Search

Based on the favourable properties of previously used one-dimensional (1D) atomic model potentials, we introduce a novel 1D atomic model potential for the 1D simulation of the quantum dynamics of a single active electron atom driven by a strong, linearly polarized near-infrared laser pulse. By comparing numerical simulation results of typical strong-field physics scenarios in 1D and 3D, we show that this novel 1D model potential gives single atom HHG spectra with impressively increased accuracy for the most frequently used driving laser pulse parameters.

A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is independent from the excited material system to a large extent, and allows us to focus on the properties of the electromagnetic fields. Technically, the Hamiltonian known for parametric down-conversion is adopted, where photons in the $n$th harmonic mode are created in exchange of annihilating $n$ photons from the fundamental mode. In our treatment, initially the fundamental mode is in a coherent state corresponding to large photon numbers, while the high harmonic modes are in vacuum state. Due to the interaction, the latter modes get populated while the fundamental one loses photons. Analytical approximations are presented for the time evolution that are verified by numerically exact calculations. For multimode, finite bandwith excitation, the time dependence of the high-order harmonic radiation is also given.

We present a general mathematical procedure to handle interactions described by a Morse potential in the presence of a strong harmonic excitation. We account for permanent and field-induced terms and their gradients in the dipole moment function, and we derive analytic formulae for the bond-length change and for the shifted energy eigenvalues of the vibrations, by using the Kramers-Henneberger frame. We apply these results to the important cases of $\mathrm{H}_{2}$ and $\mathrm{LiH}$, driven by a near- or mid-infrared laser in the $10^{13}$ $\mathrm{ W/cm^2}$ intensity range.

We investigate the liberation of an atomic electron by a linearly polarized single-cycle near-infrared laser pulse having a peak intensity that ensures tunneling. Based on phase space analysis and energy distribution in the instantaneous potential, we reveal the importance of quantum interference between tunneling and over-the-barrier pathways of escape. Tunneling is blurred both in space and time, and the contribution of tunneling at the mean energy is almost negligible. We suggest and justify improved initial conditions for a classical particle approximation of strong-field ionization, based on the quantum momentum function, and we show how to reconstruct them from the detected momentum of an escaped electron.

We present results on the accurate one-dimensional (1D) modeling of simple atomic and molecular systems excited by strong laser fields. We use atomic model potentials that we derive from the corrections proposed earlier using the reduced ground state density of a three-dimensional (3D) single-active electron atom. The correction involves a change of the asymptotics of the 1D Coulomb model potentials while maintaining the correct ground state energy. We present three different applications of this method: we construct correct 1D models of the hydrogen molecular ion, the helium atom and the hydrogen molecule using improved parameters of existing soft-core Coulomb potential forms. We test these 1D models by comparing the corresponding numerical simulation results with their 3D counterparts in typical strong-field physics scenarios with near- and mid-infrared laser pulses, having peak intensities in the $10^{14}-10^{15}\,\mathrm{W/cm}^2$ range, and we find an impressively increased accuracy in the dynamics of the most important atomic quantities on the time scale of the excitation. We also present the high-order harmonic spectra of the He atom, computed using our 1D atomic model potentials. They show a very good match with the structure and phase obtained from the 3D simulations in an experimentally important range of excitation amplitudes.

We analyze tunnel ionization of a single atom based on the Wigner function over the classical phase space which inspires improved classical electron trajectories: these start with exit momenta based on the quantum momentum function and correspond very well to the subsequent quantum evolution. We derive an approximate analytic formula to reconstruct the tunnel exit time and exit momentum from electron momentum data that can be measured e.g. with a usual time-of-flight electron detector.

Based on a plausible requirement for the ground state density, we introduce a novel one-dimensional (1D) atomic model potential for the 1D simulation of the quantum dynamics of a single active electron atom driven by a strong, linearly polarized few-cycle laser pulse. The form of this density-based 1D model potential also suggests improved parameters for other well-known 1D model potentials. We test these 1D model potentials in numerical simulations of typical strong-field physics scenarios and we find an impressively increased accuracy of the low-frequency features of the most important physical quantities. The structure and the phase of the high-order harmonic spectra also have a very good match to those resulting from the three-dimensional simulations, which enables to fit the corresponding power spectra with the help of a simple scaling function.

A proposal for a novel source of isolated attosecond XUV -- soft X-ray pulses with a well controlled carrier-envelope phase difference (CEP) is presented in the framework of nonlinear Thomson-backscattering. Based on the analytic solution of the Newton-Lorentz equations, the motion of a relativistic electron is calculated explicitly, for head-on collision with an intense fs laser pulse. By using the received formulae, the collective spectrum and the corresponding temporal shape of the radiation emitted by a mono-energetic electron bunch can be easily computed. For certain suitable and realistic parameters, single-cycle isolated pulses of ca. 20 as length are predicted in the XUV -- soft X-ray spectral range, including the 2.33-4.37 nm water window. According to our analysis, the generated almost linearly polarized beam is extremely well collimated around the initial velocity of the electron bunch, with considerable intensity and with its CEP locked to that of the fs laser pulse., Comment: 11 pages, 6 figures, reviewed, corrected and extended work, regarding the intensity dependence of the emitted attosecond pulse

We investigate the time-evolution of quantum entanglement between an electron, liberated by a strong few-cycle laser pulse, and its parent ion-core. Since the standard procedure is numerically prohibitive in this case, we propose a novel way to quantify the quantum correlation in such a system: we use the reduced density matrices of the directional subspaces along the polarization of the laser pulse and along the transverse directions as building blocks for an approximate entanglement entropy. We present our results, based on accurate numerical simulations, in terms of several of these entropies, for selected values of the peak electric field strength and the carrier-envelope phase difference of the laser pulse. The time evolution of the mutual entropy of the electron and the ion-core motion along the direction of the laser polarization is similar to our earlier results based on a simple one-dimensional model. However, taking into account also the dynamics perpendicular to the laser polarization reveals a surprisingly different entanglement dynamics above the laser intensity range corresponding to pure tunneling: the quantum entanglement decreases with time in the over-the-barrier ionization regime.

We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier frequency. The time evolution of this secondary radiation is analyzed in terms of the expectation values of the photon number operators for a large number of electromagnetic modes that are initially in the vacuum state. Our method is based on a multimode version of the Jaynes-Cummings-Paul model and can be generalized to different radiating systems as well. We show, that after the exciting pulse, the final distribution of the photon numbers is close to the conventional (Fourier transform-based) power spectrum of the secondary radiation. The details of the high harmonic spectra are also analyzed, for many-cycle excitations a clear physical interpretation can be given in terms of the Floquet quasi-energies. A first step towards the determination of the photon statistics of the HHG modes reveals states with slightly super-Poissonian distribution., Comment: 9 pages, 6 figures, v2: minor changes according to the suggestions of the PRA referee

We present a novel numerical method and algorithm for the solution of the 3D axially symmetric time-dependent Schr\"odinger equation in cylindrical coordinates, involving singular Coulomb potential terms besides a smooth time-dependent potential. We use fourth order finite difference real space discretization, with special formulae for the arising Neumann and Robin boundary conditions along the symmetry axis. Our propagation algorithm is based on merging the method of the split-operator approximation of the exponential operator with the implicit equations of second order cylindrical 2D Crank-Nicolson scheme. We call this method hybrid splitting scheme because it inherits both the speed of the split step finite difference schemes and the robustness of the full Crank-Nicolson scheme. Based on a thorough error analysis, we verified both the fourth order accuracy of the spatial discretization in the optimal spatial step size range, and the fourth order scaling with the time step in the case of proper high order expressions of the split-operator. We demonstrate the performance and high accuracy of our hybrid splitting scheme by simulating optical tunneling from a hydrogen atom due to a few-cycle laser pulse with linear polarization.

Transport properties of massive Dirac particles are investigated through an oscillating barrier. The Floquet quasienergies related to the time-dependent potential appear both in transmission and reflection as sidebands around the incoming electron's energy. We take all relevant sidebands into account and present time averaged transmission and reflection probabilities in a wide energy range. Most qualitative features of scattering on a static barrier -- like Klein paradox -- are still visible, but the transmission probability in the evanescent regime observably increases due to the oscillation of the potential. The strongly inelastic scattering process is shown to lead to multiple Fano-type resonances and temporal trapping of the particles inside the oscillating potential. We also present a detailed study of the time evolution of the wave packets generated in the scattering process. Our results can be relevant for graphene with an induced energy gap.

We study the time evolution of quantum entanglement between an electron and its parent ion during the rescattering due to a strong few-cycle laser pulse. Based on a simple one-dimensional model, we compute the Neumann entropy during the process for several values of the carrier-envelope phase. The local maxima of the oscillations in the Neumann entropy coincide with the zero crossings of the electric field of the laser pulse. We employ the Wigner function to qualitatively explain the quantum dynamics of rescattering in the phase space., Comment: 2 pages

We follow the emergence of quantum entanglement in a scattering event between two initially uncorrelated distinguishable quantum particles interacting via a delta potential. We calculate the time dependence of the Neumann entropy of the one-particle reduced density matrix. By using the exact propagator for the delta potential, we derive an approximate analytic formula for the asymptotic form of the two-particle wave function which is sufficiently accurate to account for the entanglement features of the system.

We construct the exact time dependent density profile for a superposition of the ground and singly excited states of a harmonically trapped one dimensional Bose-Einstein condensate in the limit of strongly interacting particles, the Tonks-Girardeau gas. Results of an off resonant light scattering experiment probing the system could allow to determine the number of particles contained in the gas, as well as the coefficients of the superposition.

The time evolution of anharmonic molecular wave packets is investigated under the influence of the environment consisting of harmonic oscillators. These oscillators represent photon or phonon modes and assumed to be in thermal equilibrium. Our model explicitly incorporates the fact that in the case of a nonequidistant spectrum the rates of the environment induced transitions are different for each transition. The nonunitary time evolution is visualized by the aid of the Wigner function related to the vibrational state of the molecule. The time scale of decoherence is much shorter than that of dissipation, and gives rise to states which are mixtures of localized states along the phase space orbit of the corresponding classical particle. This behavior is to a large extent independent of the coupling strength, the temperature of the environment and also of the initial state., Comment: 7 pages, 4 figures

The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to the environment, there are collective, subradiant states, that have no dipole coupling to photon modes, and therefore they are expected to decay slower. This property also implies that these type of states, which form an N-1 dimensional subspace of the atomic subsytem, also decohere slower. We propose a scheme which will create such states. First the two-level atoms are placed in a strongly detuned cavity and one of the atoms, called the control atom is excited. The time evolution of the coupled atom-cavity system leads to an appropriately entangled state of the atoms. By applying subsequent laser pulses at a well defined time instant, it is possible to drive the atomic state into the subradiant, i. e., decoherence free subspace. Up to a certain average number of the photons, the result is independent of the state of the cavity. The analysis of the conditions shows that this scheme is feasible with present day techniques achieved in atom cavity interaction experiments., Comment: 5 pages

We investigate the time evolution of a superposition of macroscopically distinct quantum states in a system of two-level atoms interacting with a thermal environment of photon modes. We show that the atomic coherent states are robust against decoherence, therefore we call their superpositions atomic Schr\"{o}dinger cat states. The initial fast regime of the time evolution is associated with the process of decoherence, and it is directed towards the statistical mixture of the constituent coherent states of the original state for most of the initial conditions. However, certain superpositions, called symmetric, exhibit exceptionally slow decoherence. By introducing a new measure, we generalize the usual decoherence scheme regarding the evolution of the state to account also for the symmetric case. To stress the fact that the environment preserves symmetric superpositions much longer than the other ones,we present Wigner function images of the decoherence of a suitably oriented four component cat state., Comment: 9 pages, 6 figures. High quality figures can be downloaded from http://www.jate.u-szeged.hu/~benedict/. To appear in Phys. Rev. A, March 2001