Search

Simple Summary: This study aims to quantify the effects of smoke originating from boreal biomass-burning fires on solar radiation propagating through the atmosphere. The wildfires that took place in summer 2017 along Greenland's west coast and northern Canada produced a considerable amount of particles that were transported north and northeast, respectively, and were detected at the Thule High Arctic Atmospheric Observatory (THAAO; 76.53 ∘ N, 68.74 ∘ W). Solar radiation measurements carried out at THAAO, satellite data, and modeled radiations allowed the estimation of surface cooling and the warming aloft at two atmospheric layers (at altitudes of approximately 5 and 11 km asl) due to the presence of the biomass-burning aerosol particles. Boreal fires have increased during the last years and are projected to become more intense and frequent as a consequence of climate change. Wildfires produce a wide range of effects on the Arctic climate and ecosystem, and understanding these effects is crucial for predicting the future evolution of the Arctic region. This study focuses on the impact of the long-range transport of biomass-burning aerosol into the atmosphere and the corresponding radiative perturbation in the shortwave frequency range. As a case study, we investigate an intense biomass-burning (BB) event which took place in summer 2017 in Canada and subsequent northeastward transport of gases and particles in the plume leading to exceptionally high values (0.86) of Aerosol Optical Depth (AOD) at 500 nm measured in northwestern Greenland on 21 August 2017. This work characterizes the BB plume measured at the Thule High Arctic Atmospheric Observatory (THAAO; 76.53 ∘ N, 68.74 ∘ W) in August 2017 by assessing the associated shortwave aerosol direct radiative impact over the THAAO and extending this evaluation over the broader region ( 60 ∘ N– 80 ∘ N, 110 ∘ W– 0 ∘ E). The radiative transfer simulations with MODTRAN6.0 estimated an aerosol heating rate of up to 0.5 K/day in the upper aerosol layer (8–12 km). The direct aerosol radiative effect (ARE) vertical profile shows a maximum negative value of −45.4 Wm − 2 for a 78 ∘ solar zenith angle above THAAO at 3 km altitude. A cumulative surface ARE of −127.5 TW is estimated to have occurred on 21 August 2017 over a portion (∼ 3.1 × 10 6 km 2 ) of the considered domain ( 60 ∘ N– 80 ∘ N, 110 ∘ W– 0 ∘ E). ARE regional mean daily values over the same portion of the domain vary between −65 and −25 Wm − 2 . Although this is a limited temporal event, this effect can have significant influence on the Arctic radiative budget, especially in the anticipated scenario of increasing wildfires. [ABSTRACT FROM AUTHOR]

This study examines the relationships linking methanesulfonic acid (MSA, arising from the atmospheric oxidation of the biogenic dimethylsulfide, DMS) in atmospheric aerosol, satellite-derived chlorophyll a (Chl- a ), and oceanic primary production (PP), also as a function of sea ice melting (SIM) and extension of the ice free area in the marginal ice zone (IF-MIZ) in the Arctic. MSA was determined in PM 10 samples collected over the period 2010–2012 at two Arctic sites, Ny Ålesund (78.9°N, 11.9°E), Svalbard islands, and Thule Air Base (76.5°N, 68.8°W), Greenland. PP is calculated by means of a bio-optical, physiologically based, semi-analytical model in the potential source areas located in the surrounding oceanic regions (Barents and Greenland Seas for Ny Ålesund, and Baffin Bay for Thule). Chl- a peaks in May in the Barents sea and in the Baffin Bay, and has maxima in June in the Greenland sea; PP follows the same seasonal pattern of Chl- a , although the differences in absolute values of PP in the three seas during the blooms are less marked than for Chl- a . MSA shows a better correlation with PP than with Chl- a , besides, the source intensity (expressed by PP) is able to explain more than 30% of the MSA variability at the two sites; the other factors explaining the MSA variability are taxonomic differences in the phytoplanktonic assemblages, and transport processes from the DMS source areas to the sampling sites. The taxonomic differences are also evident from the slopes of the correlation plots between MSA and PP: similar slopes (in the range 34.2–36.2 ng m −3 of MSA/(gC m −2 d −1 )) are found for the correlation between MSA at Ny Ålesund and PP in Barents Sea, and between MSA at Thule and PP in the Baffin Bay; conversely, the slope of the correlation between MSA at Ny Ålesund and PP in the Greenland Sea in summer is smaller (16.7 ng m −3 of MSA/(gC m −2 d −1 )). This is due to the fact that DMS emission from the Barents Sea and Baffin Bay is mainly related to the MIZ diatoms, which are prolific DMS producers, whereas in the Greenland Sea the DMS peak is related to an offshore pelagic bloom where low-DMS producer species are present. The sea ice dynamic plays a key role in determining MSA concentration in the Arctic, and a good correlation between MSA and SIM (slope = 39 ng m −3 of MSA/10 6 km 2 SIM) and between MSA and IF-MIZ (slope = 56 ng m −3 of MSA/10 6 km 2 IF-MIZ) is found for the cases attributable to bloomings of diatoms in the MIZ. Such relationships are calculated by combining the data sets from the two sites and suggest that PP is related to sea ice melting and to the extension of marginal sea ice areas, and that these factors are the main drivers for MSA concentrations at the considered Arctic sites. [ABSTRACT FROM AUTHOR]