Search

Abstract Carbon capture and storage (CCS) is now known to be an effective way to reduce greenhouse gas emissions especially CO 2 to the atmosphere. Amino acid salt (AAS) solutions are regarded as promising CO 2 absorbents compared to traditional amine solutions, as they are environmentally being with lower evaporation as well as fewer degradation issues. This paper is intended to review recent developments in CO 2 capture using AASs. The thermodynamics and kinetics of CO 2 and different AASs are illustrated in detail. We will also discuss the blended solutions containing AASs in terms of applications and absorption or regeneration performance. Additionally, we will present specific directions for future research on CO 2 -AAS systems. This paper could provide a guideline for effective carbon capture by new absorbents. Highlights • A comprehensive review of amino acid salts fundamentals is introduced. • Detailed thermodynamics and kinetics between CO 2 and various amino acid salts are discussed. • The developments of CO 2 capture by amino acid salts in the fields of biogas upgrading, natural gas and flue gas purification are illustrated. [ABSTRACT FROM AUTHOR]

Traditional technologies of carbon capture and storage (CCS) are being focused on capturing CO 2 in large-scale demonstrations, which has been proved to result in the high cost and energy penalty. Meanwhile, typical innovative measures, commonly defined as the second generation CCS technologies, elude conventional ones by integrating with solar energy and thus contributing to a more energy-efficient conversion of CO 2 . However, few reviews pay attention to thermodynamic processes and parameters of these novel technologies, and there is a lack of systematic evaluation and comparison among them. This paper firstly presents a guided tour on the state-of-art of typical and innovative CCS technologies integrated with solar energy. An overview on thermodynamic processes, including chemical reactions, operating conditions and efficiency indexes of five typical technologies is presented so that the current development level can be clarified. Since the high energy requirement and related operating cost are the main barriers to the application of existing CCS technologies, the minimum work and second-law efficiency are applied as the main indicators in the second part of this paper which relates to performance evaluation. In addition, the performance windows for innovative technologies are illustrated for the comparison of technological maturity. The results show that energy requirement of innovative CCS technologies from the flue gas is avg. 100–200 kJ/mol CO 2 and the second-law efficiency of them is only 5–12%. Therefore, the maturity and popularity of these novel technologies are still relatively low. But the well-integrated systems and diversified output of these technologies can benefit existing energy infrastructures in a long period. [ABSTRACT FROM AUTHOR]

Meeting the Paris Agreement will most likely require the combination of CO 2 capture and biomass in the industrial sector, resulting in net negative emissions. CO 2 capture within the industry has been extensively investigated. However, biomass options have been poorly explored, with literature alluding to technical and economic barriers. In addition, a lack of consistency among studies makes comparing the performance of CO 2 capture and/or biomass use between studies and sectors difficult. These inconsistencies include differences in methodology, system boundaries, level of integration, costs, greenhouse gas intensity of feedstock and energy carriers, and capital cost estimations. Therefore, an integrated evaluation of the techno-economic performance regarding CO 2 capture and biomass use was performed for five energy-intensive industrial sub-sectors. Harmonization results indicate that CO 2 mitigation potentials vary for each sub-sector, resulting in reductions of 1.4–2.7 t CO 2 /t steel (77%–149%), 0.7 t CO 2 /t cement (92%), 0.2 t CO 2 /t crude oil (68%), 1.9 t CO 2 /t pulp (1663%–2548%), and 34.9 t CO 2 /t H 2 (313%). Negative emissions can be reached in the steel, paper and H 2 sectors. Novel bio-based production routes might enable net negative emissions in the cement and (petro)chemical sectors as well. All the above-mentioned potentials can be reached for 100 €/t CO 2 or less. Implementing mitigation options could reduce industrial CO 2 emissions by 10 Gt CO 2 /y by 2050, easily meeting the targets of the 2 °C scenario by the International Energy Agency (1.8 Gt CO 2 /y reduction) for the industrial sector and even the Beyond 2 °C scenario (4.2 Gt CO 2 /y reduction). • Literature review on CO 2 mitigation in steel, cement, chemical, H 2 and paper sectors. • Introduction harmonized methodology to allow comparison between industrial sectors. • All investigated sectors have large reduction potentials for <100 €/t CO 2 avoided. • Negative emissions possible in iron/steel, H 2 and paper sectors. • Potential CO 2 emission reduction of 10 Gt/yr in 2050, easily meeting climate target. [ABSTRACT FROM AUTHOR]

The long-term energy strategy issued by the German government in 2010 and 2011 embraces a substantial reduction of CO 2 emissions and high shares of renewable energy in electricity production, along with energy efficiency improvements and an accelerated nuclear phase-out. While several studies illustrate scenarios reaching these targets, there are substantial uncertainties pertaining to key assumptions, particularly long-term electricity demand and the large-scale availability of offshore wind and carbon capture and storage (CCS). This paper explores conditions under which model-based scenarios for the German electricity sector comply with the official targets for CO 2 emission reductions and renewable shares. We apply the energy system model LIMES-D, which allows for a joint optimization of generation and transmission capacities. The results indicate that reducing electricity demand plays a crucial role for attaining the government׳s targets. Scenarios for which either offshore wind or CCS is not available show an even stronger need for a decreasing electricity demand to reach the targets and a different pattern of transmission capacity expansion than is the case with full technology availability. Hence, a broad technology portfolio could in turn hedge against future power demand increases that may challenge the joint attainment of the German decarbonization and renewable energy targets. [ABSTRACT FROM AUTHOR]

Abstract: Climate change is fast becoming the major environmental and energy concern worldwide. There is a major dilemma between the continued reliance on fossil fuel for our energy supply and the pressing need to address the problem of greenhouse gas (GHG) emissions from combustion process. This paper reviews the potential for carbon capture and storage (CCS) as a part of the climate change mitigation strategy for the Malaysian electricity sector using a technology assessment framework. The nation''s historical trend of high reliance on fossil fuel for its electricity sector makes it a prime candidate for CCS adoption. The suitability and practicality of the technology was reviewed from a broad perspective with consideration of Malaysia-specific conditions. It is apparent from this assessment that CCS has the potential to play an important role in Malaysia''s climate change mitigation strategy provided that key criteria are fulfilled. [Copyright &y& Elsevier]