1. Strain-Induced Plasmon Confinement in Polycrystalline Graphene
- Author
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Simone Zanotto, Luca Bonatti, Maria F. Pantano, Vaidotas Mišeikis, Giorgio Speranza, Tommaso Giovannini, Camilla Coletti, Chiara Cappelli, Alessandro Tredicucci, Alessandra Toncelli, Zanotto, Simone, Bonatti, Luca, Pantano, Maria F, Mišeikis, Vaidota, Speranza, Giorgio, Giovannini, Tommaso, Coletti, Camilla, Cappelli, Chiara, Tredicucci, Alessandro, and Toncelli, Alessandra
- Subjects
terahertz ,plasmon ,strain ,graphene ,conductivity of polycrystalline 2D material ,Electrical and Electronic Engineering ,atomistic simulations ,Atomic and Molecular Physics, and Optics ,Drude-Smith ,Settore CHIM/02 - Chimica Fisica ,Biotechnology ,Electronic, Optical and Magnetic Materials - Abstract
Terahertz spectroscopy is a perfect tool to investigate the electronic intraband conductivity of graphene, but a phenom-enological model (Drude-Smith) is often needed to describe disorder. By studying the THz response of isotropically strained polycrystalline graphene and using a fully atomistic computational approach to fit the results, we demonstrate here the connection between the Drude-Smith parameters and the microscopic behavior. Importantly, we clearly show that the strain-induced changes in the conductivity originate mainly from the increased separation between the single-crystal grains, leading to enchanced localization of the plasmon excitations. Only at the lowest strain values explored, a behavior consistent with the deformation of the individual grains can instead be observed.
- Published
- 2023
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