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As a rapidly expanding family of 2D materials, MXenes have recently gained considerable attention. Herein, by developing a coating method that enables transfer‐free and layer‐by‐layer film coating, the nonlinear optical absorption (NOA) of Ti3C2Tx MXene films is investigated. Using the Z‐scan technique, the NOA of the MXene films is characterized at ≈800 nm. The results show that there is a strong and layer‐dependent NOA behavior, transitioning from reverse saturable absorption (RSA) to saturable absorption (SA) as the layer number increases from 5 to 30. Notably, the nonlinear absorption coefficient β changes significantly from ≈7.13 × 102 cm GW−1 to ≈−2.69 × 102 cm GW−1 within this range. The power‐dependent NOA of the MXene films is also characterized, and a decreasing trend in β is observed for increasing laser intensity. Finally, the NOA of 2D MXene films at ≈1550 nm is characterized by integrating them onto silicon nitride waveguides, where an SA behavior is observed for the films including 5 and 10 layers of MXene, in contrast to the RSA observed at ≈800 nm. These results reveal intriguing nonlinear optical properties of 2D MXene films, highlighting their versatility and potential for implementing high‐performance nonlinear photonic devices. [ABSTRACT FROM AUTHOR]

The engineering of thermo-optic effects has found broad applications in integrated photonic devices, facilitating efficient light manipulation to achieve various functionalities. Here, we perform both an experimental characterization and a theoretical analysis of these effects in integrated microring resonators made from high-index doped silica, which have had many applications in integrated photonics and nonlinear optics. By fitting the experimental results with theory, we obtain fundamental parameters that characterize their thermo-optic performance, including the thermo-optic coefficient, the efficiency of the optically induced thermo-optic process, and the thermal conductivity. The characteristics of these parameters are compared to those of other materials commonly used for integrated photonic platforms, such as silicon, silicon nitride, and silica. These results offer a comprehensive insight into the thermo-optic properties of doped silica-based devices. Understanding these properties is essential for efficiently controlling and engineering them in many practical applications. [ABSTRACT FROM AUTHOR]

Enhanced supercontinuum generation (SCG) is experimentally demonstrated in integrated silicon nitride (Si3N4) waveguides incorporating highly nonlinear graphene oxide (GO) in the form of 2D films. On‐chip integration of the 2D GO films with precise control of their thickness is realized by using a transfer‐free and layer‐by‐layer coating method. The control of the film length and coating position is achieved via window opening in the upper silica cladding of the photonic integrated chips. Detailed SCG measurements are performed using the fabricated devices with different waveguide geometries and GO film thicknesses, and the results are compared with devices without GO. Significantly improved spectral broadening of ultrashort optical pulses with ultrahigh peak powers exceeding 1000 W is observed for the hybrid devices, achieving up to 2.4 times improvement in the spectral bandwidth relative to devices without GO. Theoretical analyses for the influence of GO film thickness, coating length, coating position, and waveguide geometry are also provided by fitting the experimental results with theory, showing that there is still significant room for further improvement. This work opens up a new avenue toward improving the SCG performance of photonic integrated devices by incorporating functional 2D materials. [ABSTRACT FROM AUTHOR]

Integrated photonic devices operating via optical nonlinearities offer a powerful solution for all‐optical information processing, yielding processing speeds that are well beyond that of electronic processing as well as providing the added benefits of compact footprint, high stability, high scalability, and small power consumption. The increasing demand for high‐performance nonlinear integrated photonic devices has facilitated the hybrid integration of novel materials to address the limitations of existing integrated photonic platforms. Recently, graphene oxide (GO), with its large optical nonlinearity, high flexibility in altering its properties, and facile fabrication processes, has attracted significant attention, enabling many hybrid nonlinear integrated photonic devices with improved performance and novel capabilities. This paper reviews the applications of GO to nonlinear integrated photonics. First, an overview of GO's optical properties and the fabrication technologies needed for its on‐chip integration is provided. Next, the state‐of‐the‐art GO nonlinear integrated photonic devices are reviewed, followed by comparisons of the nonlinear optical performance of different integrated platforms incorporating GO as well as hybrid integrated devices including different kinds of 2D materials. Finally, the current challenges and future opportunities in this field are discussed. [ABSTRACT FROM AUTHOR]

All-optical signal processing based on nonlinear optical devices is promising for ultrafast information processing in optical communication systems. Recent advances in two-dimensional (2D) layered materials with unique structures and distinctive properties have opened up new avenues for nonlinear optics and the fabrication of related devices with high performance. This paper reviews the recent advances in research on third-order optical nonlinearities of 2D materials, focusing on all-optical processing applications in the optical telecommunications band near 1550 nm. First, we provide an overview of the material properties of different 2D materials. Next, we review different methods for characterizing the third-order optical nonlinearities of 2D materials, including the Z-scan technique, third-harmonic generation (THG) measurement, and hybrid device characterization, together with a summary of the measured n2 values in the telecommunications band. Finally, the current challenges and future perspectives are discussed. [ABSTRACT FROM AUTHOR]

We experimentally demonstrate enhanced spectral broadening of femtosecond optical pulses after propagation through silicon-on-insulator (SOI) nanowire waveguides integrated with two-dimensional (2D) graphene oxide (GO) films. Owing to the strong mode overlap between the SOI nanowires and the GO films with a high Kerr nonlinearity, the self-phase modulation (SPM) process in the hybrid waveguides is significantly enhanced, resulting in greatly improved spectral broadening of the femtosecond optical pulses. A solution-based, transfer-free coating method is used to integrate GO films onto the SOI nanowires with precise control of the film thickness. Detailed SPM measurements using femtosecond optical pulses are carried out, achieving a broadening factor of up to ~4.3 for a device with 0.4-mm-long, 2 layers of GO. By fitting the experimental results with the theory, we obtain an improvement in the waveguide nonlinear parameter by a factor of ~3.5 and in the effective nonlinear figure of merit (FOM) by a factor of ~3.8, relative to the uncoated waveguide. Finally, we discuss the influence of GO film length on the spectral broadening and compare the nonlinear optical performance of different integrated waveguides coated with GO films. These results confirm the improved nonlinear optical performance of silicon devices integrated with 2D GO films. [ABSTRACT FROM AUTHOR]

We demonstrate photonic RF phase encoding based on an integrated micro-comb source. By assembling single-cycle Gaussian pulse replicas using a transversal filtering structure, phase encoded waveforms can be generated by programming the weights of the wavelength channels. This approach eliminates the need for RF signal generators for RF carrier generation or arbitrary waveform generators for phase encoded signal generation. A large number of wavelengths—up to 60—were provided by the microcomb source, yielding a high pulse compression ratio of 30. Reconfigurable phase encoding rates ranging from 2 to 6 Gb/s were achieved by adjusting the length of each phase code. This article demonstrates the significant potentials of this microcomb-based approach to achieve high-speed RF photonic phase encoding with low cost and footprint. [ABSTRACT FROM AUTHOR]

Integrated silicon nitride (SiN) waveguides with anomalous dispersion have the potential to bring practical nonlinear optics to mainstream photonic integrated circuits. However, high-stress and high-processing temperatures remain an obstacle to mass adoption. We report low-stress, high-confinement, dispersion-engineered SiN waveguides utilizing low temperature grown reactive sputtered thin-films. We demonstrate a microring resonator with an intrinsic quality factor of 6.6 × 105, which enabled us to generate a native free spectral range spaced frequency comb with an estimated on-chip pump power of 850 mW. Importantly, the peak processing temperature is 400 °C making this approach fully back-end compatible for hybrid integration with preprocessed CMOS substrates and temperature sensitive photonic platforms such as lithium niobate on insulator. [ABSTRACT FROM AUTHOR]

We report a broadband RF channelizer based on an integrated optical frequency Kerr micro-comb source, with an RF channelizing bandwidth of 90 GHz, a high RF spectral slice resolution of 1.04 GHz, and experimentally verify the RF performance up to 19 GHz. This approach of realizing RF channelizers offers reduced complexity, size, and potential cost for a wide range of applications to microwave signal detection. [ABSTRACT FROM AUTHOR]

Over the past decade, optical frequency combs generated by high-Q microresonators, or optical microcombs, which feature compact device footprints, low power consumption, and high repetition rates in broad optical bandwidths, have led to a revolution in a wide range of fields including metrology, telecommunications, radio frequency (RF) photonics, spectroscopy, sensing, and quantum optics. Among these, an application that has attracted great interest is the use of optical microcombs for RF photonics, where they offer enhanced functionalities as well as reduced size and power consumption over other approaches. This paper reviews the recent advances in this emerging field. We provide an overview of the main achievements that have been obtained to date, and highlight the strong potential of optical microcombs for RF photonics applications. We also discuss some of the open challenges and limitations that need to be addressed for practical applications. [ABSTRACT FROM AUTHOR]

Nonlinear photonic chips can generate and process signals all-optically with far superior performance to that possible electronically - particularly with respect to speed. Although silicon-on-insulator has been the leading platform for nonlinear optics, its high two-photon absorption at telecommunication wavelengths poses a fundamental limitation. We review recent progress in non-silicon CMOS-compatible platforms for nonlinear optics, with a focus on Si3N4 and Hydex®. These material systems have opened up many new capabilities such as on-chip optical frequency comb generation and ultrafast optical pulse generation and measurement. We highlight their potential future impact as well as the challenges to achieving practical solutions for many key applications. [ABSTRACT FROM AUTHOR]

We demonstrate temporal measurements of sub-picosecond optical pulses via time-to-frequency conversion in a 45-cm-long CMOS compatible high-index glass spiral waveguide. The measurements are based on efficient four-wave mixing in the C-band, using around 1 W of peak pump power. We achieve a resolution of 400 fs over a time window of 100 ps, representing a time-bandwidth product > 250. [ABSTRACT FROM PUBLISHER]

Abstract: All-optical switching devices are based on a material possessing a nonlinear optical response, enabling light to control light, and are enjoying renewed interest. Photonic crystals are a promising platform for realizing compact all-optical switches operating at very low power and integrated on an optical integrated circuit. In this review, we show that by making photonic crystals from a highly nonlinear chalcogenide glass, we have the potential to integrate a variety of active devices into a photonic chip. We describe the fabrication and testing of two-dimensional Ge33As12 Se55 chalcogenide glass photonic crystal membrane devices (waveguides and microcavities). We then demonstrate the ability to post-tune the devices using the material photosensitivity. In one proposal we hope to introduce a double-heterostructure microcavity using the photosensitivity alone. [Copyright &y& Elsevier]