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Interference in photons emitted from multiple atoms has been studied extensively. We show that a single atom can induce interference in its emitted light when tunnelling in a double-well potential coupled to an optical cavity. The phase in the cavity field interference can be modulated by the double-well spacing. By controlling the coherent tunnelling, blockade of single-photon excitations is found in the destructive interference regime, where super-Poissonian bunched light is generated. Furthermore, we show that the atomic flux of the coherent tunnelling motion generates chiral cavity fields. The direction of the chirality oscillates for many cycles before the decoherence of the atomic motion and the decay of the cavity photons. Our work opens new ways for manipulating photons with controllable quantum states of atoms for quantum information applications., 4 pages, 5 figures; SM: 6 pages, 2 figures

We investigate speeding up of relaxation of Markovian open quantum systems with the Liouvillian exceptional point (LEP), where the slowest decay mode degenerate with a faster decay mode. The degeneracy significantly increases the gap of the Liouvillian operator, which determines the timescale of such systems in converging to stationarity, and hence accelerates the relaxation process. We explore an experimentally relevant three level atomic system, whose eigenmatrices and eigenspectra are obtained completely analytically. This allows us to gain insights in the LEP and examine respective dynamics with details. We illustrate that the gap can be further widened through Floquet engineering, which further accelerates the relaxation process. Finally, we extend this approach to analyze laser cooling of trapped ions, where vibrations (phonons) couple to the electronic states. An optimal cooling condition is obtained analytically, which agrees with both existing experiments and numerical simulations. Our study provides analytical insights in understanding LEP, as well as in controlling and optimizing dissipative dynamics of atoms and trapped ions.

Trapped ions provide a platform for quantum technologies that offers long coherence times and high degrees of scalability and controllability. Here, we use this platform to develop a realistic model of a thermal device consisting of two laser-driven, strongly coupled Rydberg ions in a harmonic trap. We show that the translational degrees of freedom of this system can be utilized as a flywheel storing the work output that is generated by a cyclic thermodynamic process applied to its electronic degrees of freedom. Mimicking such a process through periodic variations of external control parameters, we use a mean-field approach underpinned by exact numerical and analytical calculations to identify relevant physical processes and to determine the charging rate of the flywheel. Our work paves the way for the design of microscopic thermal machines based on Rydberg ions that can be equipped with both many-body working media and universal work storages., 11 pages, 5 figures

It is challenging to probe ergodicity breaking trends of a quantum many-body system when dissipation inevitably damages quantum coherence originated from coherent coupling and dispersive two-body interactions. Rydberg atoms provide a test bed to detect emergent exotic many-body phases and non-ergodic dynamics where the strong Rydberg atom interaction competes with and overtakes dissipative effects even at room temperature. Here we report experimental evidence of a transition from ergodic towards ergodic breaking dynamics in driven-dissipative Rydberg atomic gases. The broken ergodicity is featured by the long-time phase oscillation, which is attributed from the formation of Rydberg excitation clusters in limit cycle phases. The broken symmetry in the limit cycle is a direct manifestation of many-body interactions, which is verified by tuning atomic densities in our experiment. The reported result reveals that Rydberg many-body systems are a promising candidate to probe ergodicity breaking dynamics, such as limit cycles, and enable the benchmark of non-equilibrium phase transition.

Greenberger-Horne-Zeilinger and W states feature genuine tripartite entanglement that cannot be converted into each other by local operations and classical communication. Here, we present a dissipative protocol for deterministic interconversion between Greenberger-Horne-Zeilinger and W states of three neutral $^{87}$Rb atoms arranged in an equilateral triangle of a two-dimensional array. With three atomic levels and diagonal van der Waals interactions of Rydberg atoms, the interconversion between tripartite entangled states can be efficiently accomplished in the Floquet-Lindblad framework through the periodic optical pump and dissipation engineering. We evaluate the feasibility of the existing methodology using the experimental parameters accessible to current neutral-atom platforms. We find that our scheme is robust against typical noises, such as laser phase noise and geometric imperfections of the atom array. In addition, our scheme can integrate the Gaussian soft quantum control technique, which further reduces the overall conversion time and increases the resilience to timing errors and interatomic distance fluctuations. The high-fidelity and robust tripartite entanglement interconversion protocol provides a route to save physical resources and enhance the computational efficiency of quantum networks formed by neutral-atom arrays., Comment: 18 pages, 14 figures, accepted by Physical Review Applied

We propose a nontrivial two-qubit gate scheme in which Rydberg atoms are subject to designed pulses resulting from geometric evolution processes. By utilizing a hybrid robust non-adiabatic and adiabatic geometric operations on the control atom and target atom, respectively, we improve the robustness of two-qubit Rydberg gate against Rabi control errors as well as blockade errors in comparison with the conventional two-qubit blockade gate. Numerical results with the current state-of-the-art experimental parameters corroborates the above mentioned robustness. We also evaluated the influence induced by the motion-induced dephasing and the dipole-dipole interaction and imperfection excitation induced leakage errors, which both could decrease the gate fidelity. Our scheme provides a promising route towards systematic control error (Rabi error) as well as blockade error tolerant geometric quantum computation on neutral atom system., Comment: 14 pages, 13 figures, 2 tables. Accepted by Physical Review Applied

Multipartite entangled states involving non-locality are one of the most fascinating characteristics of quantum mechanics. In this work, we propose a generation of Schrödinger cat states in Rydberg atom arrays against the thermal dephasing. Unlike the previous work for producing large-scale entanglement [A. Omran et al, Science 365, 570 (2019)], we encode logical 1 on dressed states rather than Rydberg states. Such treatment can increase the lifetime of multipartite entanglement coherence to around 3 times compared to the previous work [A. Omran et al, Science 365, 570 (2019)], at the same system size, and therefore induce solid fidelities of Schrödinger cat states generation. The current work theoretically verifies the advantages of Rydberg dressed state in many-body quantum entanglement, which is meaningful for large-scale quantum computation and many-body Rydberg quantum simulation., 9 pages, 8 figures, 1 table

We study signatures of quantum chaos in dynamics of Rydberg dressed bosonic atoms held in a one dimensional triple-well potential. Long-range nearest-neighbor and next-nearest-neighbor interactions, induced by laser dressing atoms to strongly interacting Rydberg states, affect drastically mean field and quantum many-body dynamics. By analyzing the mean field dynamics, classical chaos regions with positive and large Lyapunov exponents are identified as a function of the potential well tilting and dressed interactions. In the quantum regime, it is found that level statistics of the eigen-energies gains a Wigner-Dyson distribution when the Lyapunov exponents are large, giving rise to signatures of strong quantum chaos. We find that both the time averaged entanglement entropy and survival probability of the initial state have distinctively large values in the quantum chaos regime. We further show that population variances could be used as an indicator of the emergence of quantum chaos. This might provide a way to directly probe quantum chaotic dynamics through analyzing population dynamics in individual potential wells., Comment: 13 pages, 7 figures

We investigate the thermal Casimir-Polder (CP) potential of \textsuperscript{87}Rb atoms in Rydberg $n$S-states near single- and double-layer graphene. The dependence of the CP potential on parameters such as atom-surface distance, temperature, principal quantum number $n$ and graphene Fermi energy are explored. Through large scale numerical simulations, we show that, in the non-retarded regime, the CP potential is dominated by the non-resonant and evanescent-wave terms which are monotonic, and that, in the retarded regime, the CP potential exhibits spatial oscillations. We identify that the most important contributions to the resonant component of the CP potential come from the $n$S-$n$P and $n$S-$(n-1)$P transitions. Scaling of the CP potential as a function of the principal quantum number and temperature is obtained. A heterostructure comprising hexagonal boron nitride layers sandwiched between two graphene layers is also studied. When the boron nitride layer is sufficiently thin, the CP potential can be weakened by changing the Fermi energy of the top graphene layer. Our study provides insights for understanding and controlling CP potentials experienced by Rydberg atoms near single and multi-layer graphene-based van der Waals heterostructures.

We study steady state phases of a one-dimensional array of Rydberg atoms coupled by a microwave (MW) field where the higher energy Rydberg state decays to the lower energy one via single-body and collective (superradiant) decay. Using mean-field approaches, we examine the interplay among the MW coupling, intra-state van der Waals (vdW) interaction, and single-body and collective dissipation between Rydberg states. A linear stability analysis reveals that a series of phases, including uniform, antiferromagnetic, oscillatory, and bistable and multistable phases can be obtained. Without the vdW interaction, only uniform phases are found. In the presence of the vdW interaction, multistable solutions are enhanced when increasing the strength of the superradiant decay rate. Our numerical simulations show that the bistable and multistable phases are stabilized by superradiance in a long chain. The critical point between the uniform and multistable phases and its scaling with the atom number is obtained. Through numerically solving the master equation of a finite chain, we show that the mean-field multistable phase could be characterized by expectation values of Rydberg populations and two-body correlations between Rydberg atoms in different sites.

Stabilizing important physical quantities to atom-based standards lies at the heart of modern atomic, molecular and optical physics, and is widely applied to the field of precision metrology. Of particular importance is the atom-based microwave field amplitude stabilizer, the so-called atomic candle. Previous atomic candles are realized with atoms in their ground state, and hence suffer from the lack of frequency band tunability and small stabilization bandwidth, severely limiting their development and potential applications. To tackle these limitations, we employ microwave-dressed Rydberg atoms to realize a novel atomic candle that features multi-band frequency tunability and large stabilization bandwidth. We demonstrate amplitude stabilization of microwave field from C-band to Ka-band, which could be extended to quasi-DC and terahertz fields by exploring abundant Rydberg levels. Our atomic candle achieves stabilization bandwidth of 100 Hz, outperforming previous ones by more than two orders of magnitude. Our simulation indicates the stabilization bandwidth can be further increased up to 100 kHz. Our work paves a route to develop novel electric field control and applications with a noise-resilient, miniaturized, sensitive and broadband atomic candle.

The generation of squeezed light in semiconductor materials opens opportunities for building on-chip devices that are operated at the quantum level. Here we study theoretically a squeezed light source of polariton dark solitons confined in a geometric potential well of semiconductor microcavities in the strong coupling regime. We show that polariton dark solitons of odd and even parities can be created by tuning the potential depth. When driving the potential depth linearly, a bistability of solitons with the two different parities can be induced. Strong intensity squeezing is obtained near the turning point of the bistability due to the large nonlinear interaction, which can be controlled by Feshbach resonance. The phase diagram of the bistability and squeezing of the dark solitons is obtained through large scale numerical calculations. Our study contributes to the current efforts in realizing topological excitations and squeezed light sources with solid-state devices., 8 pages, 4 figures

In this report, we (SuperHelix team) present our solution to KDD Cup 2021-PCQM4M-LSC, a large-scale quantum chemistry dataset on predicting HOMO-LUMO gap of molecules. Our solution, Lite Geometry Enhanced Molecular representation learning (LiteGEM) achieves a mean absolute error (MAE) of 0.1204 on the test set with the help of deep graph neural networks and various self-supervised learning tasks. The code of the framework can be found in https://github.com/PaddlePaddle/PaddleHelix/tree/dev/competition/kddcup2021-PCQM4M-LSC/.

We analyze the excitation dynamics numerically in a one-dimensional Rydberg atomic chain, using the methods of discrete truncated Wigner approximation (dTWA) and artificial neural networks (ANN), for both van der Waals and dipolar interactions. In particular, we look at how the number of excitations dynamically grows or evolves in the system for an initial state where all atoms are in their electronic ground state. Further, we calculate the maximum number of excitations attained at any instant and the average number of excitations. For a small system size of ten atoms, we compare the results from dTWA and ANN with that of exact numerical calculations of the Schr\"odinger equation. The collapse and revival dynamics in the number of Rydberg excitations are also characterized in detail. Though we find good agreement at shorter periods, both dTWA and ANN failed to capture the dynamics accurately at longer times. By increasing the number of hidden units, the accuracy of ANN has improved but suffered by numerical instabilities, especially for large interaction strengths. Finally, we look at the dynamics of a large system size of two-hundred atoms using dTWA., Comment: 21 pages, 11 figures

Quantum holonomic gates hold built-in resilience to local noises and provide a promising approach for implementing fault-tolerant quantum computation. We propose to realize high-fidelity holonomic $(N+1)$-qubit controlled gates using Rydberg atoms confined in optical arrays or superconducting circuits. We identify the scheme, deduce the effective multi-body Hamiltonian, and determine the working condition of the multiqubit gate. Uniquely, the multiqubit gate is immune to systematic errors, i.e., laser parameter fluctuations and motional dephasing, as the $N$ control atoms largely remain in the much stable qubit space during the operation. We show that $C_N$-NOT gates can reach same level of fidelity at a given gate time for $N\leq5$ under a suitable choice of parameters, and the gate tolerance against errors in systematic parameters can be further enhanced through optimal pulse engineering. In case of Rydberg atoms, the proposed protocol is intrinsically different from typical schemes based on Rydberg blockade or antiblockade. Our study paves a new route to build robust multiqubit gates with Rydberg atoms trapped in optical arrays or with superconducting circuits. It contributes to current efforts in developing scalable quantum computation with trapped atoms and fabricable superconducting devices., Comment: Accepted to publish in Physical Review Applied

In this paper, we propose a scheme to implement the two-qubit controlled-Z gate via the Stark-tuned F��rster interaction of Rydberg atoms, where the F��rster defect is driven by a time-dependent electric field of a simple sinusoidal function while the matrix elements of the dipole-dipole interaction are time-independent. It is shown that when the system is initially in a specific state, it makes a cyclic evolution after a preset interaction time, returning to the initial state, but picks up a phase, which can be used for realizing a two-atom controlled-Z gate. Due to the interference of sequential Landau-Zener transitions, the population and phase of the state is quasi-deterministic after the cyclic evolution and therefore the gate fidelity is insensitive to fluctuations of the interaction time and the dipole-dipole matrix elements. Feasibility of the scheme realized with Cs atoms is discussed in detail, which shows that the two-qubit gate via Landau-Zener control can be realized with the state-of-the-art experimental setup., 8 pages, 8 figures

Realizing single light bullets and vortices that are stable in high dimensions is a long-standing goal in the study of nonlinear optical physics. On the other hand, the storage and retrieval of such stable high dimensional optical pulses may offer a variety of applications. Here we present a scheme to generate such optical pulses in a cold Rydberg atomic gas. By virtue of electromagnetically induced transparency, strong, long-range atom-atom interaction in Rydberg states is mapped to light fields, resulting in a giant, fast-responding nonlocal Kerr nonlinearity and the formation of light bullets and vortices carrying orbital angular momenta, which have extremely low generation power, very slow propagation velocity, and can stably propagate, with the stability provided by the combination of local and the nonlocal Kerr nonlinearities. We demonstrate that the light bullets and vortices obtained can be stored and retrieved in the system with high efficiency and fidelity. Our study provides a new route for manipulating high-dimensional nonlinear optical processes via the controlled optical nonlinearities in cold Rydberg gases.

Recent experiments have realized an all-optical photon transistor using a cold atomic gas. This approach relies on electromagnetically induced transparency (EIT) in conjunction with the strong interaction among atoms excited to high-lying Rydberg states. The transistor is gated via a so-called Rydberg spinwave, in which a single Rydberg excitation is coherently shared by the whole ensemble. In its absence the incoming photon passes through the atomic ensemble by virtue of EIT while in its presence the photon is scattered rendering the atomic gas opaque. An important current challenge is to preserve the coherence of the Rydberg spinwave during the operation of the transistor, which would enable for example its coherent optical read-out and its further processing in quantum circuits. With a combined field theoretical and quantum jump approach and by employing a simple model description we investigate systematically and comprehensively how the coherence of the Rydberg spinwave is affected by photon scattering. With large-scale numerical calculations we show how coherence becomes increasingly protected with growing interatomic interaction strength. For the strongly interacting limit we derive analytical expressions for the spinwave fidelity as a function of the optical depth and bandwidth of the incoming photon., Comment: 7 pages. 4 figures

We study the dynamic structure factor of two coherent bright solitary waves in attractive Bose- Einstein condensates confined in a harmonic trap. We demonstrate that the wave function of the two solitary waves with a fixed relative phase shows interference in momentum space. The fringes are shifted depending on the values of the phase. This momentum interference can be extracted from the dynamic structure factor of the system using stimulated two-photon Bragg scattering. Thus our method provides a way to measure the relative phase directly., Comment: 5 pages, 4 figures

We construct the invisible quantum barrier which represents the phenomenon of quantum reflection using the available data. We use the Abel equation to invert the data. The resulting invisible quantum barrier is double-valued in both axes. We study this invisible barrier in the case of atom and Bose-Einstein Condensate reflection from a solid silicon surface. A time-dependent, one-spatial dimension Gross-Pitaevskii equation is solved for the BEC case. We found that the BEC behaves very similarly to the single atom except for size effects, which manifest themselves in a maximum in the reflectivity at small distances from the wall. The effect of the atom-atom interaction on the BEC reflection and correspondingly on the invisible barrier is found to be appreciable at low velocities and comparable to the finite size effect. The trapping of ultracold atoms or BEC between two walls is discussed., Comment: 12 pages, 5 figures; This submission has been withdrawn by the authors.

We consider a novel system of two-component atomic Bose-Einstein condensate in a double-well potential. Based on the well-known two-mode approximation, we demonstrate that there are obvious avoided level-crossings when both interspecies and intraspecies interactions of two species are increased. The quantum dynamics of the system exhibits revised oscillating behaviors compared with a single component condensate. We also examine the entanglement of two species. Our numerical calculations show the onset of entanglement can be signed as a violation of Cauchy-Schwarz inequality of second-order cross correlation function. Consequently, we use Von Neumann entropy to quantity the degree of entanglement.