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Large Polarons as Key Quasiparticles in SrTiO_{3} and SrTiO_{3}-Based Heterostructures.
- Source :
-
Physical review letters [Phys Rev Lett] 2020 Sep 18; Vol. 125 (12), pp. 126401. - Publication Year :
- 2020
-
Abstract
- Despite its simple structure and low degree of electronic correlation, SrTiO_{3} (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight into the nature of the quasiparticles shaping the electronic and conduction properties of STO is needed. We studied the low-energy excitations of bulk STO and of the LaAlO_{3}/SrTiO_{3} two-dimensional electron gas (2DEG) by Ti L_{3} edge resonant inelastic x-ray scattering. In all samples, we find the hallmark of polarons in the form of intense dd+phonon excitations, and a decrease of the LO3-mode electron-phonon coupling when going from insulating to highly conducting STO single crystals and heterostructures. Both results are attributed to the dynamic screening of the large polaron self-induced polarization, showing that the low-temperature physics of STO and STO-based 2DEGs is dominated by large polaron quasiparticles.
Details
- Language :
- English
- ISSN :
- 1079-7114
- Volume :
- 125
- Issue :
- 12
- Database :
- MEDLINE
- Journal :
- Physical review letters
- Publication Type :
- Academic Journal
- Accession number :
- 33016714
- Full Text :
- https://doi.org/10.1103/PhysRevLett.125.126401