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We propose a method for material characterization using Spectral X-ray Computed Tomography (SCT). Our SCT method takes advantage of recently-developed MultiX ME 100 photon counting detectors to simultaneously measure the energy dependence of a material's linear attenuation coefficient (LAC). Relative electron density ( ρ e ) and effective atomic number (Ze) are estimated directly from the energy-dependent LAC measurements. The method employs a spectral correction algorithm and automated selection and weighting of the energy bins for optimized performance. When examining materials with Ze ≤ 23, this method achieves accuracy comparable to traditional dual-energy CT, which is often realized through consecutive data acquisitions, and is compatible with any spectral detector. The method disregards data in photon starved energy channels improving the detection of highly attenuating materials, compared to techniques that use energy integrating detectors.

Laser experiments, such as those planned at the National Ignition Facility (NIF) and the Omega facility, use small targets with the goal of studying high-energy density physics and inertial confinement fusion. One particular application is a target with layers whose density changes in a carefully designed gradient (from 0.2 to 1.2 g/cm 3 ) for use in isentropic compression experiments (ICE). We are nondestructively determining the density of these layers using two X-ray microscopes. Because of the many interfaces that comprise the layers, a plethora of X-ray phase contrast fringes appear in the images, leading to many radiographic and tomographic artifacts which compromise the ability to infer the density of the layer. In this paper, we describe how we are attacking this problem with a variety of radiographic standards and through radiographic simulation using the HADES radiographic simulation code.

A gamma-ray-based, active (A) and passive (P) computed tomography (CT) technology has been developed that locates, identifies and quantifies gamma-ray emitting isotopes, transuranic (TRU) and others, in nuclear waste drums. ACT uses a collimated external source and a HPGe detector to measure selected mono-energetic gamma-rays that are attenuated by waste-drum contents; a separate PCT measurement uses the HPGe detector to record the spectra of gamma-rays emitted from within a drum. The ACT attenuation images and the PCT emission spectra are coupled to quantitatively assay drum contents for ∼0.1–200 g of TRU isotopes. Calibration requires a single measurement of a known radioactive standard; construction of waste-drum surrogates is not required. Fixed and mobile systems demonstrated compliance with a DOE quality assurance program via several independent blind tests.

We are developing a new technique using both active (A) and passive (P) computed tomography (CT) to overcome problems in the quantitative analysis of plutonium contents in the molten salt extract (MSE) plutonium buttons. Our first three dimensional image of the MSE button using ACT scan has already shown heterogeneous behavior throughout the button as opposed to the model of a homogeneous button as previously thought. An image from a PCT scan, although it does not have sufficient spatial resolution and data, also seems to support the heterogeneous picture.

X-ray computerized tomography (CAT or CT) is a sophisticated imaging technique that provides cross-sectional views of materials, components and assemblies for industrial nondestructive evaluation (NDE). We have studied the feasibility of using CT as an inspection tool for reinforced concrete and the use of multi-energy, linear, attenuation techniques to deduce variations in density (ρ) and/or atomic number (Z) that could be caused by varying the types of concrete mixes and/or compaction in the concrete itself. To perform this study, we designed and built a prototype medium-/high-energy (200- to 2000 keV) CT scanner — ZCAT — to image small concrete samples (± 30 cm in diameter and ± 75 cm in height) with a spatial resolution of about 2 mm. We used ZCAT to quantitatively inspect a 20 cm concrete cube with 1.27 cm diameter reinforcing bars (rebars) and to measure p and/or Z variations in a 20 cm diameter concrete cylinder. We describe the ZCAT scanner design, some of its physical limitations and the data-acquisition parameters used in our study. Our results and those of others [1,2] show that CT can be used to inspect reinforced concrete and to distinguish material p and/or Z variations within concrete.

x-Ray computed axial tomography (CT) provides cross-sectional views of materials, components, and assemblies for industrial non-destructive evaluation. We have applied CT imaging to quantitatively measure the 3-D distribution ogf x-ray attenuation at reasonably high resolutions. In our industrial x-ray CT-studies, we have centered on two technical approaches: a first-generation translate/rotate CT system that consist of well-collimated (∼ 0.55 mm) photon source detector, and a third-generation scanner that uses a fluoroscopy detector.

Considerable effort is being applied to develop multiple-energy industrial CT techniques for materials characterization. Multiple-energy CT can provide reliable estimates of effective Z (Z{sub eff}), weight fraction, and rigorous calculations of absolute density, all at the spatial resolution of the scanner. Currently, a wide variety of techniques exist for CT scanners, but each has certain problems and limitations. Ultimately, the best multi-energy CT technique would combine the qualities of accuracy, reliability, and wide range of application, and would require the smallest number of additional measurements. We have developed techniques for calculating material properties of industrial objects that differ somewhat from currently used methods. In this paper, we present our methods for calculating Z{sub eff}, weight fraction, and density. We begin with the simplest case -- methods for multiple-energy CT using isotopic sources -- and proceed to multiple-energy work with x-ray machine sources. The methods discussed here are illustrated on CT scans of PBX-9502 high explosives, a lexan-aluminum phantom, and a cylinder of glass beads used in a preliminary study to determine if CT can resolve three phases: air, water, and a high-Z oil. In the CT project at LLNL, we have constructed several CT scanners of varying scanning geometries usingmore » {gamma}- and x-ray sources. In our research, we employed two of these scanners: pencil-beam CAT for CT data using isotopic sources and video-CAT equipped with an IRT micro-focal x-ray machine source.« less

Proton beams with energies of 5 and 7 MeV are focused to 5 μm and used to produce tomograms of capillary tubes and low-density foams. In this energy range, proton energy loss is primarily due to interactions with electrons. Therefore, by measuring the residual energy of protons transmitted through samples in a manner similar to that used for Scanning Transmission Ion Microscopy (STIM), and reconstructing a cross-sectional image from multiple projections, we can map out spatial variations in electron density due to sample geometry and composition. In our experimental arrangement, the sample is translated and rotated in a stationary proton beam. Transmitted proton energies are measured using a silicon surface barrier detector. Tomographie reconstructions are produced from the calculated line-average densities using a procedure based on a filtered backprojection algorithm developed for X-ray computed tomography (CT) systems. The technique is especially useful in characterizing samples where large variations in Z or low total density limit the applicability of X-ray CT analysis.