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Large Polarons as Key Quasiparticles in SrTiO_{3} and SrTiO_{3}-Based Heterostructures.

Authors :
Geondzhian A
Sambri A
De Luca GM
Di Capua R
Di Gennaro E
Betto D
Rossi M
Peng YY
Fumagalli R
Brookes NB
Braicovich L
Gilmore K
Ghiringhelli G
Salluzzo M
Source :
Physical review letters [Phys Rev Lett] 2020 Sep 18; Vol. 125 (12), pp. 126401.
Publication Year :
2020

Abstract

Despite its simple structure and low degree of electronic correlation, SrTiO_{3} (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight into the nature of the quasiparticles shaping the electronic and conduction properties of STO is needed. We studied the low-energy excitations of bulk STO and of the LaAlO_{3}/SrTiO_{3} two-dimensional electron gas (2DEG) by Ti L_{3} edge resonant inelastic x-ray scattering. In all samples, we find the hallmark of polarons in the form of intense dd+phonon excitations, and a decrease of the LO3-mode electron-phonon coupling when going from insulating to highly conducting STO single crystals and heterostructures. Both results are attributed to the dynamic screening of the large polaron self-induced polarization, showing that the low-temperature physics of STO and STO-based 2DEGs is dominated by large polaron quasiparticles.

Details

Language :
English
ISSN :
1079-7114
Volume :
125
Issue :
12
Database :
MEDLINE
Journal :
Physical review letters
Publication Type :
Academic Journal
Accession number :
33016714
Full Text :
https://doi.org/10.1103/PhysRevLett.125.126401