123 results on '"Glen A. Warren"'
Search Results
2. Flight activity and dispersal of Rhyzopertha dominica (F.) (Coleoptera: Bostrichidae) and Tribolium castaneum (Herbst) (Coleoptera: Tenebrionidae) across a mixed agricultural landscape in southern Australia
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Mark M. Stevens, Gregory J. Daglish, Beverley A. Orchard, Glen N. Warren, Jianhua Mo, and Jessica L. Hoskins
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Insect Science ,Horticulture ,Agronomy and Crop Science ,Food Science - Published
- 2023
3. Topical and dietary toxicity of emamectin benzoate, chlorantraniliprole, cyantraniliprole and indoxacarb to larvae of the common armyworm Mythimna convecta (Lepidoptera: Noctuidae)
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Jianhua Mo, Glen N Warren, and Mark M. Stevens
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Integrated pest management ,Insecticides ,Helicoverpa armigera ,Moths ,Spodoptera ,Toxicology ,Insecticide Resistance ,chemistry.chemical_compound ,Oxazines ,Cyantraniliprole ,Animals ,ortho-Aminobenzoates ,Mythimna convecta ,Ivermectin ,biology ,Indoxacarb ,Frass ,fungi ,Australia ,General Medicine ,biology.organism_classification ,chemistry ,Insect Science ,Larva ,Noctuidae ,Pyrazoles ,PEST analysis ,Agronomy and Crop Science - Abstract
BACKGROUND The common armyworm Mythimna convecta is an important pest of pastures and graminaceous crops in Australia, but materials currently registered for its control are limited to broad-spectrum compounds incompatible with integrated pest management (IPM) systems. In this study we assessed the response of M. convecta larvae to four alternative compounds using topical and dietary bioassays. RESULTS Emamectin benzoate [LC50 (lethal concentration for 50% of insects tested) values 2.69 μg mL-1 topical, 0.017 μg active ingredient (AI) g-1 dietary] and chlorantraniliprole (LC50 values 4.87 μg mL-1 topical, 0.080 μg AI g-1 dietary) were significantly more active than either indoxacarb or cyantraniliprole. Our results showed strong parallels with data on the more extensively studied Australian strains of Helicoverpa armigera, with the most notable differences being the higher contact toxicity of emamectin benzoate to M. convecta and the lower acute dietary activity of formulated cyantraniliprole to this species, which was linked to feeding deterrence. Cyantraniliprole at dietary concentrations of ≥0.02 μg AI g-1 significantly reduced the weight of surviving larvae and frass production (an indirect measure of food consumption) over the seven-day exposure period. There was also some evidence of chlorantraniliprole deterring larval feeding, although to a much more limited extent. CONCLUSIONS Both emamectin benzoate and chlorantraniliprole are suitable for use against M. convecta. The decision as to which of these compounds should be prioritized for further development should be based on their potential effects on beneficial species once their optimal field rates have been determined.
- Published
- 2021
4. Testing requirements for active interrogation systems
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Glen A. Warren, Richard T. Kouzes, Edward R. Siciliano, and Jennifer E. Tanner
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Radiation transport ,Physics ,Nuclear and High Energy Physics ,010308 nuclear & particles physics ,Special nuclear material ,External beam radiation ,Technical standard ,010403 inorganic & nuclear chemistry ,01 natural sciences ,Particle detector ,0104 chemical sciences ,0103 physical sciences ,Electromagnetic shielding ,Systems engineering ,Nuclear resonance fluorescence ,Interrogation ,Instrumentation - Abstract
The role of active-interrogation systems for nuclear security is to detect the presence of special nuclear material inside an object by observing the radiation emitted by that object when it has been exposed to known sources of external radiation. Because of the cost, complexity, and the need to avoid irradiating occupants, active-interrogation systems are intended for cargo applications where shielding can prevent detection by passive radiation detection systems. To ensure that active-interrogation systems for detection of special nuclear material are designed and tested to a consistent level of performance, technical standards are needed for evaluating such systems. This paper addresses the testing standards needed for active-interrogation systems to detect high atomic number materials, fissionable materials, and specific special nuclear materials. Because the use of special nuclear material for a testing standard is not practical, this work focuses on the determination of materials that could be used as surrogates in that they provide a similar response as targets of special nuclear materials. The results of this paper, determined through analytic calculations and radiation transport modeling, are based upon scenarios constructed and applied to specific active-interrogation modalities.
- Published
- 2019
5. Neutron-neutron correlations in the photofission of U238
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J. Burggraf, Glen A. Warren, Sean C. Stave, E. Church, S. Behling, T. A. Forest, and D. S. Dale
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Nuclear physics ,Physics ,Photofission ,Neutron - Published
- 2020
6. Exclusive π+ electroproduction off the proton from low to high -t
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R. J. Holt, S. Basnet, L. G. Tang, X. Zheng, MathML\\'> F, V. Tadevosyan, H. Breuer, A. J. Sarty, Tanja Horn, Glen A. Warren, S. Jin, W. B. Li, A. Matsumura, V. A. Punjabi, D. G. Meekins, J. Volmer, G. M. Huber, P. M. King, Rolf Ent, Jin Liu, M. E. Christy, C. E. Keppel, C. C. Chang, C. F. Perdrisat, K. A. Aniol, E. J. Beise, I. Niculescu, Y. Okayasu, W. Kim, D. Gaskell, Geoffrey Smith, H. P. Blok, msub, D. J. Margaziotis, G. J. Lolos, Pete Markowitz, S. A. Wood, C. Xu, W.U. Boeglin, J. Reinhold, E. F. Gibson, D. J. Mack, H. Mkrtchyan, W. F. Vulcan, E. J. Brash, M. K. Jones, V. Kovaltchouk, Lubomir Pentchev, J. Arrington, V. Tvaskis, mrow> π, P. E. Reimer, J. Roche, Toshinobu Miyoshi, D. H. Potterveld, and Student Lab and Education
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SDG 16 - Peace ,generalized parton distribution ,Proton ,accelerator ,Hadron ,Degrees of freedom (physics and chemistry) ,interference ,Regge ,Parton ,nonperturbative ,01 natural sciences ,7. Clean energy ,energy [beam] ,High Energy Physics - Experiment ,Nuclear physics ,Cross section (physics) ,0103 physical sciences ,ddc:530 ,structure ,010306 general physics ,Nuclear Experiment ,production [meson] ,Quantum chromodynamics ,Physics ,Range (particle radiation) ,010308 nuclear & particles physics ,background ,momentum transfer ,SDG 16 - Peace, Justice and Strong Institutions ,electroproduction ,Justice and Strong Institutions ,Amplitude ,kinematics ,High Energy Physics::Experiment ,distribution function [parton] ,Jefferson Lab ,photoproduction - Abstract
Background: Measurements of exclusive meson production are a useful tool in the study of hadronic structure. In particular, one can discern the relevant degrees of freedom at different distance scales through these studies. Purpose: To study the transition between non-perturbative and perturbative Quantum Chromodyanmics as the square of four momentum transfer to the struck proton, -t, is increased. Method: Cross sections for the $^1$H(e,e'$\pi^+$)n reaction were measured over the -t range of 0.272 to 2.127 GeV$^2$ with limited azimuthal coverage at fixed beam energy of 4.709 GeV, Q$^2$ of 2.4 GeV$^2$ and W of 2.0 GeV at the Thomas Jefferson National Accelerator Facility (JLab) Hall C. Results: The -t dependence of the measured $\pi^+$ electroproduction cross section generally agrees with prior data from JLab Halls B and C. The data are consistent with a Regge amplitude based theoretical model, but show poor agreement with a Generalized Parton Distribution (GPD) based model. Conclusion: The agreement of cross sections with prior data implies small contribution from the interference terms, and the confirmation of the change in t-slopes between the low and high -t regions previously observed in photoproduction indicates the changing nature of the electroproduction reaction in our kinematic regime., Comment: 9 pages, 5 figures Physical Review C, in press
- Published
- 2019
7. Design considerations for future radionuclide aerosol monitoring systems
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Judah I. Friese, Michael E. Swanwick, Glen A. Warren, Brian T. Schrom, J. L. Burnett, Lance S. Lidey, Paul W. Eslinger, Sheldon Stokes, Clive L. Devoy, Harry S. Miley, Joel B. Forrester, Ariane B. Chepko, Scott J. Morris, and John E. Smart
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Aerosols ,Radionuclide ,business.industry ,Health, Toxicology and Mutagenesis ,Monitoring system ,Context (language use) ,General Medicine ,Modular design ,Pollution ,law.invention ,Aerosol ,Upgrade ,law ,Air Pollutants, Radioactive ,Radiation Monitoring ,Nuclear power plant ,Systems engineering ,Environmental Chemistry ,Radiation monitoring ,Environmental science ,Fukushima Nuclear Accident ,business ,Waste Management and Disposal - Abstract
Pacific Northwest National Laboratory (PNNL) staff developed the Radionuclide Aerosol Sampler Analyzer (RASA) for worldwide aerosol monitoring in the 1990s. Recently, researchers at PNNL and Creare, LLC, have investigated possibilities for how RASA could be improved, based on lessons learned from more than 15 years of continuous operation, including during the Fukushima Daiichi Nuclear Power Plant disaster. Key themes addressed in upgrade possibilities include having a modular approach to additional radionuclide measurements, optimizing the sampling/analyzing times to improve detection location capabilities, and reducing power consumption by using electrostatic collection versus classic filtration collection. These individual efforts have been made in a modular context that might constitute retrofits to the existing RASA, modular components that could improve a manual monitoring approach, or a completely new RASA. Substantial optimization of the detection and location capabilities of an aerosol network is possible and new missions could be addressed by including additional measurements.
- Published
- 2019
8. A practical approach to determining soil-sample detection efficiency in field gamma-ray spectroscopy
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Glen A. Warren and Mital A. Zalavadia
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Radionuclide ,Radiation ,Soil test ,Field (physics) ,Detector ,Reproducibility of Results ,Context (language use) ,Sample (statistics) ,Function (mathematics) ,Empirical Research ,010403 inorganic & nuclear chemistry ,01 natural sciences ,030218 nuclear medicine & medical imaging ,0104 chemical sciences ,Spectrometry, Gamma ,03 medical and health sciences ,0302 clinical medicine ,Calibration ,Soil Pollutants, Radioactive ,Environmental science ,Gamma spectroscopy ,Remote sensing - Abstract
Field measurements of radionuclide activities in soil samples via gamma spectroscopy measurements are conducted for many applications. One example application space is on-site inspection for the Comprehensive Nuclear-Test-Ban Treaty. To extract isotopic activities from observed peak counting rates, it is necessary to understand the absolute efficiency of the detector system for a sample. In principle, this efficiency is a function of many parameters, such as sample geometry, soil elemental composition, and soil density. The demands of field measurements within the context of on-site inspections, however, places a premium on an easy-to-implement approach at the possible expense of accuracy given the need to process many samples in a short period of time. This paper presents a semi-empirical approach, using a calibrated standard and a correction that depends only on the relative differences in density of the sample and the standard. Field measurements were conducted to demonstrate the validity of the approach.
- Published
- 2021
9. Alpha and conversion electron spectroscopy of 238,239Pu and 241Am and alpha-conversion electron coincidence measurements
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Michael P. Dion, Glen A. Warren, and Brian W. Miller
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Physics ,Nuclear and High Energy Physics ,Electron spectrometer ,Silicon drift detector ,Physics::Instrumentation and Detectors ,Electron capture ,Alpha-particle spectroscopy ,Energy-dispersive X-ray spectroscopy ,Alpha particle ,Electron ,010403 inorganic & nuclear chemistry ,01 natural sciences ,Electron spectroscopy ,030218 nuclear medicine & medical imaging ,0104 chemical sciences ,03 medical and health sciences ,0302 clinical medicine ,Atomic physics ,Instrumentation - Abstract
A technique to determine the isotopic constituents of a mixed actinide sample has been proposed by a coincident alpha-conversion electron measurement. This presents a unique signature to allow the unfolding of isotopes that possess overlapping alpha particle energy and reduce backgrounds of an unseparated sample. The work presented here are results of conversion electron spectroscopy of 241 Am, 238 Pu and 239 Pu using a dual-stage peltier-cooled 25 mm 2 silicon drift detector and alpha spectroscopy with a passivated ion implanted planar silicon detector. The conversion electron spectra were evaluated from 20–55 keV based on fits to the dominant conversion electron emissions, which allowed the relative conversion electron emission intensities to be determined. These measurements provide crucial singles spectral information and calibration to aid in the coincident measurement approach. Furthermore, an alpha-conversion electron spectrometer was assembled using the silicon based detectors described and results of a coincident spectrum analysis is reported for 241 Am.
- Published
- 2016
10. On-Site Inspection RadioIsotopic Spectroscopy (Osiris) System-Integration and Field-Testing Report
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C. J. Wharton, Brian D. Milbrath, Glen A. Warren, M. A. Zalavadia, A.J. Caffrey, Nathan G. Wimer, and Kenneth M. Krebs
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Physics ,Field (physics) ,biology ,business.industry ,System integration ,Osiris ,biology.organism_classification ,Spectroscopy ,business ,Remote sensing - Published
- 2018
11. Measurements of the separated longitudinal structure function FL from hydrogen and deuterium targets at low Q2
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Bogdan Wojtsekhowski, E. McGrath, T. Angelescu, D. H. Potterveld, B. L. Berman, B. Zihlmann, P. E. Reimer, E. R. Kinney, G. Chang, T. Horn, V. V. Frolov, C. Yan, J. Arrington, Y. Liang, G. M. Huber, A. Lung, G. S. Adams, Rolf Ent, James J. Kelly, J. Telfeyan, D. G. Meekins, T. Dodario, Curtis Smith, E. Segbefia, T. Ostapenko, H. E. Jackson, H. Mkrtchyan, Glen A. Warren, K. Hafidi, Donal Day, A. Uzzle, W. F. Vulcan, W. U. Boeglin, V. Tvaskis, E. J. Brash, N. S. Chant, M. E. Christy, G. Mbianda, I. Niculescu, P. Stoler, Joerg Reinhold, M. Ungaro, X. Jiang, O. K. Baker, Z. Papandreou, G. R. Smith, H. C. Fenker, M. M. Dalton, H. P. Blok, H. Breuer, A. Tvaskis, V. P. Kubarovsky, Cynthia Keppel, A. S. Biselli, J. Kuhn, Paul Gueye, S. A. Wood, A. Ahmidouch, J. A. Dunne, D. Abbott, Simon Henry Connell, S. Vidakovic, V. Tadevosyan, D. J. Mack, K. Garrow, R. J. Holt, Avraham Klein, Jim Napolitano, Stephen Avery, N. Benmouna, S. Danagoulian, S. E. Rock, N. El Khayari, E. Schulte, G. Niculescu, S. Malace, P. Bosted, F. R. Wesselmann, G. J. Lolos, J. Roche, M. Nozar, L. Todor, A. N. Villano, D. Mckee, T. Navasardyan, M. K. Jones, Dipanwita Dutta, R. Asaturyan, Pete Markowitz, D. Gaskell, W. Hinton, Ronald Gilman, Andrei Afanasev, K. Joo, and L. G. Tang
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Physics ,Proton ,010308 nuclear & particles physics ,Scattering ,Momentum transfer ,Parton ,Deep inelastic scattering ,01 natural sciences ,Molecular physics ,Nuclear physics ,Deuterium ,0103 physical sciences ,Neutron ,Nuclear Experiment ,010306 general physics ,Nucleon - Abstract
Structure functions, as measured in lepton-nucleon scattering, have proven to be very useful in studying the partonic dynamics within the nucleon. However, it is experimentally difficult to separately determine the longitudinal and transverse structure functions, and consequently there are substantially less data available in particular for the longitudinal structure function. Here, we present separated structure functions for hydrogen and deuterium at low four-momentum transfer squared, Q2
- Published
- 2018
12. Soil Sample Efficiency Approach for OSIRIS
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Glen A. Warren and Mital A. Zalavadia
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biology ,Environmental science ,Osiris ,biology.organism_classification ,Sample (graphics) ,Remote sensing - Published
- 2018
13. Separated Kaon Electroproduction Cross Section and the Kaon Form Factor from 6 GeV JLab Data
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L. G. Tang, S. Jin, W. Kim, H. Breuer, Tanja Horn, H. P. Blok, C. E. Keppel, E. F. Gibson, Glen A. Warren, A. Vargas, A. Matsumura, D. J. Margaziotis, W. F. Vulcan, H. C. Fenker, C. Xu, P. E. Reimer, Jin Liu, R. J. Holt, M. E. Christy, S. A. Wood, C. C. Chang, S. Vidakovic, V. Tadevosyan, W.U. Boeglin, I. Niculescu, V. Tvaskis, D. J. Mack, V. Kovaltchouk, Jlab Fpi, Lubomir Pentchev, G. J. Lolos, J. Reinhold, A. J. Sarty, Rolf Ent, G. Niculescu, J. Volmer, J. Roche, Toshinobu Miyoshi, G. M. Huber, V. A. Punjabi, D. G. Meekins, E. J. Brash, E. J. Beise, M. Carmignotto, D. H. Potterveld, J. Arrington, K. A. Aniol, Richard Trotta, Y. Okayasu, Ian L. Pegg, P. M. King, Pete Markowitz, M. K. Jones, Brynle Barrett, C. F. Perdrisat, A. Dittmann, Geoffrey Smith, H. Mkrtchyan, D. Gaskell, X. Zheng, Shaikh Faruque Ali, and Student Lab and Education
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perturbation theory [quantum chromodynamics] ,Particle physics ,Meson ,interference ,Regge ,FOS: Physical sciences ,Parton ,nucl-ex ,Atomic ,01 natural sciences ,Cross section (physics) ,momentum transfer [form factor] ,Particle and Plasma Physics ,Pion ,Factorization ,0103 physical sciences ,ddc:530 ,Nuclear ,Nuclear Experiment (nucl-ex) ,010306 general physics ,Nuclear Experiment ,form factor [K] ,Quantum chromodynamics ,Physics ,distribution amplitude [parton] ,+electron+K%2B+Lambda%22">electron p --> electron K+ Lambda ,model ,factorization [quantum chromodynamics] ,010308 nuclear & particles physics ,Form factor (quantum field theory) ,Molecular ,Perturbative QCD ,Nuclear & Particles Physics ,transverse [cross section] ,electroproduction [K] ,High Energy Physics::Experiment ,longitudinal [cross section] ,distribution function [parton] ,experimental results ,Jefferson Lab - Abstract
The H1(e,e′K+)Λ reaction was studied as a function of the Mandelstam variable -t using data from the E01-004 (FPI-2) and E93-018 experiments that were carried out in Hall C at the 6 GeV Jefferson Laboratory. The cross section was fully separated into longitudinal and transverse components, and two interference terms at four-momentum transfers Q2 of 1.00, 1.36, and 2.07GeV2. The kaon form factor was extracted from the longitudinal cross section using the Regge model by Vanderhaeghen et al. [Phys. Rev. C 57, 1454 (1998)PRVCAN0556-281310.1103/PhysRevC.57.1454]. The results establish the method, previously used successfully for pion analyses, for extracting the kaon form factor. Data from 12 GeV Jefferson Laboratory experiments are expected to have sufficient precision to distinguish between theoretical predictions, for example, recent perturbative QCD calculations with modern parton distribution amplitudes. The leading-twist behavior for light mesons is predicted to set in for values of Q2 between 5 and 10GeV2, which makes data in the few-GeV regime particularly interesting. The Q2 dependence at fixed x and -t of the longitudinal cross section that we extracted seems consistent with the QCD factorization prediction within the experimental uncertainty.
- Published
- 2018
- Full Text
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14. Scenarios and Spectra Set for CTBT OSI Information Barrier Testing
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Glen A. Warren and Brian D. Milbrath
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Set (abstract data type) ,Environmental science ,Data mining ,computer.software_genre ,computer ,Spectral line - Published
- 2017
15. A program to generate simulated radioxenon beta–gamma data for concentration verification and validation and training exercises
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Amanda M. Prinke, Glen A. Warren, Brian T. Schrom, A. Ringbom, Thomas J. Suckow, Matthew W. Cooper, and Justin I. McIntyre
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Dead sea ,010308 nuclear & particles physics ,BETA (programming language) ,business.industry ,Computer science ,Health, Toxicology and Mutagenesis ,Public Health, Environmental and Occupational Health ,Training (meteorology) ,010403 inorganic & nuclear chemistry ,01 natural sciences ,Pollution ,Field (computer science) ,0104 chemical sciences ,Analytical Chemistry ,Nuclear Energy and Engineering ,0103 physical sciences ,Radiology, Nuclear Medicine and imaging ,Decay chain ,Nuclear medicine ,business ,computer ,Spectroscopy ,Simulation ,Verification and validation ,computer.programming_language - Abstract
PNNL developed a beta–gamma simulator (BGSim) that incorporated GEANT-modeled data sets from radioxenon decay chains, as well as functionality to use nuclear detector-acquired data sets to create new beta–gamma spectra with varying amounts of background, 133Xe, 131mXe, 133mXe, 135Xe, and 222Rn and its decay products. After BGSim was developed, additional uses began to be identified for the program output: training sets of two-dimensional spectra for data analysts at the IDC and other NDC, and spectra for exercises such as the Integrated Field Exercise 2014 held in Jordan at the Dead Sea.
- Published
- 2015
16. Development of a low background liquid scintillation counter for a shallow underground laboratory
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Shannon M. Morley, Craig E. Aalseth, Michael E. Wright, Erin S. Fuller, Matthew Douglas, Glen A. Warren, Bruce E. Bernacki, Mark E. Panisko, John L. Orrell, Russell O. Williams, Jennifer L. Erchinger, Crystal A. Mullen, and Martin E. Keillor
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Physics - Instrumentation and Detectors ,Radiation ,Physics::Instrumentation and Detectors ,Nuclear engineering ,Liquid scintillation counting ,FOS: Physical sciences ,Instrumentation and Detectors (physics.ins-det) ,complex mixtures ,Charged particle ,Nuclear physics ,Overburden ,Shield ,Scintillation counter ,Underground laboratory ,Environmental science ,Nuclear Experiment (nucl-ex) ,Nuclear Experiment ,National laboratory - Abstract
Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of low-concentration levels of radioactive isotopes in samples collected from the environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., $\beta$, $\alpha$) emitting isotopes with no (or very weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately-designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35 meters-water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the scintillation counter's shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements.
- Published
- 2015
- Full Text
- View/download PDF
17. Liquid scintillation counting of environmental radionuclides: a review of the impact of background reduction
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Erin C. Finn, Bruce E. Bernacki, Glen A. Warren, Crystal A. Mullen, Michael E. Wright, Martin E. Keillor, Shannon M. Morley, Erin S. Fuller, Matthew Douglas, Eric W. Hoppe, John L. Orrell, Jennifer L. Erchinger, and Mark E. Panisko
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Radionuclide ,Chemistry ,Health, Toxicology and Mutagenesis ,Nuclear engineering ,Radiochemistry ,Liquid scintillation counting ,Public Health, Environmental and Occupational Health ,010403 inorganic & nuclear chemistry ,01 natural sciences ,Pollution ,030218 nuclear medicine & medical imaging ,0104 chemical sciences ,Analytical Chemistry ,Reduction (complexity) ,03 medical and health sciences ,0302 clinical medicine ,Nuclear Energy and Engineering ,Scintillation counter ,Radiology, Nuclear Medicine and imaging ,sense organs ,National laboratory ,Spectroscopy - Abstract
Liquid scintillation counting (LSC) supports a range of environmental science measurements. At Pacific Northwest National Laboratory, we are constructing an LSC system with an expected background reduction of 10–100 relative to values reported in the literature. In this paper, a number of current measurement applications of LSC have been considered with an emphasis on determining which aspects of such measurements would gain the greatest benefit: improved minimum detectable activity (MDA), reduction in sample size, and reduction in total analysis time.
- Published
- 2015
18. Real-time stack monitoring at the BaTek medical isotope production facility
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Michael D. Ripplinger, Johannes Robert Dumais, William A. Sliger, Vincent T. Woods, Justin I. McIntyre, Agung Agusbudiman, Amanda M. Prinke, K. Khrustalev, Harry S. Miley, Abdelhakim Gheddou, Paul W. Eslinger, Pujadi Marsoem, Gatot Suhariyono, Susilo Widodo, Ulrich Stoehlker, Mika Nikkinen, Glen A. Warren, Brian T. Schrom, and Ian M. Cameron
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Waste management ,Health, Toxicology and Mutagenesis ,Radiochemistry ,Public Health, Environmental and Occupational Health ,Monitoring system ,Background concentrations ,010502 geochemistry & geophysics ,010403 inorganic & nuclear chemistry ,01 natural sciences ,Pollution ,0104 chemical sciences ,Analytical Chemistry ,Nuclear Energy and Engineering ,Stack (abstract data type) ,Environmental science ,Production (economics) ,Radiology, Nuclear Medicine and imaging ,National laboratory ,Spectroscopy ,0105 earth and related environmental sciences - Abstract
Radioxenon emissions from fission-based radiopharmaceutical production are a major source of background concentrations affecting the radioxenon detection systems of the international monitoring system (IMS). Collection of real-time emissions data from production facilities makes it possible to screen out some medical isotope signatures from the IMS radioxenon data sets. This paper describes an effort to obtain and analyze real-time stack emissions data with the design, construction and installation of a small stack monitoring system developed by a joint CTBTO-IDC, BATAN, and Pacific Northwest National Laboratory team at the BaTek medical isotope production facility near Jakarta, Indonesia.
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- 2015
19. Lead Slowing-Down Spectrometry Analysis of Data from Measurements on Nuclear Fuel
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Glen A. Warren, Adam Weltz, Jonathan A. Kulisek, A. Gavron, Jason Harris, Trevor N. Stewart, Yaron Danon, and Kevin K. Anderson
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Lead (geology) ,Nuclear Energy and Engineering ,Nuclear fuel ,Nuclear safeguards ,Nuclear engineering ,Environmental science ,Nondestructive assay ,Mass spectrometry ,health care economics and organizations ,Spent nuclear fuel - Abstract
Improved nondestructive assay of isotopic masses in used nuclear fuel would be valuable for nuclear safeguards operations associated with the transport, storage, and reprocessing of used nuclear fu...
- Published
- 2015
20. Detectors for Accelerator-Based Security Applications
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Erin A. Miller, Sean C. Stave, and Glen A. Warren
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business.industry ,Computer science ,Electromagnetic shielding ,SIGNAL (programming language) ,Detector ,Stockpile ,business ,Interdiction ,High input ,Computer hardware ,Spent nuclear fuel ,Earth-Surface Processes - Abstract
We present a review of detector systems used in accelerator-based security applications. The applications discussed span stockpile stewardship, material interdiction, treaty verification, and spent nuclear fuel assay. The challenge for detectors in accelerator-based applications is the separation of the desired signal from the background, frequently during high input count rates. Typical techniques to address the background challenge include shielding, timing, selection of sensitive materials, and choice of accelerator.
- Published
- 2015
21. Impact of Monoenergetic Photon Sources on Nonproliferation Applications Final Report
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John Valentine, Bernhard Ludewigt, Glen A. Warren, Marie-Anne Descalle, Matt Kinlaw, Sara A. Pozzi, Cameron A. Miller, David Chichester, Cameron Geddes, Brian J. Quiter, and Scott J. Thompson
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Physics ,Nuclear physics ,Photon ,Nuclear engineering - Published
- 2017
22. Assessment of Impact of Monoenergetic Photon Sources on Prioritized Nonproliferation Applications: Simulation Study Report
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Sara A. Pozzi, Matt Kinlaw, Cameron A. Miller, Brian J. Quiter, Cameron Geddes, David Chichester, Scott J. Thompson, Glen A. Warren, Marie-Anne Descalle, John Valentine, and Bernhard Ludewigt
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Photon ,Study report ,Computer science ,Nuclear engineering - Published
- 2016
23. Assaying Used Nuclear Fuel Assemblies Using Lead Slowing-Down Spectroscopy and Singular Value Decomposition
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Christopher J. Gesh, Glen A. Warren, Kevin K. Anderson, Jonathan A. Kulisek, and Andrew M. Casella
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Nuclear and High Energy Physics ,Engineering ,Fissile material ,business.industry ,Nuclear engineering ,Monte Carlo method ,Nuclear reactor ,Spent nuclear fuel ,Matrix decomposition ,law.invention ,Neutron spectroscopy ,Nuclear Energy and Engineering ,law ,Singular value decomposition ,Calibration ,Electrical and Electronic Engineering ,business - Abstract
This study investigates the use of a Lead Slowing-Down Spectrometer (LSDS) for the direct and independent measurement of fissile isotopes in light-water nuclear reactor fuel assemblies. The current study applies MCNPX, a Monte Carlo radiation transport code, to simulate the measurement of the assay of the used nuclear fuel assemblies in the LSDS. An empirical model has been developed based on the calibration of the LSDS to responses generated from the simulated assay of six well-characterized fuel assemblies. The effects of self-shielding are taken into account by using empirical basis vectors calculated from the singular value decomposition (SVD) of a matrix containing the self-shielding functions from the assay of assemblies in the calibration set. The performance of the empirical algorithm was tested on version 1 of the Next-Generation Safeguards Initiative (NGSI) used fuel library consisting of 64 assemblies, as well as a set of 27 diversion assemblies, both of which were developed by Los Alamos National Laboratory. The potential for direct and independent assay of the sum of the masses of Pu-239 and Pu-241 to within 2%, on average, has been demonstrated.
- Published
- 2013
24. Requirements for testing of active interrogation systems
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Glen A. Warren, Richard T. Kouzes, and Peter John Chiaro Jr
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Engineering ,Cargo container ,Fissile material ,business.industry ,Acoustics ,Special nuclear material ,External beam radiation ,Electrical engineering ,Interrogation ,Object (computer science) ,business - Abstract
ACTIVE-INTERROGATION (AI) systems automatically determine if special nuclear material (SNM) is present in an object (e.g., an intermodal cargo container) by observing the radiation emitted by the object when it has been exposed to an external radiation source. Active interrogation systems range from those that only indicate the presence of high-Z materials, to fissionable material detection, to those that detect specific SNM materials [1].
- Published
- 2016
25. Background characterization of an ultra-low background liquid scintillation counter
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Craig M. Marianno, John L. Orrell, Craig E. Aalseth, Crystal A. Mullen, Glen A. Warren, Martin E. Keillor, Bruce E. Bernacki, M. Douglas, Mark E. Panisko, Shannon M. Morley, Erin S. Fuller, and Jennifer L. Erchinger
- Subjects
Physics ,Radiation ,business.industry ,Orders of magnitude (temperature) ,Liquid scintillation counting ,010403 inorganic & nuclear chemistry ,01 natural sciences ,0104 chemical sciences ,Characterization (materials science) ,010309 optics ,Nuclear physics ,Optics ,0103 physical sciences ,Scintillation counter ,National laboratory ,business - Abstract
The Ultra-Low Background Liquid Scintillation Counter developed by Pacific Northwest National Laboratory will expand the application of liquid scintillation counting by enabling lower detection limits and smaller sample volumes. By reducing the overall count rate of the background environment approximately 2 orders of magnitude below that of commercially available systems, backgrounds on the order of tens of counts per day over an energy range of ~3–3600 keV can be realized. Initial test results of the ULB LSC show promising results for ultra-low background detection with liquid scintillation counting.
- Published
- 2016
26. Further developments of a robust absolute calibration method utilizing beta/gamma coincidence techniques
- Author
-
Brian T. Schrom, James H. Ely, Glen A. Warren, Derek A. Haas, Justin I. McIntyre, and Matthew W. Cooper
- Subjects
Chemistry ,business.industry ,Health, Toxicology and Mutagenesis ,Nuclear engineering ,Detector ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Extrapolation ,Pollution ,Particle detector ,Analytical Chemistry ,Nuclear Energy and Engineering ,Range (statistics) ,Calibration ,Radiation monitoring ,Radiology, Nuclear Medicine and imaging ,Radiation protection ,business ,Spectroscopy ,Energy (signal processing) - Abstract
Performing accurate and verifiable measurements is often the most challenging goal for any radiation detector and is especially challenging for the radio-xenon detectors deployed by the International Monitoring System (IMS) of the Preparatory Commission of the Comprehensive Test Ban Treaty Organization (CTBTO). Often the accuracy of the measurement is directly tied to how well the detector is calibrated, in both energy and efficiency. Standard methods often rely on using certified sealed sources to determine the absolute efficiency. Similarly, efforts to calibrate the absolute efficiency of radioactive gas cell detectors utilize a number of methodologies which allow adequate calibration but are time consuming and prone to a host of difficulties to determine uncertainties (McIntyre et al, J Radioanal Nucl Chem 282(3):755–759, 2009; Anderson et al, Stat Probab Lett 77(88):769–773, 2007). Utilizing methods developed in the 1960s for absolute measurements of activity with beta–gamma detector systems it has become clear that it is possible to achieve higher precision results that are consistent across a range of isotopes and activities (National Council on Radiation Protection and Measurement, A handbook of radioactivity measurements procedure NCPR report, 1985). Even more compelling is the ease with which this process can be used on routine samples to determine the total activity present in the detector. Additionally, recent advances in the generation of isotopically pure radio-xenon samples of 131mXe, 133Xe, and 135Xe allow these measurement techniques to achieve much better results than have previously been possible when using mixed isotopic radio-xenon sources (Haas et al, J Radioanal Nucl Chem 282(3):677–680, 2009). This paper will discuss the beta/gamma absolute detection efficiency techniques of direct measurement of the efficiencies and the extrapolation method and compare the results using modeled and measured pure sources of 133Xe and 135Xe.
- Published
- 2012
27. New concepts for radiometric measurements of environmental samples
- Author
-
Robert C. Runkle and Glen A. Warren
- Subjects
Fission products ,Health, Toxicology and Mutagenesis ,System of measurement ,Detector ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Sampling (statistics) ,chemistry.chemical_element ,Pollution ,Particle detector ,Analytical Chemistry ,Plutonium ,Nuclear Energy and Engineering ,Interference (communication) ,chemistry ,Environmental science ,Radiology, Nuclear Medicine and imaging ,Coincidence counting ,Spectroscopy ,Remote sensing - Abstract
The Radiation Detection and Nuclear Sciences Group at Pacific Northwest National Laboratory has a long history in conducting measurements of radioisotopes for various applications. This experience includes ultra-low background measurements, arrays of germanium detectors, automated sampling and measurement systems and coincidence measurement systems. A recent lab-supported effort has been studying how these capabilities, both in terms of hardware and experience, can be leveraged to enable environmental sampling measurements. One area of interest is the release of fission products and actinides into the environment from a reactor incident. While the initial survey of this area is still under way, one isotope of interest that surfaced early in the study is 238Pu. Existing techniques to assay this isotope suffer from measurement challenges. In alpha counting, there can be significant interference with 241Am, while in mass spectrometry, there can be interference with 238U. The authors are developing the concept for a detector that through coincidence counting techniques can distinguish 238Pu and 241Am. In addition, we will design the system to conduct radiometric measurements of other plutonium isotopes to enable a direct comparison of those isotopes. We will present our concept of the detector system for 238Pu, as well as discuss other radiometric measurements of fission products and actinides with which we intend to advance the state of the art for environmental measurements.
- Published
- 2012
28. The design, construction, and initial characterization of an ultra-low-background gas-proportional counting system
- Author
-
Glen A. Warren, Anthony R. Day, Martin E. Keillor, Craig E. Aalseth, Cory T. Overman, Erin S. Fuller, Eric W. Hoppe, Allen Seifert, and Emily K. Mace
- Subjects
Health, Toxicology and Mutagenesis ,Nuclear engineering ,Detector ,Public Health, Environmental and Occupational Health ,chemistry.chemical_element ,Proportional counter ,Radon ,Scintillator ,Pollution ,Neutron temperature ,Particle detector ,Analytical Chemistry ,Nuclear Energy and Engineering ,chemistry ,Electromagnetic shielding ,Measuring instrument ,Environmental science ,Radiology, Nuclear Medicine and imaging ,Spectroscopy - Abstract
Over the past several years, the Pacific Northwest National Laboratory (PNNL) has developed an ultra-low-background proportional counter (ULBPC) technology. The resulting detector is the product of an effort to produce a low-background, physically robust gas proportional counter for applications like radon emanation measurements, groundwater tritium, and 37Ar. In order to fully take advantage of the inherent low-background properties designed into the ULBPC, a comparably low-background dedicated counting system is required. An ultra-low-background counting system (ULBCS) was recently built in the new shallow underground laboratory at PNNL. With a design depth of 30 m water-equivalent, the shallow underground laboratory provides approximately 100× fewer fast neutrons and 6× fewer muons than a surface location. The ULBCS itself provides additional shielding in the form of active anti-cosmic veto (via 2-in-thick plastic scintillator paddles) and passive borated poly (1 in.), lead (6 in.), and copper (~3 in.) shielding. This work will provide details on PNNL’s new shallow underground laboratory, examine the motivation for the design of the counting system, and provide results from the characterization of the ULBCS, including initial detector background.
- Published
- 2012
29. Digital pulse-shape discrimination applied to an ultra-low-background gas-proportional counting system: first results
- Author
-
A.W. Myers, Mark E. Panisko, Glen A. Warren, Anthony R. Day, Martin E. Keillor, Richard M. Williams, Emily K. Mace, Cory T. Overman, Craig E. Aalseth, Erin S. Fuller, Eric W. Hoppe, and Allen Seifert
- Subjects
Physics ,Signal processing ,Health, Toxicology and Mutagenesis ,Acoustics ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Proportional counter ,Context (language use) ,Pollution ,Sample (graphics) ,Particle detector ,Analytical Chemistry ,Nuclear Energy and Engineering ,Measuring instrument ,Radiology, Nuclear Medicine and imaging ,Sensitivity (control systems) ,Spectroscopy ,Background radiation - Abstract
A new ultra-low-background proportional counter design was recently developed at Pacific Northwest National Laboratory (PNNL). This design, along with an ultra-low-background counting system which provides passive and active shielding with radon exclusion, has been developed to complement a new shallow underground laboratory (~30 m water-equivalent) constructed at PNNL. After these steps to mitigate dominant backgrounds (cosmic rays, external gamma-rays, radioactivity in materials), remaining background events do not exclusively arise from ionization of the proportional counter gas. Digital pulse-shape discrimination (PSD) is thus employed to further improve measurement sensitivity. In this work, a template shape is generated for each individual sample measurement of interest, a “self-calibrating” template. Differences in event topology can also cause differences in pulse shape. In this work, the temporal region analyzed for each event is refined to maximize background discrimination while avoiding unwanted sensitivity to event topology. This digital PSD method is applied to sample and background data, and initial measurement results from a biofuel methane sample are presented in the context of low-background measurements currently being developed.
- Published
- 2012
30. On the Search for Nuclear Resonance Fluorescence Signatures of $^{235}{\rm U}$ and $^{238}{\rm U}$ Above 3 MeV
- Author
-
Robert J. Ledoux, Glen A. Warren, Joseph A. Caggiano, William H. Park, Stephen E. Korbly, and William Bertozzi
- Subjects
Physics ,Nuclear and High Energy Physics ,Gamma ray ,Bremsstrahlung ,Resonance ,chemistry.chemical_element ,Uranium ,Enriched uranium ,Particle detector ,Nuclear physics ,Nuclear Energy and Engineering ,Resonance fluorescence ,chemistry ,Nuclear resonance fluorescence ,Electrical and Electronic Engineering ,Nuclear Experiment - Abstract
Nuclear resonance fluorescence is a physical process that provides an isotope-specific signature that could be used for the identification and characterization of materials. The technique involves the detection of prompt discrete-energy photons emitted from a sample that is exposed to photons in the MeV energy range. Potential applications of the technique range from detection of high explosives to characterization of special nuclear materials such as 235U. Pacific Northwest National Laboratory and Passport Systems have collaborated to conduct a a pair of measurements to search for a nuclear resonance fluorescence response of 235U above 3 MeV and of 238U above 5 MeV using an 8 g sample of highly enriched uranium and a 90 g sample of depleted uranium. No new signatures were observed. The minimum detectable integrated cross section for 235U is presented.
- Published
- 2010
31. Design and construction of an ultra-low-background 14-crystal germanium array for high efficiency and coincidence measurements
- Author
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James E. Fast, Brian J. Hyronimus, Glen A. Warren, Allen Seifert, Eric W. Hoppe, Harry S. Miley, Anthony R. Day, Martin E. Keillor, Todd W. Hossbach, and Craig E. Aalseth
- Subjects
Cryostat ,Physics ,Spectrum analyzer ,business.industry ,Health, Toxicology and Mutagenesis ,Detector ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Pollution ,Analytical Chemistry ,Semiconductor detector ,Optics ,Nuclear Energy and Engineering ,Cleanroom ,Radiology, Nuclear Medicine and imaging ,Gamma spectroscopy ,business ,Sensitivity (electronics) ,Active filter ,Spectroscopy - Abstract
Physics experiments, environmental surveillance, and treaty verification techniques continue to require increased sensitivity for detecting and quantifying radionuclides of interest. This can be done by detecting a greater fraction of gamma emissions from a sample (higher detection efficiency) and reducing instrument backgrounds. A current effort for increased sensitivity in high resolution gamma spectroscopy will produce an intrinsic germanium (HPGe) array designed for high detection efficiency, ultra-low-background performance, and useful coincidence efficiencies. The system design is optimized to accommodate filter paper samples, e.g. samples collected by the Radionuclide Aerosol Sampler/Analyzer (RASA). The system will provide high sensitivity for weak collections on atmospheric filter samples, as well as offering the potential to gather additional information from more active filters using gamma cascade coincidence detection. The current effort is constructing an ultra-low-background HPGe crystal array consisting of two vacuum cryostats, each housing a hexagonal array of 7 crystals on the order of 70% relative efficiency per crystal. Traditional methods for constructing ultra-low-background detectors are used, including use of materials known to be low in radioactive contaminants, use of ultra pure reagents, clean room assembly, etc. The cryostat will be constructed mainly from copper electroformed into near-final geometry at PNNL. Details of the detector design, simulation of efficiency and coincidence performance, HPGe crystal testing, and progress on cryostat construction are presented.
- Published
- 2009
32. Design and construction of a low-background, internal-source proportional counter
- Author
-
Todd W. Hossbach, Anthony R. Day, Martin E. Keillor, Eric W. Hoppe, Brian J. Hyronimus, Kevin E. Litke, Allen Seifert, Esther E. Mintzer, Glen A. Warren, and Craig E. Aalseth
- Subjects
Physics ,Spectrometer ,Health, Toxicology and Mutagenesis ,Nuclear engineering ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Proportional counter ,chemistry.chemical_element ,Pollution ,Copper ,Particle detector ,Analytical Chemistry ,Semiconductor detector ,Nuclear Energy and Engineering ,chemistry ,Electroforming ,Thermal ,Measuring instrument ,Radiology, Nuclear Medicine and imaging ,Spectroscopy - Abstract
High-purity copper has emerged as a preferred construction material for ultra-low-background HPGe spectrometers and offers excellent bulk radiopurity along with good electrical, thermal, and vacuum properties. Recently, these materials and techniques have been applied to the construction of low-background internal-source gas proportional counters. This work describes the design, construction, and testing of an ultra-low-background internal-source gas proportional counter built primarily of high purity electroformed copper. Energy resolution of ~10% FWHM at 59.5 keV has been achieved, a low-energy threshold of ~3 keV has been reached, and gas gain stability over a 4-week period has been demonstrated. Progress toward low-background operation is described.
- Published
- 2009
33. A High-Efficiency Fieldable Germanium Detector Array
- Author
-
Glen A. Warren, Brian J. Hyronimus, James E. Fast, Craig E. Aalseth, Todd W. Hossbach, Joseph A. Caggiano, Robert C. Runkle, Erin S. Fuller, and Anthony R. Day
- Subjects
Cryostat ,Nuclear and High Energy Physics ,Materials science ,business.industry ,Detector ,chemistry.chemical_element ,Germanium ,Cryogenics ,Semiconductor detector ,Germanium radiation detectors ,Nuclear Energy and Engineering ,chemistry ,Optoelectronics ,Electrical and Electronic Engineering ,business ,Hpge detector - Abstract
Historically, large germanium arrays for field applications have consisted of multiple detectors each housed in their own cryostat. In order to ruggedize the detectors for field use these cryostats have had additional support material introduced that significantly impacted cryogenic performance. This paper presents the development of a new cryostat design suitable for deployment of ~10 kg of high purity germanium detectors that achieves outstanding cryogenic performance (~5 W at 80 K) while providing the high detection efficiency required for stand-off measurements and the ruggedization required for use in a variety of field applications.
- Published
- 2009
34. A method for removing surface contamination on ultra-pure copper spectrometer components
- Author
-
Harry S. Miley, Justin I. McIntyre, Eric W. Hoppe, Anthony R. Day, Craig E. Aalseth, Orville T. Farmer, Glen A. Warren, John E. Smart, Allen Seifert, and Todd W. Hossbach
- Subjects
Spectrometer ,Chemistry ,Health, Toxicology and Mutagenesis ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Proportional counter ,Contamination ,Pollution ,Analytical Chemistry ,Nuclear Energy and Engineering ,Double beta decay ,Electromagnetic shielding ,Measuring instrument ,Radiology, Nuclear Medicine and imaging ,Decay chain ,Spectroscopy ,Radioactive decay - Abstract
Spectrometers for the lowest-level radiometric measurements require materials of extreme radiopurity. Measurements of rare nuclear decays, e.g., neutrinoless double-beta decay, can require construction and shielding materials with bulk radiopurity reaching one micro-Becquerel per kilogram or less. When such extreme material purity is achieved, surface contamination, particularly solid daughters in the natural radon decay chains, can become the limiting background. High-purity copper is an important material for ultra-low-background spectrometers and thus is the focus of this work. A method for removing surface contamination at very low levels without attacking the bulk material is described. An assay method using a low-background proportional counter made of the material under examination is employed, and the preliminary result of achievable surface contamination levels is presented.
- Published
- 2008
35. Modeling of gamma-ray spectra to direct efficient chemical separations
- Author
-
Craig E. Aalseth, Matthew Douglas, Paula P. Bachelor, Judah I. Friese, Orville T. Farmer, Glen A. Warren, Andrea D. Choiniere, and Shannon M. Schulte
- Subjects
Fission products ,Nuclear fission product ,Isotope ,Chemistry ,Astrophysics::High Energy Astrophysical Phenomena ,Health, Toxicology and Mutagenesis ,Nuclear engineering ,Public Health, Environmental and Occupational Health ,Analytical chemistry ,Fission product yield ,Pollution ,Spectral line ,Analytical Chemistry ,Chemical separation ,Nuclear Energy and Engineering ,Interference (communication) ,Coincident ,Radiology, Nuclear Medicine and imaging ,Spectroscopy - Abstract
A project has been undertaken at Pacific Northwest National Laboratory (PNNL) to tailor a series of efficient chemical separations to allow the rapid quantification of gamma-ray emitting isotopes in mixed fission product (MFP) samples. In support of that goal, modeling of singles and coincident gamma-ray spectra that would result from various chemical separation strategies has been performed. These simulated spectra have identified likely instances of spectral interference and have provided an estimate of the time window available for the detection of radionuclides following various chemical separation schemes. A description of results to date is presented here, demonstrating the utility of this approach for improved processing and analysis of fission product samples.
- Published
- 2008
36. Prompt determination of evacuee radiation dose from a nuclear event
- Author
-
Richard W. Perkins, Justin I. McIntyre, Judah I. Friese, Paula P. Bachelor, Glen A. Warren, Craig E. Aalseth, and Harry S. Miley
- Subjects
medicine.medical_specialty ,business.industry ,Health, Toxicology and Mutagenesis ,Public Health, Environmental and Occupational Health ,Radiation ,Neutron radiation ,Pollution ,Triage ,Analytical Chemistry ,Radiation exposure ,Nuclear Energy and Engineering ,medicine ,Neutron source ,Radiology, Nuclear Medicine and imaging ,Medical physics ,Neutron ,Neutron activation analysis ,Radiation protection ,Nuclear medicine ,business ,Spectroscopy - Abstract
In anticipation of a nuclear detonation, techniques to quickly assess the radiation exposure of evacuees should be developed. Based on experience relating neutron radiation exposures to activation products, measurement of activation products can be performed in a few minutes. Personal items exposed to significant levels of radiation allows neutron dose assessment via the activation products. This approach allows prompt collection of important data on human exposure following a nuclear attack. Data collected will facilitate triage decisions for emergency medical treatment to ameliorate the radiation effects on exposed individuals. Activation experiments with everyday items exposed to a neutron source are presented.
- Published
- 2008
37. Use of electrodeposition for sample preparation and rejection rate prediction for assay of electroformed ultra high purity copper for 232Th and 238U prior to inductively coupled plasma mass spectrometry (ICP/MS)
- Author
-
Orville T. Farmer, John E. Smart, Todd W. Hossbach, Anthony R. Day, Esther E. Mintzer, Harry S. Miley, Eric W. Hoppe, Ronald L. Brodzinski, Glen A. Warren, Craig E. Aalseth, Justin I. McIntyre, and Allen Seifert
- Subjects
Chemistry ,Health, Toxicology and Mutagenesis ,Radiochemistry ,Public Health, Environmental and Occupational Health ,Thorium ,chemistry.chemical_element ,Uranium ,Pollution ,Copper ,Analytical Chemistry ,Nuclear Energy and Engineering ,Plating ,Electroforming ,Radiology, Nuclear Medicine and imaging ,Sample preparation ,Electroplating ,Inductively coupled plasma mass spectrometry ,Spectroscopy - Abstract
The search for neutrinoless double beta decay in 76Ge has driven the need for ultra-low background Ge detectors shielded by electroformed copper of ultra-high radiopurity (
- Published
- 2008
38. Cleaning and passivation of copper surfaces to remove surface radioactivity and prevent oxide formation
- Author
-
Allen Seifert, Harry S. Miley, Glen A. Warren, Kevin E. Litke, Justin I. McIntyre, Eric W. Hoppe, Todd W. Hossbach, Paula P. Bachelor, John E. Smart, Craig E. Aalseth, Danny J. Edwards, Shannon M. Schulte, and Anthony R. Day
- Subjects
Physics ,Nuclear and High Energy Physics ,Passivation ,Metallurgy ,Oxide ,chemistry.chemical_element ,Copper ,chemistry.chemical_compound ,chemistry ,Cleanroom ,Nitric acid ,Hydrogen peroxide ,Instrumentation ,Waste disposal ,Polonium - Abstract
High-purity copper is an attractive material for constructing ultra-low-background radiation measurement devices. Many low-background experiments using high-purity copper have indicated surface contamination emerges as the dominant background. Radon daughters plate out on exposed surfaces, leaving a residual 210Pb background that is difficult to avoid. Dust is also a problem; even under cleanroom conditions, the amount of U and Th deposited on surfaces can represent the largest remaining background. To control these backgrounds, a copper cleaning chemistry has been developed. Designed to replace an effective, but overly aggressive concentrated nitric acid etch, this peroxide-based solution allows for a more controlled cleaning of surfaces. The acidified hydrogen peroxide solution will generally target the Cu+/Cu2+ species which are the predominant surface participants, leaving the bulk of copper metal intact. This preserves the critical tolerances of parts and eliminates significant waste disposal issues. Accompanying passivation chemistry has also been developed that protects copper surfaces from oxidation. Using a high-activity polonium surface spike, the most difficult-to-remove daughter isotope of radon, the performance of these methods are quantified. © 2001 Elsevier Science. All rights reserved
- Published
- 2007
39. On-Site Inspection RadioIsotopic Spectroscopy (Osiris) System Development
- Author
-
N. G. Wilmer, Kenneth M. Krebs, Glen A. Warren, Brian D. Milbrath, Ann E. Egger, Gus J. Caffrey, and David V. Jordan
- Subjects
Engineering ,System development ,Fission products ,biology ,business.industry ,Nuclear engineering ,Field tests ,biology.organism_classification ,Data acquisition ,Forensic engineering ,Gamma spectroscopy ,Osiris ,business ,Spectroscopy - Published
- 2015
40. Optical design considerations for efficient light collection from liquid scintillation counters
- Author
-
Erin S. Fuller, Jennifer L. Erchinger, Mark E. Panisko, Matthew Douglas, Bruce E. Bernacki, Glen A. Warren, Shannon M. Morley, Crystal A. Mullen, John L. Orrell, Martin E. Keillor, and Michael E. Wright
- Subjects
Physics ,Scintillation ,Photomultiplier ,Naturally occurring radioactive material ,Physics::Instrumentation and Detectors ,business.industry ,Detector ,Liquid scintillation counting ,Atomic and Molecular Physics, and Optics ,Optics ,Scintillation counter ,Light emission ,Electrical and Electronic Engineering ,business ,Engineering (miscellaneous) ,Nonimaging optics - Abstract
Liquid scintillation counters measure charged particle-emitting radioactive isotopes and are used for environmental studies, nuclear chemistry, and life science. Alpha and beta emissions arising from the material under study interact with the scintillation cocktail to produce light. The prototypical liquid scintillation counter employs low-level photon-counting detectors to measure the arrival of the scintillation. For reliable operation, the counting instrument must convey the scintillation light to the detectors efficiently and predictably. Current best practices employ the use of two or more detectors for coincidence processing to discriminate true scintillation events from background events due to instrumental effects such as photomultiplier tube dark rates, tube flashing, or other light emission not generated in the scintillation cocktail vial. In low-background liquid scintillation counters, additional attention is paid to shielding the scintillation cocktail from naturally occurring radioactive material present in the laboratory and within the instrument’s construction materials. Low-background design is generally at odds with optimal light collection. This study presents the evolution of a light collection design for liquid scintillation counting (LSC) in a low-background shield. The basic approach to achieve both good light collection and a low-background measurement is described. The baseline signals arising from the scintillation vial are modeled and methods to efficiently collect scintillation light are presented as part of the development of a customized low-background, high-sensitivity LSC system.
- Published
- 2015
41. Determining activities of radionuclides from coincidence signatures
- Author
-
Andrei B. Valsan, Craig E. Aalseth, L. Eric Smith, Todd W. Hossbach, Glen A. Warren, and Edward Ellis
- Subjects
Nuclear physics ,Physics ,Nuclear and High Energy Physics ,Radionuclide ,Identification (information) ,Photon ,Isotope ,Physics::Instrumentation and Detectors ,Detector ,Spectral analysis ,Instrumentation ,Coincidence ,Signature (logic) - Abstract
The spectral analysis of simultaneously observed photons in separate detectors may provide an invaluable tool for radioisotope identification applications. A general recursive method to determine the activity of an isotope from the observed coincidence signature rate is discussed. The method coherently accounts for effects of true coincidence summing within a single detector and detection efficiencies. A verification of the approach with computer simulations is also discussed.
- Published
- 2006
42. Generalized multicoincidence analysis methods
- Author
-
Leon E. Smith, Craig E. Aalseth, Glen A. Warren, Wondwosen Mengesha, A.B. Valsan, and J.E. Ellis
- Subjects
Physics ,Nuclear and High Energy Physics ,Spectrometer ,Nuclear forensics ,Detector ,Scintillator ,Coincidence ,Semiconductor detector ,Nuclear physics ,Nuclear Energy and Engineering ,Coincident ,otorhinolaryngologic diseases ,sense organs ,Sample collection ,Electrical and Electronic Engineering ,Remote sensing - Abstract
The ability to conduct automated trace radionuclide analysis at or near the sample collection point would provide a valuable tool for emergency response, nuclear forensics and environmental monitoring. Pacific Northwest National Laboratory is developing systems for this purpose based on dual gamma-ray spectrometers, e.g. NaI(TI) or HPGe, combined with thin organic scintillator sensors to detect light charged particles. Translating the coincident signatures recorded by these systems, which include /spl beta//spl gamma/, /spl gamma//spl gamma/ and /spl beta//spl gamma//spl gamma/, into the concentration of detectable radionuclides in the sample requires generalized multicoincidence analysis tools. The development and validation of the Coincidence Lookup Library, which currently contains the probabilities of single and coincidence signatures from more than 420 isotopes, is described. Also discussed is a method to calculate the probability of observing a coincidence signature which incorporates true coincidence summing effects. These effects are particularly important for high-geometric-efficiency detection systems. Finally, a process for validating the integrated analysis software package is demonstrated using GEANT 4 simulations of the prototype detector systems.
- Published
- 2006
43. Final State Interaction Effects in 3He(e ,e'p)
- Author
-
Ernst-Wilhelm Otten, R. Skibiński, Werner Heil, P. Merle, Michael Seimetz, Ingo Sick, Hiroyuki Kamada, Simon Širca, R. Böhm, M. Weis, Ch. Normand, M. Kohl, A. Nogga, J. Bermuth, M. Potokar, Th. Walcher, H. Schmieden, W. Glöckle, M. Hauger, J.M. Friedrich, Jörg Schmiedeskamp, R. Neuhausen, M. O. Distler, Harald Merkel, J. Jourdan, Jacek Golak, Glen A. Warren, H. Wöhrle, A. Klein, D. Baumann, M. Zeier, M. Ding, Daniela Rohe, P. Bartsch, Th. Pospischil, C. Carasco, D. Bosnar, K. W. Krygier, G. Testa, U. Müller, Henryk Witała, and P. Jennewein
- Subjects
Physics ,Nuclear and High Energy Physics ,Current (mathematics) ,3He-structure ,010308 nuclear & particles physics ,Operator (physics) ,Continuum (design consultancy) ,Momentum transfer ,Kinematics ,State (functional analysis) ,01 natural sciences ,Exact solutions in general relativity ,Quantum mechanics ,Quantum electrodynamics ,0103 physical sciences ,Final-state interaction ,Polarized electron scattering ,010306 general physics ,Ground state - Abstract
Asymmetries in quasi-elastic 3 He ( e → , e ′ p ) have been measured at a momentum transfer of 0.67 (GeV/ c ) 2 and are compared to a calculation which takes into account relativistic kinematics in the final state and a relativistic one-body current operator. With an exact solution of the Faddeev equation for the 3 He -ground state and an approximate treatment of final state interactions in the continuum good agreement is found with the experimental data.
- Published
- 2003
44. Performance of a compact detector package for the out-of-plane spectrometer system
- Author
-
Nilanga Liyanage, Ricardo Alarcon, S. Dolfini, J. R. Comfort, S. Kowalski, J. Zhao, Shalev Gilad, C. Vellidis, S. Sobczynski, K. Joo, P. Bourgeois, K. A. Dow, J. Kirkpatrick, R. S. Hicks, T. McIlvain, A. Dooley, Costas N. Papanicolas, D. S. Dale, S. Georgakopoulos, C. Mertz, C. Tschalaer, S. B. Soong, I. Nakagawa, Jian-Ping Chen, E. Six, R. A. Miskimen, M. Farkhondeh, D. J. Margaziotis, J. R. Calarco, G. A. Peterson, W. Turchinetz, C. Kunz, Nikolaos Sparveris, M. O. Distler, D. R. Tieger, N. I. Kaloskamis, A. Hotta, Glen A. Warren, D. Jordan, J. Shaw, A. J. Sarty, Ross Milner, S. Stiliaris, F. Casagrande, T. Zwart, Tancredi Botto, M. Pavan, Aron M. Bernstein, Z.-L. Zhou, Joseph B. Mandeville, S. E. Williamson, Tadaaki Tamae, X. Jiang, M. Holtrop, S. Širca, W. Boeglin, Larry Weinstein, William Bertozzi, G. Tsentalovich, A. F. Ramirez, G. W. Dodson, Yutaro Sato, S. Stave, A. Karabarbounis, R. Beck, M. B. Epstein, A. Young, and D. Rowntree
- Subjects
Physics ,Nuclear physics ,Nuclear and High Energy Physics ,Pion ,Spectrometer ,Detector ,Compton scattering ,Electron ,Nuclear Experiment ,Instrumentation ,Electron scattering ,Linear particle accelerator ,Particle identification - Abstract
We report on the design and performance of compact detector packages currently installed in the four magnetic out-of-plane spectrometers for electron scattering experiments at the MIT-Bates Linear Accelerator Center. The detector packages have been designed to meet the mechanical requirements arising from out-of-plane particle detection. They offer good trajectory and momentum reconstruction, particle identification and time-of-flight measurements for electrons, pions, protons, and deuterons with large momentum bites and in broad kinematical ranges and high luminosities. The detectors have so far been used with great success in out-of-plane measurements of 12 C ( e → , e ′ p ) , 2 H ( e → , e ′ p ) , virtual Compton scattering below pion threshold and in studies of the N → Δ transition in both exclusive reaction channels 1 H ( e → , e ′ p ) π 0 and 1 H ( e → , e ′ π + )n .
- Published
- 2002
45. The horizontal drift chambers for the focal plane proton-polarimeter of the 3-spectrometer setup at MAMI
- Author
-
A. Kozlov, Glen A. Warren, P. Bartsch, J. Sanner, D. Baumann, M. Ding, Ronald Ransome, G. Rosner, K. W. Krygier, Michael Seimetz, Ingo Sick, S. Grözinger, Klemen Bohinc, M. Kahrau, Achim Richter, M. Weis, D. Elsner, O. Strähle, R. Geiges, Justin I. McIntyre, R. Neuhausen, F. Klein, N. Clawiter, U. Müller, I. Ewald, X. Q. Wu, P. König, S. Derber, Th. Walcher, A. Wagner, J.M. Friedrich, M. Hamdorf, P. Jennewein, R. Böhm, S. Hedicke, Th. Pospischil, S. Malov, A. Süle, P. Merle, M. Potokar, E. A. J. M. Offermann, A. Liesenfeld, H. Schmieden, Harald Merkel, J. Jourdan, H. Kramer, J. Lac, and M. O. Distler
- Subjects
Physics ,Nuclear and High Energy Physics ,Argon ,Proton ,Spectrometer ,Physics::Instrumentation and Detectors ,business.industry ,chemistry.chemical_element ,Polarimeter ,Cardinal point ,Optics ,chemistry ,business ,Instrumentation ,Image resolution - Abstract
Large-area horizontal drift chambers have been built for use in a proton polarimeter. A gas mixture of 20% argon and 80% ethane is used. The left–right assignment is achieved by measuring the difference of the signals induced on neighboring potential wires. A spatial resolution of 300 μm is achieved.
- Published
- 2002
46. Precise neutron magnetic form factors
- Author
-
Glen A. Warren, T. Petitjean, P. Bartsch, Ingo Sick, H. Schmieden, J.M. Friedrich, I. Ewald, Harald Merkel, Ch. Normand, J. Jourdan, D. Baumann, M. O. Distler, Klemen Bohinc, G. Rosner, G. Kubon, U. Mueller, Simon Širca, M. Hauger, M. Weis, M. ZeierJ. Zhao, W.U. Boeglin, R. Boehm, P. Jennewein, C. Carasco, P. Trueb, H. Woehrle, Daniela Rohe, Th. Pospischil, H. Anklin, K. W. Krygier, A. Wagner, A. Honegger, R. Neuhausen, Th. Walcher, B. Zihlmann, M. Potokar, A. Liesenfeld, and M. Kahrau
- Subjects
Nuclear physics ,Physics ,Momentum ,Nuclear and High Energy Physics ,Magnetic form factor ,Nucleon form factors ,FOS: Physical sciences ,Neutron ,Radius ,Neutron magnetic radius ,Nuclear Experiment (nucl-ex) ,Nuclear Experiment ,Value (mathematics) - Abstract
Precise data on the neutron magnetic form factor G_{mn} have been obtained with measurements of the ratio of cross sections of D(e,e'n) and D(e,e'p) up to momentum transfers of Q^2 = 0.9 (GeV/c)^2. Data with typical uncertainties of 1.5% are presented. These data allow for the first time to extract a precise value of the magnetic radius of the neutron., Comment: 10 pages, 2 figures, submitted to Physics Letters B
- Published
- 2002
47. Concepts for alpha coincidence detection
- Author
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G. Tatishvili, Michael P. Dion, Glen A. Warren, and Brian W. Miller
- Subjects
Physics ,Resolution (mass spectrometry) ,Health, Toxicology and Mutagenesis ,Public Health, Environmental and Occupational Health ,Alpha-particle spectroscopy ,Actinide ,Pollution ,Coincidence ,Analytical Chemistry ,Alpha (programming language) ,Nuclear Energy and Engineering ,Environmental monitoring ,Radiology, Nuclear Medicine and imaging ,Atomic physics ,Biological system ,Spectroscopy ,Energy (signal processing) ,Coincidence detection in neurobiology - Abstract
The effectiveness of conventional measurement techniques for environmental monitoring is limited by background and other interferences. We are exploring a new measurement approach involving the detection of α particles in coincidence with conversion electrons as a means to simultaneously assay environmental samples for multiple actinides without chemical separation. The initial target isotopes studied in this work are 238Pu, 239Pu, 240Pu and 241Am. We explore various aspects of the design, such as impact of the mounting of the source material, energy resolution requirements and impact of a background on isotopic uncertainties. We conclude that a dual gas-proportional counter and a dual-sided, large-area silicon detector could provide similar performance for the measurement scenario examined.
- Published
- 2014
48. Measurement of the Recoil Polarization in thep(e→,e′p→)π0Reaction at theΔ(1232)Resonance
- Author
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I. Ewald, Justin I. McIntyre, R. D. Ransome, Glen A. Warren, U. Müller, H. Schmieden, Th. Walcher, J.M. Friedrich, Michael Seimetz, Ingo Sick, D. Baumann, Harald Merkel, G. Rosner, Daniela Rohe, F. Klein, P. Bartsch, A. Wagner, J. Lac, Klemen Bohinc, S. Hedicke, M. O. Distler, M. Kahrau, P. Merle, R. Böhm, S. S. Kamalov, S. Širca, M. Ding, M. Weis, D. Elsner, A. Süle, R. Geiges, J. Bermuth, M. Potokar, L. Tiator, S. Derber, P. Jennewein, K. W. Krygier, Th. Pospischil, R. Neuhausen, A. Liesenfeld, and Dieter Drechsel
- Subjects
Physics ,Parallel kinematics ,Recoil proton ,Recoil ,General Physics and Astronomy ,Atomic physics ,Polarization (waves) - Abstract
The recoil proton polarization has been measured in the $p(\stackrel{\ensuremath{\rightarrow}}{e}{,e}^{\ensuremath{'}}\stackrel{\ensuremath{\rightarrow}}{p}){\ensuremath{\pi}}^{0}$ reaction in parallel kinematics around $W\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}1232\phantom{\rule{0ex}{0ex}}\mathrm{MeV}$, ${Q}^{2}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}0.121\phantom{\rule{0ex}{0ex}}(\mathrm{GeV}/c{)}^{2}$, and $\ensuremath{\epsilon}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}0.718$ using the polarized cw electron beam of the Mainz Microtron. All three proton polarization components, ${P}_{x}/{P}_{e}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}(\ensuremath{-}11.4\ifmmode\pm\else\textpm\fi{}1.3\ifmmode\pm\else\textpm\fi{}1.4)%$, ${P}_{y}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}(\ensuremath{-}43.1\ifmmode\pm\else\textpm\fi{}1.3\ifmmode\pm\else\textpm\fi{}2.2)%$, and ${P}_{z}/{P}_{e}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}(56.2\ifmmode\pm\else\textpm\fi{}1.5\ifmmode\pm\else\textpm\fi{}2.6)%$, could be measured simultaneously. The Coulomb quadrupole to magnetic dipole ratio, $\mathrm{CMR}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}(\ensuremath{-}6.4\ifmmode\pm\else\textpm\fi{}{0.7}_{\mathrm{stat}}\ifmmode\pm\else\textpm\fi{}{0.8}_{\mathrm{syst}})%$, was determined from ${P}_{x}$ in the framework of the Mainz Unitary Isobar Model. The consistency among the reduced polarizations and the extraction of the ratio of longitudinal-to-transverse response is discussed.
- Published
- 2001
49. A high-precision polarimeter
- Author
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J. Jourdan, B. Zihlmann, J. Zhao, T. Petitjean, Ingo Sick, D. Crabb, John C. Mitchell, A. Tobias, M. Zeier, Rolf Ent, Glen A. Warren, A. Honegger, G. Kubon, Daniela Rohe, H. Woehrle, and M. Hauger
- Subjects
Physics ,Nuclear and High Energy Physics ,Physics::Instrumentation and Detectors ,business.industry ,FOS: Physical sciences ,Polarimeter ,Electron ,Polarization (waves) ,Coincidence ,Superconducting solenoid ,Optics ,Physics::Atomic and Molecular Clusters ,Cathode ray ,Astrophysics::Solar and Stellar Astrophysics ,Physics::Accelerator Physics ,Nuclear Experiment (nucl-ex) ,Nuclear Experiment ,business ,Instrumentation ,Saturation (magnetic) - Abstract
We have built a polarimeter in order to measure the electron beam polarization in hall C at JLAB. Using a superconducting solenoid to drive the pure-iron target foil into saturation, and a symmetrical setup to detect the Moller electrons in coincidence, we achieve an accuracy of, 17 pages, 9 figures, submitted to N.I.M
- Published
- 2001
50. Polarization transfer in the 4HeH reaction
- Author
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Ronald Ransome, Glen A. Warren, James J. Kelly, D. Baumann, J.M. Friedrich, G. Rosner, Daniela Rohe, Michael Seimetz, C. Glashausser, Ingo Sick, Javier R. Vignote, Th. Pospischil, M. Weis, K. W. Krygier, R. Neuhausen, A. Wagner, S. Derber, Steffen Strauch, U. Müller, Klemen Bohinc, A. Liesenfeld, J. Bermuth, M. Kohl, Th. Walcher, R. Böhm, A. Kozlov, G. J. Kumbartzki, J. Lac, M. Hauger, P. Jennewein, M. O. Distler, M. Ding, Sonja Dieterich, P. Bartsch, Damir Bosnar, I. Ewald, J. Jourdan, J. M. Udías, H. Schmieden, Ronald Gilman, and Harald Merkel
- Subjects
Physics ,Nuclear and High Energy Physics ,Proton ,Scattering ,Nuclear Theory ,chemistry.chemical_element ,Polarization (waves) ,Nuclear physics ,Transverse plane ,chemistry ,Physics::Accelerator Physics ,Nuclear Experiment ,Microtron ,Helium - Abstract
Polarization transfer in the 4He ( e → ,e′ p → ) 3 H reaction at a Q2 of 0.4 (GeV/c)2 was measured at the Mainz Microtron MAMI. The ratio of the transverse to the longitudinal polarization components of the ejected protons was compared with the same ratio for elastic ep scattering. The results are consistent with a recent fully relativistic calculation which includes a predicted medium modification of the proton form factor based on a quark–meson coupling model.
- Published
- 2001
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