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We present a deterministic protocol for the preparation of arbitrary entangled states in the symmetric Dicke subspace of $N$ spins coupled to a common cavity mode. By combining a new geometric phase gate, an analytic solution of the noisy quantum channel dynamics and optimal control methods, the protocol prepares entangled states that are useful for quantum sensing, achieving a precision significantly better than the standard quantum limit in the presence of photon cavity loss, spontaneous emission and dephasing. This work opens the way to entanglement-enhanced sensing with cold trapped atoms in cavities and is also directly relevant for experiments with trapped ions.

We consider stabilizer measurements for surface codes with neutral atoms and identify gate protocols that minimize logical error rates in the presence of a fundamental error source -- spontaneous emission from Rydberg states. We demonstrate that logical error rates are minimized by protocols that prevent the propagation of Rydberg leakage errors and not by protocols that minimize the physical two-qubit error rate. We provide laser-pulse-level gate protocols to counter these errors. These protocols significantly reduce the logical error rate for implementations of surface codes involving one or two species of atoms. Our work demonstrates the importance of optimizing quantum gates for logical errors in addition to gate fidelities and opens the way to the efficient realization of surface codes with neutral atoms.

High-rate quantum error correcting (QEC) codes with moderate overheads in qubit number and control complexity are highly desirable for achieving fault-tolerant quantum computing. Recently, quantum error correction has experienced significant progress both in code development and experimental realizations, with neutral atom qubit architecture rapidly establishing itself as a leading platform in the field. Scalable quantum computing will require processing with QEC codes that have low qubit overhead and large error suppression, and while such codes do exist, they involve a degree of non-locality that has yet to be integrated into experimental platforms. In this work, we analyze a family of high-rate Low-Density Parity-Check (LDPC) codes with limited long-range interactions and outline a near-term implementation in neutral atom registers. By means of circuit-level simulations, we find that these codes outperform surface codes in all respects when the two-qubit nearest neighbour gate error probability is below $\sim 0.1\%$. We show how these codes can be natively integrated in two-dimensional static neutral atom qubit architectures with open boundaries, where the desired long-range connectivity can be targeted via Rydberg-blockade interaction. Our protocol solely requires multiple laser colors to enable transitions to different Rydberg states for different interatomic distances., Comment: 12 pages, 6 figures

Many-particle entanglement is a key resource for achieving the fundamental precision limits of a quantum sensor. Optical atomic clocks, the current state-of-the-art in frequency precision, are a rapidly emerging area of focus for entanglement-enhanced metrology. Augmenting tweezer-based clocks featuring microscopic control and detection with the high-fidelity entangling gates developed for atom-array information processing offers a promising route towards leveraging highly entangled quantum states for improved optical clocks. Here we develop and employ a family of multi-qubit Rydberg gates to generate Schr\"odinger cat states of the Greenberger-Horne-Zeilinger (GHZ) type with up to 9 optical clock qubits in a programmable atom array. In an atom-laser comparison at sufficiently short dark times, we demonstrate a fractional frequency instability below the standard quantum limit using GHZ states of up to 4 qubits. However, due to their reduced dynamic range, GHZ states of a single size fail to improve the achievable clock precision at the optimal dark time compared to unentangled atoms. Towards overcoming this hurdle, we simultaneously prepare a cascade of varying-size GHZ states to perform unambiguous phase estimation over an extended interval. These results demonstrate key building blocks for approaching Heisenberg-limited scaling of optical atomic clock precision., Comment: 22 pages, 7 figures, 2 tables, added additional Methods sections and gate error modeling

Standard cavity cooling of atoms or dielectric particles is based on the action of dispersive optical forces in high-finesse cavities. We investigate here a complementary regime characterized by large cavity losses, resembling the standard Doppler cooling technique. For a single two-level emitter a modification of the cooling rate is obtained from the Purcell enhancement of spontaneous emission in the large cooperativity limit. This mechanism is aimed at cooling of quantum emitters without closed transitions, which is the case for molecular systems, where the Purcell effect can mitigate the loss of population from the cooling cycle. We extend our analytical formulation to the many particle case governed by weak individual coupling but exhibiting collective strong Purcell enhancement to a cavity mode., Comment: 9+5 pages, 7 figures

The disorder-induced quantum phase transition between superfluid and non-superfluid states of bosonic particles in one dimension is generally expected to be of the Berezinskii-Kosterlitz-Thouless (BKT) type. Here, we show that hard-core lattice bosons with integrable power-law hopping decaying with distance as $1/r^\alpha$ - corresponding in spin language to a $XY$ model with power-law couplings - undergo a non-BKT continuous phase transition instead. We use exact quantum Monte-Carlo methods to determine the phase diagram for different values of the exponent $\alpha$, focusing on the regime $\alpha > 2$. We find that the scaling of the superfluid stiffness with the system size is scale-invariant at the transition point for any $\alpha\leq 3$ - a behavior incompatible with the BKT scenario and typical of continuous phase transitions in higher dimension. By scaling analysis near the transition point, we find that our data are consistent with a correlation length exponent satisfying the Harris bound $\nu \geq 2$ and demonstrate a new universal behavior of disordered bosons in one dimension. For $\alpha>3$ our data are consistent with a BKT scenario where the liquid is pinned by infinitesimal disorder.

The development of scalable, high-fidelity qubits is a key challenge in quantum information science. Neutral atom qubits have progressed rapidly in recent years, demonstrating programmable processors and quantum simulators with scaling to hundreds of atoms. Exploring new atomic species, such as alkaline earth atoms, or combining multiple species can provide new paths to improving coherence, control and scalability. For example, for eventual application in quantum error correction, it is advantageous to realize qubits with structured error models, such as biased Pauli errors or conversion of errors into detectable erasures. In this work, we demonstrate a new neutral atom qubit, using the nuclear spin of a long-lived metastable state in ${}^{171}$Yb. The long coherence time and fast excitation to the Rydberg state allow one- and two-qubit gates with fidelities of 0.9990(1) and 0.980(1), respectively. Importantly, a significant fraction of all gate errors result in decays out of the qubit subspace, to the ground state. By performing fast, mid-circuit detection of these errors, we convert them into erasure errors; during detection, the induced error probability on qubits remaining in the computational space is less than $10^{-5}$. This work establishes metastable ${}^{171}$Yb as a promising platform for realizing fault-tolerant quantum computing.

We present two protocols for implementing deterministic non-local multi-qubit quantum gates on qubits coupled to a common cavity mode. The protocols rely only on a classical drive of the cavity modes, while no external drive of the qubits is required. In the first protocol, the state of the cavity follows a closed trajectory in phase space and accumulates a geometric phase depending on the state of the qubits. The second protocol uses an adiabatic evolution of the combined qubit-cavity system to accumulate a dynamical phase. Repeated applications of this protocol allow for the realization of phase gates with arbitrary phases, e.g. phase-rotation gates and multi-controlled-Z gates. For both protocols, we provide analytic solutions for the error rates, which scale as $\sim N/\sqrt{C}$, with $C$ the cooperativity and $N$ the qubit number. Our protocols are applicable to a variety of systems and can be generalized by replacing the cavity by a different bosonic mode, such as a phononic mode. We provide estimates of gate fidelities and durations for atomic and molecular qubits coupled to optical or microwave cavities, and suggest applications for quantum error correction., Comment: v1: 7 pages + 7 pages supplementary information, 3 figures; v2: Updated references, minor edits; v3: 11 pages + 7 pages supplement, clarified and extended derivations

We analyze the spectral and transport properties of the interacting disordered Tavis-Cummings model at half excitation filling. We demonstrate that a Poissonian level statistics coexists with eigenfunctions that are multifractal (extended, but non-ergodic) in the Hilbert space, for all strengths of light-matter interactions. This is associated with a lack of thermalization for a local perturbation. We find that the bipartite entanglement entropy grows logarithmically with time, similarly to many-body localized systems, while the spin imbalance tends to zero for strong coupling, in analogy to ergodic phases. We show that these effects are due to the combination of finite interactions and integrability of the model. When a small integrability-breaking perturbation (nearest-neighbor hopping) is introduced, typical eigenfunctions become ergodic, seemingly turning the system into a near-perfect conductor, contrary to the single-excitation noninteracting case. We propose a realization of this model with cold atoms.

We analyze the propagation of excitons in a $d$-dimensional lattice with power-law hopping $\propto 1/r^\alpha$ in the presence of dephasing, described by a generalized Haken-Strobl-Reineker model. We show that in the strong dephasing (quantum Zeno) regime the dynamics is described by a classical master equation for an exclusion process with long jumps. In this limit, we analytically compute the spatial distribution, whose shape changes at a critical value of the decay exponent $\alpha_{\rm cr} = (d+2)/2$. The exciton always diffuses anomalously: a superdiffusive motion is associated to a L\'evy stable distribution with long-range algebraic tails for $\alpha\leq\alpha_{\rm cr}$, while for $\alpha > \alpha_{\rm cr}$ the distribution corresponds to a surprising mixed Gaussian profile with long-range algebraic tails, leading to the coexistence of short-range diffusion and long-range L\'evy-flights. In the many-exciton case, we demonstrate that, starting from a domain-wall exciton profile, algebraic tails appear in the distributions for any $\alpha$, which affects thermalization: the longer the hopping range, the faster equilibrium is reached. Our results are directly relevant to experiments with cold trapped ions, Rydberg atoms and supramolecular dye aggregates. They provide a way to realize an exclusion process with long jumps experimentally., Comment: 5 pages, 2 figures

Robust gate sequences are widely used to reduce the sensitivity of gate operations to experimental imperfections. Typically, the optimization minimizes the average gate error, however, recent work in quantum error correction has demonstrated that the performance of encoded logical qubits is sensitive to not only the average error rate, but also the type of errors that occur. Here, we present a family of Rydberg blockade gates for neutral atom qubits that are robust against two common, major imperfections: intensity inhomogeneity and Doppler shifts. These gates outperform existing gates for moderate or large imperfections. We also consider the logical performance of these gates in the context of an erasure-biased qubit based on metastable $~^{171}$Yb. In this case, we observe that the robust gates outperform existing gates for even very small values of the imperfections, because they maintain the native large bias towards erasure errors for these qubits. These results significantly reduce the laser stability and atomic temperature requirements to achieve fault-tolerant quantum computing with neutral atoms. The approach of optimizing gates for logical qubit performance may be applied to other qubit platforms., Comment: v3: Added discussion of AC-Stark shifts; v2: Updated references

All-to-all interacting, disordered quantum many-body models have a wide range of applications across disciplines, from spin glasses in condensed-matter physics, over holographic duality in high-energy physics, to annealing algorithms in quantum computing. Typically, these models are abstractions that do not find unambiguous physical realisations in nature. Here, we realise an all-to-all interacting, disordered spin system by subjecting an atomic cloud in a cavity to a controllable light shift. Adjusting the detuning between atom resonance and cavity mode, we can tune between disordered versions of a central-mode model and a Lipkin-Meshkov-Glick model. By spectroscopically probing the low-energy excitations of the system, we explore the competition of interactions with disorder across a broad parameter range. We show how disorder in the central-mode model breaks the strong collective coupling, making the dark state manifold cross over to a random distribution of weakly-mixed light-matter, "grey", states. In the Lipkin-Meshkov-Glick model the ferromagnetic finite-size ground state evolves towards a paramagnet as disorder is increased. In that regime, semi-localised eigenstates emerge, as we observe by extracting bounds on the participation ratio. These results present significant steps towards freely programmable cavity-mediated interactions for the design of arbitrary spin Hamiltonians., Comment: 8 pages, 4 figures, methods, supplementary material

We identify time-optimal laser pulses to implement the controlled-Z gate and its three qubit generalization, the C$_2$Z gate, for Rydberg atoms in the blockade regime. Pulses are optimized using a combination of numerical and semi-analytical quantum optimal control techniques that result in smooth Ans\"atze with just a few variational parameters. For the CZ gate, the time-optimal implementation corresponds to a global laser pulse that does not require single site addressability of the atoms, simplifying experimental implementation of the gate. We employ quantum optimal control techniques to mitigate errors arising due to the finite lifetime of Rydberg states and finite blockade strengths, while several other types of errors affecting the gates are directly mitigated by the short gate duration. For the considered error sources, we achieve theoretical gate fidelities compatible with error correction using reasonable experimental parameters for CZ and C$_2$Z gates., Comment: added link to data repository with pulses in csv format, minor changes

Collectively coupling molecular ensembles to a cavity has been demonstrated to modify chemical reactions akin to catalysis. Theoretically understanding this experimental finding remains to be an important challenge. In particular the role of quantum effects in such setups is an open question of fundamental and practical interest. Theoretical descriptions often neglect quantum entanglement between nuclear and electro-photonic degrees of freedom, e.g.~by computing Ehrenfest dynamics. Here we discover that disorder can strongly enhance the build-up of this entanglement on short timescales after incoherent photo-excitation. We find that this can have direct consequences for reaction coordinate dynamics. We analyze this phenomenon in a disordered Holstein-Tavis-Cummings model, a minimal toy model that includes all fundamental degrees of freedom. Using a numerical technique based on matrix product states we simulate the exact quantum dynamics of more than 100 molecules. Our results highlight the importance of beyond Born-Oppenheimer theories in polaritonic chemistry., Comment: 8 pages, 5 figures (+ 8 pages Appendix)

We provide an exact solution of large random arrowhead Hamiltonians with diagonal disorder, a minimal model for inhomogeneously broadened quantum emitters coupled to a cavity mode. We find that the distribution of energy spacing can be continuously tuned between Poisson statistics and a distribution that is very close to semi-Poisson statistics - the latter being usually associated to the critical point of "Anderson" localization-delocalization transitions. We demonstrate that all the eigenstates - including two polaritons and a continuum of dark states - are multifractal, which indicates the existence of a critical "semi-localized" phase for all values of the light-matter coupling strength, where dark states are localized over multiple, arbitrarily-distant sites. By computing the escape probability from an initial site, we find that the system has a peculiar diffusive-like behavior with an escape probability growing linearly with time for any finite coupling strength, and that the escape rate can be controlled by selecting the energy of the initial site. The escape rate averaged over the disorder configurations is found to exhibit a maximum for intermediate coupling strengths, before saturating at a lower value in the collective strong coupling limit - a "cavity protection" effect. Surprisingly, we show that the saturation value increases with the disorder, indicating that the cavity does not only protect transport against disorder but can also turn the latter into an ally improving transport. We finally investigate the system in a two-terminal configuration, and show that the steady-state excitation current exhibits similar features as the escape probability, thereby extending our cavity-protected transport scenario to out-of-equilibrium situations. We finally demonstrate that dark states can provide the major contribution to long-distance transport in disordered systems.

In the absence of frustration, interacting bosons in the ground state exist either in the superfluid or insulating phases. Superfluidity corresponds to frictionless flow of the matter field, and in optical conductivity is revealed through a distinct $\delta$-functional peak at zero frequency with the amplitude known as the Drude weight. This characteristic low-frequency feature is instead absent in insulating phases, defined by zero static optical conductivity. Here we demonstrate that bosonic particles in disordered one dimensional, $d=1$, systems can also exist in a conducting, non-superfluid, phase when their hopping is of the dipolar type, often viewed as short-ranged in $d=1$. This phase is characterized by finite static optical conductivity, followed by a broad anti-Drude peak at finite frequencies. Off-diagonal correlations are also unconventional: they feature an integrable algebraic decay for arbitrarily large values of disorder. These results do not fit the description of any known quantum phase and strongly suggest the existence of a novel conducting state of bosonic matter in the ground state., Comment: 8 pages, 6 figures

We study a simple model for photoinduced electron transfer reactions for the case of many donor-acceptor pairs that are collectively and homogeneously coupled to a photon mode of a cavity. We describe both coherent and dissipative collective effects resulting from this coupling within the framework of a quantum optics Lindblad master equation. We introduce a method to derive an effective rate equation for electron transfer, by adiabatically eliminating donor and acceptor states and the cavity mode. The resulting rate equation is valid both for weak and strong coupling to the cavity mode, and describes electronic transfer through both the cavity coupled bright states and the uncoupled dark states. We derive an analytic expression for the instantaneous electron transfer rate that depends non-trivially on the time-varying number of pairs in the ground state. We find that under proper resonance conditions, and in the presence of an incoherent drive, reaction rates can be enhanced by the cavity. This enhancement persists, and can even be largest, in the weak light-matter coupling regime. We discuss how the cavity effect is relevant for realistic experiments., Comment: 17 pages, 5 figures

We present a sufficient criterion for the emergence of cluster phases in an ensemble of interacting classical particles with repulsive two-body interactions. Through a zero-temperature analysis in the low density region we determine the relevant characteristics of the interaction potential that make the energy of a two-particle cluster-crystal become smaller than that of a simple triangular lattice in two dimensions. The method leads to a mathematical condition for the emergence of cluster crystals in terms of the sum of Fourier components of a regularized interaction potential, which can be in principle applied to any arbitrary shape of interactions. We apply the formalism to several examples of bounded and unbounded potentials with and without cluster-forming ability. In all cases, the emergence of self-assembled cluster crystals is well captured by the presented analytic criterion and verified with known results from molecular dynamics simulations at vanishingly temperatures. Our work generalises known results for bounded potentials to repulsive potentials of arbitrary shape., Comment: 9 pages, 5 figures

We study a disordered ensemble of quantum emitters collectively coupled to a lossless cavity mode. The latter is found to modify the localization properties of the "dark" eigenstates, which exhibit a character of being localized on multiple, noncontiguous sites. We denote such states as semi-localized and characterize them by means of standard localization measures. We show that those states can very efficiently contribute to coherent energy transport. Our paper underlines the important role of dark states in systems with strong light-matter coupling.

We propose a mechanism to realize high-yield molecular formation from ultracold atoms. Atom pairs are continuously excited by a laser, and a collective decay into the molecular ground state is induced by a coupling to a lossy cavity mode. Using a combination of analytical and numerical techniques, we demonstrate that the molecular yield can be improved by simply increasing the number of atoms, and can overcome efficiencies of state-of-the-art association schemes. We discuss realistic experimental setups for diatomic polar and nonpolar molecules, opening up collective light matter interactions as a tool for quantum state engineering, enhanced molecule formation, collective dynamics, and cavity mediated chemistry., Comment: 15 pages, 5 figures

We consider an ensemble of cavity-coupled two-level emitters interacting via full (coherent and dissipative) dipole-dipole interactions. Using an adiabatic elimination procedure we derive effective equations of motion for a subsystem consisting of the cavity and a single emitter. Those equations can be used for schemes to enhance the cavity-coupling of single emitters as shown in [S. Sch\"{u}tz, J. Schachenmayer, D. Hagenm\"{u}ller, G. K. Brennen, T. Volz, V. Sandoghdar, T. W. Ebbesen, C. Genes, and G. Pupillo, e-print arXiv:1904.08888]. We analyze limitations of effective subsystem parameters, and study how joint dissipative decay processes in the subsystem affect cavity-coupling properties of the single emitter and cavity transmission spectra., Comment: Accompanying manuscript of arXiv:1904.08888

Power-law interactions play a key role in a large variety of physical systems. In the presence of disorder, these systems may undergo many-body localization for a sufficiently large disorder. Within the many-body localized phase the system presents in time an algebraic growth of entanglement entropy, $S_{vN}(t)\propto t^{\gamma}$. Whereas the critical disorder for many-body localization depends on the system parameters, we find by extensive numerical calculations that the exponent $\gamma$ acquires a universal value $\gamma_c\simeq 0.33$ at the many-body localization transition, for different lattice models and decay powers. Moreover, our results suggest an intriguing relation between $\gamma_c$ and the critical minimal decay power of interactions necessary for the observation of many-body localization., Comment: 5 pages, 3 figures, plus Supplementary Material

Light-matter interactions have generated considerable interest as a means to manipulate material properties. Light-induced superconductivity has been demonstrated using pulsed lasers. An attractive alternative possibility is to exploit strong light-matter interactions arising by coupling phonons to the vacuum electromagnetic field of a cavity mode as has been suggested and theoretically studied. Here we explore this possibility for two very different superconductors, namely YBCO (YBa$_2$Cu$_3$O$_{6+x}$) and Rb$_3$C$_{60}$, coupled to surface plasmon polaritons, using a novel cooperative effect based on the presence of a strongly coupled vibrational environment allowing efficient dressing of the otherwise weakly coupled phonon bands of these compounds. By placing the superconductor-surface plasmon system in a SQUID magnetometer, we find that the superconducting transition temperatures ($T_{c}$) for both compounds are modified in the absence of any external laser field. For YBCO, $T_{c}$ decreases from 92 K to 86 K while for Rb$_3$C$_{60}$, it increases from 30 K to 45 K at normal pressures. In the latter case, a simple theoretical framework is provided to understand these results based on an enhancement of the electron-phonon coupling. This proof-of-principle study opens a new tool box to not only modify superconducting materials but also to understand the mechanistic details of different superconductors., Comment: 25 pages, 4 figures

An array of ultracold atoms in an optical lattice (Mott insulator) excited to a state where single electron wave-functions spatially overlap would represent a new and ideal platform to simulate exotic electronic many-body phenomena in the condensed phase. However, this highly excited non-equilibrium system is expected to be so short-lived that it has eluded observation so far. Here, we demonstrate the first step toward its realization by exciting high-lying electronic (Rydberg) states of the atomic Mott insulator with a coherent ultrashort laser pulse. Beyond a threshold principal quantum number where Rydberg orbitals of neighboring lattice sites overlap with each other, the atoms efficiently undergo spontaneous Penning ionization resulting in a drastic change of ion-counting statistics, sharp increase of avalanche ionization and the formation of an ultracold plasma. These observations signal the actual creation of exotic electronic states with overlapping wave functions, which is further confirmed by a significant difference in ionization dynamics between a Bose-Einstein condensate and a Mott insulator.

We investigate the $T=0$ phase diagram of a variant of the one-dimensional extended Hubbard model where particles interact via a finite-range soft-shoulder potential. Using Density Matrix Renormalization Group (DMRG) simulations, we evidence the appearance of Cluster Luttinger Liquid (CLL) phases, similarly to what first predicted in a hard-core bosonic chain [M. Mattioli, M. Dalmonte, W. Lechner, and G. Pupillo, Phys. Rev. Lett. 111, 165302]. As the interaction strength parameters change, we find different types of clusters, that encode the order of the ground state in a semi-classical approximation and give rise to different types of CLLs. Interestingly, we find that the conventional Tomonaga Luttinger Liquid (TLL) is separated by a critical line with a central charge $c=5/2$, along which the two (spin and charge) bosonic degrees of freedom (corresponding to $c=1$ each) combine in a supersymmetric way with an emergent fermionic excitation ($c=1/2$). We also demonstrate that there are no significant spin correlations., Comment: Submission to SciPost

We investigate the ground state properties of one-dimensional hard-core bosons interacting via a variable long-range potential using the density matrix renormalization group. We demonstrate that restoring energy extensivity in the system, which is done by rescaling the interaction potential with a suitable size-dependent factor known as Kac's prescription, has a profound influence on the low-energy properties in the thermodynamic limit. While an insulating phase is found in the absence of Kac's rescaling, the latter leads to a new metallic phase that does not fall into the conventional Luttinger liquid paradigm. Our results in one dimension illustrate the subtlety of determining the thermodynamic properties of generic long-range quantum systems.

Strong, long-range interactions present a unique challenge for the theoretical investigation of quantum many-body lattice models, due to the generation of large numbers of competing states at low energy. Here, we investigate a class of extended bosonic Hubbard models with off-site terms interpolating between short and infinite range, thus allowing for an exact numerical solution for all interaction strengths. We predict a novel type of stripe crystal at strong coupling. Most interestingly, for intermediate interaction strengths we demonstrate that the stripes can turn superfluid, thus leading to a self-assembled array of quasi-one-dimensional superfluids. These bosonic superstripes turn into an isotropic supersolid with decreasing the interaction strength. The mechanism for stripe formation is based on cluster self-assembling in the corresponding classical ground state, reminiscent of classical soft-matter models of polymers, different from recently proposed mechanisms for cold gases of alkali or dipolar magnetic atoms., Comment: 6+3 pages, 5+4 figures

We analyze the disorder driven localization of the two dimensional Bose-Hubbard model by evaluating the full low energy quasiparticle spectrum via a recently developed fluctuation operator expansion method. For any strength of the local interaction we find a mobility edge that displays an approximately exponential decay with increasing disorder strength. We determine the finite-size scaling collapse and exponents at this critical line finding that the localization of excitations is characterized by weak multi-fractality and a thermal-like critical gap ratio. A direct comparison to a recent experiment yields an excellent match of the predicted finite-size transition point and scaling of single particle correlations., Comment: 5+2 pages, 4 figures (added 12 pages Supplemental Material)

Quasicrystals remain among the most intriguing materials in physics and chemistry. Their structure results in many unusual properties including anomalously low friction as well as poor electrical and thermal conductivity but it also supports superconductivity, which shows that quantum effects in quasicrystals can be quite unique. Here we theoretically study superfluidity in a model quantum cluster quasicrystal. Using path-integral Monte Carlo simulations, we explore a 2D ensemble of bosons with the Lifshitz-Petrich-Gaussian pair potential, finding that moderate quantum fluctuations do not destroy the dodecagonal quasicrystalline order. This quasicrystal is characterized by a small yet finite superfluidity, demonstrating that particle clustering combined with the local cogwheel structure can underpin superfluidity even in the almost classical regime. This type of distributed superfluidity may also be expected in certain open crystalline lattices. Large quantum fluctuations are shown to induce transitions to cluster solids, supersolids and superfluids, which we characterize fully quantum-mechanically., Comment: 5 pages, 3 figures

We discuss a technique to strongly couple a single target quantum emitter to a cavity mode, which is enabled by virtual excitations of a nearby mesoscopic ensemble of emitters. A collective coupling of the latter to both the cavity and the target emitter induces strong photon non-linearities in addition to polariton formation, in contrast to common schemes for ensemble strong coupling. We demonstrate that strong coupling at the level of a single emitter can be engineered via coherent and dissipative dipolar interactions with the ensemble, and provide realistic parameters for a possible implementation with SiV$^{-}$ defects in diamond. Our scheme can find applications, amongst others, in quantum information processing or in the field of cavity-assisted quantum chemistry., Comment: 13 pages, 6 figures; substantially revised manuscript; see arXiv:1912.12703 for mathematical derivations

We investigate light-matter coupling in metallic crystals where plasmons coexist with phonons exhibiting large oscillator strength. We demonstrate theoretically that this coexistence can lead to strong light-matter interactions without external resonators. When the frequencies of plasmons and phonons are comparable, hybridization of these collective matter modes occurs in the crystal. We show that the coupling of these modes to photonic degrees of freedom gives rise to intrinsic surface plasmon-phonon polaritons, which offer the unique possibility to control the phonon properties by tuning the electron density and the crystal thickness. In particular, dressed phonons with reduced frequency and large wave vectors arise in the case of quasi-2D crystals, which leads to large enhancements of the electron-phonon scattering in the vibrational ultrastrong coupling regime. This suggests that photons can play a key role in determining the quantum properties of certain materials. A non-perturbative self-consistent Hamiltonian method is presented that is valid for arbitrarily large coupling strengths., Comment: 17 pages, 3 figures

We analyze the effects of disorder on the correlation functions of one-dimensional quantum models of fermions and spins with long-range interactions that decay with distance $\ell$ as a power-law $1/\ell^\alpha$. Using a combination of analytical and numerical results, we demonstrate that power-law interactions imply a long-distance algebraic decay of correlations within disordered-localized phases, for all exponents $\alpha$. The exponent of algebraic decay depends only on $\alpha$, and not, e.g., on the strength of disorder. We find a similar algebraic localization for wave-functions. These results are in contrast to expectations from short-range models and are of direct relevance for a variety of quantum mechanical systems in atomic, molecular and solid-state physics., Comment: 7+6 pages, 4+4 figures

We present a new type of phase-change behavior relevant for information storage applications, that can be observed in 2D systems with cluster-forming ability. The temperature-based control of the ordering in 2D particle systems depends on the existence of a crystal-to-glass transition. We perform molecular dynamics simulations of models with soft interactions, demonstrating that the crystalline and amorphous structures can be easily tuned by heat pulses. The physical mechanism responsible for this behavior is a self-assembled polydispersity, that depends on the cluster-forming ability of the interactions. Therefore, the range of real materials that can perform such a transition is very wide in nature, reading from colloidal suspensions to vortex matter. The state of the art in soft matter experimental setups, controlling interactions, polydispersity and dimensionality, makes it a very fertile ground for practical applications.

We study the interplay between charge transport and light-matter interactions in a confined geometry, by considering an open, mesoscopic chain of two-orbital systems resonantly coupled to a single bosonic mode close to its vacuum state. We introduce and benchmark different methods based on self-consistent solutions of non-equilibrium Green's functions and numerical simulations of the quantum master equation, and derive both analytical and numerical results. It is shown that in the dissipative regime where the cavity photon decay rate is the largest parameter, the light-matter coupling is responsible for a steady-state current enhancement scaling with the cooperativity parameter. We further identify different regimes of interest depending on the ratio between the cavity decay rate and the electronic bandwidth. Considering the situation where the lower band has a vanishing bandwidth, we show that for a high-finesse cavity, the properties of the resonant Bloch state in the upper band are transfered to the lower one, giving rise to a delocalized state along the chain. Conversely, in the dissipative regime with low cavity quality factors, we find that the current enhancement is due to a collective decay of populations from the upper to the lower band., Comment: 52 pages, 11 figures

We theoretically investigate charge transport through electronic bands of a mesoscopic one-dimensional system, where inter-band transitions are coupled to a confined cavity mode, initially prepared close to its vacuum. This coupling leads to light-matter hybridization where the dressed fermionic bands interact via absorption and emission of dressed cavity-photons. Using a self-consistent non-equilibrium Green's function method, we compute electronic transmissions and cavity photon spectra and demonstrate how light-matter coupling can lead to an enhancement of charge conductivity in the steady-state. We find that depending on cavity loss rate, electronic bandwidth, and coupling strength, the dynamics involves either an individual or a collective response of Bloch states, and explain how this affects the current enhancement. We show that the charge conductivity enhancement can reach orders of magnitudes under experimentally relevant conditions.

We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of two colliding ${^{87}}\mathrm{Rb}$ atoms, we demonstrate that the effective optical length and pole strength of this Rydberg optical Feshbach resonance can be tuned over several orders of magnitude, while incoherent processes and losses are minimised. Given the ubiquity of Rydberg molecular states, this technique should be generally applicable to homo-nuclear atomic pairs as well as to atomic mixtures with s-wave (or even p-wave) scattering., Comment: 8 pages, 5 figures. Accepted in Phys. Rev. A

We show that the entangled-plaquette variational ansatz can be adapted to study the two-dimensional $t-J$ model in the presence of two mobile holes. Specifically, we focus on a square lattice comprising up to $N=256$ sites in the parameter range $0.4\leq J/ t\leq2.0$. Ground state energies are obtained via the optimization of a wave function in which the weight of a given configuration is expressed in terms of variational coefficients associated with square and linear entangled plaquettes. Our estimates are in excellent agreement with exact results available for the $N=16$ lattice. By extending our study to considerably larger systems we find, based on the analysis of the long distance tail of the probability of finding two holes at spatial separation $r$, and on our computed two-hole binding energies, the existence of a two-hole bound state for all the values of $J/t$ explored here. It is estimated that d-wave binding of the two holes does not occur for $J/t

We study interactions between polaritons, arising when photons strongly couple to collective excitations in an array of two-level atoms trapped in an optical lattice inside a cavity. We consider two types of interactions between atoms: Dipolar forces and atomic saturability, which ranges from hard-core repulsion to Rydberg blockade. We show that, in spite of the underlying repulsion in the subsystem of atomic excitations, saturability induces a broadband bunching of photons for two-polariton scattering states. We interpret this bunching as a result of interference, and trace it back to the mismatch of the quantization volumes for atomic excitations and photons. We examine also bound bipolaritonic states: These include states created by dipolar forces, as well as a gap bipolariton, which forms solely due to saturability effects in the atomic transition. Both types of bound states exhibit strong bunching in the photonic component. We discuss the dependence of bunching on experimentally relevant parameters.

We investigate the out-of-equilibrium physics of monodisperse bosonic ensembles on a square lattice. The effective Hamiltonian description of these systems is given in terms of an extended Hubbard model with cluster-forming interactions relevant to experimental realizations with cold Rydberg-dressed atoms. The ground state of the model, recently investigated in Phys. Rev. Lett. 123, 045301 (2019), features, aside from a superfluid and a stripe crystalline phase occurring at small and large interaction strength $V$, respectively, a rare first-order transition between an isotropic and an anisotropic stripe supersolid at intermediate $V$. By means of quantum Monte Carlo calculations we show that the equilibrium crystal may be turned into a glass by simulated temperature quenches and that out-of-equilibrium isotropic (super)solid states may emerge also when their equilibrium counterparts are anisotropic. These out-of-equilibrium states are of experimental interest, their excess energy with respect to the ground state being within the energy window typically accessed in cold atom experiments. We find, after quenching, no evidence of coexistence between superfluid and glassy behavior. Such an absence of superglassiness is qualitatively explained., Comment: 8 pages, 6 figures

At low enough temperatures and high densities, the equilibrium configuration of an ensemble of ultrasoft particles is a self-assembled, ordered, cluster-crystal. In the present work we explore the out-of-equilibrium dynamics for a two-dimensional realization, which is relevant to superconducting materials with multi-scale intervortex forces. We find that for small temperatures following a quench, the suppression of the thermally-activated particle hopping hinders the ordering. This results in a glass transition for a monodispersed ensemble, for which we derive a microscopic explanation in terms of an "effective polydispersity" induced by multi-scale interactions. This demonstrates that a vortex glass can form in clean systems of thin films of "type-1.5" superconductors. An additional setup to study this physics can be layered superconducting systems, where the shape of the effective vortex-vortex interactions can be engineered.

We theoretically investigate the dynamics of a gas of strongly interacting Rydberg atoms subject to a time-domain Ramsey interferometry protocol. The many-body dynamics is governed by an Ising-type Hamiltonian with long range interactions of tunable strength. We analyze and model the contrast degradation and phase accumulation of the Ramsey signal and identify scaling laws for varying interrogation times, ensemble densities, and ensemble dimensionalities., Comment: 16 pages, 3 figures

We demonstrate theoretically that photon-photon attraction can be engineered in the continuum of scattering states for pairs of photons propagating in a hollow-core photonic crystal fiber filled with cold atoms. The atoms are regularly spaced in an optical lattice configuration and the photons are resonantly tuned to an internal atomic transition. We show that the hard-core repulsion resulting from saturation of the atomic transitions induces bunching in the photonic component of the collective atom-photon modes (polaritons). Bunching is obtained in a frequency range as large as tens of GHz, and can be controlled by the inter-atomic separation. We provide a fully analytical explanation for this phenomenon by proving that correlations result from a mismatch of the quantization volumes for atomic excitations and photons in the continuum. Even stronger correlations can be observed for in-gap two-polariton bound states. Our theoretical results use parameters relevant for current experiments with Rb atoms excited on the D2-line., Comment: 9 pages, 3 figures

We deal with the problem of studying the effective theories and the symmetries of long-range models around critical points. We focus in particular on the Kitaev chain with long-range pairings decaying with distance as power-law with exponent $\alpha$. This is a quadratic solvable model, yet displaying non-trivial quantum phase transitions. By renormalization group approach we derive first the effective theory close to the critical line at positive chemical potential. This is the sum of two terms: a Dirac action $S_D$, found in the short-range Ising universality class, and a CS breaking term $S_{AN}$. While $S_D$ originates from low-energy excitations, $S_{AN}$ derives from the higher energy modes where singularities develop, due to the long-range nature of the model. At criticality $S_{AN}$ flows to zero if $\alpha > 2$, while if $\alpha < 2$ it dominates and determines the breakdown of the CS. Out of criticality $S_{AN}$ breaks, in the considered approximation, the effective Lorentz invariance (ELI) for every finite $\alpha$. As $\alpha$ increases, such ELI breakdown becomes less and less pronounced and in the short-range limit $\alpha \to \infty$ the ELI is restored. To test the validity of the effective theory, we compared the two-fermion static correlations and the von Neumann entropy obtained from them with the ones calculated on the lattice, finding agreement. From the effective theory one can also see that new phases emerge for $\alpha < 1$. Finally we show that at every finite $\alpha$ the critical exponents are the same as for the short-range ($\alpha \to \infty$) model. At variance, for the critical line with negative chemical potential, only $S_{AN}$ ($S_D$) is present for $1 < \alpha < 2$ (for $\alpha > 2$). Close to this line, where the minimum of the spectrum coincides with the momentum where singularities develop, the critical exponents change exactly where CS is broken., Comment: 18+9 pages, 3+3 figures, accepted Ann. Phys

We analyze the quantum phases, correlation functions and edge modes for a class of spin-1/2 and fermionic models related to the 1D Ising chain in the presence of a transverse field. These models are the Ising chain with anti-ferromagnetic long-range interactions that decay with distance $r$ as $1/r^\alpha$, as well as a related class of fermionic Hamiltonians that generalise the Kitaev chain, where both the hopping and pairing terms are long-range and their relative strength can be varied. For these models, we provide the phase diagram for all exponents $\alpha$, based on an analysis of the entanglement entropy, the decay of correlation functions, and the edge modes in the case of open chains. We demonstrate that violations of the area law can occur for $\alpha \lesssim1$, while connected correlation functions can decay with a hybrid exponential and power-law behaviour, with a power that is $\alpha$-dependent. Interestingly, for the fermionic models we provide an exact analytical derivation for the decay of the correlation functions at every $\alpha$. Along the critical lines, for all models breaking of conformal symmetry is argued at low enough $\alpha$. For the fermionic models we show that the edge modes, massless for $\alpha \gtrsim 1$, can acquire a mass for $\alpha < 1$. The mass of these modes can be tuned by varying the relative strength of the kinetic and pairing terms in the Hamiltonian. Interestingly, for the Ising chain a similar edge localization appears for the first and second excited states on the paramagnetic side of the phase diagram, where edge modes are not expected. We argue that, at least for the fermionic chains, these massive states correspond to the appearance of new phases, notably approached via quantum phase transitions without mass gap closure. Finally, we discuss the possibility to detect some of these effects in experiments with cold trapped ions., Comment: 15 pages, 8 figures

Many-body correlations govern a variety of important quantum phenomena such as the emergence of superconductivity and magnetism. Understanding quantum many-body systems is thus one of the central goals of modern sciences. Here we demonstrate an experimental approach towards this goal by utilizing an ultracold Rydberg gas generated with a broadband picosecond laser pulse. We follow the ultrafast evolution of its electronic coherence by time-domain Ramsey interferometry with attosecond precision. The observed electronic coherence shows an ultrafast oscillation with a period of 1 femtosecond, whose phase shift on the attosecond timescale is consistent with many-body correlations among Rydberg atoms beyond mean-field approximations. This coherent and ultrafast many-body dynamics is actively controlled by tuning the orbital size and population of the Rydberg state, as well as the mean atomic distance. Our approach will offer a versatile platform to observe and manipulate non-equilibrium dynamics of quantum many-body systems on the ultrafast timescale.

We investigate the quantum phases of monodispersed bosonic gases confined to a triangular lattice and interacting via a class of soft-shoulder potentials. The latter correspond to soft-core potentials with an additional hard-core onsite interaction. Using exact quantum Monte Carlo simulations, we show that the low temperature phases for weak and strong interactions following a temperature quench are a homogeneous superfluid and a glass, respectively. The latter is an insulating phase characterized by inhomogeneity in the density distribution and structural disorder. Remarkably, we find that for intermediate interaction strengths a {\it superglass} occurs in an extended region of the phase diagram, where glassy behavior coexists with a sizable finite superfluid fraction. This glass phase is obtained in the absence of geometrical frustration or external disorder and is a result of the competition of quantum fluctuations and cluster formation in the corresponding classical ground state. For high enough temperature, the glass and superglass turn into a floating stripe solid and a supersolid, respectively. Given the simplicity and generality of the model, these phases should be directly relevant for state-of-the-art experiments with Rydberg-dressed atoms in optical lattices., Comment: 5.5+3.5 pages, 4+4 figures