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1. THE GLOBAL AEROSOL SYNTHESIS AND SCIENCE PROJECT (GASSP): Measurements and Modeling to Reduce Uncertainty: Novel methodologies for quantifying model uncertainty are combined with an extensive new database of in situ aerosol microphysical and chemical measurements to reduce uncertainty in aerosol effects on climate

Author: Reddington, C.L., Carslaw, K.S., Stier, P., Schutgens, N., Coe, H., Liu, D., Allan, J., Browse, J., Pringle, K.J., Lee, L.A., Yoshioka, M., Johnson, J.S., Regayre, L.A., Spracklen, D.V., Mann, G.W., Clarke, A., Hermann, M., Henning, S., Wex, H., Kristensen, T.B., Leaitch, W.R., Poschl, U., Rose, D., Andreae, M.O., Schmale, J., Kondo, Y., Oshima, N., Schwarz, J.P., Nenes, A., Anderson, B., Roberts, G.C., Snider, J.R., Leck, C., Quinn, P.K., Chi, X., Ding, A., Jimenez, J.L., and Zhang, Q.
Subjects: United States. National Aeronautics and Space Administration -- Analysis, Online databases -- Methods -- Analysis, Climate models -- Methods -- Analysis, Online database, Business, Earth sciences
Abstract: The largest uncertainty in the historical radiative forcing of climate is caused by changes in aerosol particles due to anthropogenic activity. Sophisticated aerosol microphysics processes have been included in many [...]
Published: 2017
Full Text: View/download PDF

2. EUREC4A

Author: Stevens, B, Bony, S, Farrell, D, Ament, F, Blyth, A, Fairall, C, Karstensen, J, Quinn, P, Speich, S, Acquistapace, C, Aemisegger, F, Albright, A, Bellenger, H, Bodenschatz, E, Caesar, K, Chewitt-Lucas, R, De Boer, G, Delanoe, J, Denby, L, Ewald, F, Fildier, B, Forde, M, George, G, Gross, S, Hagen, M, Hausold, A, Heywood, K, Hirsch, L, Jacob, M, Jansen, F, Kinne, S, Klocke, D, Kolling, T, Konow, H, Lothon, M, Mohr, W, Naumann, A, Nuijens, L, Olivier, L, Pincus, R, Pohlker, M, Reverdin, G, Roberts, G, Schnitt, S, Schulz, H, Pier Siebesma, A, Stephan, C, Sullivan, P, Touze-Peiffer, L, Vial, J, Vogel, R, Zuidema, P, Alexander, N, Alves, L, Arixi, S, Asmath, H, Bagheri, G, Baier, K, Bailey, A, Baranowski, D, Baron, A, Barrau, S, Barrett, P, Batier, F, Behrendt, A, Bendinger, A, Beucher, F, Bigorre, S, Blades, E, Blossey, P, Bock, O, Boing, S, Bosser, P, Bourras, D, Bouruet-Aubertot, P, Bower, K, Branellec, P, Branger, H, Brennek, M, Brewer, A, Brilouet, P, Brugmann, B, Buehler, S, Burke, E, Burton, R, Calmer, R, Canonici, J, Carton, X, Cato, G, Charles, J, Chazette, P, Chen, Y, Chilinski, M, Choularton, T, Chuang, P, Clarke, S, Coe, H, Cornet, C, Coutris, P, Couvreux, F, Crewell, S, Cronin, T, Cui, Z, Cuypers, Y, Daley, A, Damerell, G, Dauhut, T, Deneke, H, Desbios, J, Dorner, S, Donner, S, Douet, V, Drushka, K, Dutsch, M, Ehrlich, A, Emanuel, K, Emmanouilidis, A, Etienne, J, Etienne-Leblanc, S, Faure, G, Feingold, G, Ferrero, L, Fix, A, Flamant, C, Flatau, P, Foltz, G, Forster, L, Furtuna, I, Gadian, A, Galewsky, J, Gallagher, M, Gallimore, P, Gaston, C, Gentemann, C, Geyskens, N, Giez, A, Gollop, J, Gouirand, I, Gourbeyre, C, De Graaf, D, De Groot, G, Grosz, R, Guttler, J, Gutleben, M, Hall, K, Harris, G, Helfer, K, Henze, D, Herbert, C, Holanda, B, Ibanez-Landeta, A, Intrieri, J, Iyer, S, Julien, F, Kalesse, H, Kazil, J, Kellman, A, Kidane, A, Kirchner, U, Klingebiel, M, Korner, M, Kremper, L, Kretzschmar, J, Kruger, O, Kumala, W, Kurz, A, L'Hegaret, P, Labaste, M, Lachlan-Cope, T, Laing, A, Landschutzer, P, Lang, T, Lange, D, Lange, I, Laplace, C, Lavik, G, Laxenaire, R, Lebihan, C, Leandro, M, Lefevre, N, Lena, M, Lenschow, D, Li, Q, Lloyd, G, Los, S, Losi, N, Lovell, O, Luneau, C, Makuch, P, Malinowski, S, Manta, G, Marinou, E, Marsden, N, Masson, S, Maury, N, Mayer, B, Mayers-Als, M, Mazel, C, Mcgeary, W, Mcwilliams, J, Mech, M, Mehlmann, M, Meroni, A, Mieslinger, T, Minikin, A, Minnett, P, Moller, G, Avalos, Y, Muller, C, Musat, I, Napoli, A, Neuberger, A, Noisel, C, Noone, D, Nordsiek, F, Nowak, J, Oswald, L, Parker, D, Peck, C, Person, R, Philippi, M, Plueddemann, A, Pohlker, C, Portge, V, Poschl, U, Pologne, L, Posyniak, M, Prange, M, Melendez, E, Radtke, J, Ramage, K, Reimann, J, Renault, L, Reus, K, Reyes, A, Ribbe, J, Ringel, M, Ritschel, M, Rocha, C, Rochetin, N, Rottenbacher, J, Rollo, C, Royer, H, Sadoulet, P, Saffin, L, Sandiford, S, Sandu, I, Schafer, M, Schemann, V, Schirmacher, I, Schlenczek, O, Schmidt, J, Schroder, M, Schwarzenboeck, A, Sealy, A, Senff, C, Serikov, I, Shohan, S, Siddle, E, Smirnov, A, Spath, F, Spooner, B, Katharina Stolla, M, Szkolka, W, De Szoeke, S, Tarot, S, Tetoni, E, Thompson, E, Thomson, J, Tomassini, L, Totems, J, Ubele, A, Villiger, L, Von Arx, J, Wagner, T, Walther, A, Webber, B, Wendisch, M, Whitehall, S, Wiltshire, A, Wing, A, Wirth, M, Wiskandt, J, Wolf, K, Worbes, L, Wright, E, Wulfmeyer, V, Young, S, Zhang, C, Zhang, D, Ziemen, F, Zinner, T, Zoger, M, Stevens B., Bony S., Farrell D., Ament F., Blyth A., Fairall C., Karstensen J., Quinn P. K., Speich S., Acquistapace C., Aemisegger F., Albright A. L., Bellenger H., Bodenschatz E., Caesar K. -A., Chewitt-Lucas R., De Boer G., Delanoe J., Denby L., Ewald F., Fildier B., Forde M., George G., Gross S., Hagen M., Hausold A., Heywood K. J., Hirsch L., Jacob M., Jansen F., Kinne S., Klocke D., Kolling T., Konow H., Lothon M., Mohr W., Naumann A. K., Nuijens L., Olivier L., Pincus R., Pohlker M., Reverdin G., Roberts G., Schnitt S., Schulz H., Pier Siebesma A., Stephan C. C., Sullivan P., Touze-Peiffer L., Vial J., Vogel R., Zuidema P., Alexander N., Alves L., Arixi S., Asmath H., Bagheri G., Baier K., Bailey A., Baranowski D., Baron A., Barrau S., Barrett P. A., Batier F., Behrendt A., Bendinger A., Beucher F., Bigorre S., Blades E., Blossey P., Bock O., Boing S., Bosser P., Bourras D., Bouruet-Aubertot P., Bower K., Branellec P., Branger H., Brennek M., Brewer A., Brilouet P. -E., Brugmann B., Buehler S. A., Burke E., Burton R., Calmer R., Canonici J. -C., Carton X., Cato G., Charles J. A., Chazette P., Chen Y., Chilinski M. T., Choularton T., Chuang P., Clarke S., Coe H., Cornet C., Coutris P., Couvreux F., Crewell S., Cronin T., Cui Z., Cuypers Y., Daley A., Damerell G. M., Dauhut T., Deneke H., Desbios J. -P., Dorner S., Donner S., Douet V., Drushka K., Dutsch M., Ehrlich A., Emanuel K., Emmanouilidis A., Etienne J. -C., Etienne-Leblanc S., Faure G., Feingold G., Ferrero L., Fix A., Flamant C., Flatau P. J., Foltz G. R., Forster L., Furtuna I., Gadian A., Galewsky J., Gallagher M., Gallimore P., Gaston C., Gentemann C., Geyskens N., Giez A., Gollop J., Gouirand I., Gourbeyre C., De Graaf D., De Groot G. E., Grosz R., Guttler J., Gutleben M., Hall K., Harris G., Helfer K. C., Henze D., Herbert C., Holanda B., Ibanez-Landeta A., Intrieri J., Iyer S., Julien F., Kalesse H., Kazil J., Kellman A., Kidane A. T., Kirchner U., Klingebiel M., Korner M., Kremper L. A., Kretzschmar J., Kruger O., Kumala W., Kurz A., L'Hegaret P., Labaste M., Lachlan-Cope T., Laing A., Landschutzer P., Lang T., Lange D., Lange I., Laplace C., Lavik G., Laxenaire R., LeBihan C., Leandro M., Lefevre N., Lena M., Lenschow D., Li Q., Lloyd G., Los S., Losi N., Lovell O., Luneau C., Makuch P., Malinowski S., Manta G., Marinou E., Marsden N., Masson S., Maury N., Mayer B., Mayers-Als M., Mazel C., McGeary W., McWilliams J. C., Mech M., Mehlmann M., Meroni A. N., Mieslinger T., Minikin A., Minnett P., Moller G., Avalos Y. M., Muller C., Musat I., Napoli A., Neuberger A., Noisel C., Noone D., Nordsiek F., Nowak J. L., Oswald L., Parker D. J., Peck C., Person R., Philippi M., Plueddemann A., Pohlker C., Portge V., Poschl U., Pologne L., Posyniak M., Prange M., Melendez E. Q., Radtke J., Ramage K., Reimann J., Renault L., Reus K., Reyes A., Ribbe J., Ringel M., Ritschel M., Rocha C. B., Rochetin N., Rottenbacher J., Rollo C., Royer H., Sadoulet P., Saffin L., Sandiford S., Sandu I., Schafer M., Schemann V., Schirmacher I., Schlenczek O., Schmidt J., Schroder M., Schwarzenboeck A., Sealy A., Senff C. J., Serikov I., Shohan S., Siddle E., Smirnov A., Spath F., Spooner B., Katharina Stolla M., Szkolka W., De Szoeke S. P., Tarot S., Tetoni E., Thompson E., Thomson J., Tomassini L., Totems J., Ubele A. A., Villiger L., Von Arx J., Wagner T., Walther A., Webber B., Wendisch M., Whitehall S., Wiltshire A., Wing A. A., Wirth M., Wiskandt J., Wolf K., Worbes L., Wright E., Wulfmeyer V., Young S., Zhang C., Zhang D., Ziemen F., Zinner T., Zoger M., Stevens, B, Bony, S, Farrell, D, Ament, F, Blyth, A, Fairall, C, Karstensen, J, Quinn, P, Speich, S, Acquistapace, C, Aemisegger, F, Albright, A, Bellenger, H, Bodenschatz, E, Caesar, K, Chewitt-Lucas, R, De Boer, G, Delanoe, J, Denby, L, Ewald, F, Fildier, B, Forde, M, George, G, Gross, S, Hagen, M, Hausold, A, Heywood, K, Hirsch, L, Jacob, M, Jansen, F, Kinne, S, Klocke, D, Kolling, T, Konow, H, Lothon, M, Mohr, W, Naumann, A, Nuijens, L, Olivier, L, Pincus, R, Pohlker, M, Reverdin, G, Roberts, G, Schnitt, S, Schulz, H, Pier Siebesma, A, Stephan, C, Sullivan, P, Touze-Peiffer, L, Vial, J, Vogel, R, Zuidema, P, Alexander, N, Alves, L, Arixi, S, Asmath, H, Bagheri, G, Baier, K, Bailey, A, Baranowski, D, Baron, A, Barrau, S, Barrett, P, Batier, F, Behrendt, A, Bendinger, A, Beucher, F, Bigorre, S, Blades, E, Blossey, P, Bock, O, Boing, S, Bosser, P, Bourras, D, Bouruet-Aubertot, P, Bower, K, Branellec, P, Branger, H, Brennek, M, Brewer, A, Brilouet, P, Brugmann, B, Buehler, S, Burke, E, Burton, R, Calmer, R, Canonici, J, Carton, X, Cato, G, Charles, J, Chazette, P, Chen, Y, Chilinski, M, Choularton, T, Chuang, P, Clarke, S, Coe, H, Cornet, C, Coutris, P, Couvreux, F, Crewell, S, Cronin, T, Cui, Z, Cuypers, Y, Daley, A, Damerell, G, Dauhut, T, Deneke, H, Desbios, J, Dorner, S, Donner, S, Douet, V, Drushka, K, Dutsch, M, Ehrlich, A, Emanuel, K, Emmanouilidis, A, Etienne, J, Etienne-Leblanc, S, Faure, G, Feingold, G, Ferrero, L, Fix, A, Flamant, C, Flatau, P, Foltz, G, Forster, L, Furtuna, I, Gadian, A, Galewsky, J, Gallagher, M, Gallimore, P, Gaston, C, Gentemann, C, Geyskens, N, Giez, A, Gollop, J, Gouirand, I, Gourbeyre, C, De Graaf, D, De Groot, G, Grosz, R, Guttler, J, Gutleben, M, Hall, K, Harris, G, Helfer, K, Henze, D, Herbert, C, Holanda, B, Ibanez-Landeta, A, Intrieri, J, Iyer, S, Julien, F, Kalesse, H, Kazil, J, Kellman, A, Kidane, A, Kirchner, U, Klingebiel, M, Korner, M, Kremper, L, Kretzschmar, J, Kruger, O, Kumala, W, Kurz, A, L'Hegaret, P, Labaste, M, Lachlan-Cope, T, Laing, A, Landschutzer, P, Lang, T, Lange, D, Lange, I, Laplace, C, Lavik, G, Laxenaire, R, Lebihan, C, Leandro, M, Lefevre, N, Lena, M, Lenschow, D, Li, Q, Lloyd, G, Los, S, Losi, N, Lovell, O, Luneau, C, Makuch, P, Malinowski, S, Manta, G, Marinou, E, Marsden, N, Masson, S, Maury, N, Mayer, B, Mayers-Als, M, Mazel, C, Mcgeary, W, Mcwilliams, J, Mech, M, Mehlmann, M, Meroni, A, Mieslinger, T, Minikin, A, Minnett, P, Moller, G, Avalos, Y, Muller, C, Musat, I, Napoli, A, Neuberger, A, Noisel, C, Noone, D, Nordsiek, F, Nowak, J, Oswald, L, Parker, D, Peck, C, Person, R, Philippi, M, Plueddemann, A, Pohlker, C, Portge, V, Poschl, U, Pologne, L, Posyniak, M, Prange, M, Melendez, E, Radtke, J, Ramage, K, Reimann, J, Renault, L, Reus, K, Reyes, A, Ribbe, J, Ringel, M, Ritschel, M, Rocha, C, Rochetin, N, Rottenbacher, J, Rollo, C, Royer, H, Sadoulet, P, Saffin, L, Sandiford, S, Sandu, I, Schafer, M, Schemann, V, Schirmacher, I, Schlenczek, O, Schmidt, J, Schroder, M, Schwarzenboeck, A, Sealy, A, Senff, C, Serikov, I, Shohan, S, Siddle, E, Smirnov, A, Spath, F, Spooner, B, Katharina Stolla, M, Szkolka, W, De Szoeke, S, Tarot, S, Tetoni, E, Thompson, E, Thomson, J, Tomassini, L, Totems, J, Ubele, A, Villiger, L, Von Arx, J, Wagner, T, Walther, A, Webber, B, Wendisch, M, Whitehall, S, Wiltshire, A, Wing, A, Wirth, M, Wiskandt, J, Wolf, K, Worbes, L, Wright, E, Wulfmeyer, V, Young, S, Zhang, C, Zhang, D, Ziemen, F, Zinner, T, Zoger, M, Stevens B., Bony S., Farrell D., Ament F., Blyth A., Fairall C., Karstensen J., Quinn P. K., Speich S., Acquistapace C., Aemisegger F., Albright A. L., Bellenger H., Bodenschatz E., Caesar K. -A., Chewitt-Lucas R., De Boer G., Delanoe J., Denby L., Ewald F., Fildier B., Forde M., George G., Gross S., Hagen M., Hausold A., Heywood K. J., Hirsch L., Jacob M., Jansen F., Kinne S., Klocke D., Kolling T., Konow H., Lothon M., Mohr W., Naumann A. K., Nuijens L., Olivier L., Pincus R., Pohlker M., Reverdin G., Roberts G., Schnitt S., Schulz H., Pier Siebesma A., Stephan C. C., Sullivan P., Touze-Peiffer L., Vial J., Vogel R., Zuidema P., Alexander N., Alves L., Arixi S., Asmath H., Bagheri G., Baier K., Bailey A., Baranowski D., Baron A., Barrau S., Barrett P. A., Batier F., Behrendt A., Bendinger A., Beucher F., Bigorre S., Blades E., Blossey P., Bock O., Boing S., Bosser P., Bourras D., Bouruet-Aubertot P., Bower K., Branellec P., Branger H., Brennek M., Brewer A., Brilouet P. -E., Brugmann B., Buehler S. A., Burke E., Burton R., Calmer R., Canonici J. -C., Carton X., Cato G., Charles J. A., Chazette P., Chen Y., Chilinski M. T., Choularton T., Chuang P., Clarke S., Coe H., Cornet C., Coutris P., Couvreux F., Crewell S., Cronin T., Cui Z., Cuypers Y., Daley A., Damerell G. M., Dauhut T., Deneke H., Desbios J. -P., Dorner S., Donner S., Douet V., Drushka K., Dutsch M., Ehrlich A., Emanuel K., Emmanouilidis A., Etienne J. -C., Etienne-Leblanc S., Faure G., Feingold G., Ferrero L., Fix A., Flamant C., Flatau P. J., Foltz G. R., Forster L., Furtuna I., Gadian A., Galewsky J., Gallagher M., Gallimore P., Gaston C., Gentemann C., Geyskens N., Giez A., Gollop J., Gouirand I., Gourbeyre C., De Graaf D., De Groot G. E., Grosz R., Guttler J., Gutleben M., Hall K., Harris G., Helfer K. C., Henze D., Herbert C., Holanda B., Ibanez-Landeta A., Intrieri J., Iyer S., Julien F., Kalesse H., Kazil J., Kellman A., Kidane A. T., Kirchner U., Klingebiel M., Korner M., Kremper L. A., Kretzschmar J., Kruger O., Kumala W., Kurz A., L'Hegaret P., Labaste M., Lachlan-Cope T., Laing A., Landschutzer P., Lang T., Lange D., Lange I., Laplace C., Lavik G., Laxenaire R., LeBihan C., Leandro M., Lefevre N., Lena M., Lenschow D., Li Q., Lloyd G., Los S., Losi N., Lovell O., Luneau C., Makuch P., Malinowski S., Manta G., Marinou E., Marsden N., Masson S., Maury N., Mayer B., Mayers-Als M., Mazel C., McGeary W., McWilliams J. C., Mech M., Mehlmann M., Meroni A. N., Mieslinger T., Minikin A., Minnett P., Moller G., Avalos Y. M., Muller C., Musat I., Napoli A., Neuberger A., Noisel C., Noone D., Nordsiek F., Nowak J. L., Oswald L., Parker D. J., Peck C., Person R., Philippi M., Plueddemann A., Pohlker C., Portge V., Poschl U., Pologne L., Posyniak M., Prange M., Melendez E. Q., Radtke J., Ramage K., Reimann J., Renault L., Reus K., Reyes A., Ribbe J., Ringel M., Ritschel M., Rocha C. B., Rochetin N., Rottenbacher J., Rollo C., Royer H., Sadoulet P., Saffin L., Sandiford S., Sandu I., Schafer M., Schemann V., Schirmacher I., Schlenczek O., Schmidt J., Schroder M., Schwarzenboeck A., Sealy A., Senff C. J., Serikov I., Shohan S., Siddle E., Smirnov A., Spath F., Spooner B., Katharina Stolla M., Szkolka W., De Szoeke S. P., Tarot S., Tetoni E., Thompson E., Thomson J., Tomassini L., Totems J., Ubele A. A., Villiger L., Von Arx J., Wagner T., Walther A., Webber B., Wendisch M., Whitehall S., Wiltshire A., Wing A. A., Wirth M., Wiskandt J., Wolf K., Worbes L., Wright E., Wulfmeyer V., Young S., Zhang C., Zhang D., Ziemen F., Zinner T., and Zoger M.
Abstract: The science guiding the EUREC4A campaign and its measurements is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic - eastward and southeastward of Barbados. Through its ability to characterize processes operating across a wide range of scales, EUREC4A marked a turning point in our ability to observationally study factors influencing clouds in the trades, how they will respond to warming, and their link to other components of the earth system, such as upper-ocean processes or the life cycle of particulate matter. This characterization was made possible by thousands (2500) of sondes distributed to measure circulations on meso- (200 km) and larger (500 km) scales, roughly 400 h of flight time by four heavily instrumented research aircraft; four global-class research vessels; an advanced ground-based cloud observatory; scores of autonomous observing platforms operating in the upper ocean (nearly 10 000 profiles), lower atmosphere (continuous profiling), and along the air-sea interface; a network of water stable isotopologue measurements; targeted tasking of satellite remote sensing; and modeling with a new generation of weather and climate models. In addition to providing an outline of the novel measurements and their composition into a unified and coordinated campaign, the six distinct scientific facets that EUREC4A explored - from North Brazil Current rings to turbulence-induced clustering of cloud droplets and its influence on warm-rain formation - are presented along with an overview of EUREC4A's outreach activities, environmental impact, and guidelines for scientific practice. Track data for all platforms are standardized and accessible at 10.25326/165 , and a film documenting the campaign is provided as a video supplement.
Published: 2021

3. Rainforest aerosols as biogenic nuclei of clouds and precipitation in the Amazon

Author: Poschl, U., Martin, S.T., Sinha, B., Chen, Q., Gunthe, S.S., Huffman, J.A., Borrmann, S., Farmer, D.K., Garland, R.M., Helas, G., Jimenez, J.L., King, S.M., Manzi, A., Mikhailov, E., Pauliquevis, T., Petters, M.D., Prenni, A.J., Roldin, P., Rose, D., Schneider, J., Su, H., Zorn, S.R., Artaxo, P., and Andreae, M.O.
Subjects: Amazon River region -- Environmental aspects, Rain forests -- Evaluation, Aerosols -- Environmental aspects, Science and technology
Abstract: The Amazon is one of the few continental regions where atmospheric aerosol particles and their effects on climate are not dominated by anthropogenic sources. During the wet season, the ambient conditions approach those of the pristine pre-industrial era. We show that the fine submicrometer particles accounting for most cloud condensation nuclei are predominantly composed of secondary organic material formed by oxidation of gaseous biogenic precursors. Supermicrometer particles, which are relevant as ice nuclei, consist mostly of primary biological material directly released from rainforest biota. The Amazon Basin appears to be a biogeochemical reactor, in which the biosphere and atmospheric photochemistry produce nuclei for clouds and precipitation sustaining the hydrological cycle. The prevailing regime of aerosol-cloud interactions in this natural environment is distinctly different from polluted regions. 10.1126/science.1191056
Published: 2010
Full Text: View/download PDF

4. Arctic Ozone Loss Due to Denitrification

Author: Waibel, A. E., Peter, Th., Carslaw, K. S., Oelhaf, H., Wetzel, G., Crutzen, P. J., Poschl, U., Tsias, A., Reimer, E., and Fischer, H.
Published: 1999

5. Real-time detection of Bioaerosols by Mass Spectrometry and Fluorescence methods during the BIODETECT 2014 campaign at CEA/LSCE/ACTRIS SUPERSITE (Saclay, France)

Author: Sarda-Esteve, Roland, Sciare, Jean, Bonnaire, N., Junot, C., Fennaille, F., Bercher, F., Thibaudon, M., Baisnee, B., Gallagher, M., Gabey, A., Foot, V.E., Huffman, J.A., Poschl, U., Su, H., Kiselev, D., Sampo, S., Favez, Olivier, Jayne, John, Croteau, Philip, Prevot, A., Vlachou, A., El Haddad, Imad, Roux, J.M., Nadal, M.H., Bossuet, C., Olmedo, L., and Civs, Gestionnaire
Subjects: [SDE] Environmental Sciences
Abstract: The French Atomic Energy Commission (CEA) has developed a new on line mass spectrometry method to detect atmospheric fungal spores (Sarda Esteve et al., AAAR 2013) under the Bio Chemical Collectors (BCC) research project. This method has been compared with a traditional method from the National Network of Survey for Airborne contaminants (RNSA) to identify Cladosporium events and has shown good agreement with microscopy techniques. Real-time measurements of bio-aerosols using light-induced fluorescence (LIF) techniques have also been performed widely, both for bio-aerosol quantification and to support ice nucleation studies (e.g. Despres et al., 2012). Recent work has sought to better understand the variability in observed fluorescence recorded using LIF instruments (Huffman et al., 2013, O'Connor et al., 2014). Novel data analysis methods are also required to effectively interpret the datasets produced by such instruments, which can exhibit high dimensionality. Robinson et al., (2013) successfully distinguished between calibration particles measured using a WIBS 4A by applying a clustering algorithm to the data. They went on to apply this algorithm to ambient datasets and attributed particular clusters to bacteria and fungal spores (Crawford et al., 2014). To understand the major processes affecting fluorescent aerosol particles, it is necessary to intercompare these real-time methods with measurements of biological targets that provide more detailed chemical information, such as real-time mass spectrometry. An intensive measurement campaign, BIODETECT 2014, will take place at the LSCE-SIRTA ACTRIS supersite outside Paris in summer between the 7th of July and the 8th of August. This study may help identify potential new technologies for monitoring the spread of airborne pathogens and other bio-aerosols. During this period of the year, bacteria and fungal spore are expected to be emitted to the air in high concentration. These bio-aerosol events can be used as proxies for airborne pathogens spreading through an urban/suburban influenced environment.
Published: 2014

6. Size distributions and temporal variations of biological aerosol particles in the Amazon rainforest characterized by microscopy and real-time UV-APS fluorescence techniques during AMAZE-08

Author: Poschl, U
Subjects: FÍSICA ATMOSFÉRICA
Published: 2012

7. Introduction: European Integrated Project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI) - integrating aerosol research from nano to global scales

Author: Kulmala M, Asmi A, Lappalainen HK, Carslaw KS, Poschl U, Baltensperger U, Hov O, Brenquier JL, Pandis SN, Facchini MC, Hansson, H.C, Wiedensohler A, and O'Dowd CD
Subjects: GAS-PARTICLE INTERACTIONS, DROPLET GROWTH-KINETICS, KINETIC-MODEL FRAMEWORK, SOURCE ATTRIBUTION, SUBMICRON ORGANIC AEROSOLS
Abstract: The European Aerosol Cloud Climate and Air Quality Interactions project EUCAARI is an EU Research Framework 6 integrated project focusing on understanding the interactions of climate and air pollution. EUCAARI works in an integrative and multidisciplinary way from nano-to global scale. EUCAARI brings together several leading European research groups, state-of-the-art infrastructure and some key scientists from third countries to investigate the role of aerosol on climate and air quality. Altogether 48 partners from 25 countries are participating in EUCAARI. During the first 16 months EUCAARI has built operational systems, e. g. established pan-European measurement network for Lagrangian studies and four stations in developing countries. Also an improved understanding of nanoscale processes (like nucleation) has been implemented in global models. Here we present the research methods, organisation, operations and first results of EUCAARI.
Published: 2009

8. Isoprene and monoterpene fluxes from Central Amazonian rainforest inferred from tower-based and airborne measurements, and implications on the atmospheric chemistry and the local carbon budget

Author: Kuhn U., Andreae M. O., Ammann C., Araujo A. C., Brancaleoni E., Ciccioli P., Dindorf T., Frattoni M., Gatti L.V., Ganzeveld L., Kruijt B., Lelieveld J., Lloyd J., Meixner F.X., Nobre A.D., Poschl U., Spirig C., and Stefani P.
Subjects: Basso rapporto Isoprenoisi/NEE, Elevate Concentrazioni radicali OH, Foresta Amazzonica, Flussi isoprene e monoterpeni
Abstract: Flussi di isoprene e monoterpeni sono stati determinati in un sito della foresta Amazzonica mediante tre differenti metodi micro-meteorologici. Le misure degli isoprenoidi e dei loro prodotti di ossidazione ha permesso di stabilire che, in contrato con quello che si pensava comunemente, alte concentrazioni di radicali OH sono presenti nell'Atmospheric Boundary Layer di questi siti remoti. E' stato inoltre confermato che l'emissione di isoprenoidi rappresenta una frazione molto piccola della frazione di CO2 assimilata.
Published: 2007

9. Isoprene and its oxidation products methyl vinyl ketone, methacrolein, and isoprene related peroxides measured online over the tropical rain forest of Surinam in March 1998

Author: Warneke, C., Holzinger, R., Hansel, A., Jordan, A., Lindinger, W., Poschl, U., Williams, J., Hoor, P., Fischer, H., Pj, Crutzen, Bert Scheeren, Lelieveld, J., and Isotope Research
Subjects: methylvinylketone, OZONE, IMPACT, methacrolein, PHOTOSYNTHESIS, box model, VOLATILE ORGANIC-COMPOUNDS, isoprene oxidation products, NONMETHANE HYDROCARBONS, TROPOSPHERIC CHEMISTRY, isoprene, tropical forest boundary layer, EMISSION, PPTV, TEMPERATURE
Abstract: Airborne measurements of volatile organic compounds (VOC) were performed over the tropical rainforest in Surinam (0-12 km altitude, 2 degrees -7 degrees N, 54 degrees -58 degrees W) using the proton transfer reaction mass spectrometry (PTR-MS) technique, which allows online monitoring of compounds like isoprene, its oxidation products methyl vinyl ketone, methacrolein, tentatively identified hydroxy-isoprene-hydroperoxides, and several other organic compounds. Isoprene volume mixing ratios (VMR) varied from below the detection limit at the highest altitudes to about 7 nmol/mol in the planetary boundary layer shortly before sunset. Correlations between isoprene and its product compounds were made for different times of day and altitudes, with the isoprene-hydroperoxides showing the highest correlation. Model calculated mixing ratios of the isoprene oxidation products using a detailed hydrocarbon oxidation mechanism, as well as the intercomparison measurement with air samples collected during the flights in canisters and later analysed with a GC-FID, showed good agreement with the PTR-MS measurements, in particular at the higher mixing ratios. Low OH concentrations in the range of 1-3 x 10(5) molecules cm(-3) averaged over 24 hours were calculated due to loss of OH and HO(2) in the isoprene oxidation chain, thereby strongly enhancing the lifetime of gases in the forest boundary layer.
Published: 2001

10. High spatial and temporal resolution measurements of primary organics and their oxidation products over the tropical forests of Surinam

Author: Pj, Crutzen, Williams, J., Poschl, U., Hoor, P., Fischer, H., Warneke, C., Holzinger, R., Hansel, A., Lindinger, W., Bert Scheeren, Lelieveld, J., and Isotope Research
Subjects: methyl vinyl ketone, UPPER TROPOSPHERE, ACETONE, methacrolein, proton transfer mass spectrometer (PTR-MS), GASES, upper tropospheric HO(x), tropical rainforest emissions, volatile organic compounds (VOC), isoprene oxidation products, CHEMISTRY, HYDROGEN RADICALS, isoprene, EMISSIONS
Abstract: Tropical forests with emissions greater than 10(15) g C of reactive hydrocarbons per year strongly affect atmospheric chemistry. Here we report aircraft-borne measurements of organics during March 1998 in Surinam, a largely unpolluted region which is optimally located to study chemical processes induced by tropical forest emissions. Isoprene and its degradation products methylvinyl ketone (MVK) and methacrolein (MACR) and possibly isoprene hydroperoxides (ISOHP), were measured in the nmol mol(-1) volume mixing ratio (VMR) range, consistent with estimated emissions and model calculations. In addition, high VMRs of some non-isoprene-derived organics were measured, such as acetone (approximate to 2-4 nmol mol(1) up to 12 km altitude), an important source of HO and HO(2) in the upper troposphere. Moreover, several masses were measured at significant mixing ratios which could not be identified by reference to previous field measurements or gas-phase isoprene chemistry. High VMRs, almost 0.4 nmol mol(-1), were also recorded for a compound which is most likely dimethyl sulphide (DMS). If so, boundary layer loss of HO by reactions with hydrocarbons and their oxidation products strongly prolongs the lifetime of DMS, allowing its transport deep into the Amazon forest south of the intertropical convergence zone (ITCZ). We postulate greater sulphate production and deposition north than south of the (ITCZ) with possible consequences for cloud and ecosystem properties. (C) 2000 Elsevier Science Ltd. All rights reserved.
Published: 2000

11. General overview: European Integrated project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI) - integrating aerosol research from nano to global scales

Author: Kulmala, M., Asmi, A., Lappalainen, H.K., Baltensperger, U., Brenguier, J.-L., Facchini, M.C., Hansson, H.-C., Hov, Ø., O'Dowd, C.D., Poschl, U., Wiedensohler, A., Boers, R., Boucher, O., de Leeuw, G., Denier van der Gon, H.A.C., Feichter, J., Krejci, R., Laj, P., Lihavainen, H., Lohmann, U., McFiggans, G., Mentel, T., Pilinis, C., Riipinen, I., Schulz, M., Stohl, A., Swietlicki, E., Vignati, E., Alves, C., Amann, M., Ammann, M., Arabas, S., Artaxo, P., Baars, H., Beddows, D.C.S., Bergstrom, R., Beukes, J.P., Bilde, M., Burkhart, J.F., Canonaco, F., Clegg, S.L., Coe, H., Crumeyrolle, S., D'Anna, B., Decesari, S., Gilardoni, S., Fischer, M., Fjaeraa, A.M., Fountoukis, C., George, C., Gomes, L., Halloran, P., Hamburger, T., Harrison, R.M., Herrmann, H., Hoffmann, T., Hoose, C., Hu, M., Hyvarinen, A., Horrak, U., Iinuma, Y., Iversen, T., Josipovic, M., Kanakidou, M., Kiendler-Scharr, A., Kirkevag, A., Kiss, G., Klimont, Z., Kolmonen, P., Komppula, M., Kristjansson, J.-E., Laakso, L., Laaksonen, A., Labonnote, L., Lanz, V.A., Lehtinen, K.E.J., Rizzo, L.V., Makkonen, R., Manninen, H.E., McMeeking, G., Merikanto, J., Minikin, A., Mirme, S., Morgan, W.T., Nemitz, E., O'Donnell, D., Panwar, T. S., Pawlowska, H., Petzold, A., Pienaar, J.J., Pio, C., Plass-Duelmer, C., Prevot, A.S.H., Pryor, S., Reddington, C.L., Roberts, G., Rosenfeld, D., Schwarz, J., Seland, O., Sellegri, K., Shen, X.J., Shiraiwa, M., Siebert, H., Sierau, B., Simpson, D., Sun, J.Y., Topping, D., Tunved, P., Vaattovaara, P., Vakkari, V., Veefkind, J.P., Visschedijk, A., Vuollekoski, H., Vuolo, R., Wehner, B., Wildt, J., Woodward, S., Worsnop, D.R., van Zadelhoff, G.-J., Zardini, A.A., Zhang, K., van Zyl, P.G., Kerminen, V.-M., Carslaw, K.S., Pandis, S.N., Kulmala, M., Asmi, A., Lappalainen, H.K., Baltensperger, U., Brenguier, J.-L., Facchini, M.C., Hansson, H.-C., Hov, Ø., O'Dowd, C.D., Poschl, U., Wiedensohler, A., Boers, R., Boucher, O., de Leeuw, G., Denier van der Gon, H.A.C., Feichter, J., Krejci, R., Laj, P., Lihavainen, H., Lohmann, U., McFiggans, G., Mentel, T., Pilinis, C., Riipinen, I., Schulz, M., Stohl, A., Swietlicki, E., Vignati, E., Alves, C., Amann, M., Ammann, M., Arabas, S., Artaxo, P., Baars, H., Beddows, D.C.S., Bergstrom, R., Beukes, J.P., Bilde, M., Burkhart, J.F., Canonaco, F., Clegg, S.L., Coe, H., Crumeyrolle, S., D'Anna, B., Decesari, S., Gilardoni, S., Fischer, M., Fjaeraa, A.M., Fountoukis, C., George, C., Gomes, L., Halloran, P., Hamburger, T., Harrison, R.M., Herrmann, H., Hoffmann, T., Hoose, C., Hu, M., Hyvarinen, A., Horrak, U., Iinuma, Y., Iversen, T., Josipovic, M., Kanakidou, M., Kiendler-Scharr, A., Kirkevag, A., Kiss, G., Klimont, Z., Kolmonen, P., Komppula, M., Kristjansson, J.-E., Laakso, L., Laaksonen, A., Labonnote, L., Lanz, V.A., Lehtinen, K.E.J., Rizzo, L.V., Makkonen, R., Manninen, H.E., McMeeking, G., Merikanto, J., Minikin, A., Mirme, S., Morgan, W.T., Nemitz, E., O'Donnell, D., Panwar, T. S., Pawlowska, H., Petzold, A., Pienaar, J.J., Pio, C., Plass-Duelmer, C., Prevot, A.S.H., Pryor, S., Reddington, C.L., Roberts, G., Rosenfeld, D., Schwarz, J., Seland, O., Sellegri, K., Shen, X.J., Shiraiwa, M., Siebert, H., Sierau, B., Simpson, D., Sun, J.Y., Topping, D., Tunved, P., Vaattovaara, P., Vakkari, V., Veefkind, J.P., Visschedijk, A., Vuollekoski, H., Vuolo, R., Wehner, B., Wildt, J., Woodward, S., Worsnop, D.R., van Zadelhoff, G.-J., Zardini, A.A., Zhang, K., van Zyl, P.G., Kerminen, V.-M., Carslaw, K.S., and Pandis, S.N.
Abstract: In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan-European aerosol emissions inventory was developed and evaluated, a new cluster spectrometer was built and tested in the field and several new aerosol parameterizations and computations modules for chemical transport and global climate models were developed and evaluated. These achievements and related studies have substantially improved our understanding and reduced the uncertainties of aerosol radiative forcing and air quality-climate interactions. The EUCAARI results can be utilized in European and global environmental policy to assess the aerosol impacts and the corresponding abatement strategies.
Published: 2011

12. Introduction: European Integrated Project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI) : integrating aerosol research from nano to global scales

Author: Kulmala, M., Asmi, A., Lappalainen, H.K., Carslaw, K.S., Poschl, U., Baltensperger, U., Hov, O., Brenquier, J.L., Pandis, S.N., Facchini, M.C., Hansson, H.-C., Wiedensohler, A., O'Dowd, C.D., Kulmala, M., Asmi, A., Lappalainen, H.K., Carslaw, K.S., Poschl, U., Baltensperger, U., Hov, O., Brenquier, J.L., Pandis, S.N., Facchini, M.C., Hansson, H.-C., Wiedensohler, A., and O'Dowd, C.D.
Abstract: The European Aerosol Cloud Climate and Air Quality Interactions project EUCAARI is an EU Research Framework 6 integrated project focusing on understanding the interactions of climate and air pollution. EUCAARI works in an integrative and multidisciplinary way from nano-to global scale. EUCAARI brings together several leading European research groups, state-of-the-art infrastructure and some key scientists from third countries to investigate the role of aerosol on climate and air quality. Altogether 48 partners from 25 countries are participating in EUCAARI. During the first 16 months EUCAARI has built operational systems, e. g. established pan-European measurement network for Lagrangian studies and four stations in developing countries. Also an improved understanding of nanoscale processes (like nucleation) has been implemented in global models. Here we present the research methods, organisation, operations and first results of EUCAARI.
Published: 2009
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13. Atmospheric composition change: global and regional air quality

Author: Monks, P. S, Granier, C., Fuzzi, S., Stohl, A., Williams, M. L., Akimoto, H., Amann, M., Baklanov, A., Baltensperger, U., Bey, I., Blake, N., Blake, R. S., Carslaw, K., Cooper, O. R., Dentener, F., Fowler, D., Fragkou, E., Frost, G. J., Generoso, S., Ginoux, P., Grewe, V., Guenther, A., Hanson, H. C., Henne, S., Hjorth, J., Hofzumahaus, A., Huntrieser, H., Isaksen, I. S. A., Jenkin, M. E., Kaiser, J., Kanakidou, M., Klimont, Z., Kulmala, M., Laj, P., Lawrence, M. G., Lee, J. D., Liousse, C., Maione, M., McFiggans, G., Metzger, A., Mieville, A., Moussiopoulos, N., Orlando, J. J., O'Dowd, C. D., Palmer, P. I., Parrish, D. D., Petzold, A., Platt, U., Poschl, U., Prevot, A. S. H., Reeves, C. E., Reimann, S., Rudich, Y., Sellegri, K., Steinbrecher, R., Simpson, D., ten Brink, H., Theloke, J., van der Werf, G. R., Vautard, R., Vestreng, V., Vlachokostas, Ch., von Glasow, R., Monks, P. S, Granier, C., Fuzzi, S., Stohl, A., Williams, M. L., Akimoto, H., Amann, M., Baklanov, A., Baltensperger, U., Bey, I., Blake, N., Blake, R. S., Carslaw, K., Cooper, O. R., Dentener, F., Fowler, D., Fragkou, E., Frost, G. J., Generoso, S., Ginoux, P., Grewe, V., Guenther, A., Hanson, H. C., Henne, S., Hjorth, J., Hofzumahaus, A., Huntrieser, H., Isaksen, I. S. A., Jenkin, M. E., Kaiser, J., Kanakidou, M., Klimont, Z., Kulmala, M., Laj, P., Lawrence, M. G., Lee, J. D., Liousse, C., Maione, M., McFiggans, G., Metzger, A., Mieville, A., Moussiopoulos, N., Orlando, J. J., O'Dowd, C. D., Palmer, P. I., Parrish, D. D., Petzold, A., Platt, U., Poschl, U., Prevot, A. S. H., Reeves, C. E., Reimann, S., Rudich, Y., Sellegri, K., Steinbrecher, R., Simpson, D., ten Brink, H., Theloke, J., van der Werf, G. R., Vautard, R., Vestreng, V., Vlachokostas, Ch., and von Glasow, R.
Abstract: Air quality transcends all scales with in the atmosphere from the local to the global with handovers and feedbacks at each scale interaction. Air quality has manifold effects on health, ecosystems, heritage and climate. In this review the state of scientific understanding in relation to global and regional air quality is outlined. The review discusses air quality, in terms of emissions, processing and transport of trace gases and aerosols. New insights into the characterization of both natural and anthropogenic emissions are reviewed looking at both natural (e.g. dust and lightning) as well as plant emissions. Trends in anthropogenic emissions both by region and globally are discussed as well as biomass burning emissions. In terms of chemical processing the major air quality elements of ozone, non-methane hydrocarbons, nitrogen oxides and aerosols are covered. A number of topics are presented as a way of integrating the process view into the atmospheric context; these include the atmospheric oxidation efficiency, halogen and HOx chemistry, nighttime chemistry, tropical chemistry, heat waves, megacities, biomass burning and the regional hot spot of the Mediterranean. New findings with respect to the transport of pollutants across the scales are discussed, in particular the move to quantify the impact of long-range transport on regional air quality. Gaps and research questions that remain intractable are identified. The review concludes with a focus of research and policy questions for the coming decade. In particular, the policy challenges for concerted air quality and climate change policy (co-benefit) are discussed.
Published: 2009

14. Temperature and humidity dependence of secondary organic aerosol yield from the ozonolysis of beta-pinene

Author: von Hessberg, C, von Hessberg, P, Poschl, U, Bilde, M, Nielsen, OJ, Moortgat, GK, von Hessberg, C, von Hessberg, P, Poschl, U, Bilde, M, Nielsen, OJ, and Moortgat, GK
Published: 2009

15. Isoprene and monoterpene fluxes from central amazonian rainforest inferred from tower-based and airborne measurements, and implications on the atmospheric chemistry and the local carbon budget

Author: Kuhn, U., Andreae, M.O., Ammann, C., de Araujo, A.C., Brancaleoni, E., Ciccioli, P., Dindorf, T., Frattoni, M., Gatti, L.V., Ganzeveld, L., Kruijt, B., Lelieveld, J., Lloyd, J., Meixner, F.X., Nobre, A.D., Poschl, U., Spirig, C., Stefani, P., Thielmann, A., Valentini, R., Kesselmeier, J., Kuhn, U., Andreae, M.O., Ammann, C., de Araujo, A.C., Brancaleoni, E., Ciccioli, P., Dindorf, T., Frattoni, M., Gatti, L.V., Ganzeveld, L., Kruijt, B., Lelieveld, J., Lloyd, J., Meixner, F.X., Nobre, A.D., Poschl, U., Spirig, C., Stefani, P., Thielmann, A., Valentini, R., and Kesselmeier, J.
Published: 2007
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16. ChemInform Abstract: Synthesis, Reactivity, and Spectroscopy of Phenylated Cyclotetrasilanes and Cyclopentasilanes

Author: POSCHL, U., primary, SIEGL, H., additional, and HASSLER, K., additional
Published: 2010
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17. Nitration of Allergens Triggers Allergic Immune Responses.

Author: Muller, B, primary, Poschl, U, additional, Zhang, Y, additional, Yang, H, additional, Teich, R, additional, and Garn, H, additional
Published: 2009
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18. Combined particle emission reduction and heat recovery from combustion exhaust—A novel approach for small wood-fired appliances

Author: MESSERER, A, primary, SCHMATLOCH, V, additional, POSCHL, U, additional, and NIESSNER, R, additional
Published: 2007
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19. Exploring the severe winter haze in Beijing: the impact of synoptic weather, regional transport and heterogeneous reactions.

Author: Zheng, G. J., Duan, F. K., Su, H., Ma, Y. L., Cheng, Y., Zheng, B., Zhang, Q., Huang, T., Kimoto, T., Chang, D., Poschl, U., Cheng, Y. F., and He, K. B.
Subjects: HAZE, SYNOPTIC climatology, SYNOPTIC meteorology, WEATHER, GAS phase reactions
Abstract: Extreme haze episodes repeatedly shrouded Beijing during the winter of 2012-2013, causing major environmental and health problems. To better understand these extreme events, we performed a model-assisted analysis of the hourly observation data of PM2.5 and its major chemical compositions. The synthetic analysis shows that (1) the severe winter haze was driven by stable synoptic meteorological conditions over northeastern China, and not by an abrupt increase in anthropogenic emissions. (2) Secondary species, including organics, sulfate, nitrate, and ammonium, were the major constituents of PM2.5 during this period. (3) Due to the dimming effect of high loading of aerosol particles, gaseous oxidant concentrations decreased significantly, suggesting a reduced production of secondary aerosols through gas-phase reactions. Surprisingly, the observational data reveals an enhanced production rate of secondary aerosols, suggesting an important contribution from other formation pathways, most likely heterogeneous reactions. These reactions appeared to be more efficient in producing secondary inorganics aerosols than organic aerosols resulting in a strongly elevated fraction of inorganics during heavily polluted periods. (4) Moreover, we found that high aerosol concentration was a regional phenomenon. The accumulation process of aerosol particles occurred successively from cities southeast of Beijing. The apparent sharp increase in PM2.5 concentration of up to several hundred pgm-3 per hour recorded in Beijing represented rapid recovery from an interruption to the continuous pollution accumulation over the region, rather than purely local chemical production. This suggests that regional transport of pollutants played an important role during these severe pollution events. [ABSTRACT FROM AUTHOR]
Published: 2015
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20. Liquid- and Gas-Phase Nitration of Bovine Serum Albumin Studied by LC−MS and LC−MS/MS Using Monolithic Columns

Author: Walcher, W., Franze, T., Weller, M. G., Poschl, U., and Huber, C. G.
Abstract: Post-translational nitration of proteins was analyzed by capillary reversed-phase high-performance liquid chromatography (RP-HPLC) on-line interfaced to electrospray ionization mass spectrometry (ESI−MS) or tandem mass spectrometry (ESI−MS/MS). Both methods were compared using a tryptic digest of bovine serum albumin (BSA) and yielded sequence coverages of 95% and 33% with RP-HPLC−ESI−MS and RP-HPLC−ESI−MS/MS, respectively. At least 95% of the tyrosines were covered by the former method, whereas the latter method only detected less than 50% of the tyrosine-containing peptides. Upon liquid-phase nitration of BSA in aqueous solution using an excess of tetranitromethane, at least 16 of the 20 tyrosine residues were found to be nitrated. After exposure of solid BSA samples to gaseous nitrogen dioxide and ozone at atmospherically relevant concentration levels, only 3 nitrated peptides were detected. By use of such a model system, RP-HPLC−ESI−MS proved to be a rapid and highly efficient method for the comprehensive and quantitative detection of protein nitration. Keywords: proteins, peptides • monolithic capillary columns • nitration • reversed-phase liquid chromatography • electrospray ionization mass spectrometry • nitrogen dioxide, ozone • tetranitromethane
Published: 2003

21. Interaction of Ozone and Water Vapor with Spark Discharge Soot Aerosol Particles Coated with Benzo[a]pyrene: O<INF>3</INF> and H<INF>2</INF>O Adsorption, Benzo[a]pyrene Degradation, and Atmospheric Implications

Author: Poschl, U., Letzel, T., Schauer, C., and Niessner, R.
Abstract: The interaction of ozone and water vapor with spark discharge soot particles coated with the five-ring polycyclic aromatic hydrocarbon benzo[a]pyrene (BaP) has been investigated in aerosol flow tube experiments at ambient temperature and pressure (296 K, 1 atm). The investigated range of ozone volume mixing ratio (VMR) and relative humidity (RH) was 0−1 ppm and 0−25%, respectively. The observed gas-phase ozone losses and pseudo-first-order BaP decay rate coefficients exhibited Langmuir-type dependencies on gas-phase ozone concentration and were reduced in the presence of water vapor, which indicates rapid, reversible and competitive adsorption of O3 and H2O on the particles followed by a slower surface reaction between adsorbed O3 and BaP. At low ozone VMR and RH, the half-life of surface BaP molecules was found to be shorter than previously reported (~ 5 min at 30 ppb O3 under dry conditions). At higher RH and for multilayer BaP surface coverage, however, a strong increase of BaP half-life was observed and can be attributed to competitive H2O adsorption and to surface/bulk shielding effects, respectively. From four independent sets of ozone loss and BaP decay measurement data the following parameters have been derived: O3 and H2O Langmuir adsorption equilibrium constants KO3 = (2.8 ± 0.2) × 10^-13 cm³ and KH2O = (2.1 ± 0.4) × 10^-17 cm³, maximum pseudo-first-order BaP decay rate coefficient k1,4 = (0.015 ± 0.001) s^-1, adsorption site surface concentration [SS]S = (5.7 ± 1.7) × 10¹⁴ cm^-2. On the basis of these values, a second-order BaP−O3 surface reaction rate coefficient k2,s = (2.6 ± 0.8) × 10^-17 cm² s^-1 can be calculated, and estimates for the mean surface residence times and adsorption enthalpies of O3 and H2O have been derived: τO3 ≈ 5−18 s; τH2O ≈ 3 ms, ΔHads,O3 ≈ −(80−90) kJ mol^-1, ΔHads,H2O ≈ −50 kJ mol^-1. The results and their atmospheric implications are discussed in view of related studies.
Published: 2001

22. Microstructural rearrangement of sodium chloride condensation aerosol particles on interaction with water vapor

Author: Kramer, L., Poschl, U., and Niessner, R.
Published: 2000
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23. Mass Accommodation Coefficient of H<INF>2</INF>SO<INF>4</INF> Vapor on Aqueous Sulfuric Acid Surfaces and Gaseous Diffusion Coefficient of H<INF>2</INF>SO<INF>4</INF> in N<INF>2</INF>/H<INF>2</INF>O

Author: Poschl, U., Canagaratna, M., Jayne, J. T., Molina, L. T., Worsnop, D. R., Kolb, C. E., and Molina, M. J.
Abstract: The experimental determination of the mass accommodation coefficient of H2SO4 vapor on aqueous sulfuric acid and the gas-phase diffusion coefficient of H2SO4 vapor in N2/H2O at 303 K is reported. The measurements were carried out under laminar flow conditions in a coated wall tubular flow reactor coupled to a chemical ionization mass spectrometer for gas-phase detection. Wall loss rates of H2SO4 vapor, from which both the mass accommodation coefficient and the gas diffusion coefficient were determined, were measured as a function of total reactor pressure, water vapor concentration, and sulfuric acid vapor concentration. The observed wall loss rate coefficient depends linearly on the inverse of the total reactor pressure (0.54−10 Torr) and is independent of the aqueous sulfuric acid composition over the range 73−98 wt %, which was varied by the addition of water vapor. A kinetic model based on the additivity of kinetic resistances that couples gas-phase diffusion and mass accommodation to the measured H2SO4 vapor loss rate has been applied to the data. The model yields a lower limit of 0.43 with a best fit value of 0.65. The mass accommodation coefficient is independent of the liquid H2SO4/H2O composition over the range investigated. The gas-phase diffusion coefficient for H2SO4 vapor in N2/H2O (H2O mixing ratio ≤0.32) was determined to be 66.8 ± 1.1 Torr cm² s^-1. The resistance model agrees well with a more rigorous approximate solution to the full continuity equation describing mass transport and kinetics. The atmospheric implications of the reported results are discussed.
Published: 1998

24. Pressure and Temperature Dependence of the Gas-Phase Reaction of SO<INF>3</INF> with H<INF>2</INF>O and the Heterogeneous Reaction of SO<INF>3</INF> with H<INF>2</INF>O/H<INF>2</INF>SO<INF>4</INF> Surfaces

Author: Jayne, J. T., Poschl, U., Chen, Y.-m., Dai, D., Molina, L. T., Worsnop, D. R., Kolb, C. E., and Molina, M. J.
Abstract: The gas-phase reaction of SO3 with H2O and the heterogeneous reaction of SO3 with H2O−H2SO4 surfaces have been studied in a fast flow reactor coupled to a chemical ionization mass spectrometer (CIMS) for species detection. The gas-phase reaction was studied under turbulent flow conditions over the pressure range from 100 to 760 Torr N2 and the temperature range from 283 to 370 K. The loss rate of SO3 was measured under pseudo-first-order conditions; it exhibits a second-order dependence on water vapor concentration and has a strong negative temperature dependence. The first-order rate coefficient for the SO3 loss by gas-phase reaction shows no significant pressure dependence and can be expressed as k^I(s^-1) = 3.90 × 10^-41 exp(6830.6/T)[H2O]² where [H2O] is in units of molecule cm^-3 and T is in Kelvin. The overall uncertainty of our experimentally determined rate coefficients is estimated to be ±20%. At sufficiently low SO3 concentrations (<10¹² molecule cm^-3) the rate coefficient is independent of the initial SO3 level, as expected for a gas-phase reaction mechanism involving one SO3 and two H2O molecules. However, at higher concentrations and lower temperatures, increased rate coefficients were observed, indicating a fast heterogeneous reaction after the onset of binary homogeneous nucleation of acid hydrate clusters leading to particle formation, which was verified by light-scattering experiments. The heterogeneous loss of SO3 to the reactor walls has also been investigated under low pressure (1.1−12.5 Torr) laminar flow conditions. The loss rate is highly dependent on the humidity of the surface. In the presence of excess water the reactive sticking coefficient approaches unity and the wall loss rate is gas diffusion limited; under dry conditions it approaches zero, as expected. The atmospheric implications of the homogeneous and heterogeneous SO3−water reaction are discussed.
Published: 1997

25. High acetone concentrations throughout the 0-12 km altitude range over the tropical rainforest in Surinam

Author: Poschl, U., Williams, J., Hoor, P., Fischer, H., Pj, Crutzen, Warneke, C., Holzinger, R., Hansel, A., Jordan, A., Lindinger, W., Bert Scheeren, Wouter Peters, Lelieveld, J., and Isotope Research
Subjects: biomass burning, UPPER TROPOSPHERE, PHOTOCHEMISTRY, proton-transfer reaction mass spectrometry, acetone, VOLATILE ORGANIC-COMPOUNDS, tropical rainforest emissions, carbon monoxide, Surinam, acetonitrile, SULFUR-DIOXIDE, MASS-SPECTROMETER, CHEMISTRY, 2-propanol, HYDROGEN RADICALS, TRACE GAS, LOWER STRATOSPHERE, EMISSIONS
Abstract: Airborne measurements of acetone were performed over the tropical rainforest in Surinam (2 degrees -7 degrees N, 54 degrees -58 degrees W, 0-12 km altitude) during the LBA-CLAIRE campaign in March 1998, using a novel proton transfer reaction mass spectrometer (PTR-MS) that enables the on-line monitoring of volatile organic compounds (VOC) with a higher proton affinity than water. The measured acetone volume mixing ratios ranged from similar to0.1 nmol/mol up to similar to8 nmol/mol with an overall average of 2.6 nmol/mol and a standard deviation of 1.0 nmol/mol. The observed altitude profile and correlations with CO, acetonitrile, propane and wind direction are discussed with respect to potential acetone sources. No linear correlation between acetone and CO mixing ratios was observed, at variance with results of previous measurement campaigns. The mean acetone/CO ratio (0.022) was substantially higher than typical values found before. The abundance of acetone appears to be influenced, but not dominated, by biomass burning, thus suggesting large emissions of acetone and/or acetone precursors, such as possibly 2-propanol, from living plants or decaying litter in the rainforest.

26. Amorphous and crystalline aerosol particles interacting with water vapor: Conceptual framework and experimental evidence for restructuring, phase transitions and kinetic limitations

Author: Eugene Mikhailov, Vlasenko, S., Martin, St, Koop, T., and Poschl, U.
Subjects: lcsh:Chemistry, lcsh:QD1-999, lcsh:Physics, lcsh:QC1-999
Abstract: Interactions with water are crucial for the properties, transformation and climate effects of atmospheric aerosols. Here we present a conceptual framework for the interaction of amorphous aerosol particles with water vapor, outlining characteristic features and differences in comparison to crystalline particles. We used a hygroscopicity tandem differential mobility analyzer (H-TDMA) to characterize the hydration and dehydration of crystalline ammonium sulfate, amorphous oxalic acid and amorphous levoglucosan particles (diameter ~100 nm, relative humidity 5–95% at 298 K). The experimental data and accompanying Köhler model calculations provide new insights into particle microstructure, surface adsorption, bulk absorption, phase transitions and hygroscopic growth. The results of these and related investigations lead to the following conclusions: (1) Many organic substances, including carboxylic acids, carbohydrates and proteins, tend to form amorphous rather than crystalline phases upon drying of aqueous solution droplets. Depending on viscosity and microstructure, the amorphous phases can be classified as glasses, rubbers, gels or viscous liquids. (2) Amorphous organic substances tend to absorb water vapor and undergo gradual deliquescence and hygroscopic growth at lower relative humidity than their crystalline counterparts. (3) In the course of hydration and dehydration, certain organic substances can form rubber- or gel-like structures (supramolecular networks) and undergo transitions between swollen and collapsed network structures. (4) Organic gels or (semi-)solid amorphous shells (glassy, rubbery, ultra-viscous) with low molecular diffusivity can kinetically limit the uptake and release of water and may influence the hygroscopic growth and activation of aerosol particles as cloud condensation nuclei (CCN) and ice nuclei (IN). Moreover, (semi-)solid amorphous phases may influence the uptake of gaseous photo-oxidants and the chemical transformation and aging of atmospheric aerosols. (5) The shape and porosity of amorphous and crystalline particles formed upon dehydration of aqueous solution droplets depend on chemical composition and drying conditions. The apparent volume void fractions of particles with highly porous structures can range up to ~50% or more (xerogels, aerogels). (6) For efficient description of water uptake and phase transitions of aerosol particles, we propose not to limit the terms deliquescence and efflorescence to equilibrium phase transitions of crystalline substances. Instead we propose generalized definitions according to which amorphous and crystalline components can undergo gradual or prompt, partial or full deliquescence or efflorescence. We suggest that (semi-)solid amorphous phases may be important not only in the upper atmosphere as suggested in recent studies of glass formation at low temperatures. Depending on relative humidity, (semi-)solid phases and moisture-induced glass transitions may also play a role in gas-particle interactions at ambient temperatures in the lower atmosphere.

27. Synthesis and Spectroscopy of Halogenated Cyclopentasilanes

Author: Poschl, U. and Hassler, K.
Abstract: Nonahalocyclopentasilanes, HSi5X9, and octahalocyclopentasilanes, H2Si5X8 (X = Cl, Br, I), were prepared by dearylation of the corresponding phenylated cyclosilanes HSi5Ph9 and H2Si5Ph8 with gaseous hydrogen halides and catalytic amounts of aluminum halides (HX/AlX3) dissolved in benzene. The products were identified and characterized by IR and NMR spectroscopy (¹H and ²⁹Si, including Si−H and Si−Si coupling constants). The halogenation of trans-1,3-H2Si5Ph8 led to isomeric mixtures of cis-1,3-H2Si5X8 and trans-1,3-H2Si5X8 in equimolar amounts.
Published: 1996

28. Isoprene and its oxidation products methyl vinyl ketone, methacrolein, and isoprene related peroxides measured online over the tropical rain forest of Surinam in March 1998

Author: Williams, J., Lelieveld, J., Crutzen, P. J., Scheeren, H. A., Poschl, U., Warneke, C., Hoor, P., Lindinger, W., Hansel, A., Fischer, H., Jordan, A., and Holzinger, R.
Subjects: ATMOSPHERIC chemistry, FORESTS & forestry, GAS chromatography, HYDROXYL group, SIMULATION methods & models, SPECTROMETRY, STATISTICS, INSTRUMENTATION technicians, ORGANIC compounds, REACTIVITY (Chemistry)
Abstract: Airborne measurements of volatile organic compounds (VOC) were performed over the tropical rainforest in Surinam (0-12 km altitude, 2 deg. -7 deg. N, 54 deg. -58 deg. W) using the proton transfer reactionmass spectrometry (PTR-MS) technique, which allows online monitoringof compounds like isoprene, its oxidation products methyl vinyl ketone, methacrolein, tentatively identified hydroxy-isoprene-hydroperoxides, and several other organic compounds. Isoprene volume mixing ratios (VMR) varied from below the detection limit at the highest altitudes to about 7 nmol/mol in the planetary boundary layer shortly beforesunset. Correlations between isoprene and its product compounds weremade for different times of day and altitudes, with the isoprene-hydroperoxides showing the highest correlation. Model calculated mixing ratios of the isoprene oxidation products using a detailed hydrocarbon oxidation mechanism, as well as the intercomparison measurement with air samples collected during the flights in canisters and later analysed with a GC-FID, showed good agreement with the PTR-MS measurements, in particular at the higher mixing ratios. Low OH concentrations in the range of 1-3 x 105 molecules cm-3 averaged over 24 hours were calculated due to loss of OH and HO2 in the isoprene oxidation chain, thereby strongly enhancing the lifetime of gases in the forest boundary layer. [ABSTRACT FROM AUTHOR]
Published: 2001
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29. High acetone concentrations throughout the 0-12 km altitude range over the tropical rainforest in Surinam

Author: Crutzen, P. J., Peters, W., Lelieveld, J., Williams, J., Jordan, A., Warneke, C., Scheeren, H. A., Poschl, U., Holzinger, R., Hoor, P., Lindinger, W., Hansel, A., and Fischer, H.
Subjects: SPECTROMETRY, STATISTICS, METEOROLOGY, INSTRUMENTATION technicians, CARBON monoxide, ATMOSPHERIC chemistry, BIOMASS
Abstract: Airborne measurements of acetone were performed over the tropical rainforest in Surinam (2 deg. -7 deg. N, 54 deg. -58 deg. W, 0-12 km altitude) during the LBA-CLAIRE campaign in March 1998, using a novelproton transfer reaction mass spectrometer (PTR-MS) that enables theon-line monitoring of volatile organic compounds (VOC) with a higherproton affinity than water. The measured acetone volume mixing ratios ranged from ?0.1 nmol/mol up to ?8 nmol/mol with an overall averageof 2.6 nmol/mol and a standard deviation of 1.0 nmol/mol. The observed altitude profile and correlations with CO, acetonitrile, propane and wind direction are discussed with respect to potential acetone sources. No linear correlation between acetone and CO mixing ratios was observed, at variance with results of previous measurement campaigns.The mean acetone/CO ratio (0.022) was substantially higher than typical values found before. The abundance of acetone appears to be influenced, but not dominated, by biomass burning, thus suggesting large emissions of acetone and/or acetone precursors, such as possibly 2-propanol, from living plants or decaying litter in the rainforest. [ABSTRACT FROM AUTHOR]
Published: 2001
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30. An atmospheric chemistry interpretation of mass scans obtained from a proton transfer mass spectrometer flown over the tropical rainforest of Surinam

Author: Hansel, A., Crutzen, P. J., Warneke, C., Poschl, U., Holzinger, R., Lindinger, W., Williams, J., and Lelieveld, J.
Subjects: ATMOSPHERIC chemistry, FORESTS & forestry, INSTRUMENTATION technicians, SIMULATION methods & models, SPECTROMETRY, ORGANIC compounds, REACTIVITY (Chemistry)
Abstract: Data on a variety of organic gases are presented, obtained with a proton transfer mass spectrometer (PTR-MS) operated during the March 1998 LBA/CLAIRE airborne measurement campaign, between 60 and 12500 m over the rainforest in Surinam (2 deg. N-5 deg. N, 54 deg. W-57 deg. W). The instrument can detect molecules with a proton affinity greater than water, including alkenes, dialkenes, carbonyls, alcohols, and nitriles. Many such molecules are emitted from the rainforest (e.g., isoprene) or formed from the oxidation of primary emissions (e.g., methylvinylketone (MVK) and methacrolein (MACR)). From a comparison with modelled data; the variation with altitude; previously reported biogenic emissions and the time and location of the measurement, possible and probable identities for the significant masses encountered inthe range 33-140 amu have been deduced. The main observed protonatedmasses, postulated identities and observed average boundary layer mixing ratios over the rainforest were: 33 methanol (1.1 nmol/mol); 42 acetonitrile (190 pmol/mol); 43 multiple possibilities (5.9 nmol/mol), 45 acetaldehyde (1.7 nmol/mol), 47 formic acid (not quantified); 59acetone (2.9 nmol/mol), 61 acetic acid (not quantified), 63 dimethylsulphide (DMS) (289 pmol/mol), 69 isoprene (1.7 nmol/mol), 71 MVK + MACR (1.3 nmol/mol), 73 methyl ethyl ketone (1.8 nmol/mol), 75 hydroxyacetone (606 pmol/mol), 83 C5 isoprene hydroxy carbonyls C5H8O2, methyl furan, and cis 3-hexen-1-ol (732 pmol/mol), 87 C5 carbonyls and methacrylic acid, 95 possibly 2-vinyl furan (656 pmol/mol), 97 unknown (305 pmol/mol), 99 cis hexenal (512 pmol/mol) and 101 isoprene C5 hydroperoxides (575 pmol/mol). Some species agreed well with those derivedfrom an isoprene only photochemical model (e.g., mass 71 MVK + MACR)while others did not and were observed at higher than previously reported mixing ratios (e.g., mass 59 acetone, mass 63 DMS). Monoterpenes were [ABSTRACT FROM AUTHOR]
Published: 2001
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31. ChemInform Abstract: Synthesis, Reactivity, and Spectroscopy of Phenylated Cyclotetrasilanes and Cyclopentasilanes.

Author: POSCHL, U., SIEGL, H., and HASSLER, K.
Published: 1996
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32. EUREC4A

Author: B. Stevens, S. Bony, D. Farrell, F. Ament, A. Blyth, C. Fairall, J. Karstensen, P. K. Quinn, S. Speich, C. Acquistapace, F. Aemisegger, A. L. Albright, H. Bellenger, E. Bodenschatz, K.-A. Caesar, R. Chewitt-Lucas, G. de Boer, J. Delanoë, L. Denby, F. Ewald, B. Fildier, M. Forde, G. George, S. Gross, M. Hagen, A. Hausold, K. J. Heywood, L. Hirsch, M. Jacob, F. Jansen, S. Kinne, D. Klocke, T. Kölling, H. Konow, M. Lothon, W. Mohr, A. K. Naumann, L. Nuijens, L. Olivier, R. Pincus, M. Pöhlker, G. Reverdin, G. Roberts, S. Schnitt, H. Schulz, A. P. Siebesma, C. C. Stephan, P. Sullivan, L. Touzé-Peiffer, J. Vial, R. Vogel, P. Zuidema, N. Alexander, L. Alves, S. Arixi, H. Asmath, G. Bagheri, K. Baier, A. Bailey, D. Baranowski, A. Baron, S. Barrau, P. A. Barrett, F. Batier, A. Behrendt, A. Bendinger, F. Beucher, S. Bigorre, E. Blades, P. Blossey, O. Bock, S. Böing, P. Bosser, D. Bourras, P. Bouruet-Aubertot, K. Bower, P. Branellec, H. Branger, M. Brennek, A. Brewer, P.-E. Brilouet, B. Brügmann, S. A. Buehler, E. Burke, R. Burton, R. Calmer, J.-C. Canonici, X. Carton, G. Cato Jr., J. A. Charles, P. Chazette, Y. Chen, M. T. Chilinski, T. Choularton, P. Chuang, S. Clarke, H. Coe, C. Cornet, P. Coutris, F. Couvreux, S. Crewell, T. Cronin, Z. Cui, Y. Cuypers, A. Daley, G. M. Damerell, T. Dauhut, H. Deneke, J.-P. Desbios, S. Dörner, S. Donner, V. Douet, K. Drushka, M. Dütsch, A. Ehrlich, K. Emanuel, A. Emmanouilidis, J.-C. Etienne, S. Etienne-Leblanc, G. Faure, G. Feingold, L. Ferrero, A. Fix, C. Flamant, P. J. Flatau, G. R. Foltz, L. Forster, I. Furtuna, A. Gadian, J. Galewsky, M. Gallagher, P. Gallimore, C. Gaston, C. Gentemann, N. Geyskens, A. Giez, J. Gollop, I. Gouirand, C. Gourbeyre, D. de Graaf, G. E. de Groot, R. Grosz, J. Güttler, M. Gutleben, K. Hall, G. Harris, K. C. Helfer, D. Henze, C. Herbert, B. Holanda, A. Ibanez-Landeta, J. Intrieri, S. Iyer, F. Julien, H. Kalesse, J. Kazil, A. Kellman, A. T. Kidane, U. Kirchner, M. Klingebiel, M. Körner, L. A. Kremper, J. Kretzschmar, O. Krüger, W. Kumala, A. Kurz, P. L'Hégaret, M. Labaste, T. Lachlan-Cope, A. Laing, P. Landschützer, T. Lang, D. Lange, I. Lange, C. Laplace, G. Lavik, R. Laxenaire, C. Le Bihan, M. Leandro, N. Lefevre, M. Lena, D. Lenschow, Q. Li, G. Lloyd, S. Los, N. Losi, O. Lovell, C. Luneau, P. Makuch, S. Malinowski, G. Manta, E. Marinou, N. Marsden, S. Masson, N. Maury, B. Mayer, M. Mayers-Als, C. Mazel, W. McGeary, J. C. McWilliams, M. Mech, M. Mehlmann, A. N. Meroni, T. Mieslinger, A. Minikin, P. Minnett, G. Möller, Y. Morfa Avalos, C. Muller, I. Musat, A. Napoli, A. Neuberger, C. Noisel, D. Noone, F. Nordsiek, J. L. Nowak, L. Oswald, D. J. Parker, C. Peck, R. Person, M. Philippi, A. Plueddemann, C. Pöhlker, V. Pörtge, U. Pöschl, L. Pologne, M. Posyniak, M. Prange, E. Quiñones Meléndez, J. Radtke, K. Ramage, J. Reimann, L. Renault, K. Reus, A. Reyes, J. Ribbe, M. Ringel, M. Ritschel, C. B. Rocha, N. Rochetin, J. Röttenbacher, C. Rollo, H. Royer, P. Sadoulet, L. Saffin, S. Sandiford, I. Sandu, M. Schäfer, V. Schemann, I. Schirmacher, O. Schlenczek, J. Schmidt, M. Schröder, A. Schwarzenboeck, A. Sealy, C. J. Senff, I. Serikov, S. Shohan, E. Siddle, A. Smirnov, F. Späth, B. Spooner, M. K. Stolla, W. Szkółka, S. P. de Szoeke, S. Tarot, E. Tetoni, E. Thompson, J. Thomson, L. Tomassini, J. Totems, A. A. Ubele, L. Villiger, J. von Arx, T. Wagner, A. Walther, B. Webber, M. Wendisch, S. Whitehall, A. Wiltshire, A. A. Wing, M. Wirth, J. Wiskandt, K. Wolf, L. Worbes, E. Wright, V. Wulfmeyer, S. Young, C. Zhang, D. Zhang, F. Ziemen, T. Zinner, M. Zöger, Max Planck Institute for Meteorology (MPI-M), Max-Planck-Gesellschaft, Laboratoire de Météorologie Dynamique (UMR 8539) (LMD), Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-École des Ponts ParisTech (ENPC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Caribbean Institute for Meteorology and Hydrology (CIMH), Meteorological Institute [Hamburg], University of Hamburg, National Centre for Atmospheric Science [Leeds] (NCAS), Natural Environment Research Council (NERC), NOAA Earth System Research Laboratory (ESRL), National Oceanic and Atmospheric Administration (NOAA), Helmholtz Centre for Ocean Research [Kiel] (GEOMAR), NOAA Pacific Marine Environmental Laboratory [Seattle] (PMEL), Institute for Geophysics and Meteorology [Köln] (IGM), University of Cologne, Institute for Atmospheric and Climate Science [Zürich] (IAC), Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology [Zürich] (ETH Zürich), Max Planck Institute for Dynamics and Self-Organization (MPIDS), NOAA Physical Sciences Laboratory (PSL), SPACE - LATMOS, Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), University of Leeds, Deutsches Zentrum für Luft- und Raumfahrt (DLR), Deutscher Wetterdienst [Offenbach] (DWD), Ludwig-Maximilians-Universität München (LMU), Laboratoire d'aérologie (LAERO), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Universität Hamburg (UHH), Max Planck Institute for Marine Microbiology, Delft University of Technology (TU Delft), Processus et interactions de fine échelle océanique (PROTEO), Laboratoire d'Océanographie et du Climat : Expérimentations et Approches Numériques (LOCEAN), Muséum national d'Histoire naturelle (MNHN)-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité)-Muséum national d'Histoire naturelle (MNHN)-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado [Boulder]-National Oceanic and Atmospheric Administration (NOAA), Max-Planck-Institut für Chemie (MPIC), Centre national de recherches météorologiques (CNRM), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Scripps Institution of Oceanography (SIO - UC San Diego), University of California [San Diego] (UC San Diego), University of California (UC)-University of California (UC), Universität zu Köln = University of Cologne, National Center for Atmospheric Research [Boulder] (NCAR), Hydrometeorological Service [Georgetown], Ministry of Agriculture [Guyana], Institute of Marine Affairs (IMA), Institute of Geophysics [Warsaw], Polska Akademia Nauk = Polish Academy of Sciences (PAN), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), United Kingdom Met Office [Exeter], Institute of Physics and Meteorology [Stuttgart] (IPM), University of Hohenheim, Woods Hole Oceanographic Institution (WHOI), Queen Elizabeth Hospital [Bridgetown, St. Michael, Barbados] (QEH), Department of Atmospheric Sciences [Seattle], University of Washington [Seattle], École nationale des sciences géographiques (ENSG), Institut National de l'Information Géographique et Forestière [IGN] (IGN)-Université Gustave Eiffel, Institut de Physique du Globe de Paris (IPGP (UMR_7154)), Institut national des sciences de l'Univers (INSU - CNRS)-Université de La Réunion (UR)-Institut de Physique du Globe de Paris (IPG Paris)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), Equipe Marine Mapping & Metrology (Lab-STICC_M3), Laboratoire des sciences et techniques de l'information, de la communication et de la connaissance (Lab-STICC), École Nationale d'Ingénieurs de Brest (ENIB)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Institut Mines-Télécom [Paris] (IMT)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL)-IMT Atlantique (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT)-École Nationale d'Ingénieurs de Brest (ENIB)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Institut Mines-Télécom [Paris] (IMT)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL)-IMT Atlantique (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT), École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne), University of Manchester [Manchester], Institut de Recherche sur les Phénomènes Hors Equilibre (IRPHE), Aix Marseille Université (AMU)-École Centrale de Marseille (ECM)-Centre National de la Recherche Scientifique (CNRS), University of Warsaw (UW), NOAA Chemical Sciences Laboratory (CSL), Max-Planck-Institut für Meteorologie (MPI-M), St. Christopher Air and Sea Port (SCASPA), Service des Avions Français Instrumentés pour la Recherche en Environnement (SAFIRE), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France, Laboratoire d'Océanographie Physique et Spatiale (LOPS), Institut de Recherche pour le Développement (IRD)-Institut Français de Recherche pour l'Exploitation de la Mer (IFREMER)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS), Saint Vincent and the Grenadines Meteorological Services, Grenada Meteorological Services, Chimie Atmosphérique Expérimentale (CAE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université Paris Cité (UPCité), University of California [Santa Cruz] (UC Santa Cruz), University of California (UC), Cayman Islands National Weather Service, Laboratoire d’Optique Atmosphérique - UMR 8518 (LOA), Institut national des sciences de l'Univers (INSU - CNRS)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Météorologie Physique (LaMP), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Clermont Auvergne (UCA), Massachusetts Institute of Technology (MIT), Centre for Ocean and Atmospheric Sciences [Norwich] (COAS), School of Environmental Sciences [Norwich], University of East Anglia [Norwich] (UEA)-University of East Anglia [Norwich] (UEA), College of Earth, Ocean and Atmospheric Sciences [Corvallis] (CEOAS), Oregon State University (OSU), Leibniz Institute for Tropospheric Research (TROPOS), Department of Meteorology and Geophysics [Vienna], Universität Wien, Leipziger Institut für Meteorologie (LIM), Universität Leipzig, Meteorological Department (St. Maarten), Università degli Studi di Milano-Bicocca = University of Milano-Bicocca (UNIMIB), TROPO - LATMOS, NOAA Atlantic Oceanographic and Meteorological Laboratory (AOML), Department of Earth and Planetary Sciences [Albuquerque] (EPS), The University of New Mexico [Albuquerque], University of Miami [Coral Gables], Farallon Institute, Division technique INSU/SDU (DTI), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Deutsches Zentrum für Luft- und Raumfahrt [Oberpfaffenhofen-Wessling] (DLR), Regional Security System [Barbados], Max Planck Institute for Chemistry (MPIC), Applied Physics Laboratory [Seattle] (APL-UW), Barbados Coast Guard, Développement Instrumental et Techniques Marines (DITM), Institut Français de Recherche pour l'Exploitation de la Mer (IFREMER), Austral, Boréal et Carbone (ABC), Institut Pythéas (OSU PYTHEAS), Institut de Recherche pour le Développement (IRD)-Aix Marseille Université (AMU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut National de Recherche pour l’Agriculture, l’Alimentation et l’Environnement (INRAE), Nucleus for European Modeling of the Ocean (NEMO R&D ), Laboratoire d'études en Géophysique et océanographie spatiales (LEGOS), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), European Project: 694768,EUREC4A, European Project: 820829,CONSTRAIN H2020, European Project: 741120,COMPASS, European Project: 817578,TRIATLAS(2019), École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris), Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS), Laboratoire d'aérologie (LA), Centre National de la Recherche Scientifique (CNRS)-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées, Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Muséum national d'Histoire naturelle (MNHN)-Institut de Recherche pour le Développement (IRD)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP)-École normale supérieure - Paris (ENS Paris), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP)-Sorbonne Université (SU)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Muséum national d'Histoire naturelle (MNHN)-Institut de Recherche pour le Développement (IRD)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Institut national des sciences de l'Univers (INSU - CNRS)-Météo France-Centre National de la Recherche Scientifique (CNRS), Scripps Institution of Oceanography (SIO), University of California-University of California, Universität zu Köln, Queen Elizabeth Hospital [Bridgetown, St. Michael, Barbados], Institut de Physique du Globe de Paris (IPGP), Institut national des sciences de l'Univers (INSU - CNRS)-IPG PARIS-Université de La Réunion (UR)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Institut Mines-Télécom [Paris] (IMT)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT)-École Nationale d'Ingénieurs de Brest (ENIB)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP), Université Fédérale Toulouse Midi-Pyrénées-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP)-Institut de Recherche pour le Développement (IRD)-Muséum national d'Histoire naturelle (MNHN)-Centre National de la Recherche Scientifique (CNRS)-Sorbonne Université (SU)-Institut Pierre-Simon-Laplace (IPSL (FR_636)), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-École polytechnique (X)-Centre National d'Études Spatiales [Toulouse] (CNES)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Paris (UP)-Institut de Recherche pour le Développement (IRD)-Muséum national d'Histoire naturelle (MNHN)-Centre National de la Recherche Scientifique (CNRS)-Sorbonne Université (SU), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), École Nationale d'Ingénieurs de Brest (ENIB)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Institut Mines-Télécom [Paris] (IMT)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique), Institut Mines-Télécom [Paris] (IMT)-École Nationale d'Ingénieurs de Brest (ENIB)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Institut Mines-Télécom [Paris] (IMT)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique), Centre National de la Recherche Scientifique (CNRS)-Aix Marseille Université (AMU)-École Centrale de Marseille (ECM), Centre National de la Recherche Scientifique (CNRS)-Météo France-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES), Institut de Recherche pour le Développement (IRD)-Institut Français de Recherche pour l'Exploitation de la Mer (IFREMER)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), University of California [Santa Cruz] (UCSC), University of California, Universität Leipzig [Leipzig], Università degli Studi di Milano-Bicocca [Milano] (UNIMIB), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS), Stevens, B, Bony, S, Farrell, D, Ament, F, Blyth, A, Fairall, C, Karstensen, J, Quinn, P, Speich, S, Acquistapace, C, Aemisegger, F, Albright, A, Bellenger, H, Bodenschatz, E, Caesar, K, Chewitt-Lucas, R, De Boer, G, Delanoe, J, Denby, L, Ewald, F, Fildier, B, Forde, M, George, G, Gross, S, Hagen, M, Hausold, A, Heywood, K, Hirsch, L, Jacob, M, Jansen, F, Kinne, S, Klocke, D, Kolling, T, Konow, H, Lothon, M, Mohr, W, Naumann, A, Nuijens, L, Olivier, L, Pincus, R, Pohlker, M, Reverdin, G, Roberts, G, Schnitt, S, Schulz, H, Pier Siebesma, A, Stephan, C, Sullivan, P, Touze-Peiffer, L, Vial, J, Vogel, R, Zuidema, P, Alexander, N, Alves, L, Arixi, S, Asmath, H, Bagheri, G, Baier, K, Bailey, A, Baranowski, D, Baron, A, Barrau, S, Barrett, P, Batier, F, Behrendt, A, Bendinger, A, Beucher, F, Bigorre, S, Blades, E, Blossey, P, Bock, O, Boing, S, Bosser, P, Bourras, D, Bouruet-Aubertot, P, Bower, K, Branellec, P, Branger, H, Brennek, M, Brewer, A, Brilouet, P, Brugmann, B, Buehler, S, Burke, E, Burton, R, Calmer, R, Canonici, J, Carton, X, Cato, G, Charles, J, Chazette, P, Chen, Y, Chilinski, M, Choularton, T, Chuang, P, Clarke, S, Coe, H, Cornet, C, Coutris, P, Couvreux, F, Crewell, S, Cronin, T, Cui, Z, Cuypers, Y, Daley, A, Damerell, G, Dauhut, T, Deneke, H, Desbios, J, Dorner, S, Donner, S, Douet, V, Drushka, K, Dutsch, M, Ehrlich, A, Emanuel, K, Emmanouilidis, A, Etienne, J, Etienne-Leblanc, S, Faure, G, Feingold, G, Ferrero, L, Fix, A, Flamant, C, Flatau, P, Foltz, G, Forster, L, Furtuna, I, Gadian, A, Galewsky, J, Gallagher, M, Gallimore, P, Gaston, C, Gentemann, C, Geyskens, N, Giez, A, Gollop, J, Gouirand, I, Gourbeyre, C, De Graaf, D, De Groot, G, Grosz, R, Guttler, J, Gutleben, M, Hall, K, Harris, G, Helfer, K, Henze, D, Herbert, C, Holanda, B, Ibanez-Landeta, A, Intrieri, J, Iyer, S, Julien, F, Kalesse, H, Kazil, J, Kellman, A, Kidane, A, Kirchner, U, Klingebiel, M, Korner, M, Kremper, L, Kretzschmar, J, Kruger, O, Kumala, W, Kurz, A, L'Hegaret, P, Labaste, M, Lachlan-Cope, T, Laing, A, Landschutzer, P, Lang, T, Lange, D, Lange, I, Laplace, C, Lavik, G, Laxenaire, R, Lebihan, C, Leandro, M, Lefevre, N, Lena, M, Lenschow, D, Li, Q, Lloyd, G, Los, S, Losi, N, Lovell, O, Luneau, C, Makuch, P, Malinowski, S, Manta, G, Marinou, E, Marsden, N, Masson, S, Maury, N, Mayer, B, Mayers-Als, M, Mazel, C, Mcgeary, W, Mcwilliams, J, Mech, M, Mehlmann, M, Meroni, A, Mieslinger, T, Minikin, A, Minnett, P, Moller, G, Avalos, Y, Muller, C, Musat, I, Napoli, A, Neuberger, A, Noisel, C, Noone, D, Nordsiek, F, Nowak, J, Oswald, L, Parker, D, Peck, C, Person, R, Philippi, M, Plueddemann, A, Pohlker, C, Portge, V, Poschl, U, Pologne, L, Posyniak, M, Prange, M, Melendez, E, Radtke, J, Ramage, K, Reimann, J, Renault, L, Reus, K, Reyes, A, Ribbe, J, Ringel, M, Ritschel, M, Rocha, C, Rochetin, N, Rottenbacher, J, Rollo, C, Royer, H, Sadoulet, P, Saffin, L, Sandiford, S, Sandu, I, Schafer, M, Schemann, V, Schirmacher, I, Schlenczek, O, Schmidt, J, Schroder, M, Schwarzenboeck, A, Sealy, A, Senff, C, Serikov, I, Shohan, S, Siddle, E, Smirnov, A, Spath, F, Spooner, B, Katharina Stolla, M, Szkolka, W, De Szoeke, S, Tarot, S, Tetoni, E, Thompson, E, Thomson, J, Tomassini, L, Totems, J, Ubele, A, Villiger, L, Von Arx, J, Wagner, T, Walther, A, Webber, B, Wendisch, M, Whitehall, S, Wiltshire, A, Wing, A, Wirth, M, Wiskandt, J, Wolf, K, Worbes, L, Wright, E, Wulfmeyer, V, Young, S, Zhang, C, Zhang, D, Ziemen, F, Zinner, T, Zoger, M, and Institut Mines-Télécom [Paris] (IMT)-École Nationale d'Ingénieurs de Brest (ENIB)-École Nationale Supérieure de Techniques Avancées Bretagne (ENSTA Bretagne)-Université de Bretagne Sud (UBS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Université Bretagne Loire (UBL)-Institut Mines-Télécom [Paris] (IMT)-IMT Atlantique Bretagne-Pays de la Loire (IMT Atlantique)
Subjects: [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere, QE1-996.5, [SDU.STU.GP]Sciences of the Universe [physics]/Earth Sciences/Geophysics [physics.geo-ph], Cloud Feedback, Geology, [SDU.STU.ME]Sciences of the Universe [physics]/Earth Sciences/Meteorology, Environmental sciences, Atmospheric circulation, Trade-wind cumulus, Field campaign, Aerosol, clouds, sea, sub-tropic, CHIM/12 - CHIMICA DELL'AMBIENTE E DEI BENI CULTURALI, [SDE]Environmental Sciences, GE1-350, Shallow convection, [SDU.OTHER]Sciences of the Universe [physics]/Other, ComputingMilieux_MISCELLANEOUS
Abstract: The science guiding the EUREC4A campaign and its measurements is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. Through its ability to characterize processes operating across a wide range of scales, EUREC4A marked a turning point in our ability to observationally study factors influencing clouds in the trades, how they will respond to warming, and their link to other components of the earth system, such as upper-ocean processes or the life cycle of particulate matter. This characterization was made possible by thousands (2500) of sondes distributed to measure circulations on meso- (200 km) and larger (500 km) scales, roughly 400 h of flight time by four heavily instrumented research aircraft; four global-class research vessels; an advanced ground-based cloud observatory; scores of autonomous observing platforms operating in the upper ocean (nearly 10 000 profiles), lower atmosphere (continuous profiling), and along the air–sea interface; a network of water stable isotopologue measurements; targeted tasking of satellite remote sensing; and modeling with a new generation of weather and climate models. In addition to providing an outline of the novel measurements and their composition into a unified and coordinated campaign, the six distinct scientific facets that EUREC4A explored – from North Brazil Current rings to turbulence-induced clustering of cloud droplets and its influence on warm-rain formation – are presented along with an overview of EUREC4A's outreach activities, environmental impact, and guidelines for scientific practice. Track data for all platforms are standardized and accessible at https://doi.org/10.25326/165 (Stevens, 2021), and a film documenting the campaign is provided as a video supplement.
Published: 2021

33. Comparison of nitrotyrosine antibodies and development of immunoassays for the detection of nitrated proteins.

Author: Franze T, Weller MG, Niessner R, and Poschl U
Subjects: Animals, Antibodies, Antibodies, Monoclonal, Goats, Immunoassay methods, Mice, Rabbits, Sheep, Tyrosine immunology, Air Pollutants analysis, Environmental Monitoring methods, Tyrosine analogs & derivatives
Abstract: Three monoclonal antibodies (mAb) and three polyclonal antibodies (pAb) have been characterized and compared with respect to their cross-reactivities and affinities for 3-nitrotyrosine, eight aromatic compounds with similar chemical structures, a peptide containing a single nitrotyrosine residue, and fourteen nitrated protein standards (bovine serum albumin, BSA) containing different numbers of nitrotyrosine residues per protein molecule (0.2 to 16.8). In indirect competitive immunoassays, mAb Alexis 39B6 exhibited the highest affinity for free 3-nitrotyrosine (10(6) L mol(-1)), while the pAb Oxis 24312 from sheep exhibited the highest affinities for nitrated proteins (up to 10(8) L mol(-1)). The apparent affinities determined in the indirect competitive assays were inversely correlated with the limits of detection (LOD) determined in one-sided immunoassays. With the sheep pAb minimum LOD on the order of 10 pmol L(-1) were achieved for highly nitrated proteins, corresponding to effective LOD on the order of 100 pmol L(-1) for nitrotyrosine residues. In the one-sided assays, however, the LOD for nitrated proteins increased proportionally with increasing background concentrations of native proteins in the investigated samples. Sandwich immunoassays combining pAb and mAb for selective enrichment and detection of nitrated proteins allowed to eliminate this native protein matrix effect and to achieve LOD on the order of 300 pmol L(-1) for highly nitrated proteins independent of native protein background concentrations.
Published: 2004
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34. In-source fragmentation of partially oxidized mono- and polycyclic aromatic hydrocarbons in atmospheric pressure chemical ionization mass spectrometry coupled to liquid chromatography

Author: Letzel T, Poschl U, Rosenberg E, Grasserbauer M, and Niessner R
Abstract: Partially oxidized derivatives of polycyclic aromatic hydrocarbons (PAHs) are known to be important environmental pollutants. For the identification of these substances in complex mixtures, e.g. atmospheric aerosol samples, liquid chromatography/mass spectrometry with atmospheric pressure chemical ionization (LC/APCI-MS) has been found to be a suitable analytical technique. In this study 31 derivatives of mono- and polycyclic aromatic hydrocarbons with up to five condensed aromatic rings carrying different functional groups (carboxyl, dicarboxylic anhydride, lactone, hydroxyl, and carbonyl) were characterized by LC/APCI-MS. Each substance was measured in positive and negative ion detection mode at four different fragmentor voltages (90 to 190 V). For the first time, the results show that characteristic and well-interpretable fragmentation patterns can be obtained for these classes of compounds by in-source collision-induced dissociation in a single quadrupole LC/APCI-MS system. For each class of compounds typical spectral features and optimum measurement conditions are reported, and fragmentation pathways are proposed. The study demonstrates the applicability of LC/APCI-MS for the determination of most of the investigated compounds at trace levels, and it provides a database for the identification of unknown partially oxidized aromatic hydrocarbons. Copyright 1999 John Wiley & Sons, Ltd.
Published: 1999
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34. In-source fragmentation of partially oxidized mono- and polycyclic aromatic hydrocarbons in atmospheric pressure chemical ionization mass spectrometry coupled to liquid chromatography

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