1. Robust coherent dynamics of homogeneously limited anisotropic excitons in two-dimensional layered ReS2
- Author
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Chowdhury, Rup Kumar, Islam, Md Samiul, Barthelemy, Marie, Beyer, Nicolas, Engel, Lorry, Pelle, Jean-Sebastien, Rastei, Mircea, Barsella, Alberto, and Fras, Francois
- Subjects
Condensed Matter - Mesoscale and Nanoscale Physics ,Physics - Optics ,Quantum Physics - Abstract
The discovery of in-plane anisotropic excitons in two-dimensional layered semiconductors enables state-of-the-art nanophotonic applications. A fundamental yet unknown parameter of these quasiparticles is the coherence time (T_2 ), which governs the quantum dephasing timescale, over which the coherent superposition of excitons can be maintained and manipulated. Here, we report the direct measurement of T_2 within the sub-picosecond range, along with multiple population decay timescales (T_1 ) at resonance for anisotropic excitons in pristine layered rhenium disulfide (ReS2). We observe a notable weak dependence on layer thickness for T_2 , and a quasi-independence for T_1 . The excitonic coherence in few-layer ReS2 exhibits exceptional robustness against optical density and temperature compared to other two-dimensional semiconductors, enabling quantum features even at room temperature. No photon echo fingerprints were observed in pristine ReS2, highlighting the homogeneous character of the anisotropic excitonic transitions and a particularly low level of disorder in exfoliated flakes. Lastly, our results for mono- to bulk-like ReS2 support a direct gap band structure regardless their layer thickness, addressing the ongoing discussion about its nature.
- Published
- 2024