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New high-repetition-rate x-ray free electron lasers (XFELs) require for their operation highly reliable ultrafast laser systems with high pulse energy, high repetition rate, and high average power. In this Letter, we present high-average-power scaling of near-infrared optical parametric chirped pulse amplification (OPCPA) in potassium titanyl arsenate (KTA) with tunable center wavelengths from 1.5 to 2.0 μm. Using a three-stage amplification scheme and a kW-level InnoSlab Yb:YAG pump amplifier for the final non-collinear KTA stage, we demonstrate an amplified output power of 106.2 W at a center wavelength of 1.75 μm and 100 kHz. Idler absorption introduces a potential upper limit on the average power scaling of center wavelengths

Laser amplifiers at high repetition rate are critical for many applications in the chemical, physical and biological sciences. A variety of laser sources from XUV to THz can be derived from Ti:Sapphire laser amplifiers at moderate to low conversion efficiencies. High repetition rate applications require NIR and IR sources based on optical parametric chirped pulse amplifier (OPCPA) to drive these sources, offsetting the conversion efficiency losses with an even higher average power beam to drive the frequency conversion processes. We use these technologies at next generation free-electron laser (FEL) facilities. The Linac Coherent Light Source (LCLS), LCLS-II upgrade, will provide sub-femtosecond and femtosecond X-ray pulses at 100 kHz, and later up to 1 MHz repetition rate. The higher repetition rate benefits pump-probe experiments for weakly scattering samples and serves a variety of experiments which require attenuation to avoid perturbation and damage of the sample by the X-ray probe. A millijoule R&D laser amplifier was developed to test experimental conditions for optical laser beam delivery at LCLS-II. The laser can be operated at two distinct wavelength ranges. At 800 nm center wavelength we use the second harmonic of an Yb:YAG amplifier system to pump an OPCPA in a BBO crystal. A second tunable version operates between 1.45-2 m center wavelength using the fundamental Yb:YAG beam to pump a KTA OPCPA with average output powers in excess of 100 W. Currently the amplifier is operated 24 hours, 7 days a week. It is based on a simple and robust design, which ensures long term stability with good output beam quality.

We present the experimental thermal study of a 88.6 W average power optical parametric chirped pulse amplifier (OPCPA) system operating at 100 kHz, delivering sub-20 fs pulses at a center wavelength of 800 nm. A 15 W pump laser at 1030 nm is used to derive the seed pulses via white-light continuum generation and to pre-amplify the seed pulses to a 1 W level. Further amplification takes place in two high power stages, that are pumped with a frequency doubled Yb:YAG InnoSlab amplifier. The system is a prototype for the future LCLS-II pump-probe laser system.

The Free-electron LASer in Hamburg (FLASH) has been extended with a new undulator line FLASH2 in 2014. A compact grazing-incident wide-spectral-range spectrometer based on spherical-variable-line-spacing (SVLS) gratings in the extreme ultraviolet (XUV) region was constructed to optimize and characterize the free-electron laser (FEL) performance at FLASH2. The spectrometer is equipped with three different concave SVLS gratings covering a spectral range from 1 to 62 nm to analyze the spectral characteristics of the XUV radiation. Wavelength calibration and evaluation of the spectral resolution were performed at the plane grating monochromator beamline PG2 at FLASH1 before the installation at FLASH2, and compared with analytical simulations. The first light using self-amplified spontaneous emission from FLASH2 was observed by the spectrometer during a simultaneous operation of both undulator lines—FLASH1 and FLASH2. In addition, the spectral resolution of the spectrometer was evaluated by comparing the measured spectrum from FLASH2 with FEL simulations.

We design and realize an arrival time diagnostic for ultrashort X-ray pulses achieving unprecedented high sensitivity in the soft X-ray regime via cross-correlation with a ≈1550 nm optical laser. An interferometric detection scheme is combined with a multi-layer sample design to greatly improve the sensitivity of the measurement. We achieve up to 275% of relative signal change when exposed to 1.6 mJ/cm2 of soft X-rays at 530 eV, more than a hundred-fold improvement in sensitivity as compared to previously reported techniques. The resolution of the arrival time measurement is estimated to around 2.8 fs (rms). The demonstrated X-ray arrival time monitor paves the way for sub-10 fs-level timing jitter at high repetition rate X-ray facilities.

We study the feasibility of using small angle X-ray scattering (SAXS) as a new experimental diagnostic for intense laser-solid interactions. By using X-ray pulses from a hard X-ray free electron laser, we can simultaneously achieve nanometer and femtosecond resolution of laser-driven samples. This is an important new capability for the Helmholtz international beamline for extreme fields at the high energy density endstation currently built at the European X-ray free electron laser. We review the relevant SAXS theory and its application to transient processes in solid density plasmas and report on first experimental results that confirm the feasibility of the method. We present results of two test experiments where the first experiment employs ultra-short laser pulses for studying relativistic laser plasma interactions, and the second one focuses on shock compression studies with a nanosecond laser system.

High power OPCPAs above 10 W at short-wave IR wavelengths (SWIR: 1.4 - 3 μm) may be limited because of thermal heat dissipation in the nonlinear crystals. In this work we provide up-to-date measurements of the absorption coefficients of the nonlinear crystals used at these wavelengths and simulations of the thermal effects on critical parameters. In particular, power scaling limits will be discussed.

We present a 100 kHz, sub-20 fs optical parametric chirped-pulse amplifier (OPCPA) system delivering 88.6 W average power at a center wavelength of 800 nm. The seed pulses are derived from the pump laser via white-light continuum generation and are amplified in three non-collinear OPCPA stages. The final two high-power stages are pumped with a 661 W Yb:YAG InnoSlab amplifier. A simple and robust design is used for the OPCPA system to avoid thermal effects and enhance long-term stability, resulting in excellent beam quality and high conversion efficiency. To the best of our knowledge, this is the highest average power OPCPA system reported to date.

Review of scientific instruments 87(10), 103701 (2016). doi:10.1063/1.4963906, We describe the phase-contrast imaging instrument at the Matter in Extreme Conditions (MEC) endstation of the Linac Coherent Light Source. The instrument can image phenomena with a spatial resolution of a few hundreds of nanometers and at the same time reveal the atomic structure through X-ray diffraction, with a temporal resolution better than 100 fs. It was specifically designed for studies relevant to high-energy-density science and can monitor, e.g., shock fronts, phase transitions, or void collapses. This versatile instrument was commissioned last year and is now available to the MEC user community., Published by American Institute of Physics, [S.l.]

Next-generation X-ray sources have allowed new opportunities for ultrafast imaging, but such schemes require femtosecond synchronization between the pump and probe laser pulses. Here, researchers present few-femtosecond timing between a free-electron laser and an external laser exploiting terahertz radiation.

We report on investigations of high-order harmonic generation from solid surfaces in the coherent wake emission regime with relativistically intense few-cycle (8 fs) laser pulses. Significant spectral broadening compared to previous experiments with many-cycle pulses and the appearance of substructures on the harmonics are observed that strongly fluctuate from shot-to-shot. Measurements in which the linear polarization was rotated or ellipticity of the laser pulse was varied exhibit a strong dependence of the harmonic emission on the polarization state of the incident pulse. We show that the observed spectral features are ultimately connected to the sub-cycle electron dynamics in the laser-solid interaction and thus proof of the few-cycle nature of the observed harmonic emission. Using a simple model we have investigated the factors that play an important role in the shape of the emitted spectrum.

Quasi-phase matching (QPM) can be used to increase the conversion efficiency of the high harmonic generation (HHG) process. We observed QPM with an improved dual-gas foil target with a 1 kHz, 10 mJ, 30 fs laser system. Phase tuning and enhancement were possible within a spectral range from 17 nm to 30 nm. Furthermore analytical calculations and numerical simulations were carried out to distinguish QPM from other effects, such as the influence of adjacent jets on each other or the laser gas interaction. The simulations were performed with a 3 dimensional code to investigate the phase matching of the short and long trajectories individually over a large spectral range.

Optical parametric chirped-pulse amplification (OPCPA) is the most promising method for providing compact, wavelength tunable, high power, femtosecond lasers. We have recently achieved a 112 W OPCPA with wavelength tunability around 800 nm and 30 fs pulse duration in burst mode (100 kHz in a 800 µs burst at 10 Hz). In this work, we discuss the various laser architectures and the critical parameters in achieving similar laser parameters but in continuous operation.

The use of temporally shaped pump pulses for optical parametric chirped-pulse amplification can increase the efficiency and suppress possible spectral distortions in this process. With this goal in mind a novel method for shaping narrowband picosecond pulses has been developed. The method is based on the pulse stacking principle, where replicas of the incoming pulse are created in a specially designed four-beam interferometer. The replicas are recombined with appropriate relative delays. The interferometer design allows for a unique flexibility in varying the pulse shape, since all relevant degrees of freedom, such as relative intensities and delays between the pulse replicas are independently adjustable. Here we describe the design of our device in detail and report on the experimental demonstration of its pulse-shaping capabilities.

We report on the pulse contrast-ratio characterization of a few-cycle 0.2 TW optical parametric chirped pulse amplifier system operating at 20 Hz. A specially designed third-order correlator was used to characterize and optimize the contrast of the system. We demonstrate that the pulse contrast depends much more on the temporal overlap between the pump and the seed pulse than the shape of the amplified spectrum. The best amplified pulse contrast-ratio was 10-4 at Δt=±25 ps and >10-9 at Δt=±150 ps delays.

This manuscript serves as a reference to describe the optical laser sources and capabilities at the Linac Coherent Light Source., Ultrafast optical lasers play an essential role in exploiting the unique capabilities of recently commissioned X-ray free-electron laser facilities such as the Linac Coherent Light Source (LCLS). Pump–probe experimental techniques reveal ultrafast dynamics in atomic and molecular processes and reveal new insights in chemistry, biology, material science and high-energy-density physics. This manuscript describes the laser systems and experimental methods that enable cutting-edge optical laser/X-ray pump–probe experiments to be performed at LCLS.

Optical parametric chirped-pulse amplifiers with high average power are possible with novel high-power Yb:YAG amplifiers with kW-level output powers. We demonstrate a compact wavelength-tunable sub-30-fs amplifier with 11.4 W average power with 20.7% pump-to-signal conversion efficiency. For parametric amplification, a beta-barium borate crystal is pumped by a 140 W, 1 ps Yb: YAG InnoSlab amplifier at 3.25 MHz repetition rate. The broadband seed is generated via supercontinuum generation in a YAG crystal.

The potential of borate crystals, BBO, LBO and BiBO, for high average power scaling of optical parametric chirped-pulse amplifiers is investigated. Up-to-date measurements of the absorption coefficients at 515 nm and the thermal conductivities are presented. The measured absorption coefficients are a factor of 10-100 lower than reported by the literature for BBO and LBO. For BBO, a large variation of the absorption coefficients was found between crystals from different manufacturers. The linear and nonlinear absorption coefficients at 515 nm as well as thermal conductivities were determined for the first time for BiBO. Further, different crystal cooling methods are presented. In addition, the limits to power scaling of OPCPAs are discussed.

A conceptual design of a high power, ultrabroadband optical parametric chirped-pulse amplifier (OPCPA) was carried out comparing nonlinear crystals (LBO and BBO) for 810 nm centered, sub-7.0 fs pulses with energies above 1 mJ. These amplifiers are only possible with a parallel development of kilowatt-level OPCPA-pump amplifiers. It is therefore important to know good strategies to use the available OPCPA-pump energy efficiently. Numerical simulations, including self- and cross-phase modulation, were used to investigate the critical parameters to achieve sufficient spectral and spatial quality. At high output powers, thermal absorption in the nonlinear crystals starts to degrade the output beam quality. Strategies to minimize thermal effects and limits to the maximum average power are discussed.

The high repetition rate laser systems providing the ELI-ALPS facility with TW-to-PW peak intensity pulses are designed to generate secondary light sources with a duration of tens of attosecond for basic and applied researches.

Nature Communications 4, 1731 (2013). doi:10.1038/ncomms2754, The resolution of ultrafast studies performed at extreme ultraviolet and X-ray free-electron lasers is still limited by shot-to-shot variations of the temporal pulse characteristics. Here we show a versatile single-shot temporal diagnostic tool that allows the determination of the extreme ultraviolet pulse duration and the relative arrival time with respect to an external pump-probe laser pulse. This method is based on time-resolved optical probing of the transient reflectivity change due to linear absorption of the extreme ultraviolet pulse within a solid material. In this work, we present measurements performed at the FLASH free-electron laser. We determine the pulse duration at two distinct wavelengths, yielding (184±14) fs at 41.5 nm and (21±19) fs at 5.5 nm. Furthermore, we demonstrate the feasibility to operate the tool as an online diagnostic by using a 20-nm-thin Si3N4 membrane as target. Our results are supported by detailed numerical and analytical investigations., Published by Nature Publishing Group, London

Attosecond science is enabled by the ability to convert femtosecond near-infrared laser light into coherent harmonics in the extreme ultraviolet spectral range. While attosecond sources have been utilized in experiments that have not demanded high intensities, substantially higher photon flux would provide a natural link to the next significant experimental breakthrough. Numerical simulations of dual-gas high harmonic generation indicate that the output in the cutoff spectral region can be selectively enhanced without disturbing the single-atom gating mechanism. Here, we summarize the results of these simulations and present first experimental findings to support these predictions.

An Yb:YAG thin-disk multipass laser amplifier system was developed operating in a 10 Hz burst operation mode with 800 µs burst duration and 100 kHz intra-burst repetition rate. Methods for the suppression of parasitic amplified spontaneous emission are presented. The average output pulse energy is up to 44.5 mJ and 820 fs compressed pulse duration. The average power of 4.45 kW during the burst is the highest reported for this type of amplifier.

An Yb:YAG thin-disk laser amplifier is presented capable of amplifying pulses to a maximum average power of 4.45 kW at burst repetition rates of 100 kHz as pump amplifier for an optical parametric amplifier system.

Physical review letters 107, 175002 (2011). doi:10.1103/PhysRevLett.107.175002, Published by APS, College Park, Md.

Improved performance of Free Electron Laser (FEL) light sources in terms of timing stability, pulse shape and spectral properties of the amplified FEL pulses is of interest in many fields of science. A promising scheme is direct seeding with High-Harmonic Generation (HHG) in a noble gas target. A Free-Electron-Laser seeded by an external XUV-source is planned for FLASH II at DESY in Hamburg. The requirements for the XUV/soft X-ray source can be summarized as follows: A repetition rate of at least 100 kHz in a 10 Hz burst is needed at variable wavelengths from 10 to 40 nm and pulse energies of several nJ within single harmonics. This application requires a laser amplifier system with exceptional parameters, mJ-level pulse energy, sub-10 fs pulse duration at 100 kHz (1 MHz) burst repetition rate. A new OPCPA system is under development in order to meet these requirements, and very promising results has been achieved. In parallel to this development, a new High- Harmonic Generation concept is necessary to sustain the high average power of the driving laser system and for the need of high conversion efficiencies. Highest conversion efficiency in High Harmonic Generation has been shown using gas-filled capillary targets, up to now. For our application, only a free-jet target is applicable for high harmonic generation at high repetition rate, to overcome damage threshold limitations of HHG target optics. A new multi-jet target is under development and first tests show a good performance of this nozzle configuration.

We present a new dual-gas multi-jet HHG source which can be perfectly controlled via phasematching of the long and short trajectory contributions and is applicable for high average power driver laser systems.

We report on a Yb:YAG Innoslab laser amplifier system for generation of subpicsecond high energy pump pulses for optical parametric chirped pulse amplification (OPCPA) at high repetition rates. Pulse energies of up to 20 mJ (at 12.5 kHz) and repetition rates of up to 100 kHz were attained with pulse durations of 830 fs and average power in excess of 200 W. We further investigate the possibility to use subpicosecond pulses to derive a stable continuum in a YAG crystal for OPCPA seeding.

Ultra-fast laser sources have revolutionized many fields in science. As technology improves, new applications can be made accessible. The OPCPA technique has shown potential to be the key technology for future amplifier systems, but hasn’t achieved a breakthrough such as Ti:Sapphire laser technology, mostly due to the complex pump amplifier design. We present an operationally stable OPCPA system that might turn the tide for OPCPA technology. This first prototype system will be used in the accelerator environment at the FLASH free electron laser at DESY in Hamburg. The envisioned key parameters for this amplifier are >1 mJ pulse energy with a repetition rate of 100 kHz and a pulse duration of

High-order relativistic harmonics produced in the interaction of 8fs multi-TW pulses with solids are shown to be significantly broadened as compared to the case of multi-cycle driving pulses. Their potential for single-attosecond-pulse generation is discussed.

We report on the performance of a 60 kHz repetition rate sub-10 fs, optical parametric chirped pulse amplifier system with 2 W average power and 3 GW peak power. This is to our knowledge the highest average power sub-10 fs kHz-amplifier system reported to date. The amplifier is conceived for applications at free electron laser facilities and is designed such to be scalable in energy and repetition rate.

We demonstrate the amplification of broadband pulses from a Ti:Sapphire oscillator by non-collinear optical parametric chirped-pulse amplification technique in a type-I BBO crystal to energies of 90 mJ. Partial compression of the amplified pulses is demonstrated down to a 10 fs duration. These parameters come in combination with good spatial quality and focusability of the amplified beam.

We report the first generation of three-cycle, 8 fs, 125 mJ optical pulses in a noncollinear optical parametric chirped-pulse amplifier (NOPCPA) operating at 805 nm central wavelength. These 16 TW laser pulses are compressed to within 5% of their Fourier limit. These parameters come in combination with an amplified pulse contrast-ratio of 10−5 at Δt=±5ps and ≫10−7 at t≪−5ps limited by the detection barrier. Numerical split-step simulations are performed to investigate potential improvements for the NOPCPA laser system.

We report on an electron accelerator based on few-cycle (8 fs full width at half maximum) laser pulses, with only 40 mJ energy per pulse, which constitutes a previously unexplored parameter range in laser-driven electron acceleration. The produced electron spectra are monoenergetic in the tens-of-MeV range and virtually free of low-energy electrons with thermal spectrum. The electron beam has a typical divergence of 5-10 mrad. The accelerator is routinely operated at 10 Hz and constitutes a promising source for several applications. Scalability of the few-cycle driver in repetition rate and energy implies that the present work also represents a step towards user friendly laser-based accelerators.

We report generation of three-cycle, 8 fs, 125 mJ optical pulses in a noncollinear optical parametric chirped-pulse amplifier (NOPCPA). These 16 TW laser pulses are compressed to within 6% of their Fourier limit.

We report the amplification of three-cycle, 8.5 fs optical pulses in a near-infrared noncollinear optical parametric chirped-pulse amplifier (OPCPA) up to energies of 80 mJ. Improved dispersion management in the amplifier by means of a combination of reflection grisms and a chirped-mirror stretcher allowed us to recompress the amplified pulses to within 6% of their Fourier limit. The novel ultrabroad, ultraprecise dispersion control technology presented in this work opens the way to scaling multiterawatt technology to even shorter pulses by optimizing the OPCPA bandwidth.

We report about the experimental realization and detailed characterization of a 7 TW optical parametric chirped pulse amplifier which produces 14 fs pulses with an energy of 100 mJ.

We present the design of the 10 TW OPCPA system which is currently being constructed for the Laser and Attosecond Physics laboratory at the Max-Planck Institute for Quantum Optics and perform a detailed characterization of a newly developed picosecond pump source. The setup consists of a broadband femtosecond seed oscillator, three OPCPA stages and an independent 80-ps pump laser, whose repetition rate is actively synchronized to the repetition rate of a fs- oscillator. The pump laser is a Nd:YAG flash-lamp pumped system consisting of a Nd:YVO/sub 4/ based picosecond pulse oscillator, a regenerative amplifier, a two-pass pre-amplifier. and two power amplifiers. At the output system produces more than 1.4 J of 1064 nm in 90-ps pulses at a 10-Hz repetition rate. These pulses are frequency doubled in a DKDP crystal yielding about 700-mJ. 80-ps pulses at 532-nm with a multimode spatial profile and a nearly Gaussian temporal profile. The near-field pump beam profile is relay-imaged from the doubling crystal of the pump laser on each nonlinear crystal in order to have the best amplification efficiency.

Optical parametric chirped pulse amplification provides a promising alternative for amplification of high-power few-cycle pulses. Our objective is to explore the feasibility of this concept in amplifying 7 fs phase-stabilized pulses till 10 TW power.

An improved dual-gas quasi-phase matching (QPM) foil target for high harmonic generation (HHG) is presented. The target can be setup with 12 individual gas inlets each feeding multiple nozzles separated by a minimum distance of 10 μm. Three-dimensional gas density profiles of these jets were measured using a Mach-Zehnder Interferometer. These measurements reveal how the jets influence the density of gas in adjacent jets and how this leads to increased local gas densities. The analysis shows that the gas profiles of the jets are well defined up to a distance of about 300 μm from the orifice. This target design offers experimental flexibility, not only for HHG/QPM investigations, but also for a wide range of experiments due to the large number of possible jet configurations. We demonstrate the application to controlled phase tuning in the extreme ultraviolet using a 1 kHz-10 mJ-30 fs-laser system where interference between two jets in the spectral range from 17 to 30 nm was observed.

The long-term stability of optical parametric chirped-pulse amplifiers is hindered by thermal path length drifts affecting the temporal pump-to-signal overlap. A kilowatt-pumped burst amplifier is presented delivering broadband 1.4 mJ pulses with a spectral bandwidth supporting sub-7 fs pulse duration. Active temporal overlap control can be achieved by feedback of optical timing signals from cross-correlation or spectral measurements. Using a balanced optical cross-correlator, we achieve a pump-to-signal synchronization with a residual jitter of only (46 ± 2) fs rms. Additionally, we propose passive pump-to-signal stabilization with an intrinsic jitter of (7.0 ± 0.5) fs rms using white-light continuum generation.

We have developed an easy-to-use and reliable timing tool to determine the arrival time of an optical laser and a free electron laser (FEL) pulses within the jitter limitation. This timing tool can be used from XUV to X-rays and exploits high FELs intensities. It uses a shadowgraph technique where we optically (at 800 nm) image a plasma created by an intense XUV or X-ray FEL pulse on a transparent sample (glass slide) directly placed at the pump - probe sample position. It is based on the physical principle that the optical properties of the material are drastically changed when its free electron density reaches the critical density. At this point the excited glass sample becomes opaque to the optical laser pulse. The ultra-short and intense XUV or X-ray FEL pulse ensures that a critical electron density can be reached via photoionization and subsequent collisional ionization within the XUV or X-ray FEL pulse duration or even faster. This technique allows to determine the relative arrival time between the optical laser and the FEL pulses in only few single shots with an accuracy mainly limited by the optical laser pulse duration and the jitter between the FEL and the optical laser. Considering the major interest in pump-probe experiments at FEL facilities in general, such a femtosecond resolution timing tool is of utmost importance. © 2012 IOP Publishing Ltd and Sissa Medialab srl.

We report on the simultaneous determination of non-linear dispersion functions and resolving power of three flat-field XUV grating spectrometers. A moderate-intense short-pulse infrared laser is focused onto technical aluminum which is commonly present as part of the experimental setup. In the XUV wavelength range of 10-19 nm, the spectrometers are calibrated using Al-Mg plasma emission lines. This cross-calibration is performed in-situ in the very same setup as the actual main experiment. The results are in excellent agreement with ray-tracing simulations. We show that our method allows for precise relative and absolute calibration of three different XUV spectrometers. © 2011 IOP Publishing Ltd and SISSA.

We report on the implementation of a high-count-rate charged particle imaging detector for two-color pump-probe experiments at the free electron laser in Hamburg (FLASH). In doing so, we have developed a procedure for finding the spatial and temporal overlap between the extreme UV free electron laser (FEL) pulses and the IR pulses, which allows for complete alignment of the setup in situations where the region of overlap between the FEL and the IR is not easily accessible by means of imaging optics.

Significant progress in high repetition rate ultrashort pulse sources based on fiber technology is presented. These systems enable operation at a high repetition rate of up to 500 kHz and high average power in the extreme ultraviolet wavelength range via high harmonic generation in a gas jet. High average power few-cycle pulses of a fiber amplifier pumped optical parametric chirped pulse amplifier are used to produce µW level average power for the strongest harmonic at 42.9 nm at a repetition rate of 96 kHz.

We report on a high power optical parametric amplifier delivering 8 fs pulses with 6 GW peak power. The system is pumped by a fiber amplifier and operated at 96 kHz repetition rate. The average output power is as high as 6.7 W, which is the highest average power few-cycle pulse laser reported so far. When stabilizing the seed oscillator, the system delivered carrier-envelop phase stable laser pulses. Furthermore, high harmonic generation up to the 33(th) order (21.8 nm) is demonstrated in a Krypton gas jet. In addition, the scalability of the presented laser system is discussed.

We demonstrate a new and compact Phi-plane-pumped noncollinear optical parametric chirped-pulse amplification (NOPCPA) scheme for broadband pulse amplification, which is based on two-beam-pumping (TBP) at 532 nm. We employ type-I phase-matching in a 5 mm long BBO crystal with moderate pump intensities to preserve the temporal pulse contrast. Amplification and compression of the signal pulse from 675 nm - 970 nm is demonstrated, which results in the generation of 7.1-fs light pulses containing 0.35 mJ energy. In this context, we investigate the pump-to-signal energy conversion efficiency for TBP-NOPCPA and outline details for few-cycle pulse characterization. Furthermore, it is verified, that the interference at the intersection of the two pump beams does not degrade the signal beam spatial profile. It is theoretically shown that the accumulated OPA phase partially compensates for wave-vector mismatch and leads to extended broadband amplification. The experimental outcome is supported by numerical split-step simulations of the parametric signal gain, including pump depletion and parametric fluorescence.

We present a two-stage noncollinear optical parametric chirped-pulse amplification system that generates 7.9 fs pulses containing 130 mJ of energy at an 805 nm central wavelength and 10 Hz repetition rate. These 16 TW light pulses are compressed to within 5% of their Fourier limit and are carefully characterized by the use of home-built pulse diagnostics. The contrast ratio before the main pulse has been measured as 10(-4), 10(-8), and 10(-11) at t=-3.3 ps, t=-5 ps, and t=-30 ps, respectively. This source allows for experiments in a regime of relativistic light-matter interactions and attosecond science.

FLASH, the Free-electron LASer in Hamburg, is a worldwide unique source for extremely bright ultra-short laser-like pulses tunable in a wide spectral range in the extreme ultraviolet and soft x-ray region (Ackermann et?al 2007 Nat. Photonics 1 336?42). To fully exploit the features of this new generation of light sources, a user facility with efficient radiation transport to the experimental area and novel online photon diagnostics capable of characterizing the unique parameters of the FLASH radiation has been built. It serves a broad user community active in many scientific fields ranging from atomic and molecular physics to plasma and solid state physics as well as chemistry and biology. A special focus is placed on the exploitation of the ultra-short FLASH pulses using pump?probe techniques. Thus, the facility is equipped with optical and THz sources synchronized to FLASH. This paper gives a detailed overview of the FLASH user facility.

We report on the generation of 8 fs, 125 mJ pulses in a noncollinear optical parametric chirped pulse amplifier with a temporal contrast reaching 10 orders of magnitude at 5 ps before the main pulse.