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A measurement of the $^{50}\mathrm{Ti}(d,p)^{51}\mathrm{Ti}$ reaction at 16 MeV was performed using the Super Enge Split-Pole Spectrograph to measure the magnitude of the $N=32$ subshell gap in Ti. Seven states were observed that had not been observed in previous $(d,p)$ measurements, and the $L$ transfer values for six previously measured states were either changed or measured for the first time. The results were used to determine single neutron energies for the ${p}_{3/2}$, ${p}_{1/2}$, and ${f}_{5/2}$ orbitals. The resulting single neutron energies in $^{51}\mathrm{Ti}$ confirm the existence of the $N=32$ gap in Ti. These single neutron energies and those from previous measurements in $^{49}\mathrm{Ca}$, $^{53}\mathrm{Cr}$, and $^{55}\mathrm{Fe}$ are compared to values from a covariant density functional theory calculation.

The predominant branch in the $\ensuremath{\beta}$ decay of $^{34}\mathrm{Ar}$ is the superallowed ${0}^{+}\ensuremath{\rightarrow}\phantom{\rule{0.16em}{0ex}}{0}^{+}$ transition to the ground state of $^{34}\mathrm{Cl}$. To determine its important branching ratio one must first establish the ratios for the competing Gamow-Teller branches based on the measured intensities of $\ensuremath{\gamma}$ rays subsequently emitted from the excited states they populate in $^{34}\mathrm{Cl}$. The strongest of these branches populates the ${1}^{+}$ state at 666 keV in $^{34}\mathrm{Cl}$, which has three possible $\ensuremath{\gamma}$-decay paths. We report here a measurement of the decay of this state, which we populated via resonant proton capture in the reaction $^{33}\mathrm{S}$($p,\ensuremath{\gamma}$)$^{34}\mathrm{Cl}$. We find that the intensity of the 519-keV $\ensuremath{\gamma}$-ray path is 1.46(19)% relative to that of the 666-keV path. This result is critical to new precise measurements of the superallowed decay of $^{34}\mathrm{Ar}$.

Energy production in Type Ia x-ray bursts depends on a number of nuclear reactions that become efficient in a hot environment (up to 2 GK). Model sensitivity studies have been performed in an effort to better identify the reactions that have the largest effect, but these efforts are hampered by the high level of complexity of the astrophysical model and large nuclear physics uncertainties. In a recent study, the $^{24}\mathrm{Mg}(\ensuremath{\alpha},p)^{27}\mathrm{Al}$ reaction was found to significantly affect the energy generation in x-ray bursts. This manuscript reports the first study of the $^{24}\mathrm{Mg}(\ensuremath{\alpha},{p}_{1,2}\ensuremath{\gamma})^{27}\mathrm{Al}$ reaction at energies relevant for x-ray bursts. The branches to the $^{27}\mathrm{Al}$ excited states increase to a small degree the estimates of the total astrophysical $^{24}\mathrm{Mg}(\ensuremath{\alpha},p)^{27}\mathrm{Al}$ reaction rate.

Precise antineutrino measurements are very sensitive to proper background characterization. We present an improved measurement of the $^{13}\mathrm{C}(\ensuremath{\alpha},n)^{16}\mathrm{O}$ reaction cross section which constitutes significant background for large $\overline{\ensuremath{\nu}}$ detectors. We greatly improve the precision and accuracy by utilizing a setup that is sensitive to the neutron energies while making measurements of the excited state transitions via secondary $\ensuremath{\gamma}$-ray detection. Our results shows a 54% reduction in the background contributions from the $^{16}\mathrm{O}({3}^{\ensuremath{-}},6.13\text{ }\mathrm{MeV})$ state used in the KamLAND analysis.

Carbon and oxygen burning reactions, in particular, $^{12}\mathrm{C}+^{12}\mathrm{C}$ fusion, are important for the understanding and interpretation of the late phases of stellar evolution as well as the ignition and nucleosynthesis in cataclysmic binary systems such as type Ia supernovae and x-ray superbursts. A new measurement of this reaction has been performed at the University of Notre Dame using particle-$\ensuremath{\gamma}$ coincidence techniques with SAND (a silicon detector array) at the high-intensity 5U Pelletron accelerator. New results for $^{12}\mathrm{C}+^{12}\mathrm{C}$ fusion at low energies relevant to nuclear astrophysics are reported. They show strong disagreement with a recent measurement using the indirect Trojan Horse method. The impact on the carbon burning process under astrophysical scenarios will be discussed.

Nucleosynthesis in the first generation of massive stars offers a unique setting to explore the creation of the first heavier nuclei in an environment free of impurities from earlier stellar generations. In later generations of massive stars, hydrogen burning occurs predominantly through the CNO cycles, but without the carbon, nitrogen, and oxygen to catalyze the reaction sequence, first stars would have to rely on the inefficient $pp$ chains for their energy production. Observations of second and third generation stars show pronounced abundances of carbon and oxygen isotopes, which suggests a rapid conversion of the primordial abundances to heavier elements. While the triple-alpha-process primarily facilitates this conversion, there are alternative reaction sequences, such as $^{2}\mathrm{H}(\ensuremath{\alpha},\ensuremath{\gamma})^{6}\mathrm{Li}(\ensuremath{\alpha},\ensuremath{\gamma})^{10}\mathrm{B}(\ensuremath{\alpha},n)^{13}\mathrm{N}$, that may play a significant role. To study such alternate reaction pathways for production of carbon and heavier nuclei, a number of new measurements are needed. In this work, new measurements are reported for the $^{10}\mathrm{B}(\ensuremath{\alpha},n)^{13}\mathrm{N}$ reaction, extending the cross section down to 575 keV incident $\ensuremath{\alpha}$-particle energy. The measurements were made using a state-of-the-art deuterated liquid scintillator and a spectrum unfolding technique. An $R$-matrix analysis was performed in order to facilitate a comparison of the underlying nuclear structure with the reaction measurements. An unexpected upturn is observed in the low-energy $S$ factor that indicates the presence of a new low-energy resonance. A revised reaction rate is determined that takes into account the present data as well as other previous measurements from the literature that were previously neglected.

A high-count-rate ionization chamber design with position-sensitivity has been developed and deployed at several accelerator facilities. Counting rates of ≥ 500 kHz with good Z -separation (up to 5% energy resolution) for particle identification have been demonstrated in a series of commissioning experiments. A position-sensitive capability, with a resolution of 3 mm, has been implemented for the first time to record position information and suppress pileup. The design and performance of the detectors are described.

An active target detector array, ANASEN, has been developed for nuclear reaction studies with rare isotope beams at low energies. It aims at measurements of the excitation functions for proton and α - particle elastic and inelastic scattering and direct measurements of ( α , p) reactions with exotic nuclei in inverse kinematics. ANASEN is composed of three types of charged particle detectors. The length of the active area is 340 mm and the total covered area is 1300 cm 2 (almost 3 π steradian solid angle coverage) providing high efficiency for experiments with low intensity radioactive beams. A mix of 78 conventional electronics channels (for Proportional Counter and CsI-detectors) and 480 dedicated high-density ASICs electronics channels for the silicon detector are used for readout.

A new precision half-life measurement of $^{29}\mathrm{P}$ was conducted using the TwinSol $\ensuremath{\beta}$-counting station at the University of Notre Dame Nuclear Science Laboratory. The resulting value of ${t}_{1/2}^{\mathrm{new}}=4.1055(44)\phantom{\rule{0.28em}{0ex}}\mathrm{s}$ is the most precise $^{29}\mathrm{P}$ half-life measurement to date. Utilizing this measurement and reevaluating the world data leads to a new world average of ${t}_{1/2}^{\mathrm{world}}=4.1031(58)\phantom{\rule{0.28em}{0ex}}\mathrm{s}$, which improves the Birge ratio from 3.11 to 1.45 and is 2.3 times more precise than the previous world value. The new Cabibbo-Kobayashi-Maskawa matrix element ${V}_{\mathrm{ud}}$ for $^{29}\mathrm{P}$ shifts closer into agreement with the superallowed pure Fermi value. The uncertainty in the mixed transition value of ${V}_{\mathrm{ud}}$, however, is still dominated by the Fermi to Gamow-Teller mixing ratio $\ensuremath{\rho}$. Using the new world half-life and assuming the validity of the standard model, a new predicted value for $\ensuremath{\rho}$ and its associated correlation parameters have been evaluated in order to guide future determination of $\ensuremath{\rho}$.

Carbon and oxygen burning reactions, in particular, $^{12}$C+$^{12}$C fusion, are important for the understanding and interpretation of the late phases of stellar evolution as well as the ignition and nucleosynthesis in cataclysmic binary systems such as type Ia supernovae and x-ray superbursts. A new measurement of this reaction has been performed at the University of Notre Dame using particle-$\gamma$ coincidence techniques with SAND (a silicon detector array) at the high-intensity 5U Pelletron accelerator. New results for $^{12}$C+$^{12}$C fusion at low energies relevant to nuclear astrophysics are reported. They show strong disagreement with a recent measurement using the indirect Trojan Horse method. The impact on the carbon burning process under astrophysical scenarios will be discussed., Comment: accepted for publication in Phys. Rev. Lett

Precise antineutrino measurements are very sensitive to proper background characterization. We present an improved measurement of the ^{13}C(α,n)^{16}O reaction cross section which constitutes significant background for large ν[over ¯] detectors. We greatly improve the precision and accuracy by utilizing a setup that is sensitive to the neutron energies while making measurements of the excited state transitions via secondary γ-ray detection. Our results shows a 54% reduction in the background contributions from the ^{16}O(3^{-},6.13 MeV) state used in the KamLAND analysis.

The National Ignition Facility (NIF) provides the opportunity to study nuclear reactions under controlled conditions at high temperatures and pressures at a level never before achieved. However, the timescale of the deuterium-tritium (DT) implosion is only a few nanoseconds, making data collection and diagnostics very challenging. One method that has been proposed for obtaining additional information about the conditions of the implosion is to activate a dopant material using the $\ensuremath{\alpha}$ particles produced from the DT fuel as a diagnostic. The yield of the activated material can give a measure of the mixing that occurs in the capsule. One of the reactions that has been proposed is $^{10}\mathrm{B}(\ensuremath{\alpha},n)\phantom{\rule{0.16em}{0ex}}^{13}\mathrm{N}$ as it produces a radioactive reactant product with a convenient half-life of $\ensuremath{\approx}10\phantom{\rule{0.16em}{0ex}}\mathrm{min}$. Although this reaction has several advantages for the application at hand, it has not seen much study in the present literature, resulting in large uncertainties in the cross section. Furthermore, for the current application, the cross section must be well characterized. With this motivation, the $^{10}\mathrm{B}(\ensuremath{\alpha},n)\phantom{\rule{0.16em}{0ex}}^{13}\mathrm{N}$ cross section has been remeasured for $2.2l{E}_{\ensuremath{\alpha}}l4.9\phantom{\rule{0.28em}{0ex}}\mathrm{MeV}$ with the angle-integrated ground-state cross section reported for the first time. The present results, combined with previous measurements, allow for a determination of the cross section to a significantly higher degree of accuracy and precision than obtained previously and are shown to be consistent with thick-target measurements. Preliminary calculations are performed to test the feasibility of this reaction as a diagnostic for a NIF implosion.

The Silicon Array for Branching Ratio Experiments (SABRE) has been developed for use to study reactions of interest to nuclear structure and astrophysics . The array has been incorporated into the Super Enge Split-Pole Spectrograph (SE-SPS) experimental setup at Florida State University’s John D. Fox accelerator laboratory to detect charged-particle decays in coincidence with reaction products detected by the SE-SPS focal plane detector. Its construction and electronics processing are discussed, as well as the commissioning data used to validate its performance.

The performance of the maximum likelihood expectation maximization method for unfolding neutron energy spectra using deuterated liquid scintillator is evaluated for future utilization with rare isotope beams. High-resolution neutron energy spectra as well as the detector response matrix were measured at the Edwards Accelerator Laboratory at Ohio University. Maximum-likelihood expectation maximization (MLEM) unfolded neutron spectra are compared with spectra from neutron time-of-flight. The effects of the MLEM stopping criteria and spectrum statistics are also investigated.

The 14O(α,p)17F reaction is an important trigger reaction to the α-p process in X-ray bursts. The most stringent experimental constraints on its astrophysical rate come from measurements of the time-inverse reaction, 17F(p,α)14O. Previous studies of this inverse reaction have sufficiently characterized the high-energy dependence of the cross section but there are still significant uncertainties at lower energies. A new measurement of the 17F(p,α)14O cross section is underway at the Twin Solenoid (TwinSol) facility at the University of Notre Dame using an in-flight secondary 17F beam. The initial results are promising but improvements are needed to complete the measurement. The initial data and plans for an improved measurement are presented in this manuscript.

We report a new precision half-life measurement of $^{20}\mathrm{F}$, performed using the $\ensuremath{\beta}$-counting station of the University of Notre Dame's Nuclear Science Laboratory. The measured half-life of $11.0160{(41)}_{\text{stat}}{(155)}_{\text{sys}}$ s resulting from this work will help resolve the longstanding discrepancy between two earlier sets of high-precision half-life measurements.

The influence of high-energy (1.6 MeV) Ar2+ irradiation on the interfacial interaction between cerium oxide thin films (∼15 nm) with a SiO2/Si substrate is investigated using transmission electron microscopy, ultrahigh vacuum x-ray photoelectron spectroscopy (XPS), and a carbon monoxide (CO) oxidation catalytic reaction using ambient pressure XPS. The combination of these methods allows probing the dynamics of vacancy generation and its relation to chemical interactions at the CeO2/SiO2/Si interface. The results suggest that irradiation causes amorphization of some portion of CeO2 at the CeO2/SiO2/Si interface and creates oxygen vacancies due to the formation of Ce2O3 at room temperature. The subsequent ultra-high-vacuum annealing of irradiated films increases the concentration of Ce2O3 with the simultaneous growth of the SiO2 layer. Interactions with CO molecules result in an additional reduction of cerium and promote the transition of Ce2O3 to a silicate compound. Thermal annealing of thin films exposed to oxygen or carbon monoxide shows that the silicate phase is highly stabile even at 450 °C.

Background: The precise determination of the $\mathcal{F}t$ value in $T=1/2$ mixed mirror decays is an important avenue for testing the standard model of the electroweak interaction through the determination of ${V}_{ud}$ in nuclear $\ensuremath{\beta}$ decays. $^{11}\mathrm{C}$ is an interesting case, as its low mass and small ${Q}_{EC}$ value make it particularly sensitive to violations of the conserved vector current hypothesis. The present dominant source of uncertainty in the $^{11}\mathrm{C}\phantom{\rule{4pt}{0ex}}\mathcal{F}t$ value is the half-life.Purpose: A high-precision measurement of the $^{11}\mathrm{C}$ half-life was performed, and a new world average half-life was calculated.Method: $^{11}\mathrm{C}$ was created by transfer reactions and separated using the TwinSol facility at the Nuclear Science Laboratory at the University of Notre Dame. It was then implanted into a tantalum foil, and $\ensuremath{\beta}$ counting was used to determine the half-life.Results: The new half-life, ${t}_{1/2}=1220.27(26)$ s, is consistent with the previous values but significantly more precise. A new world average was calculated, ${t}_{1/2}^{\text{world}}=1220.41(32)$ s, and a new estimate for the Gamow-Teller to Fermi mixing ratio $\ensuremath{\rho}$ is presented along with standard model correlation parameters.Conclusions: The new $^{11}\mathrm{C}$ world average half-life allows the calculation of a $\mathcal{F}{t}^{\text{mirror}}$ value that is now the most precise value for all superallowed mixed mirror transitions. This gives a strong impetus for an experimental determination of $\ensuremath{\rho}$, to allow for the determination of ${V}_{ud}$ from this decay.

Background: The $^{17}\mathrm{F}(p,\ensuremath{\gamma})^{18}\mathrm{Ne}$ reaction is part of the astrophysical ``hot CNO'' cycles that are important in astrophysical environments like novas. Its thermal reaction rate is low owing to the relatively high energy of the resonances and therefore is dominated by direct, nonresonant capture in stellar environments at temperatures below 0.4 GK.Purpose: An experimental method is established to extract the proton strength to bound and unbound states in experiments with radioactive ion beams and to determine the parameters of direct and resonant capture in the $^{17}\mathrm{F}(p,\ensuremath{\gamma})^{18}\mathrm{Ne}$ reaction.Method: The $^{17}\mathrm{F}(d,n)^{18}\mathrm{Ne}$ reaction is measured in inverse kinematics using a beam of the short-lived isotope $^{17}\mathrm{F}$ and a compact setup of neutron, proton, $\ensuremath{\gamma}$-ray, and heavy-ion detectors called resoneut.Results: The spectroscopic factors for the lowest $l=0$ proton resonances at ${\mathrm{E}}_{\mathrm{c}.\mathrm{m}.}=0.60$ and 1.17 MeV are determined, yielding results consistent within $1.4\ensuremath{\sigma}$ of previous proton elastic-scattering measurements. The asymptotic normalization coefficients of the bound ${2}_{1}^{+}$ and ${2}_{2}^{+}$ states in $^{18}\mathrm{Ne}$ are determined and the resulting direct-capture reaction rates are extracted.Conclusions: The direct-capture component of the $^{17}\mathrm{F}(p,\ensuremath{\gamma})^{18}\mathrm{Ne}$ reaction is determined for the first time from experimental data on $^{18}\mathrm{Ne}$.

An array consisting of 12 deuterated organic liquid scintillator detectors for fast-neutron spectroscopy was designed and built at Oak Ridge National Laboratory (ORNL). This versatile array is designed for measurements with low reaction yields, such as those performed with rare isotope beams, as well as at high current DC facilities used for underground nuclear astrophysics research. Because some measurements also offer limited, or no, additional timing information, the ORNL Deuterated Spectroscopic Array (ODeSA) was optimized to utilize spectrum unfolding to extract neutron energy spectra . This array was characterized for n/ γ pulse shape discrimination, light response, resolution, and intrinsic efficiency by using the neutron time-of-flight tunnel at the Edwards Accelerator Laboratory at Ohio University. Results and future plans are discussed.

Reactions on certain proton-rich, radioactive nuclei have been shown to have a significant influence on X-ray bursts. We provide an overview of two recent measurements of important X-ray burst reactions using in-flight radioactive ion beams from the RESOLUT facility at the J. D. Fox Superconducting Accelerator Laboratory at Florida State University. The 17 F(d,n) 18 Ne reaction was measured, and Asymptotic Normalization Coefficients were extracted for bound states in 18 Ne that determine the direct-capture cross section dominating the 17 F(p, γ ) 18 Ne reaction rate for T≲ 0.45 GK. Unbound resonant states were also studied, and the single-particle strength for the 4.523-MeV (3 + ) state was found to be consistent with previous results. The 19 Ne(d,n) 20 Na proton transfer reaction was used to study resonances in the 19 Ne(p, γ ) 20 Na reaction. The most important 2.65-MeV state in 20 Na was observed to decay by proton emission to both the ground and first-excited states in 19 Ne, providing strong evidence for a 3 + spin assignment and indicating that proton capture on the thermally-populated first-excited state in 19 Ne is an important contributor to the 19 Ne(p, γ ) 20 Na reaction rate.

The $^{19}\mathrm{Ne}(p,\ensuremath{\gamma})^{20}\mathrm{Na}$ reaction is the second step of a reaction chain which breaks out from the hot CNO cycle, following the $^{15}\mathrm{O}(\ensuremath{\alpha},\ensuremath{\gamma})^{19}\mathrm{Ne}$ reaction at the onset of x-ray burst events. We investigate the spectrum of the lowest proton-unbound states in $^{20}\mathrm{Na}$ in an effort to resolve contradictions in spin-parity assignments and extract reliable information about the thermal reaction rate. The proton-transfer reaction $^{19}\mathrm{Ne}(d,n)^{20}\mathrm{Na}$ is measured with a beam of the radioactive isotope $^{19}\mathrm{Ne}$ at an energy around the Coulomb barrier and in inverse kinematics. We observe three proton resonances with the $^{19}\mathrm{Ne}$ ground state, at 0.44, 0.66, and 0.82 MeV c.m. energies, which are assigned ${3}^{+}$, ${1}^{+}$, and (${0}^{+}$), respectively. In addition, we identify two resonances with the first excited state in $^{19}\mathrm{Ne}$, one at 0.20 MeV and one, tentatively, at 0.54 MeV. These observations allow us for the first time to experimentally quantify the astrophysical reaction rate on an excited nuclear state. Our experiment shows an efficient path for thermal proton capture in $^{19}\mathrm{Ne}(p,\ensuremath{\gamma})^{20}\mathrm{Na}$, which proceeds through ground state and excited-state capture in almost equal parts and eliminates the possibility for this reaction to create a bottleneck in the breakout from the hot CNO cycle.

The ^{19}Ne(p,γ)^{20}Na reaction is the second step of a reaction chain which breaks out from the hot CNO cycle, following the ^{15}O(α,γ)^{19}Ne reaction at the onset of x-ray burst events. We investigate the spectrum of the lowest proton-unbound states in ^{20}Na in an effort to resolve contradictions in spin-parity assignments and extract reliable information about the thermal reaction rate. The proton-transfer reaction ^{19}Ne(d,n)^{20}Na is measured with a beam of the radioactive isotope ^{19}Ne at an energy around the Coulomb barrier and in inverse kinematics. We observe three proton resonances with the ^{19}Ne ground state, at 0.44, 0.66, and 0.82 MeV c.m. energies, which are assigned 3^{+}, 1^{+}, and (0^{+}), respectively. In addition, we identify two resonances with the first excited state in ^{19}Ne, one at 0.20 MeV and one, tentatively, at 0.54 MeV. These observations allow us for the first time to experimentally quantify the astrophysical reaction rate on an excited nuclear state. Our experiment shows an efficient path for thermal proton capture in ^{19}Ne(p,γ)^{20}Na, which proceeds through ground state and excited-state capture in almost equal parts and eliminates the possibility for this reaction to create a bottleneck in the breakout from the hot CNO cycle.

Resonance scattering with rare isotope beams provides direct access to continuum properties of exotic nuclei and can serve as a stringent test for modern theoretical approaches. Properties of neutron deficient isotope 8B, that were studied using resonance scattering of protons of 7Be, are discussed and compared to the predictions of the ab initio theories. New experimental data on clustering in 10Be studied using 6He+α resonance elastic scattering is presented.

Many astrophysical events, such as novae and X-ray bursts, are powered by reactions with radioactive nuclei. Studying the properties of these nuclei in the laboratory can therefore further our understanding of these astrophysical explosions. The TwinSol separator at the University of Notre Dame has recently been used to produce intense (~106 pps) beams of 17F. In this article, some of the first measurements with these beams are discussed.

The 14O(α,p)17F reaction is important for understanding the αp process that occurs in X-ray bursts, but the rate of this reaction remains uncertain due to the uncertain properties of states in 18Ne. We measured the 17F(p,p)17F and 17F(p,α)14O reactions to study the properties of states in 18Ne that are important for the 14O(α,p)17F reaction using 17F radioactive beams from the RESOLUT facility at Florida State University. Double-sided silicon strip detectors were used to detect light particles, and recoiling heavy ions were detected in coincidence using a gas ionization chamber at forward angles. The performance of the system was first tested using the 17O(p,α)14N reaction. This was the first measurement using the ASIC electronics and recoil detector being developed for the Array for Nuclear Astrophysics Studies with Exotic Nuclei (ANASEN). We report on the performance and preliminary results.

Clustering phenomena in 10Be and 18O were studied by means of resonance elastic scattering of α-particles on 6He and 14C. Excitation functions for α+6He and α+14C were measured and detailed R-matrix analyses of the excitation functions was performed. We compare the experimental results with the predictions of modern theoretical approaches and discuss properties of cluster rotational bands.

We discuss the identification and properties of the states that belong to the highly clustered rotational band in A=10 nuclei, 10Be, 10B(T=1) and 10C. The band is of interest because it may correspond to an exotic α:nn:α configuration.