1. Large Polarons as Key Quasiparticles in SrTiO3 and SrTiO3-Based Heterostructures.
- Author
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Geondzhian, Andrey, Sambri, Alessia, De Luca, Gabriella M., Di Capua, Roberto, Di Gennaro, Emiliano, Betto, Davide, Rossi, Matteo, Ying Ying Peng, Fumagalli, Roberto, Brookes, Nicholas B., Braicovich, Lucio, Gilmore, Keith, Ghiringhelli, Giacomo, and Salluzzo, Marco
- Subjects
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POLARONS , *TWO-dimensional electron gas , *HETEROSTRUCTURES , *QUASIPARTICLES , *INELASTIC scattering , *SINGLE crystals - Abstract
Despite its simple structure and low degree of electronic correlation, SrTiO3 (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight into the nature of the quasiparticles shaping the electronic and conduction properties of STO is needed. We studied the low-energy excitations of bulk STO and of the LaAlO3/SrTiO3 two-dimensional electron gas (2DEG) by Ti L3 edge resonant inelastic x-ray scattering. In all samples, we find the hallmark of polarons in the form of intense dd+phonon excitations, and a decrease of the LO3-mode electron-phonon coupling when going from insulating to highly conducting STO single crystals and heterostructures. Both results are attributed to the dynamic screening of the large polaron self-induced polarization, showing that the low-temperature physics of STO and STO-based 2DEGs is dominated by large polaron quasiparticles. [ABSTRACT FROM AUTHOR]
- Published
- 2020
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