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We demonstrate an approach for a real-time, consumable-free optical system operating on a liquid jet which can be easily derived from the water distribution infrastructure. We apply a pump-probe scheme based on the acquisition and nanosecond manipulation of UV-excited fluorescence to increase the selective identification of bacterial against organic pollutants in water.

We characterized the white-light supercontinuum emission by a sub-petawatt laser system in the atmosphere via light detection and ranging measurements. As much as 1 J of supercontinuum is generated in the atmosphere, corresponding to a conversion efficiency of 30 %. This generation occurs at altitudes below 100 m. The high initial beam intensity results in the saturation of the number of self-guided filaments. Therefore, the “photon bath” surrounding the filaments strongly contributes to the white-light generation. These finding is well reproduced by numerical simulations based on the experimental parameters.

We show that the coherent manipulation of molecular wavepackets in the excited states of trp-containing dipeptides allows efficient discrimination among them. Optimal dynamic discrimination fails, however, for some dipeptide couples. When considering the limited spectral resources at play (3 nm bandwidth at 266 nm), we discuss the concept of discriminability, which appears uncorrelated to both static spectra and relaxation lifetimes.

The electric conductivity, HV discharge triggering and guiding capabilities of filaments at 3.9 micrometer in air are investigated in the perspective of lightning control applications, and compared to near-IR filaments in identical conditions

International audience; We have investigated nanocrystals of Fe(IO3)3 by polarization-sensitive second harmonic generation (SHG) microscopy. As the nonlinear optical properties of this material were only poorly characterized, we have first determined the relative values of the elements of its second-order susceptibility tensor, by the global fitting of the polarization-resolved SHG response of an ensemble of nanocrystals. This information allows one to optically retrieve the orientation of individual particles in the sample. The high SHG efficiency measured for nanocrystals of Fe(IO3)3 and their polar nature could make them very attractive for nonlinear microscopy of biological samples.

Intensity correlations and noise reduction are observed and characterized in the broadband supercontinuum generated by spatio-temporal solitons propagating in air, i.e., in filamentation of ultrashort laser pulses. Large correlations and reduction of the laser noise are observed already at the first steps of the filamentation process, while further propagation results in cascaded χ(3) broadening processes and yield complex correlation maps. The spectral range yielding an optimal laser noise reduction of 3.6 dB is found to cover 10 nm around the fundamental wavelength.

International audience; We report new experimental and numerical results on supercontinuum generation at ultraviolet/visible wavelengths produced by the propagation of infrared femtosecond laser pulses in air. Spectral broadening is shown to similarly affect single filaments over laboratory distance scales, as well as broad beams over long-range propagation distances. Numerical simulations display evidence of the crucial role of third harmonic generation in the build-up of UV-visible wavelengths, by comparison with current single-envelope models including chromatic dispersion and self-steepening.

A new ray-tracing scheme is proposed to simulate the non-linear propagation of ultra-short pulses. The results are in good agreement with experimental data and numerical solving of the non-linear Schrodinger equation in both the self-focusing and the filamentation regions. In particular, they indicate a major contribution of the ‘photon bath’ in the self-guided propagation of ultra-short pulses. The model suggests that a pure-Kerr self-guiding mode can allow filamentation without ionization.

An unexpected blue-fluorescence band (around 420 nm) from both micrometer-sized dried particles and aqueous droplets of riboflavin [7,8-dimethyl-10-(D-1′-ribityl)-isoalloxazine] is observed when the microparticles are irradiated with a pulsed UV (355- or 351-nm) laser. The intensity of the band increases quadratically with input laser energy density (fluence) and is attributable to a one-photon-excited fluorescence of lumichrome (7,8-dimethyl-alloxazine) that is produced by photo-degradation of riboflavin. The well-known greenish-yellow fluorescence band (at 560 nm for dried particles and 535 nm for aqueous droplets) from riboflavin increases sublinearly with UV-laser fluence. With a laser input fluence above 5 J/cm2 the riboflavin fluorescence decays earlier and the lumichrome fluorescence reaches a maximum later than the peak of the input laser pulse. The temporal dynamics of the 420- and 535-nm fluorescence peaks are consistent with a rate-equation simulation of photon-induced conversion of riboflavin to lumichrome and the subsequent fluorescence of lumichrome.

A four wavelength backscattering depolarization LIDAR designed for polar stratospheric cloud and stratospheric aerosol measurement is described. The system uses the following wavelengths: 355 nm, 532 nm, 750 nm, and 850 nm. These wavelengths, obtained by means of the third- and second-harmonic of a Nd: YAG laser and by means of a tunable Ti: Sapphire laser, are chosen in a way to better characterize the particel size of such stratospheric aerosols. They are not emitted simultaneously as the LIDAR system is designed with only two detection channels permitting to detect, in the analog and in the photon counting mode, both the direct and the depolarized backscattered signal. The system has been operational in northern Finland since the end of November 1991.

In 2010, we reported [1] on a demonstration of a mobile source of high-energy near-single-cycle THz pulses based on a tilted pulse front optical rectification set-up, pumped by a mobile terawatt laser (Teramobile). The absolute value of the THz pulse energy was measured with a pyroelectric detector (Coherent Molectron J4-05). The company does not provide a spectral sensitivity dependence for this detector below 3.3 THz. In the reported experiments, generated THz pulses had broad spectra centred at 0.2 THz [1]. Previously, this detector was used for measuring the energy of near-single-cycle THz pulses with an average frequency of 0.9 THz generated by an accelerator-based source [2]. Afterwards, it was reported that the sensitivity of the Coherent pyroelectric detector at 1 THz was approximately 1.8 times less than the specified sensitivity at 1.06 lm [3], and this difference has been take into account in a following publication [7]. Recently, we compared the sensitivity of the Coherent Molectron J4-05 detector with that of another widely used pyroelectric THz detector (Microtech Instruments) [3–6]. The latter detector is provided with a calibration curve of the spectral dependence of the sensitivity in the frequency range of 0.12–3 THz. As a result, we found that at frequencies of 0.2–0.5 THz, the Coherent Molectron J4-05 detector underestimates the THz pulse energy by a factor of about 3.5 with regard to the Microtech Instruments detector. This finding evidences an additional drop of the Coherent Molectron J4-05 detector sensitivity for THz wave frequencies below 1 THz. By this comparison, we conclude that the THz pulse energy in Ref. [1] should significantly be re-estimated, up to 175 lJ (instead of the initially published value of 50 lJ), which is to the best of our knowledge the highest energy of near-single-cycle THz pulses generated by tabletop sources.