction as a key component, is driving the evolution of shell structure, with the filling of the πd5/2 orbital of particular importance in this region. Finite geometry effects also play an important role in this evolution as the p orbitals approach the neutron-separation threshold, and the energy spacing between them reduces. The information gained from the nuclear structure will help to continue refining these interactions, and provide a valuable benchmark for nuclear-structure studies around the border of the island of inversion. Similar experiments to study ³⁰Al and ³¹Mg carried out recently will help to further the understanding of nuclear structure in this exotic region of the nuclear chart.
- Published
- 2022
3. Use of Bayesian Optimization to understand the structure of nuclei
- Author
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Hooker, J, Kovoor, J, Jones, KL, Kanungo, R, Alcorta, M, Allen, J, Andreoiu, C, Atar, L, Bardayan, DW, Bhattacharjee, SS, Blankstein, D, Burbadge, C, Burcher, S, Catford, WN, Cha, S, Chae, K, Connolly, D, Davids, B, Esker, N, Garcia, FH, Gillespie, S, Ghimire, R, Gula, A, Hackman, G, Hallam, S, Hellmich, M, Henderson, J, Holl, M, Jassal, P, King, S, Knight, T, Kruecken, R, Lepailleur, A, Liang, J, Morrison, L, O’Malley, PD, Pain, SD, Pereira-Lopez, X, Psaltis, A, Radich, A, Shotter, AC, Vostinar, M, Williams, M, and Workman, O
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Affordable and Clean Energy ,Bayesian optimization ,Geant4 simulation ,Low-energy reactions ,Stable ion beam ,Radioactive ion beam ,Transfer reaction ,Direct reaction ,Atomic ,Molecular ,Nuclear ,Particle and Plasma Physics ,Geochemistry ,Interdisciplinary Engineering ,Applied Physics - Abstract
Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a 12Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the 12C(d,p) reaction to well-known states in 13C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for 13Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in 13C were extracted to better than 90 keV, paving a way for extracting information on 13Be.
- Published
- 2022
4. One-neutron stripping process in the 209Bi(6Li, 5Li)210Bi* reaction reaction
- Author
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Zhang, Gao-Long, Jiao, Zhen-Wei, Zhang, Guang-Xin, Cardozo, E. N., Paes, B., Hu, Shi-Peng, Qian, Jian-Qiang, Mengoni, Daniele, Qu, Wei-Wei, Li, Cong-Bo, Zheng, Yun, Zhang, Huan-Qiao, Sun, Hui-Bin, Wang, Nan, Zhang, Chun-Lei, Valiente-Dobón, J. J., Testov, D., Mazzocco, M., Gozzelino, A., Parascandolo, C., Pierroutsakou, D., La Commara, M., Goasduff, A., Bazzacco, D., Napoli, D. R., Galtarossa, F., Recchia, F., Illana, A., Bakes, S., Zanon, I., Aydin, S., de Angelis, G., Siciliano, M., Menegazzo, R., Lenzi, S. M., Akkoyun, S., Canto, L. F., and Lubian, J.
- Published
- 2024
- Full Text
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5. Transfer reaction measurements using SNACK at KoBRA.
- Author
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Kwag, M.S., Akers, C., Lee, K.B., Shin, T., and Tshoo, K.
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PROTON transfer reactions , *NUCLEAR astrophysics , *MONTE Carlo method , *ION beams , *LINEAR accelerators , *RADIOACTIVE nuclear beams - Abstract
KoBRA can produce RI beams with energies of 5–10 MeV/u from stable ion beams (10–40 MeV/u) delivered from the superconducting linear accelerator SLC3 of RAON. In its early phase of operation, transfer reaction measurements with these RI beams can be performed for nuclear astrophysics studies. SNACK has been developed at RISP in order to measure the light ejectiles from the transfer reactions. With the beam trajectories obtained from upstream PPACs, excitation energy levels in the heavy recoils can be reconstructed by measuring light ejectile's energies and scattering angles. The expected results of transfer reaction measurements with SNACK and KoBRA beamline detectors were calculated by using a Monte Carlo simulation. [ABSTRACT FROM AUTHOR]
- Published
- 2023
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6. Changes in proton occupancies pertaining to putative neutrinoless double beta decay in 130Te and 136Xe
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Entwisle, Jonathan and Freeman, Sean
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539.7 ,Transfer reaction ,Neutrinoless double beta decay - Abstract
A systematic study of the change in proton single-particle occupancies in two neutrinoless double beta decay candidates, 130Te to 130Xe and 136Xe to 136Ba, has been performed. Final states in 129Sb, 129I, 135I and 135Cs have been populated using the (d,3He) single proton removal reaction. The deuterons were accelerated to 101 MeV using the coupled azimuthally varying field and Ring cyclotrons at the Research Center for Nuclear Physics, University of Osaka. The outgoing ejectiles were momentum analysed using the Grand Raiden magnetic spectrometer. Absolute cross sections were measured for states up to 7 MeV in excitation. Transferred angular momenta were identified through a comparison of angular distributions with those calculated using the distorted-wave Born approximation. Spectroscopic factors were extracted from the experimental cross sections. In addition to the 0v2B decay candidates the reaction was also performed on 128Te, 132Xe, 134Xe and 138Ba as a consistency check. The occupancies of the nuclei were determined from the spectroscopic factors, the reaction model was normalised using a common normalisation factor across all targets. The change in occupancies between the 0v2B decay candidates and their daughters were then determined. The change in occupancies were then compared with those calculated by interacting shell model, interacting boson model and quasiparticle random phase approximation. This comparison showed that whilst the three theories were qualitatively able to reproduce the change in occupancies, quantitatively there are significant discrepancies. These are the same models that are used to determine the nuclear matrix elements governing the rate of 0v2B decay.
- Published
- 2017
7. Investigation of the role of 10Li resonances in the halo structure of 11Li through the 11Li(p,d)10Li transfer reaction
- Author
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Wang, Z. [TRIUMF, Vancouver, BC (Canada); Simon Fraser Univ., Burnaby, BC (Canada)]
- Published
- 2016
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8. Cluster emission in massive transfer reactions based on dinuclear system model
- Author
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XU Siyu and FENG Zhaoqing
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cluster emission ,pre-equilibrium process ,transfer reaction ,dinuclear system model ,Nuclear engineering. Atomic power ,TK9001-9401 - Abstract
BackgroundThe pre-equilibrium cluster manifests the nuclear structure and reaction dynamics of collision system. The systematical investigation of cluster emission in transfer reactions is of significance in deep understanding of the synthesis of superheavy nuclei, shell evolution, new isotope production, etc.PurposeThe dynamics of pre-equilibrium cluster in a few of nucleon transfer reaction has been described by theoretical model, such as exciton model, cluster model. However, the cluster emission in massive transfer is very complicated because of the emission mechanism associated with the structure properties and also the dynamical process.MethodsIn this work, the pre-equilibrium cluster emission in massive transfer reaction has been systematically investigated within the dinuclear system model. The model has been successfully used for describing the massive fusion reaction and multi-nucleon transfer dynamics. The nucleon exchange and energy dissipation take place once the dinuclear system is formed. The nucleon transfer between the binary fragments is governed by the single-particle Hamiltonian and proceeds around the Fermi surface formed by the dinuclear system. The master equation is used for the nucleon transfer dynamics and the relative motion energy dissipation is taken into account. The dynamics of neutron, proton, deuteron, triton, 3He, 4He, 6,7Li and 8,9Be in collisions of 12C+209Bi, 40Ca+208Pb and 48Ca+238U near Coulomb barrier energies is analyzed, i.e., temporal evolution of production rate, kinetic energy spectra and angular distribution.ResultsIt is found that the emission probability of 4He is the same magnitude of proton emission and several orders larger than the one of 3He. Both the nuclear structure and dynamical effects influence the pre-equilibrium cluster production.ConclusionsThe pre-equilibrium clusters are emitted from the 'projectile-like' and 'target-like' fragments and the angular distributions manifest the similar trends. The kinetic energy spectra of clusters are shown as the Boltzmann distribution. The method is also extended to the cluster emission in weakly bound nuclei induced reactions by considering the preformation factor for the cluster construction.
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- 2023
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9. Use of Bayesian Optimization to understand the structure of nuclei.
- Author
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Hooker, J., Kovoor, J., Jones, K.L., Kanungo, R., Alcorta, M., Allen, J., Andreoiu, C., Atar, L., Bardayan, D.W., Bhattacharjee, S.S., Blankstein, D., Burbadge, C., Burcher, S., Catford, W.N., Cha, S., Chae, K., Connolly, D., Davids, B., Esker, N., and Garcia, F.H.
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NUCLEAR physics , *NUCLEAR models , *MONTE Carlo method , *RADIOACTIVE nuclear beams , *ENERGY dissipation - Abstract
Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a 12Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the 12C(d,p) reaction to well-known states in 13C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for 13Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in 13C were extracted to better than 90 keV, paving a way for extracting information on 13Be. [ABSTRACT FROM AUTHOR]
- Published
- 2022
- Full Text
- View/download PDF
10. 24Mg(p, α)21Na reaction study for spectroscopy of 21Na
- Author
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Peters, W. [Oak Ridge Associated Univ., Oak Ridge, TN (United States)]
- Published
- 2015
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11. Evolution of the nuclear spin-orbit splitting explored via the 32Si(d,p)33Si reaction using SOLARIS.
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Chen, J., Kay, B.P., Hoffman, C.R., Tang, T.L., Tolstukhin, I.A., Bazin, D., Lubna, R.S., Ayyad, Y., Beceiro-Novo, S., Coombes, B.J., Freeman, S.J., Gaffney, L.P., Garg, R., Jayatissa, H., Kuchera, A.N., MacGregor, P., Mitchell, A.J., Mittig, W., Monteagudo, B., and Munoz-Ramos, A.
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NUCLEAR structure , *NEUTRONS , *MEAN field theory , *RADIOISOTOPES , *CYCLOTRONS , *KINEMATICS - Abstract
The spin-orbit splitting between neutron 1 p orbitals at 33Si has been deduced using the single-neutron-adding (d , p) reaction in inverse kinematics with a beam of 32Si, a long-lived radioisotope. Reaction products were analyzed by the newly implemented SOLARIS spectrometer at the reaccelerated-beam facility at the National Superconducting Cyclotron Laboratory. The measurements show reasonable agreement with shell-model calculations that incorporate modern cross-shell interactions, but they contradict the prediction of proton density depletion based on relativistic mean-field theory. The evolution of the neutron 1 p -shell orbitals is systematically studied using the present and existing data in the isotonic chains of N = 17 , 19, and 21. In each case, a smooth decrease in the separation of the 1 p 3 / 2 - 1 p 1 / 2 orbitals is seen as the respective p -orbitals approach zero binding, suggesting that the finite nuclear potential strongly influences the evolution of nuclear structure in this region. [ABSTRACT FROM AUTHOR]
- Published
- 2024
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12. Chemical effect on muonic atom formation through muon transfer reaction in benzene and cyclohexane samples.
- Author
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Inagaki, Makoto, Ninomiya, Kazuhiko, Nambu, Akihiro, Kudo, Takuto, Terada, Kentaro, Sato, Akira, Kawashima, Yoshitaka, Tomono, Dai, and Shinohara, Atsushi
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HYDROGEN atom ,CYCLOHEXANE ,MOLECULAR structure ,ATOMS ,MUONS ,PROTON transfer reactions - Abstract
To investigate the chemical effect on the muon capture process through a muon transfer reaction from a muonic hydrogen atom, the formation rate of muonic carbon atoms is measured for benzene and cyclohexane molecules in liquid samples. The muon transfer rate to carbon atoms of the benzene molecule is higher than that to the carbon atoms of the cyclohexane molecule. Such a deviation has never been observed among those molecules for gas samples. This may be because the transfers occur from the excited states of muonic hydrogen atoms in the liquid system, whereas in the gas system, all the transfers occur from the 1s (ground) state of muon hydrogen atoms. The muonic hydrogen atoms in the excited states have a larger radius than those in the 1s state and are therefore considered to be affected by the steric hindrance of the molecular structure. This indicates that the excited states of muonic hydrogen atoms contribute significantly to the chemical effects on the muon transfer reaction. [ABSTRACT FROM AUTHOR]
- Published
- 2021
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13. On the donor substrate dependence of group‐transfer reactions by hydrolytic enzymes: Insight from kinetic analysis of sucrose phosphorylase‐catalyzed transglycosylation.
- Author
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Klimacek, Mario, Sigg, Alexander, and Nidetzky, Bernd
- Abstract
Chemical group‐transfer reactions by hydrolytic enzymes have considerable importance in biocatalytic synthesis and are exploited broadly in commercial‐scale chemical production. Mechanistically, these reactions have in common the involvement of a covalent enzyme intermediate which is formed upon enzyme reaction with the donor substrate and is subsequently intercepted by a suitable acceptor. Here, we studied the glycosylation of glycerol from sucrose by sucrose phosphorylase (SucP) to clarify a peculiar, yet generally important characteristic of this reaction: partitioning between glycosylation of glycerol and hydrolysis depends on the type and the concentration of the donor substrate used (here: sucrose, α‐d‐glucose 1‐phosphate (G1P)). We develop a kinetic framework to analyze the effect and provide evidence that, when G1P is used as donor substrate, hydrolysis occurs not only from the β‐glucosyl‐enzyme intermediate (E‐Glc), but additionally from a noncovalent complex of E‐Glc and substrate which unlike E‐Glc is unreactive to glycerol. Depending on the relative rates of hydrolysis of free and substrate‐bound E‐Glc, inhibition (Leuconostoc mesenteroides SucP) or apparent activation (Bifidobacterium adolescentis SucP) is observed at high donor substrate concentration. At a G1P concentration that excludes the substrate‐bound E‐Glc, the transfer/hydrolysis ratio changes to a value consistent with reaction exclusively through E‐Glc, independent of the donor substrate used. Collectively, these results give explanation for a kinetic behavior of SucP not previously accounted for, provide essential basis for design and optimization of the synthetic reaction, and establish a theoretical framework for the analysis of kinetically analogous group‐transfer reactions by hydrolytic enzymes. [ABSTRACT FROM AUTHOR]
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- 2020
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14. Serum glutamine synthetase activity as biomarker for tuberculosis diagnosis and monitoring anti-tubercular drug therapy success.
- Author
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Chattopadhyay, Dipak Kumar
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GLUTAMINE synthetase , *BLOOD serum analysis , *BIOMARKERS , *ANTITUBERCULAR agents , *TUBERCULOSIS ,PUBLIC health in developing countries - Abstract
Tuberculosis is a major public health problem in developing countries. It is one of the most widely spread human diseases globally. While the new diagnostics for tuberculosis (TB) have created greater interest, their full impact on global propaganda against tuberculosis is yet to be evaluated. Most of the TB cases are prevalent in the underdeveloped and developing regions of the world where the means to diagnose and to treat TB cases are limited. As a result, the infectious TB cases might remain undiagnosed or diagnosed late. So, the need of the hour is to launch a rapid but simple, inexpensive, sensitive and specific test to diagnose TB cases at the earliest. The abundant presence of glutamine synthetase (GS) in the culture filtrate of pathogenic mycobacteria has correlation with the occurrence of poly L-glutamate/glutamine component in the cell wall of these pathogenic mycobacteria but not in non-pathogenic mycobacteria. The GS seems to be stable in the infected host and also is present in host tissues and fluid. GS is demonstrated to be present in the serum of subjects suffering from pulmonary or extra-pulmonary tuberculosis; but not detectable at all in normal control and disease control (lung disease control) subjects. With anti-tubercular (A-TB) drug therapy in pulmonary and extra-pulmonary tubercular subjects, the serum GS levels fall significantly. To confirm that only the Mycobacterium tuberculosis (M. tuberculosis) GS is being assayed, the serum GS activity may be assayed in the presence of L-methionine-S, R-sulfoximine (MSO), a selective inhibitor of M. tuberculosis GS. The concentration of this inhibitor is so selected that it is sufficient to inhibit mycobacterial GS activity but not the human (mammalian) GS activity. It increases the specificity of the test. Thus, an ELISA or latex agglutination test might be inducted to assay the serum GS activity for the rapid and reliable detection of active or latent tubercular subjects and also detecting the presence of drug sensitivity or the emergence of resistance against A-TB drugs. Nevertheless, for rapid field study, the card assay technique might be implemented; where when a drop of serum from a suspected subject be placed on the substrate for GS; a definite colour change would mark the test positive. The assay for serum GS requires only a sample of serum from the patient and takes only few minutes to perform. Therefore, the results will be available instantaneously when the patient is at the medical facility centre or even at home and this will curtail the number of visits to the medical facility centre. This is really advantageous in developing and underdeveloped countries where in many cases the patients do not have the capability of making multiple visits to the medical facility centre. The test procedure can also be used as an assay to monitor the response and success of antitubercular drug therapy. The procedure can very well indicate whether the treatment is successful or a change in the antibiotic drug therapy would be needed. [ABSTRACT FROM AUTHOR]
- Published
- 2019
15. Measurement and analysis of 10B+12C elastic scattering at energy of 41.3MeV.
- Author
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Burtebayev, N., Nassurlla, M., Sabidolda, A., Sakuta, S. B., Karakhodjaev, A. A., Ergashev, F. X., Rusek, K., Piasecki, E., Trzcińska, A., Wolińska-Cichocka, M., Kowalczyk, Michal, Mauyey, B., Janseitov, D., Zalewski, B., Hamada, Sh., Kemper, K. W., and Ibraheem, Awad A.
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ELASTIC analysis (Engineering) , *ELASTIC scattering - Abstract
Angular distribution of the 1 0 B + 1 2 C elastic scattering was measured at E lab ( 1 0 B) = 4 1. 3 MeV. Experimental data showed a significant increase in differential cross-sections at backward angles. The optical model with phenomenological potentials reproduces well the experimental cross-sections in the region of the angles of the forward hemisphere, but is not able to explain the increase in cross-sections at large angles. The distorted wave Born approximation method was used to reproduce the experimental data at large angles (> 9 0 ∘) by taking into consideration a deuteron transfer. Spectroscopic amplitude has been extracted for the configuration 1 2 C → 1 0 B + d from the analysis. [ABSTRACT FROM AUTHOR]
- Published
- 2019
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16. Investigation of spatial manifestation of α clusters in 16O via α-transfer reactions.
- Author
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Fukui, Tokuro, Kanada-En'yo, Yoshiko, Ogata, Kazuyuki, Suhara, Tadahiro, and Taniguchi, Yasutaka
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CLUSTER theory (Nuclear physics) , *EXCITED states , *GROUND state (Quantum mechanics) , *FIELD theory (Physics) , *MOLECULAR dynamics - Abstract
Abstract Recently, we have determined surface distributions of α clusters in the ground state of Ne 20 from α -transfer cross sections, without investigating the properties of its excited states. In this paper we extend our comprehension of α -cluster structures in excited states of nuclei through reaction studies. In particular we focus on O 16 , for which attention has been paid to advances of structure theory and assignment regarding 4 + -resonance states. We study the surface manifestation of the α -cluster states in both the ground and excited states of O 16 from the analysis of the α -transfer reaction C 12 (Li 6 , d) 16 O. The α -transfer reaction is described by the distorted-wave Born approximation. We test two microscopic wave functions as an input of reaction calculations. Then a phenomenological potential model is introduced to clarify the correspondence between cluster-wave functions and transfer-cross sections. Surface peaks of the α -wave function of O 16 (0 +) are sensitively probed by transfer-cross sections at forward angles, while it remains unclear how we trace the surface behavior of O 16 (4 +) from the cross sections. From inspection of the cross sections at forward angles, we are able to specify that the α -cluster structure in the 0 1 + and 0 2 + states prominently manifests itself at the radii ∼4 and ∼4.5 fm, respectively. It is remarkable that the 4 1 + state has the C 12 + α -cluster component with the surface peak at the radius ∼4 or outer, whereas the C 12 + α -cluster component in the 4 2 + state is found not to be dominant. The 4 2 + state is difficult to be interpreted by a simple potential model assuming the C 12 + α configuration only. [ABSTRACT FROM AUTHOR]
- Published
- 2019
- Full Text
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17. Development of an Operationally Simple, Scalable, and HCN-Free Transfer Hydrocyanation Protocol Using an Air-Stable Nickel Precatalyst
- Author
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Julia C. Reisenbauer, Benjamin N. Bhawal, Nicola Jelmini, and Bill Morandi
- Subjects
HCN-free ,Organic Chemistry ,transfer reaction ,nickel catalysis ,homogeneous catalysis ,hydrocyanation ,Physical and Theoretical Chemistry - Abstract
Hydrocyanation reactions enable access to synthetically valuable nitriles from readily available alkene precursors. However, hydrocyanation reactions using hydrogen cyanide (HCN) or similarly toxic reagents on laboratory scale can be particularly challenging due to their hazardous nature. In addition, such processes typically require air- and temperature-sensitive Ni(0) precatalysts, further reducing the operational simplicity of this transformation. Herein, we report a HCN-free transfer hydrocyanation of alkenes and alkynes that employs commercially available aliphatic nitriles as sacrificial HCN donors in combination with a catalytic amount of air-stable and inexpensive NiCl2as a precatalyst and a cocatalytic Lewis acid. The scalability and robustness of the catalytic process were demonstrated by the hydrocyanation of α-methylstyrene on a 100 mmol scale (11.4 g of product obtained) using 1 mol % of the Ni catalyst. In addition, the feasibility of the dehydrocyanation protocol using the air-stable Ni(II) precatalyst and norbornadiene as a sacrificial acceptor was showcased by the selective conversion of an aliphatic nitrile into the corresponding alkene., Organic Process Research & Development, 26 (4), ISSN:1083-6160, ISSN:1520-586X
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- 2022
- Full Text
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18. Transferhydrochlorierung von internen Alkinen mittels eines metallfrei aktivierbaren HCl-Surrogats
- Author
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Weidkamp, Andreas Josef
- Subjects
organische Synthese ,catalysis ,vinyl chlorides ,Vinylchloride ,Katalyse ,hydrochlorination ,Transferreaktion ,organic synthesis ,547 Organische Chemie ,transfer reaction ,Hydrochlorierung - Abstract
Die vorliegende Dissertation behandelt die Entwicklung eines metallfrei aktivierbaren Surrogats, das zur Transferhydrochlorierung von internen Alkinen befähigt ist. Dazu wurden in einem ersten Teilprojekt Versuche zur Darstellung von substituierten Cyclononatrienen durchgeführt, die durch eine photochemische Elektrocyclisierung aktiviert werden sollten. Ein lineares Vorläufermolekül sollte zunächst durch eine WITTIG-artige Reaktion eines Acylsilans mit einem Phosphorylid erhalten werden, dies gelang allerdings nicht. Als alternativer Ansatz sollte die Kupplung eines funktionalisierten Butadienylnukleophils mit einem Alkylelektrophil dienen, auch hier wurde aber kein Produkt erhalten. Aufgrund der besseren synthetischen Zugänglichkeit stellten wir ein vinylisch chloriertes Cyclohexadien dar. Dieses erwies sich als zu instabil, um es erfolgreich als Transferreagenz einzusetzen. In einem weiteren Teilprojekt strebten wir mehrfach chlorierte Bicyclo[3.1.0]hexan-artige Surrogate an, die zwar weiterhin metallfrei, aber nicht mehr photochemisch aktiviert werden sollten. Über Dichlorcarbenadditionen stellten wir dazu mehrere potenzielle Transfer-reagenzien dar. Neue Surrogate wurden stets in einer Modellreaktion mit der LEWIS-Säure B(C6F5)3 als Katalysator getestet. Auf Basis der Transfereffizienz wurde eine Hypothese zur Struktur-Reaktivitäts-Beziehung abgeleitet. Entsprechend dieser wurde das nächste potenzielle Surrogat entworfen. Dadurch gelang die Entwicklung eines Surrogats, das pro eingesetztem Molekül Reagenz zwei Moleküle Chlorwasserstoff überträgt. Nachdem wir die Struktur des Surrogats und die weiteren Parameter der Reaktion optimiert hatten, untersuchten wir deren Anwendungsbreite. Nur alkyl(aryl)substituierte Alkine waren einsetz-bar, wobei der elektronenspendende Effekt der Arylgruppe zusätzlich in einem gewissen Bereich liegen musste. Die Toleranz funktioneller Gruppen war eingeschränkt, jedoch wurden Ether, Ester und heteroaromatische Substituenten toleriert. Vorläufige Beobachtungen legen eine Rolle der LEWIS-Säure als Katalysator und ein Vinylkation als Zwischenstufe nahe. Ein davon unabhängiges Projekt widmete sich der erstmaligen Darstellung von am Boratom verbrückten Azoazaborininen. Diese sollten aus silylierten Diazenen und B-chlorierten Azaborininen unter Freisetzung von Chlortrimethylsilan dargestellt werden. Die erhaltenen komplexen Reaktionsgemische wurden hauptsächlich mittels 19F{1H} NMR-Spektroskopie von fluorierten Aryl(silyl)diazenen untersucht. Das von Benzol abgeleitete Stammsystem der Azaborinine reagierte unsauber, bei dem Naphthalinanalogon konnte die Anzahl der Reaktionsprodukte durch sterische Modifikation des Azaborinins verringert werden. Auch mit einer Erhöhung des sterischen Anspruchs am Silyldiazen wurde dennoch kein sauberes Produkt erhalten. Ein alkylsubstituiertes Silyldiazen reagierte zwar selektiv, zersetzte sich aber innerhalb von Stunden. Aufgrund der schnellen Freisetzung von Chlortrimethylsilan erscheint eine unerwünschte Reaktion der zunächst erfolgreich gebildeten Zielmoleküle möglich., The present thesis addresses the development of a metal-free activated surrogate used for the transfer hydrochlorination of internal alkynes. In a first sub-project, attempts to synthesize substituted cyclononatrienes, which were planned to be activated by photochemical electrocyclization, were made. To this end, a linear precursor molecule was intended to be obtained by a WITTIG-type reaction of an acylsilane with a phosphorus ylide, however, this failed. We alternatively then attempted to use a coupling of a functionalized butadienyl nucleophile with an alkyl electrophile, but again no product was obtained. Due to its better synthetic availability, we produced a vinylically chlorinated cyclohexadiene. This, however, was determined to be too unstable in order to successfully employ it as a transfer reagent. In another sub-project, we aimed at multichlorinated bicyclo[3.1.0]hexane-type surrogates, which still should be activated under metal-free conditions but not necessarily by photochemical means anymore. To this end, we synthesized several potential transfer reagents using dichlorocarbene addition. All new surrogates were tested in a model reaction using the LEWIS acid B(C6F5)3 as a catalyst. Based on the observed transfer efficiency, a hypothesis regarding the structure–reactivity relationship was put forward. The next potential surrogate was then designed accordingly. Thereby, we developed a surrogate, that transfers two molecules of hydrogen chloride per molecule of reagent. After having optimized the structure of the surrogate and the other reaction parameters, we investigated the substrate scope. It became apparent, that only aryl- and alkyl-substituted alkynes could be used. Additionally, the electron-donating effect of the aryl group had to lie within a certain range. The tolerance of functional groups was limited, but ethers, esters and heteroaromatic substituents were tolerated. Preliminary observations indicate the LEWIS acid acts as a catalyst and point to a vinyl cation as a reaction intermediate. In a project independent of the others, we pursued the first synthesis of azoazaborinines with the azo bridge connected to the boron atoms. These should be formed in the reaction of silylated diazenes and B-chlorinated azaborinines while liberating chlorotrimethylsilane. The obtained complex reaction mixtures were chiefly analyzed by 19F{1H} spectroscopy of fluorinated aryl silyl diazenes.¬ The benzene-derived azaborinine system reacted unselectively, but for the naphthalene-derived analogue the amount of reaction products could be reduced by steric modification of the azaborinines. However, even after increasing the steric hindrance at the silyl diazene, no pure product was obtained. An alkyl-substituted silyl diazene did react selectively yet decomposed within few hours. Due to the fast formation of chlorotrimethylsilane, it appears possible that the target compounds are initially produced but then decompose in an undesired way.
- Published
- 2023
- Full Text
- View/download PDF
19. Deuteron interaction with 124Sn nuclei at sub-barrier energies
- Author
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Yu.N. Pavlenko, V.P. Verbytskyi, O.I. Rundel, O.V. Babak, O.K. Gorpinich, V.V. Ostashko, Yu.Ya. Karlyshev, O.D. Grygorenko, A. Korzina, A.V. Stepaniuk, I. P. Dryapachenko, and E. M. Mozhzhukhin
- Subjects
deuteron ,124Sn nucleus ,sub-barrier energies ,deuteron elastic scattering ,deuteron breakup ,transfer reaction ,Atomic physics. Constitution and properties of matter ,QC170-197 - Abstract
The measurements of cross sections for deuteron elastic scattering and (d,p) reaction on 124Sn nuclei have been performed with aim to study the features of sub-barrier deuteron interaction with heavy nuclei. Experimental data were obtained on the electrostatic Tandem accelerator EGP-10K of the Institute for Nuclear Research (Kyiv) at the deuteron beam energies Ed = 4.0; 5.0 and 5.5 MeV. Cross sections of deuteron elastic scattering were calculated in approach where the deuteron interaction potential with heavy nuclei at sub-barrier energies has been constructed in the framework of single folding model using the complex dynamic polarization potential. It is shown that the account of finite deuteron size leads to the increasing the nuclear potential in outer region of interaction and significantly improves the description of the experimental data. The calculations of elastic scattering cross sections were performed without any variations of the nuclear potential parameters. The analysis of measured integral cross sections of the 124Sn(d,p) reaction and calculated cross sections of deuteron breakup reaction 124Sn(d,p)n124Sn shows the dominant contribution of the neutron transfer reaction in the processes of the formation of protons and elastic scattering cross sections.
- Published
- 2015
20. Shape coexistence and mixing of low-lying 0+ states in 96Sr.
- Author
-
Cruz, S., Bender, P.C., Krücken, R., Wimmer, K., Ames, F., Andreoiu, C., Austin, R.A.E., Bancroft, C.S., Braid, R., Bruhn, T., Catford, W.N., Cheeseman, A., Chester, A., Cross, D.S., Diget, C.Aa., Drake, T., Garnsworthy, A.B., Hackman, G., Kanungo, R., and Knapton, A.
- Subjects
- *
MIXING , *EXCITED state energies , *NEUTRONS , *DEFORMATIONS (Mechanics) , *NUCLEAR physics experiments - Abstract
Abstract The low energy excited 0 2 , 3 + states in 96Sr are amongst the most prominent examples of shape coexistence across the nuclear landscape. In this work, the neutron [ 2 s 1 / 2 ] 2 content of the 0 1 , 2 , 3 + states in 96Sr was determined by means of the d(95Sr, p) transfer reaction at the TRIUMF-ISAC2 facility using the SHARC and TIGRESS arrays. Spectroscopic factors of 0.19(3) and 0.22(3) were extracted for the 96Sr ground and 1229 keV 0 + states, respectively, by fitting the experimental angular distributions to DWBA reaction model calculations. A detailed analysis of the γ -decay of the isomeric 0 3 + state was used to determine a spectroscopic factor of 0.33(13). The experimental results are compared to shell model calculations, which predict negligible spectroscopic strength for the excited 0 + states in 96Sr. The strengths of the excited 0 2 , 3 + states were also analyzed within a two-level mixing model and are consistent with a mixing strength of a 2 = 0.40 (14) and a difference in intrinsic deformations of | Δ β | = 0.31 (3). These results suggest coexistence of three different configurations in 96Sr and strong shape mixing of the two excited 0 + states. [ABSTRACT FROM AUTHOR]
- Published
- 2018
- Full Text
- View/download PDF
21. A new measurement of the intruder configuration in 12Be.
- Author
-
Chen, J., Lou, J.L., Ye, Y.L., Li, Z.H., Pang, D.Y., Yuan, C.X., Ge, Y.C., Li, Q.T., Hua, H., Jiang, D.X., Yang, X.F., Xu, F.R., Pei, J.C., Li, J., Jiang, W., Sun, Y.L., Zang, H.L., Zhang, Y., Aoi, N., and Ideguchi, E.
- Subjects
- *
KINEMATICS , *DEUTERON reactions , *ELASTIC scattering , *ISOMERS , *PARTICLES - Abstract
A new 11 Be( d , p ) 12 Be transfer reaction experiment was carried out in inverse kinematics at 26.9 A MeV, with special efforts devoted to the determination of the deuteron target thickness and of the required optical potentials from the present elastic scattering data. In addition a direct measurement of the cross section for the 0 2 + state was realized by applying an isomer-tagging technique. The s -wave spectroscopic factors of 0.20 − 0.04 + 0.03 and 0.41 − 0.11 + 0.11 were extracted for the 0 1 + and 0 2 + states, respectively, in 12 Be. Using the ratio of these spectroscopic factors, together with the previously reported results for the p -wave components, the single-particle component intensities in the bound 0 + states of 12 Be were deduced, allowing a direct comparison with the theoretical predictions. It is evidenced that the ground-state configuration of 12 Be is dominated by the d -wave intruder, exhibiting a dramatic evolution of the intruding mechanism from 11 Be to 12 Be, with a persistence of the N = 8 magic number broken. [ABSTRACT FROM AUTHOR]
- Published
- 2018
- Full Text
- View/download PDF
22. Methylamine-glutamate N-methyltransferase
- Author
-
Schomburg, Dietmar, editor, Schomburg, Ida, editor, and Chang, Antje, editor
- Published
- 2006
- Full Text
- View/download PDF
23. Structure of 36Ca under the Coulomb magnifying glass
- Author
-
Lalanne, L., Poves Paredes, Alfredo, and UAM. Departamento de Física Teórica
- Subjects
Liquid Hydrogen Target ,Shell Models ,Energy ,Bubble Structures ,Detection System ,Transfer Reaction ,Física ,Mirror Energy Differences ,Detector Arrays ,Radioactive Nuclei ,Mirror Nuclei - Abstract
Artículo escrito por un elevado número de autores, solo se referencian el que aparece en primer lugar, el nombre del grupo de colaboración, si le hubiere, y los autores pertenecientes a la UAM, Detailed spectroscopy of the neutron-deficient nucleus Ca36 was obtained up to 9 MeV using the Ca37(p,d)Ca36 and the Ca38(p,t)Ca36 transfer reactions. The radioactive nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid hydrogen target CRYPTA, to produce light ejectiles (the deuteron d or triton t) that were detected in the MUST2 detector array, in coincidence with the heavy residues identified by a zero-degree detection system. Our main findings are (i) a similar shift in energy for the 11+ and 21+ states by about -250 keV, as compared with the mirror nucleus S36; (ii) the discovery of an intruder 02+ state at 2.83(13) MeV, which appears below the first 2+ state, in contradiction with the situation in S36; and (iii) a tentative 03+ state at 4.83(17) MeV, proposed to exhibit a bubble structure with two neutron vacancies in the 2s1/2 orbit. The inversion between the 02+ and 21+ states is due to the large mirror energy difference (MED) of -516(130) keV for the former. This feature is reproduced by shell model calculations, using the sd-pf valence space, predicting an almost pure intruder nature for the 02+ state, with two protons (neutrons) being excited across the Z=20 magic closure in Ca36 (S36). This mirror system has the largest MEDs ever observed, if one excludes the few cases induced by the effect of the continuum
- Published
- 2022
24. Proton Decay of 21Na for 20Ne Energy Levels
- Author
-
Kim, M. J., Chae, K. Y., Cha, S. M., Ahn, S. H., Bardayan, D. W., Chipps, K. A., Cizewski, J. A., Howard, M. E., Manning, B., Ratkiewicz, A., Kozub, R. L., Kwak, K., Matos, M., O’Malley, P. D., Strauss, S., Pain, S. D., Pittman, S. T., Smith, M. S., and Peters, W. A.
- Published
- 2020
- Full Text
- View/download PDF
25. First data with the Hybrid Array of Gamma Ray Detector (HAGRiD).
- Author
-
Smith, K., Baugher, T., Burcher, S., Carter, A.B., Cizewski, J.A., Chipps, K.A., Febbraro, M., Grzywacz, R., Jones, K.L., Munoz, S., Pain, S.D., Paulauskas, S.V., Ratkiewicz, A., Schmitt, K.T., Thornsberry, C., Toomey, R., Walter, D., and Willoughby, H.
- Subjects
- *
ASTROPHYSICS , *GAMMA ray detectors , *RADIOACTIVE decay , *SCINTILLATORS , *PARTICLE detectors - Abstract
The structure of nuclei provides insight into astrophysical reaction rates that are difficult to measure directly. These studies are often performed with transfer reactions and β-decay measurements. These experiments benefit from particle-γ coincidence measurements which provide information beyond that of particle detection alone. The Hybrid Array of Gamma Ray Detectors (HAGRiD) of LaBr 3 (Ce) scintillators has been designed with this purpose in mind. The design of the array permits it to be coupled with particle detector systems, such as the Oak Ridge Rutgers University Barrel Array (ORRUBA) of silicon detectors and the Versatile Array of Neutron Detectors at Low Energy (VANDLE). It is also designed to operate with the Jet Experiments in Nuclear Structure and Astrophysics (JENSA) advanced target system. HAGRiD’s design avoids compromising the charged-particle angular resolution due to compact geometries which are often used to increase the γ efficiency in other systems. First experiments with HAGRiD coupled to VANDLE as well as ORRUBA and JENSA are discussed. [ABSTRACT FROM AUTHOR]
- Published
- 2018
- Full Text
- View/download PDF
26. High-lying excited states in Be from the Be(Be,Be)Be reaction.
- Author
-
Jiang, Wei, Ye, YanLin, Li, ZhiHuan, Lin, ChengJian, Li, QiTe, Ge, YuCheng, Lou, JianLing, Jiang, DongXing, Li, Jing, Tian, ZhengYang, Feng, Jun, Yang, Biao, Yang, ZaiHong, Chen, Jie, Zang, HongLiang, Liu, Qiang, Li, PengJie, Chen, ZhiQiang, Zhang, Yun, and Liu, Yang
- Abstract
A transfer-reaction experiment of Be(Be, Be)Be was performed at a beam energy of 45 MeV. Excited states in Be up to 18.80 MeV are produced using missing mass and invariant mass methods. Most of the observed high-lying resonant states, reconstructed from the α + He and t + Li decay channels, agree with the previously reported results. In addition, two new resonances at 15.6 and 18.8 MeV are identified from the present measurement. The 18.55 MeV state is found to decay into both the t + Li. and t + Li* (0.478 MeV) channels, with a relative branching ratio of 0.93 ± 0.33. Further theoretical investigations are encouraged to interpret this new information on cluster structure in neutron-rich light nuclei. [ABSTRACT FROM AUTHOR]
- Published
- 2017
- Full Text
- View/download PDF
27. Phosphonate dehydrogenase
- Author
-
Schomburg, Dietmar, editor and Schomburg, Ida, editor
- Published
- 2006
- Full Text
- View/download PDF
28. Transfer And Disproportionation Reaction of the Cyclo-Dextrin Glucanotransferase From Klebsiella Pneumoniae
- Author
-
Flaschel, E., Andriamboavonjy, E. R., Renken, A., Szejtli, J., editor, and Szente, L., editor
- Published
- 1996
- Full Text
- View/download PDF
29. Use of Bayesian Optimization to Understand the Structure of Nuclei
- Author
-
J. Hooker, J. Kovoor, K.L. Jones, R. Kanungo, M. Alcorta, J. Allen, C. Andreoiu, L. Atar, D.W. Bardayan, S.S. Bhattacharjee, D. Blankstein, C. Burbadge, S. Burcher, W.N. Catford, S. Cha, K. Chae, D. Connolly, B. Davids, N. Esker, F.H. Garcia, S. Gillespie, R. Ghimire, A. Gula, G. Hackman, S. Hallam, M. Hellmich, J. Henderson, M. Holl, P. Jassal, S. King, T. Knight, R. Kruecken, A. Lepailleur, J. Liang, L. Morrison, P.D. O’Malley, S.D. Pain, X. Pereira-Lopez, A. Psaltis, A. Radich, A.C. Shotter, M. Vostinar, M. Williams, and O. Workman
- Subjects
Nuclear and High Energy Physics ,Direct reaction ,FOS: Physical sciences ,Transfer reaction ,01 natural sciences ,Atomic ,Stable ion beam ,Particle and Plasma Physics ,Affordable and Clean Energy ,0103 physical sciences ,Nuclear ,Nuclear Experiment (nucl-ex) ,010306 general physics ,Instrumentation ,Nuclear Experiment ,Bayesian optimization ,Applied Physics ,010308 nuclear & particles physics ,Low-energy reactions ,Geant4 simulation ,Molecular ,Computational Physics (physics.comp-ph) ,Geochemistry ,Interdisciplinary Engineering ,Radioactive ion beam ,Physics - Computational Physics - Abstract
Monte Carlo simulations are widely used in nuclear physics to model experimental systems. In cases where there are significant unknown quantities, such as energies of states, an iterative process of simulating and fitting is often required to describe experimental data. We describe a Bayesian approach to fitting experimental data, designed for data from a $^{12}$Be(d,p) reaction measurement, using simulations made with GEANT4. Q-values from the $^{12}$C(d,p) reaction to well-known states in $^{13}$C are compared with simulations using BayesOpt. The energies of the states were not included in the simulation to reproduce the situation for $^{13}$Be where the states are poorly known. Both cases had low statistics and significant resolution broadening owing to large proton energy losses in the solid deuterium target. Excitation energies of the lowest three excited states in $^{13}$C were extracted to better than 90 keV, paving a way for extracting information on $^{13}$Be., 8 pages, 6 figures
- Published
- 2021
30. Charge Transfer across Liquid—Liquid Interfaces
- Author
-
Girault, H. H., Bockris, J. O’M., editor, Conway, B. E., editor, and White, Ralph E., editor
- Published
- 1993
- Full Text
- View/download PDF
31. Using a double folding potential for the derivation of the spectroscopic factors of the (, ) transfer reaction.
- Author
-
Condori, R. Pampa, Dias, H., and Lubian, J.
- Subjects
- *
GROUND state (Quantum mechanics) , *PHASE transitions , *NUCLEAR reactions , *DWBA (Nuclear physics) , *WAVE functions , *ELASTIC scattering - Abstract
In this paper, the reactions are revisited, with the goal of obtaining spectroscopic factors (SF) for the transition to the ground state of some residual nuclei, applying the distorted wave Born approximation (DWBA). The double-folding São Paulo Potential (SPP) was used to derive the distorted wave function in the entrance and exit channels. The derived SF are compared with the results of extensive shell model calculations showing a rather good agreement. [ABSTRACT FROM AUTHOR]
- Published
- 2016
- Full Text
- View/download PDF
32. First test experiment to produce the slowed-down RI beam with the momentum-compression mode at RIBF.
- Author
-
Sumikama, T., Ahn, D.S., Fukuda, N., Inabe, N., Kubo, T., Shimizu, Y., Suzuki, H., Takeda, H., Aoi, N., Beaumel, D., Hasegawa, K., Ideguchi, E., Imai, N., Kobayashi, T., Matsushita, M., Michimasa, S., Otsu, H., Shimoura, S., and Teranishi, T.
- Subjects
- *
MOMENTUM (Mechanics) , *NUCLEAR fission , *NUCLEAR energy , *ION beams , *NUCLEAR reactors - Abstract
The 82 Ge beam has been produced by the in-flight fission reaction of the 238 U primary beam with 345 MeV/u at the RIKEN RI beam factory, and slowed down to about 15 MeV/u using the energy degraders. The momentum-compression mode was applied to the second stage of the BigRIPS separator to reduce the momentum spread. The energy was successfully reduced down to 13 ± 2.5 MeV/u as expected. The focus was not optimized at the end of the second stage, therefore the beam size was larger than the expectation. The transmission of the second stage was half of the simulated value mainly due to out of focus. The two-stage separation worked very well for the slowed-down beam with the momentum-compression mode. [ABSTRACT FROM AUTHOR]
- Published
- 2016
- Full Text
- View/download PDF
33. Investigation of the role of 10Li resonances in the halo structure of 11Li through the [formula omitted] transfer reaction.
- Author
-
Sanetullaev, A., Kanungo, R., Tanaka, J., Alcorta, M., Andreoiu, C., Bender, P., Chen, A.A., Christian, G., Davids, B., Fallis, J., Fortin, J.P., Galinski, N., Gallant, A.T., Garrett, P.E., Hackman, G., Hadinia, B., Ishimoto, S., Keefe, M., Krücken, R., and Lighthall, J.
- Subjects
- *
NUCLEAR reactions , *DELOCALIZATION energy , *GROUND state (Quantum mechanics) , *LITHIUM spectra , *ANGULAR distribution (Nuclear physics) - Abstract
The first measurement of the one-neutron transfer reaction 11 Li(p,d) 10 Li performed using the IRIS facility at TRIUMF with a 5.7 A MeV 11 Li beam interacting with a solid H 2 target is reported. The 10 Li residue was populated strongly as a resonance peak with energy E r = 0.62 ± 0.04 MeV having a total width Γ = 0.33 ± 0.07 MeV . The angular distribution of this resonance is characterized by neutron occupying the 1 p 1 / 2 orbital. A DWBA analysis yields a spectroscopic factor of 0.67 ± 0.12 for p 1 / 2 removal strength from the ground state of 11 Li to the region of the peak. [ABSTRACT FROM AUTHOR]
- Published
- 2016
- Full Text
- View/download PDF
34. SEARCHING FOR 2p DECAY OF THE FIRST EXCITED STATE OF Ne.
- Author
-
Golovkov, M. S., Sharov, P. G., Bezbakh, A. A., Rymzhanova, S. A., Chudoba, V., Fomichev, A. S., Gorshkov, A. V., Grigorenko, L. V., Kaminski, G., Knyazev, A. G., Krupko, S. A., Mentel, M., Oganessian, Yu. Ts., Parfenova, Yu. L., Pluchinski, P., Sidorchuk, S. I., Slepnev, R. S., Stepantsov, S. V., Ter-Akopian, G. M., and Wolski, R.
- Subjects
RADIOACTIVE nuclear beams ,PROTON decay ,GRAND unified theories (Nuclear physics) ,PARTICLE beams ,PION beams - Published
- 2015
35. Isobutyryl-CoA mutase
- Author
-
Schomburg, Dietmar, Stephan, Dörte, Schomburg, Dietmar, editor, and Stephan, Dörte, editor
- Published
- 1998
- Full Text
- View/download PDF
36. Baker–Venkataraman rearrangement
- Author
-
Li, Jie Jack and Li, Jie Jack
- Published
- 2014
- Full Text
- View/download PDF
37. Chemical effect on muonic atom formation through muon transfer reaction in benzene and cyclohexane samples
- Author
-
00898455, Inagaki, Makoto, Ninomiya, Kazuhiko, Nambu, Akihiro, Kudo, Takuto, Terada, Kentaro, Sato, Akira, Kawashima, Yoshitaka, Tomono, Dai, Shinohara, Atsushi, 00898455, Inagaki, Makoto, Ninomiya, Kazuhiko, Nambu, Akihiro, Kudo, Takuto, Terada, Kentaro, Sato, Akira, Kawashima, Yoshitaka, Tomono, Dai, and Shinohara, Atsushi
- Abstract
To investigate the chemical effect on the muon capture process through a muon transfer reaction from a muonic hydrogen atom, the formation rate of muonic carbon atoms is measured for benzene and cyclohexane molecules in liquid samples. The muon transfer rate to carbon atoms of the benzene molecule is higher than that to the carbon atoms of the cyclohexane molecule. Such a deviation has never been observed among those molecules for gas samples. This may be because the transfers occur from the excited states of muonic hydrogen atoms in the liquid system, whereas in the gas system, all the transfers occur from the 1s (ground) state of muon hydrogen atoms. The muonic hydrogen atoms in the excited states have a larger radius than those in the 1s state and are therefore considered to be affected by the steric hindrance of the molecular structure. This indicates that the excited states of muonic hydrogen atoms contribute significantly to the chemical effects on the muon transfer reaction.
- Published
- 2021
38. New determination of C()O reaction rate.
- Author
-
Oulebsir, N.
- Subjects
- *
CHEMICAL kinetics , *NUCLEAR astrophysics , *SUPERGIANT stars , *ELASTIC scattering , *DWBA (Nuclear physics) - Abstract
The reaction C()O was investigated through the direct -transfer reaction (7Li,t) at 28 and 34 MeV incident energies. We determined the reduced -widths of the sub-threshold 2 and 1 states of O from the DWBA analysis of the transfer reaction C(7Li,t)O performed at two incident energies. The obtained result for the 2 and 1 sub-threshold resonances as introduced in the -matrix fitting of radiative capture and elastic-scattering data to determine the E2 and E1 -factor from 0.01MeV to 4.2MeV in the center-of-mass energy. After determining the astrophysic factor of C()O S(E) with Pierre Descouvement code, I determined numerically the new reaction rate of this reaction at a different stellar temperature (0.06 Gk-2 GK). The C()O reaction rate at T is [7.21] × 10 cm3 s mol. Some comparisons and discussions about our new C()O reaction rate are presented. The agreements of the reaction rate below T between our results and with those proposed by NACRE indicate that our results are reliable, and they could be included in the astrophysical reaction rate network. [ABSTRACT FROM AUTHOR]
- Published
- 2015
- Full Text
- View/download PDF
39. DEUTERON INTERACTION WITH 124Sn NUCLEI AT SUB-BARRIER ENERGIES.
- Author
-
Pavlenko, Yu. N., Verbytskyi, V. P., Rundel, O. I., Babak, O. V., Gorpinich, O. K., Ostashko, V. V., Karlyshev, Yu. Ya., Grygorenko, O. D., Korzina, T. A., Stepaniuk, A. V., Dryapachenko, I. P., and Mozhzhukhin, E. M.
- Subjects
- *
DEUTERON reactions , *TIN isotopes , *NUCLEAR energy , *ELASTIC scattering , *DEUTERON scattering - Abstract
The measurements of cross sections for deuteron elastic scattering and (d, p) reaction on 124Sn nuclei have been performed with aim to study the features of sub-barrier deuteron interaction with heavy nuclei. Experimental data were obtained on the electrostatic Tandem accelerator EGP-10K of the Institute for Nuclear Research (Kyiv) at the deuteron beam energies Ed = 4.0; 5.0 and 5.5 MeV. Cross sections of deuteron elastic scattering were calculated in approach where the deuteron interaction potential with heavy nuclei at sub-barrier energies has been constructed in the framework of single folding model using the complex dynamic polarization potential. It is shown that the account of finite deuteron size leads to the increasing the nuclear potential in outer region of interaction and significantly improves the description of the experimental data. The calculations of elastic scattering cross sections were performed without any variations of the nuclear potential parameters. The analysis of measured integral cross sections of the 124Sn(d, p) reaction and calculated cross sections of deuteron breakup reaction 124Sn(d, p)n124Sn shows the dominant contribution of the neutron transfer reaction in the processes of the formation of protons and elastic scattering cross sections. [ABSTRACT FROM AUTHOR]
- Published
- 2015
- Full Text
- View/download PDF
40. NACRE II: AN UPDATE AND EXTENSION OF THE NACRE COMPILATION OF CHARGED-PARTICLE-INDUCED THERMONUCLEAR REACTION RATES FOR ASTROPHYSICS.
- Author
-
XU, Y., TAKAHASHI, K., GORIELY, S., and ARNOULD, M.
- Subjects
NUCLEAR astrophysics ,NUCLEAR reactions ,RADIATIVE capture ,NUCLEAR facilities ,THERMONUCLEAR fusion ,NUCLEAR cross sections - Published
- 2013
41. Study of 60Fe(n,γ)61Fe reaction of astrophysical interest via d(60Fe,pγ) indirect reaction.
- Author
-
Giron, S., Hammache, F., de Séréville, N., Beaumel, D., Burgunder, J., Caceres, L., Clement, E., Duchene, G., Flavigny, F., De France, G., Franchoo, S., Fernandez, B., Galaviz-Redondo, D., Gasques, L., Gibelin, J., Gillibert, A., Grevy, S., Guillot, J., Heil, M., and Kiener, J.
- Subjects
- *
SUPERNOVAE , *RADIOACTIVE decay , *NUCLEOSYNTHESIS , *ASTROPHYSICS , *NUCLEAR reactions - Abstract
INTEGRAL and RHESSI spacecrafts recently detected the 1.173 and 1.333 MeV γ-ray lines coming from the 60Fe—60Co—60Ni radioactive decay chain. The long lived isotope 60Fe (T1/2 = 1.5 106y) is believed to be primarily produced in core-collapse supernovae. However the interpretation of the observations is difficult because of the large uncertainties concerning 59Fe(n,γ)60Fe and 60Fe(n,γ)61Fe cross sections, involved in 60Fe nucleosynthesis. The direct component of the 60Fe(n,γ)61Fe reaction was studied indirectly via the d(60Fe,pγ)61Fe transfer reaction. The experiment performed in GANIL in spring 2009 will allow to determine the excitation energies of the populated excited states of 61Fe and for the first time their spectroscopic factors as well as their transfer angular momentum. I will first give an overview of the astrophysical context, then I will describe the experimental setup and finally present some preliminary results of the ongoing analysis. [ABSTRACT FROM AUTHOR]
- Published
- 2010
- Full Text
- View/download PDF
42. Transfer Reactions on Neutron-rich Nuclei at REX-ISOLDE.
- Author
-
Kröll, Th., Bildstein, V., Wimmer, K., Krücken, R., Gernhäuser, R., Lutter, R., Schwerdtfeger, W., Thirolf, P., Bastin, B., Bree, N., Diriken, J., Huyse, M., Patronis, N., Raabe, R., Van Duppen, P., Vermaelen, P., Cederkäll, J., Clément, E., Van de Walle, J., and Voulot, D.
- Subjects
- *
NUCLEAR reactions , *PARTICLES (Nuclear physics) , *ISOTOPES , *DETECTORS , *RADIOACTIVE nuclear beams - Abstract
We report on one- and two-neutron transfer reactions to study the single-particle properties of nuclei at the border of the “island of inversion.” The (d, p)- and (t, p)-reactions in inverse kinematics on the neutron-rich isotope 30Mg, delivered as radioactive beam by the REX-ISOLDE facility, have been investigated. The outgoing protons have been detected and identified by a newly built array of Si detectors. The γ-decay of excited states has been detected in coincidence by the MINIBALL array. First results for 31Mg and from the search for the second, spherical, 0+ state in 32Mg are presented. [ABSTRACT FROM AUTHOR]
- Published
- 2009
- Full Text
- View/download PDF
43. The Simultaneous Investigation of the 6He+12C Reaction Observables Using Folding Potential.
- Author
-
Karakoc, M., Kucuk, Y., and Boztosun, I.
- Subjects
- *
BORN approximation , *TRANSFER functions , *DATA , *SCATTERING (Physics) , *FUNCTIONAL analysis , *APPROXIMATION theory - Abstract
We investigate the observables of the 6He+12C system by using coupled-channels Born approximation. We try to address the role of the transfer channels in explaining the reaction observables. We noticed the inclusion of the transfer channels does not have large effect. However, we present that deformation of the imaginary potential has an important effect in explaining the elastic, inelastic and transfer reaction data simultaneously for this system. [ABSTRACT FROM AUTHOR]
- Published
- 2008
- Full Text
- View/download PDF
44. Elastic 3He-transfer Reaction of 6He on the 9Be Target at 25 MeV/nucleon.
- Author
-
Pang, D. Y., Ye, Y. L., Jiang, D. X., Zheng, T., Li, Z. H., Li, X. Q., Ge, Y. C., Wu, C. E., Hua, H., Zhang, G. L., Wang, J., Lou, J. L., Lu, F., Fan, F. Y., Ozawa, A., Yamaguchi, Y., Kanungo, R., Fang, D., and Tanihata, I.
- Subjects
- *
PARTICLES (Nuclear physics) , *NUCLEON-nucleon scattering , *SPECTRUM analysis , *NUCLEAR energy , *NUCLEAR physics - Abstract
Angular distribution of the cross sections of the elastic 3He-transfer of the 6He nucleus on the 9Be target were measured at the incident energy of 25 MeV/nucleon. The experimental data at the backward angles were analyzed within the finite-range DWBA framework. A large spectroscopic amplitude of 1.41 for the 3He-cluster in the ground state of the 9Be nucleus was needed for this experiment, which is much larger than its theoretical prediction of 0.286. © 2006 American Institute of Physics [ABSTRACT FROM AUTHOR]
- Published
- 2006
- Full Text
- View/download PDF
45. Indirect measurements of nuclear astrophysics reactions at CIAE.
- Author
-
Liu, Wei-ping, Li, Zhi-hong, Bai, Xi-xiang, Wang, You-bao, Lian, Gang, Guo, Bing, Zeng, Sheng, Yan, Sheng-quan, Wang, Bao-xiang, Su, Jun, Shu, Neng-chuan, and Chen, Yong-shou
- Subjects
- *
NUCLEAR astrophysics , *INDIRECT measures , *CHEMICAL kinetics , *ION bombardment , *NUCLEAR physics - Abstract
This paper described the nuclear astrophysical studies using the unstable ion beam facility GIRAFFE, by indirect measurements. We measured the angular distributions for some single proton or neutron transfer reactions, such as 7Be(d,n)8B, 11C(d,n)12N, 8Li(d,n)9Be, 8Li(d,p)9Li and 13N(d,n)14O in inverse kinematics, and derived the astrophysical S-factors or reaction rates of 7Be(p,γ)8B, 11C(p,γ)12N, 8Li(n,γ)9Li, 13N(p,γ)14O by asymptotic normalization coefficient, spectroscopic factor, and R-matrix approach at astrophysically relevant energies. © 2006 American Institute of Physics [ABSTRACT FROM AUTHOR]
- Published
- 2006
- Full Text
- View/download PDF
46. Optical Potentials of Exotic Nuclear Systems Extracted from Transfer Reactions.
- Author
-
Lin, C. J., Yang, F., Zhou, P., Zhang, H. Q., Liu, Z. H., Ruan, M., Wu, X. K., and Zhang, C. L.
- Subjects
- *
NUCLEAR reactions , *ELASTIC scattering , *COLLISIONS (Nuclear physics) , *NUCLEAR energy , *NUCLEAR physics - Abstract
An alternative method is proposed to extract the optical potentials of exotic nuclear systems in the outgoing channels by means of transfer reactions. An example of 208Pb(7Li, 6He)209Bi is demonstrated in details. Compared to the conventional method of which the optical potentials are directly extracted from the elastic scatterings, this indirect method has many benefits. © 2006 American Institute of Physics [ABSTRACT FROM AUTHOR]
- Published
- 2006
- Full Text
- View/download PDF
47. Determination of the astrophysical 8Li(n, γ)9Li reaction rate from the measurement of 2H(8Li,9 Li)1H reaction.
- Author
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Zhihong Li, Weiping Liu, Xixiang Bai, Bing Guo, Gang Lian, Shengquan Yan, Baoxiang Wang, Sheng Zeng, Yun Lu, Jun Su, Yongshou Chen, Kaisu Wu, Nengchuan Shu, and Kajino, Toshitaka
- Subjects
- *
STARS , *CHEMICAL kinetics , *ASTROPHYSICS , *NUCLEAR physics , *NUCLEAR reactions , *ELECTROMAGNETIC waves - Abstract
The cross section of the 8Li(n, γ)9Li reaction has attracted much attention for many years because of its importance in nuclear astrophysics. The single particle spectroscopic factor, S1,3/2 for the ground state of 9Li = 8Li x n derived from the transfer reaction of 8Li(d, p)9Li was used to calculate the direct radiative capture reaction rates of 8Li(n, γ)9Li at energies of astrophysical interest. The present result shows that the 8Li(n, γ)9Li direct capture reaction may play an important role in the astrophysical environments of inhomogeneous big bang and type II supernovae. © 2006 American Institute of Physics [ABSTRACT FROM AUTHOR]
- Published
- 2006
- Full Text
- View/download PDF
48. Shell Gap Reduction In Exotic N = 17 Nuclei.
- Author
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Obertelli, A., Alamanos, N., Alvarez, M., Auger, F., Dayras, R., Drouart, A., de France, G., Gillibert1, A., Jurado, B., Keeley, N., Lapoux, V., Mittig, W., Mougeot, X., Nalpas, L., Pakou, A., Patronis, N., Pollacco, E., Rejmund, F., Rejmund, M., and Roussel-Chomaz, P.
- Subjects
- *
PARTICLES (Nuclear physics) , *NUCLEAR physics , *NEUTRONS , *KINEMATICS , *PHYSICS - Abstract
27Ne has been investigated through the one neutron transfer reaction 26Ne(d,p)27Ne in inverse kinematics at 9.7 MeV/nucleon. The results support the existence of a low lying negative parity state in 27Ne which is a signature of a reduced sd-fp shell gap in the N=16 neutron rich region, at variance with stable nuclei. © 2006 American Institute of Physics [ABSTRACT FROM AUTHOR]
- Published
- 2006
- Full Text
- View/download PDF
49. Baker–Venkataraman rearrangement
- Author
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Li, Jie Jack and Li, Jie Jack
- Published
- 2009
- Full Text
- View/download PDF
50. Nucleon-Nucleon Pairing Correlations probed in the 118Sn+206Pb Transfer Reactions
- Author
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Diklić, Josipa, Szilner, Suzana, Corradi, L., Čolovic, Petra, Colucci, G., Fioretto, E., Galtarossa, F., Goasduff, A., Gottardo, A., Grebosz, J., Illana Sisón, A., Jaworski, G., Jurado Gomez, M., Marchi, T., Mijatović, Tea, Montagnoli, G., Nurkić, Deni, Pollarolo, G., Scarlassara, F., Siciliano, M., Soić, Neven, Stefanini, A.M., Testov, D., Utepov, A., Valiente-Dobón, J.J., and Vukman, Nikola
- Subjects
Physics ,nuclear reaction ,nucleon correlations ,Nuclear Theory ,Nuclear Experiment ,transfer reaction - Abstract
Two nucleon transfer reactions at low bombarding energies are an ideal tool to investigate nucleon-nucleon correlations. With heavy ions one has the possibility to transfer several nucleon pairs, involving both neutrons and protons at the same time. In this work we will study how pair correlations can be probed in heavy ion collisions , and how the strong Coulomb field influences the reaction dynamic.
- Published
- 2021
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