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A detailed investigation on the relative isotopic distributions has been carried out for the first time in case of even-even correlated fission fragments for the $^{235}$U($n_{th}$,$f$) fission reaction. High-statistics data were obtained in a prompt $\gamma$ ray spectroscopy measurement during the EXILL campaign at ILL, Grenoble, France. The extensive off-line analysis of the coincidence data have been carried out using four different coincidence methods. Combining the results from 2-dimensional $\gamma-\gamma$ and 3-dimensional $\gamma-\gamma-\gamma$ coincidence analysis, a comprehensive picture of the relative isotopic yield distributions of the even-even neutron-rich fission fragments has emerged. The experimentally observed results have been substantiated by the theoretical calculations based on a novel approach of isospin conservation, and a reasonable agreement has been obtained. The calculations following the semi-empirical GEF model have also been carried out. The results from the GEF model calculations are found to be in fair agreement with the experimental results., Comment: Accepted in PRC; nucl-ex; nucl-th

Medium-spin excited states of the neutron-rich nucleus $^{87}$Br were observed and studied for the first time. They were populated in fission of $^{235}$U induced by the cold-neutron beam of the PF1B facility of the Institut Laue-Langevin, Grenoble. The measurement of $\gamma$ radiation following fission has been performed using the EXILL array of Ge detectors. The observed level scheme was compared with results of large valence space shell model calculations. The medium-spin level scheme consists of three band-like structures, which can be understood as bands built on the ${\pi}f_{5/2}$, ${\pi}(p_{3/2}+f_{5/2})$ and ${\pi}g_{9/2}$ configurations. The behavior of the observed ${\pi}g_{9/2}$ band at high spins shows a considerable deviation from the shell model predictions. This deviation in this band is probably the result of an increased collectivity, which can be understood assuming that the ${\pi}g_{9/2}$ high-$\it j$ proton polarizes the core.

We present recent results on the structure of the one-valence-particle $^{41}$Ca and $^{49}$Ca, and one-valence-hole $^{47}$Ca, nuclei. The isotopes of interest were populated via the cold-neutron capture reactions $^{40}$Ca(n,$\gamma$), $^{48}$Ca(n,$\gamma$) and $^{46}$Ca(n,$\gamma$), respectively. The experiments were performed at the Institut Laue-Langevin, within the EXILL campaign, which employed a large array of HPGe detectors. The $\gamma$ decay and level schemes of these nuclei were investigated by $\gamma$-ray coincidence relationships, leading to the identification of 41, 10, and 6 new transitions in $^{41}$Ca, $^{47}$Ca, and $^{49}$Ca, respectively. Branching ratios and intensities were extracted for the $\gamma$ decay from each state, and $\gamma$-ray angular correlations were performed to establish a number of transition multipolarities and mixing ratios, thus helping in the spin assignment of the states. The experimental findings are discussed along with microscopic, self-consistent beyond-mean-field calculations performed with the Hybrid Configuration Mixing model, based on a Skyrme SkX Hamiltonian. The latter suggests that a fraction of the low-spin states of the $^{41}$Ca, $^{49}$Ca, and $^{47}$Ca nuclei is characterized by the coexistence of either 2p-1h and 1p-2h excitations, or couplings between single-particle/hole degrees of freedom and collective vibrations (phonons) of the doubly-magic "core".

An extended investigation of the low-spin structure of the $^{65}$Ni nucleus was performed at the Institut Laue-Langevin, Grenoble, via the neutron capture reaction $^{64}$Ni(n,$\gamma$)$^{65}$Ni, using the FIPPS HPGe array. The level scheme of $^{65}$Ni was significantly expanded, with 2 new levels and 87 newly found transitions. Angular correlation analyses were also performed, allowing us to assign spins and parities for a number of states, and to determine multipolarity mixing ratios for selected $\gamma$ transitions. The low-energy part of the experimental level scheme (up to about 1.4 MeV) was compared with Monte Carlo Shell Model calculations, which predict spherical shapes for all states, apart from the 9/2$^+$ and the second excited 1/2$^-$ states of oblate deformation.

The low-spin structure of the semimagic 64Ni nucleus has been considerably expanded: combining four experiments, several 0+ and 2+ excited states were identified below 4.5 MeV, and their properties established. The Monte Carlo shell model accounts for the results and unveils an unexpectedly complex landscape of coexisting shapes: a prolate 0+ excitation is located at a surprisingly high energy (3463 keV), with a collective 2+ state 286 keV above it, the first such observation in Ni isotopes. The evolution in excitation energy of the prolate minimum across the neutron N = 40 subshell gap highlights the impact of the monopole interaction and its variation in strength with N.

We performed an experimental search for the bound state singlet deuteron predicted in some microscopic calculations. The predicted energy of this metastable level is in vicinity of the deuteron disintegration threshold. This state should manifest itself in two-photon transition following thermal neutron capture by protons. The experiment consists in the search for the second gamma-ray in the cascade through a high statistics measurement of $\gamma$-ray spectra after cold neutron capture by hydrogen nuclei. The upper limit $2\mu$b (2$\sigma$ level) is obtained for the cross section of the singlet deuteron production with the bound energy in the range 10-125 keV., Comment: 10 pages, 4 figures

The dispersive behavior of materials with atomic charge numbers varing from $Z = 4$ (beryllium, Be) to $Z = 82$ (lead, Pb) was investigated experimentally and theoretically at $\gamma$-ray energies up to 2 MeV. The experiment was performed at the double-crystal gamma spectrometer GAMS6 of the ILL in Grenoble. The experimental results were compared with theoretical calculations which account for all major elastic processes involved. Overall, we found a good agreement between theory and experiment. We find that for the development of refractive optics at $\gamma$-ray energies beyond those currently in use high-Z materials become increasingly attractive compared to the beryllium lens-stacks used at X-ray energies., Comment: submitted to Phys. Rev. A

The STEREO experiment is a very short baseline reactor antineutrino experiment aiming at testing the hypothesis of light sterile neutrinos as an explanation of the deficit of the observed neutrino interaction rate with respect to the predicted rate, known as the Reactor Antineutrino Anomaly. The detector center is located 10 m away from the compact, highly $^{235}$U enriched core of the research nuclear reactor of the Institut Laue Langevin in Grenoble, France. This paper describes the STEREO site, the detector components and associated shielding designed to suppress the external sources of background which were characterized on site. It reports the performances in terms of detector response and energy reconstruction., Comment: 32 pages, 17 figures

The refractive index of silicon at $\gamma$-ray energies from 181 - 1959 keV was investigated using the GAMS6 double crystal spectrometer and found to follow the predictions of the classical scattering model. This is in contrast to earlier measurements on the GAMS5 spectrometer, which suggested a sign-change in the refractive index for photon energies above 500 keV. We present a re-evaluation of the original data from 2011 as well as data from a 2013 campaign in which we show that systematic errors due to diffraction effects of the prism can explain the earlier data., Comment: submitted to Physical Review C

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

Spectra of ultracold neutrons that appeared in experiments on neutron diffraction by a moving grating were measured using the time-of-flight Fourier spectrometer. Diffraction lines of five orders were observed simultaneously. The obtained data are in good agreement with the theoretical predictions based on the multiwave dynamical theory of neutron diffraction by a moving grating., Comment: Submitted to Phys. Rev. A

We describe a new time-of-flight Fourier spectrometer for investigation of UCN diffraction by a moving grating. The device operates in the regime of a discrete set of modulation frequencies. The results of the first experiments show that the spectrometer may be used for obtaining UCN energy spectra in the energy range of 60$\div$200 neV with a resolution of about 5 neV. The accuracy of determination of the line position was estimated to be several units of $10^{-10}$ eV, Comment: Submitted to NIMA

We describe an experimental installation for a new test of the weak equivalence principle for neutron. The device is a sensitive gravitational spectrometer for ultra-cold neutrons allowing to precisely compare the gain in kinetic energy of free falling neutrons to quanta of energy ${\hbar}{\Omega}$ transferred to the neutron via a non stationary device, i.e. a quantum modulator. The results of first test experiments indicate a collection rate allowing measurements of the factor of equivalence $ { \gamma}$ with a statistical uncertainty in the order of $5{\times}10^{-3}$ per day. A number of systematic effects were found, which partially can be easily corrected. For the elimination of others more detailed investigations and analysis are needed. Some possibilities to improve the device are also discussed., Comment: Submitted to NIMA

When a rather cold electron bunch is transported during laser bubble acceleration in a strongly focusing plasma channel with typical forces of 100 GeV/m, it will form partially ordered long electron cylinders due to the relativistically longitudinal reduced repulsion between electrons, resulting in a long-range pair correlation function, when reaching energies in the laboratory above 0.5 GeV. During Compton back-scattering with a second laser, injected opposite to the electron bunch, the electron bunch will be further modulated with micro bunches and due to its ordered structure will reflect coherently, M\"ossbauer-like, resulting in a \gamma free electron laser (\gamma-FEL). Increasing the relativistic \gamma factor, the quantal regime becomes more dominant. We discuss the scaling laws with \gamma.

We study the production of radioisotopes for nuclear medicine in (gamma,gamma') photoexcitation reactions or (gamma,xn + yp) photonuclear reactions for the examples of ^195mPt, ^117mSn and ^44Ti with high flux [(10^13 - 10^15) gamma/s], small beam diameter and small energy band width (Delta E/E ~ 10^-3 -10^-4) gamma beams. In order to realize an optimum gamma-focal spot, a refractive gamma-lens consisting of a stack of many concave micro-lenses will be used. It allows for the production of a high specific activity and the use of enriched isotopes. For photonuclear reactions with a narrow gamma beam, the energy deposition in the target can be reduced by using a stack of thin target wires, hence avoiding direct stopping of the Compton electrons and e^+e^- pairs. The well-defined initial excitation energy of the compound nucleus leads to a small number of reaction channels and enables new combinations of target isotope and final radioisotope. The narrow-bandwidth gamma excitation may make use of collective resonances in gamma-width, leading to increased cross sections. (gamma,gamma') isomer production via specially selected gamma cascades allows to produce high specific activity in multiple excitations, where no back-pumping of the isomer to the ground state occurs. The produced isotopes will open the way for completely new clinical applications of radioisotopes. For example ^195mPt could be used to verify the patient's response to chemotherapy with platinum compounds before a complete treatment is performed. In targeted radionuclide therapy the short-range Auger and conversion electrons of ^195mPt and ^117mSn enable a very local treatment. The generator ^44Ti allows for a PET with an additional gamma-quantum (gamma-PET), resulting in a reduced dose or better spatial resolution., Comment: 10 pages, 7 figures

We present for the first time the concept of a seeded {\gamma} quantum Free-Electron-Laser (QFEL) at 478 keV, which has very different properties compared to a classical. The basic concept is to produce a highly brilliant {\gamma} beam via SASE. To produce highly intense and coherent {\gamma} beam, we intend to use a seeded FEL scheme. Important for the production of such a {\gamma} beam are novel refractive {\gamma} -lenses for focusing and an efficient monochromator, allowing to generate a very intense and coherent seed beam. The energy of the {\gamma} beam is 478 keV, corresponding to a wavelength in the sub-{\AA}ngstr{\o}m regime (1/38 {\AA}). To realize a coherent {\gamma} beam at 478 keV, it is necessary to use a quantum FEL design. At such high radiation energies a classical description of the {\gamma}-FEL becomes wrong.

Next-generation gamma beams beams from laser Compton-backscattering facilities like ELI-NP (Bucharest)] or MEGa-Ray (Livermore) will drastically exceed the photon flux presently available at existing facilities, reaching or even exceeding 10^13 gamma/sec. The beam structure as presently foreseen for MEGa-Ray and ELI-NP builds upon a structure of macro-pulses (~120 Hz) for the electron beam, accelerated with X-band technology at 11.5 GHz, resulting in a micro structure of 87 ps distance between the electron pulses acting as mirrors for a counterpropagating intense laser. In total each 8.3 ms a gamma pulse series with a duration of about 100 ns will impinge on the target, resulting in an instantaneous photon flux of about 10^18 gamma/s, thus introducing major challenges in view of pile-up. Novel gamma optics will be applied to monochromatize the gamma beam to ultimately Delta E/E~10^-6. Thus level-selective spectroscopy of higher multipole excitations will become accessible with good contrast for the first time. Fast responding gamma detectors, e.g. based on advanced scintillator technology (e.g. LaBr3(Ce)) allow for measurements with count rates as high as 10^6-10^7 gamma/s without significant drop of performance. Data handling adapted to the beam conditions could be performed by fast digitizing electronics, able to sample data traces during the micro-pulse duration, while the subsequent macro-pulse gap of ca. 8 ms leaves ample time for data readout. A ball of LaBr3 detectors with digital readout appears to best suited for this novel type of nuclear photonics at ultra-high counting rates., Comment: 4 pages, 1 figure, 1 table

With new gamma-beam facilities like MEGa-ray at LLNL (USA) or ELI-NP at Bucharest with 10^13 g/s and a bandwidth of Delta E_g/E_g ~10^-3, a new era of g-beams with energies <=20 MeV comes into operation, compared to the present world-leading HIGS facility (Duke Univ., USA) with 10^8 g/s and Delta E_g/E_g~0.03. Even a seeded quantum FEL for g-beams may become possible, with much higher brilliance and spectral flux. At the same time new exciting possibilities open up for focused g-beams. We describe a new experiment at the g-beam of the ILL reactor (Grenoble), where we observed for the first time that the index of refraction for g-beams is determined by virtual pair creation. Using a combination of refractive and reflective optics, efficient monochromators for g-beams are being developed. Thus we have to optimize the system of the g-beam facility, the g-beam optics and g-detectors. We can trade g-intensity for band width, going down to Delta E_g/E_g ~ 10^-6 and address individual nuclear levels. 'Nuclear photonics' stresses the importance of nuclear applications. We can address with g-beams individual nuclear isotopes and not just elements like with X-ray beams. Compared to X rays, g-beams can penetrate much deeper into big samples like radioactive waste barrels, motors or batteries. We can perform tomography and microscopy studies by focusing down to micron resolution using Nucl. Reson. Fluorescence for detection with eV resolution and high spatial resolution. We discuss the dominating M1 and E1 excitations like scissors mode, two-phonon quadrupole octupole excitations, pygmy dipole excitations or giant dipole excitations under the new facet of applications. We find many new applications in biomedicine, green energy, radioactive waste management or homeland security. Also more brilliant secondary beams of neutrons and positrons can be produced., Comment: 8 pages, 3 figures, 2 tables

The index of refraction n(E_{\gamma})=1+\delta(E_{\gamma})+i\beta(E_{\gamma}) is split into a real part \delta and an absorptive part \beta. The absorptive part has the three well-known contributions to the cross section \sigma_{abs}: the photo effect, the Compton effect and the pair creation, but there is also the inelastic Delbr\"uck scattering. Second-order elastic scattering cross sections \sigma_{sca} with Rayleigh scattering (virtual photo effect), virtual Compton effect and Delbr\"uck scattering (virtual pair creation) can be calculated by integrals of the Kramers-Kronig dispersion relations from the cross section \sigma_{abs}. The real elastic scattering amplitudes are proportional to the refractive indices \delta_{photo}, \delta_{Compton} and \delta_{pair}. While for X-rays the negative \delta_{photo} dominates, we show for the first time experimentally and theoretically that the positive \delta_{pair} dominates for \gamma rays, opening a new era of \gamma optics applications, i.e. of nuclear photonics., Comment: 4 pages, 3 figures

We have measured the neutron electric dipole moment using spin rotation in a non-centrosymmetric crystal. Our result is d_n = (2.5 +- 6.5(stat) +- 5.5(syst)) 10^{-24} e cm. The dominating contribution to the systematic uncertainty is statistical in nature and will reduce with improved statistics. The statistical sensitivity can be increased to 2 10^{-26} e cm in 100 days data taking with an improved setup. We state technical requirements for a systematic uncertainty at the same level., Comment: submitted to Phys. Lett. B

Laue lenses are an emerging technology based on diffraction in crystals that allows the concentration of soft gamma rays. This kind of optics that works in the 100 keV - 1.5 MeV band can be used to realize an high-sensitivity and high-angular resolution telescope (in a narrow field of view). This paper reviews the recent progresses that have been done in the development of efficient crystals, in the design study and in the modelisation of the answer of Laue lenses. Through the example of a new concept of 20 m focal length lens focusing in the 100 keV - 600 keV band, the performance of a telescope based on a Laue lens is presented. This lens uses the most efficient mosaic crystals in each sub-energy range in order to yield the maximum reflectivity. Imaging capabilities are investigated and shows promising results., Comment: Published in Proc. of SPIE 2009, volume 7437

An experiment using a prototype setup to search for the neutron electric dipole moment by measuring spin-rotation in a non-centrosymmetric crystal (quartz) was carried out to investigate statistical sensitivity and systematic effects of the method. It has been demonstrated that the concept of the method works. The preliminary result of the experiment is $d_{\rm n}=(2.5\pm 6.5)\cdot 10^{-24}$ e$\cdot $cm. The experiment showed that an accuracy of $\sim 2.5\cdot 10^{-26}$ e$\cdot $cm can be obtained in 100 days data taking, using available quartz crystals and neutron beams., Comment: 13 pages, 4 figures

The concept of a gamma-ray telescope based on a Laue lens offers the possibility to increase the sensitivity by more than an order of magnitude with respect to existing instruments. Laue lenses have been developed by our collaboration for several years : the main achievement of this R&D program was the CLAIRE lens prototype. Since then, the endeavour has been oriented towards the development of efficient diffracting elements (crystal slabs), the aim being to step from a technological Laue lens to a scientifically exploitable lens. The latest mission concept featuring a gamma-ray lens is the European Gamma-Ray Imager (GRI) which intends to make use of the Laue lens to cover energies from 200 keV to 1300 keV. Investigations of two promising materials, low mosaicity copper and gradient concentration silicon-germanium are presented in this paper. The measurements have been performed during three runs on beamline ID15A of the European Synchrotron Radiation Facility, and on the GAMS 4 instrument of the Institute Laue-Langevin (both in Grenoble, France) using highly monochromatic beam of energy close to 500 keV. Despite it was not perfectly homogeneous, the presented copper crystal exhibits peak reflectivity of 25% in accordance with theoretical predictions, and a mosaicity around 26 arcsec, the ideal range for the realization of a Laue lens such as GRI. Silicon-germanium featuring a constant gradient have been measured for the very first time at 500 keV. Two samples showed a quite homogeneous reflectivity reaching 26%, which is far from the 48% already observed in experimental crystals but a very encouraging beginning. This results have been used to estimate the performance of the GRI Laue lens design.

The binding energies of 29Si, 33S, and 36Cl have been measured with a relative uncertainty $< 0.59 \times 10^{-6}$ using a flat-crystal spectrometer. The unique features of these measurements are 1) nearly perfect crystals whose lattice spacing is known in meters, 2) a highly precise angle scale that is derived from first principles, and 3) a gamma-ray measurement facility that is coupled to a high flux reactor with near-core source capability. The binding energy is obtained by measuring all gamma-rays in a cascade scheme connecting the capture and ground states. The measurements require the extension of precision flat-crystal diffraction techniques to the 5 to 6 MeV energy region, a significant precision measurement challenge. The binding energies determined from these gamma-ray measurements are consistent with recent highly accurate atomic mass measurements within a relative uncertainty of $4.3 \times 10^{-7}$. The gamma-ray measurement uncertainties are the dominant contributors to the uncertainty of this consistency test. The measured gamma-ray energies are in agreement with earlier precision gamma-ray measurements., Comment: 13 pages, 4 figures