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1. Stereocontrolled syntheses of Kainoid amino acids from 7-azabicyclo[2.2.] heptadienes using tandem radical addition-homoallylic radical rearrangement

Author

Hodgson, David M., Hachisu, Shuji, and Andrews, Mark D.

Subjects
Amino acids -- Chemical properties, Pyrrole -- Chemical properties, Oxidation-reduction reaction -- Research, Biological sciences, Chemistry
Abstract

A full account of extension and adaptation of the methodology to the addition of carbon-based radicals to 7-azabicyclo[2.2.1]heptadienes is presented. Oxidative cleavage of the resulting 2-azabicyclo[2.2.1]hept-5-enes provide straightfoward access to polysubstituted pyrrolidines and in particular an efficient entry to the Kainoid amino acids.

Published
2005

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