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The number of large urban agglomerations is steadily increasing worldwide. At a local scale, their emissions lead to air pollution, directly affecting people's health. On a global scale, their emissions lead to an increase of greenhouse gases, affecting climate. In this context, in 2017 and 2018, the airborne campaign EMeRGe (Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales) investigated emissions of European and Asian major population centres (MPCs) to improve the understanding and predictability of pollution outflows. Here, we present two methods to identify and characterise pollution outflows probed during EMeRGe. First, we use a set of volatile organic compounds (VOCs) as chemical tracers to characterise air masses by specific source signals, i.e. benzene from anthropogenic pollution of targeted regions, acetonitrile from biomass burning (BB, primarily during EMeRGe-Asia), and isoprene from fresh biogenic signals (primarily during EMeRGe-Europe. Second, we attribute probed air masses to source regions and estimate their individual contribution by constructing and applying a simple emission uptake scheme for the boundary layer which combines FLEXTRA back trajectories and EDGAR carbon monoxide (CO) emission rates (acronyms are provided in the Appendix). During EMeRGe-Europe, we identified anthropogenic pollution outflows from northern Italy, southern Great Britain, the Belgium–Netherlands–Ruhr (BNR) area and the Iberian Peninsula. Additionally, our uptake scheme indicates significant long-range transport of pollution from the USA and Canada. During EMeRGe-Asia, the pollution outflow is dominated by sources in China and Taiwan, but BB signals from Southeast Asia and India contribute as well. Outflows of pre-selected MPC targets are identified in less than 20 % of the sampling time, due to restrictions in flight planning and constraints of the measurement platform itself. Still, EMeRGe combines in a unique way near- and far-field measurements, which show signatures of local and distant sources, transport and conversion fingerprints, and complex air mass compositions. Our approach provides a valuable classification and characterisation of the EMeRGe dataset, e.g. for BB and anthropogenic influence of potential source regions and paves the way for a more comprehensive analysis and various model studies.

Abstract Characterizing the size and settling velocity of pyroclastic fragments injected into the atmosphere during volcanic eruptions (i.e., tephra) is crucial to the forecasting of plume and cloud dispersal. Optical disdrometers have been integrated into volcano monitoring networks worldwide in order to best constrain these parameters in real time. Nonetheless, their accuracy during tephra fallout still needs to be assessed. A significant complication is the occurrence of particle aggregates that modify size and velocity distributions of falling tephra. We made the first use of the Thies Clima Laser Precipitation Monitor (LPM) for tephra-fallout detection at Sakurajima volcano (Japan), which is characterized by a lower size detection window with respect to more commonly used disdrometers (e.g., Parsivel2) and can more easily distinguish different falling objects. For the first time, individual particles have been distinguished from most aggregates based on disdrometer data, with the potential to provide useful grain-size information in real time. In case of negligible aggregation, LPM and collected sample-based estimates are in agreement for both grain-size and sedimentation rate. In case of significant aggregation, particle shape analyses and a dedicated drag equation are used to filter out aggregates from LPM data that also provide good agreement with collected tephra samples.

Abstract Aggregation of volcanic ash is known to significantly impact sedimentation from volcanic plumes. The study of particle aggregates during tephra fallout is crucial to increase our understanding of both ash aggregation and sedimentation. In this work, we describe key features of ash aggregates and ash sedimentation associated with eleven Vulcanian explosions at Sakurajima Volcano (Japan) based on state-of-the-art sampling techniques. We identified five types of aggregates of both Particle Cluster (PC) and Accretionary Pellet (AP) categories. In particular, we found that PCs and the first and third type of APs can coexist within the same eruption in rainy conditions. We also found that the aerodynamic properties of aggregates (e.g., terminal velocity and density) depend on their type. In addition, grainsize analysis revealed that characteristics of the grainsize distributions (GSDs) of tephra samples correlate with the typology of the aggregates identified. In fact, bimodal GSDs correlate with the presence of cored clusters (PC3) and liquid pellets (AP3), while unimodal GSDs correlate either with the occurrence of ash clusters (PC1) or with the large particles (coarse ash) coated by fine ash (PC2).

Abstract Volcanic ash has the capacity to impact human health, livestock, crops and infrastructure, including international air traffic. For recent major eruptions, information on the volcanic ash plume has been combined with relatively coarse-resolution meteorological model output to provide simulations of regional ash dispersal, with reasonable success on the scale of hundreds of kilometres. However, to predict and mitigate these impacts locally, significant improvements in modelling capability are required. Here, we present results from a dynamic meteorological-ash-dispersion model configured with sufficient resolution to represent local topographic and convectively-forced flows. We focus on an archetypal volcanic setting, Soufrière, St Vincent, and use the exceptional historical records of the 1902 and 1979 eruptions to challenge our simulations. We find that the evolution and characteristics of ash deposition on St Vincent and nearby islands can be accurately simulated when the wind shear associated with the trade wind inversion and topographically-forced flows are represented. The wind shear plays a primary role and topographic flows a secondary role on ash distribution on local to regional scales. We propose a new explanation for the downwind ash deposition maxima, commonly observed in volcanic eruptions, as resulting from the detailed forcing of mesoscale meteorology on the ash plume.

The realistic representation of atmospheric pollutant dispersal over areas of complex topography presents a challenging application for meteorological models. Here, we present results from high–resolution atmospheric modeling in order to gain insight into local processes that can affect ash transport and deposition. The nested Weather Research and Forecasting (WRF) model with the finest resolution of 50 m was used to simulate atmospheric flow over the complex topography of Sakurajima volcano, Japan, for two volcanic eruption cases. The simulated airflow results were shown to compare well against surface observations. As a preliminary application, idealized trajectory modeling for the two cases revealed that accounting for local circulations can significantly impact volcanic ash deposition leading to a total fall velocity up to 2–3 times the particle’s terminal velocity depending on the size. Such a modification of the estimated particle settling velocity over areas with complex topography can be used to parametrize the impact of orographic effects in dispersal models, in order to improve fidelity.

Vulcanian eruptions (short-lived explosions consisting of a rising thermal) occur daily in volcanoes around the world. Such small-scale eruptions represent a challenge in numerical modeling due to local-scale effects, such as the volcano’s topography impact on atmospheric circulation and near-vent plume dynamics, that need to be accounted for. In an effort to improve the applicability of Tephra2, a commonly-used advection-diffusion model, in the case of vulcanian eruptions, a number of key modifications were carried out: (i) the ability to solve the equations over bending plume, (ii) temporally-evolving three-dimensional meteorological fields, (iii) the replacement of the particle diameter distribution with observed particle terminal velocity distribution which provides a simple way to account for the settling velocity variation due to particle shape and density. We verified the advantage of our modified model (Tephra4D) in the tephra dispersion from vulcanian eruptions by comparing the calculations and disdrometer observations of tephra sedimentation from four eruptions at Sakurajima volcano, Japan. The simulations of the eruptions show that Tephra4D is useful for eruptions in which small-scale movement contributes significantly to ash transport mainly due to the consideration for orographic winds in advection.

Ground-based remote sensing equipment have the potential to be used for the nowcasting of the tephra hazard from volcanic eruptions. To do so raw data from the equipment first need to be accurately transformed to tephra-related physical quantities. In order to establish these relations for Sakurajima volcano, Japan, we propose a methodology based on high-resolution simulations. An eruption that occurred at Sakurajima on 16 July 2018 is used as the basis of a pilot study. The westwards dispersal of the tephra cloud was ideal for the observation network that has been installed near the volcano. In total, the plume and subsequent tephra cloud were recorded by 2 XMP radars, 1 lidar and 3 optical disdrometers, providing insight on all phases of the eruption, from plume generation to tephra transport away from the volcano. The Weather Research and Forecasting (WRF) and FALL3D models were used to reconstruct the transport and deposition patterns. Simulated airborne tephra concentration and accumulated load were linked, respectively, to lidar backscatter intensity and radar reflectivity. Overall, results highlight the possibility of using such a high-resolution modelling-based methodology as a reliable complementary strategy to common approaches for retrieving tephra-related quantities from remote sensing data.

At Sakurajima volcano, frequent Vulcanian eruptions have been seen at the summit crater of Minamidake since 1955. In addition to this eruption style, the eruptive activities of Strombolian type and prolonged ash emission also occur frequently. We studied the design of a simulator of advection-diffusion-fallout of volcanic ash emitted continuously. The time function of volcanic ash eruption rate is given by a linear combination of the volcanic tremor amplitude and the volume change of the pressure source obtained from the ground motion. The simulation is repeated using discretized values of the eruption rate time function at an iteration time interval of the simulation. The integrated value of the volcanic ash deposition on the ground obtained from each individual simulation is used to estimate the value of the ash fallout. The plume height is given by an empirical equation proportional to a quarter of the power of the eruption rate. Since the wind velocity field near the volcano is complicated by the influence of the volcanic topography, the predicted values published by meteorological organizations are made in high resolution by Weather Research and Forecasting (WRF) for the simulation. We confirmed that an individual simulation can be completed within a few minutes of iteration interval time, using the PUFF model as the Lagrangian method and FALL3D-8.0 as the Eulerian method on a general-purpose PC. Except during rainfall, the radar reflectivity, the count of particles per particle size, and fall velocity obtained by the disdrometers can be used for the quasi-real time matching of the plume height calculated from the eruption rate and the ash fall deposition rate obtained from the simulation. [ABSTRACT FROM AUTHOR]

The year 2021 marked a decade of holopelagic sargassum (morphotypes Sargassum natans I and VIII, and Sargassum fluitans III) stranding on the Caribbean and West African coasts. Beaching of millions of tons of sargassum negatively impacts coastal ecosystems, economies, and human health. Additionally, the La Soufrière volcano erupted in St. Vincent in April 2021, at the start of the sargassum season. We investigated potential monthly variations in morphotype abundance and biomass composition of sargassum harvested in Jamaica and assessed the influence of processing methods (shade-drying vs. frozen samples) and of volcanic ash exposure on biochemical and elemental components. S. fluitans III was the most abundant morphotype across the year. Limited monthly variations were observed for key brown algal components (phlorotannins, fucoxanthin, and alginate). Shade-drying did not significantly alter the contents of proteins but affected levels of phlorotannins, fucoxanthin, mannitol, and alginate. Simulation of sargassum and volcanic ash drift combined with age statistics suggested that sargassum potentially shared the surface layer with ash for ~50 d, approximately 100 d before stranding in Jamaica. Integrated elemental analysis of volcanic ash, ambient seawater, and sargassum biomass showed that algae harvested from August had accumulated P, Al, Fe, Mn, Zn, and Ni, probably from the ash, and contained less As. This ash fingerprint confirmed the geographical origin and drift timescale of sargassum. Since environmental conditions and processing methods influence biomass composition, efforts should continue to improve understanding, forecasting, monitoring, and valorizing sargassum, particularly as strandings of sargassum show no sign of abating. [ABSTRACT FROM AUTHOR]

Characterizing the size and settling velocity of pyroclastic fragments injected into the atmosphere during volcanic eruptions (i.e., tephra) is crucial to the forecasting of plume and cloud dispersal. Optical disdrometers have been integrated into volcano monitoring networks worldwide in order to best constrain these parameters in real time. Nonetheless, their accuracy during tephra fallout still needs to be assessed. A significant complication is the occurrence of particle aggregates that modify size and velocity distributions of falling tephra. We made the first use of the Thies Clima Laser Precipitation Monitor (LPM) for tephra-fallout detection at Sakurajima volcano (Japan), which is characterized by a lower size detection window with respect to more commonly used disdrometers (e.g., Parsivel2) and can more easily distinguish different falling objects. For the first time, individual particles have been distinguished from most aggregates based on disdrometer data, with the potential to provide useful grain-size information in real time. In case of negligible aggregation, LPM and collected sample-based estimates are in agreement for both grain-size and sedimentation rate. In case of significant aggregation, particle shape analyses and a dedicated drag equation are used to filter out aggregates from LPM data that also provide good agreement with collected tephra samples. [ABSTRACT FROM AUTHOR]

Aggregation of volcanic ash is known to significantly impact sedimentation from volcanic plumes. The study of particle aggregates during tephra fallout is crucial to increase our understanding of both ash aggregation and sedimentation. In this work, we describe key features of ash aggregates and ash sedimentation associated with eleven Vulcanian explosions at Sakurajima Volcano (Japan) based on state-of-the-art sampling techniques. We identified five types of aggregates of both Particle Cluster (PC) and Accretionary Pellet (AP) categories. In particular, we found that PCs and the first and third type of APs can coexist within the same eruption in rainy conditions. We also found that the aerodynamic properties of aggregates (e.g., terminal velocity and density) depend on their type. In addition, grainsize analysis revealed that characteristics of the grainsize distributions (GSDs) of tephra samples correlate with the typology of the aggregates identified. In fact, bimodal GSDs correlate with the presence of cored clusters (PC3) and liquid pellets (AP3), while unimodal GSDs correlate either with the occurrence of ash clusters (PC1) or with the large particles (coarse ash) coated by fine ash (PC2). [ABSTRACT FROM AUTHOR]

Volcanic plumes from small and moderate eruptions represent a challenge in the study of plume morphology due to eruption source parameter uncertainties and atmospheric influence. Sakurajima volcano, Japan, features such activity and due to its continuous eruptions in the recent years provides an ideal natural laboratory. A data set of 896 eruptions between 2009 and 2016 with well‐constrained plume heights, estimated erupted mass, and associated atmospheric conditions has been compiled. Plume heights ranged between 1,500 and 5,000 m and mainly developed under stable atmospheric stratification and low background wind speeds. The eruptions presented in the database were used to drive FPLUME, a 1‐D integral volcanic plume model, to study the simulated plume morphology. FPLUME was seen to provide consistent results under stable atmospheric stratification. A method for the real‐time monitoring of erupted mass used in the Sakurajima observatory was seen to provide appropriate first guess estimates for the eruptions, showing agreement with analytical and simulated mass flow rate calculations. Volcanic plumes from Sakurajima show significant influence by the atmospheric environment. The plume scaling parameter (Π) was used to characterize the expected degree of plume bending with results correlating well against modeled plume angles. The vertical wind profile was seen to have a significant impact on the resolved plume. Wind shear characteristics were seen to have a mechanical effect on the plume, aiding or inhibiting bending. Finally, potential issues were identified in simulations under unstable atmospheric conditions as the model either failed to provide a solution or overestimated the plume height. Key Points: A database of 896 eruptions from Sakurajima with associated atmospheric profiles is presentedDifferent plume bending regimes are quantitatively evaluated using the FPLUME modelVertical wind shear mechanically affects plume morphology by aiding or inhibiting plume bending [ABSTRACT FROM AUTHOR]

The Sakurajima volcano is characterized by frequent vulcanian eruptions at the Minamidake or Showa crater in the summit area. We installed an integrated monitoring system for the detection of volcanic ash (composed of remote sensing sensors XMP radars, lidar, and GNSS with different wave lengths) and 13 optical disdrometers on the ground covering all directions from the crater to measure drop size distribution and falling velocity. Campaign sampling of volcanic ash supports the conversion of particle counts measured by the disdrometer to the weight of volcanic ash. Seismometers and tilt/strain sensors were used to estimate the discharge rate of volcanic ash from the vents. XMP radar can detect volcanic ash clouds even under visual difficulty because of weather such as fog or clouds. A vulcanian eruption on November 13 was the largest event at the Sakurajima volcano in 2017; however, the volcanic plume was not visible due to clouds covering the summit. Radar revealed that the volcanic plume reached an elevation of 4.2-6.2 km. Post-fit phase residuals (PPR) from the GNSS analysis increased suddenly after the eruption, and large-PPR paths from the satellites to the groundbased receivers intersected each other at an elevation of 4.2 km. The height of the volcanic plume was also estimated from the discharge rate of volcanic ash to be 4.5 km, which is empirically related to seismic energy and the deflation volume obtained via ground deformation monitoring. Using the PUFF model, the weight of the ash-fall deposit was accurately forecast in the main direction of transport of the volcanic ash, which was verified by disdrometers. For further advances in forecasting of the ash-fall deposit, we must consider high-resolution wind field, shape of volcanic plume as the initial value, and the particle number distribution along the volcanic plume. [ABSTRACT FROM AUTHOR]

A high-resolution forecast methodology for the ash hazard at Sakurajima volcano, Japan, is presented. The methodology employs a combined modeling approach and utilizes eruption source parameters estimated by geophysical observations from Sakurajima, allowing for a proactive approach in forecasting. The Weather Research and Forecasting (WRF) model is used to downscale Japan Meteorological Agency (JMA) forecast data over the area of interest. The high-resolution meteorological data are then used in FALL3D model to provide a forecast for the ash dispersal and deposition. The methodology is applied for an eruption that occurred on June 16, 2018. Disdrometer observations of ashfall are used along with ash dispersal modeling to inform the choice of the total grain size distribution (TGSD). A series of pseudo-forecast ash dispersal simulations are then carried out using the proposed methodology and estimated TGSD, initialized with meteorological forecast data released up to ~13 hours before the eruption, with results showing surprising consistency up to ~10 hours before the eruption. Using forecast data up to 4 hours before the eruption was seen to constrain observation to model ratios within a factor of 2-4 depending on the timing of simulation and location. A number of key future improvements for the methodology are also highlighted. [ABSTRACT FROM AUTHOR]

This paper reports a preliminary attempt to determine volcanic ash particle size distribution using the video drop size detector (VDSD) for estimating volcanic ash amount with X-band radar. The VDSD records an image showing the size and number of particles falling into the aperture by a charge coupled device camera. Size distribution spectra of a range of particles from fine ash to small lapilli were derived in discrete form from the VDSD observation. The parameterization of the particle size distribution following Gamma function was done using volcanic ash of eruptions at the Sakurajima Volcano between December 13-21, 2014. Three Gamma distribution parameters were determined analytically. The analytical results revealed a continuous distribution of particles characterized by shape, intercept, and slope. The distribution was used to determine volcanic mass concentration, ground deposit weight, and reflectivity. Verification of these results with X-band radar observations showed that the reflectivity obtained from analytical results is similar to that fromradar observation. However, the ground deposit weight from analysis was overestimated, compared with the real weight of ash deposit on the ground. The algorithm proposed in this study is expected to provide a practical method for estimating ash distribution in the aftermath of a volcanic eruption using radar-reflectivity for cases where direct measurement at the location is not possible. An overview of the algorithm for volcanic ash retrieval from X-band radar observations is also presented. [ABSTRACT FROM AUTHOR]

Intense rainfall over active volcanoes is known to trigger dangerous volcanic hazards, from remobilizing loose volcanic surface material into lahars or mudflows to initiating explosive activity including pyroclastic flows at certain dome-forming volcanoes. However, the effect of the heated volcanic surface on the atmospheric circulation, including any feedback with precipitation, is unknown. This is investigated here, using the Weather Research and Forecasting (WRF) Model. The recent activity at the Soufrière Hills Volcano (SHV), Montserrat, is a well-documented case of such rainfall-volcano interaction and is used as a template for these experiments. The volcano is represented in the model by an idealized Gaussian mountain, with an imposed realistic surface temperature anomaly on the volcano summit. A robust increase in precipitation over the volcano is simulated for surface temperature anomalies above approximately 40°C, an area-average value that is exceeded at the SHV. For wind speeds less than 4 m s−1 and a range of realistic atmospheric conditions, the precipitation increase is well above the threshold required to trigger volcanic hazards (5-10 mm h−1). Hence, the thermal atmospheric forcing due to an active, but nonerupting, volcano appears to be an important factor in rainfall-volcano interactions and should be taken account of in future hazard studies. [ABSTRACT FROM AUTHOR]

This article explores the impact of international exhibitions and world fairs on the practices of women in smaller countries like Greece, and to argue that these exhibitions offered a model in terms of content, reason and form that was later employed and transformed to fit into a nationalist frame. Using archival material, I focus on two interrelated aspects of exhibitions: first, I attempt to follow and understand the creation of a prototype, that of women’s exhibition, in a national Greek context. Then, I discuss how women’s organisations, such as ‘Ergani Athena’ and the Lyceum Club of Greek Women employed these models to organise women’s exhibitions of arts and crafts in Greece. These exhibitions became the model for similar efforts for years to come and influenced collections and museums of decorative and folk arts. The discussion of Greek women and their involvement in both national and international exhibitions can enrich historical paradigms regarding women and world fairs, and thus contribute to the analysis of the phenomenon on a global scale. Furthermore, it provides a sharper view of the female contribution to framing modern Greek national identity in the public sphere, and allows us to connect the histories of gender, nationalism and the emergence of museum exhibits. [ABSTRACT FROM AUTHOR]

The realistic representation of atmospheric pollutant dispersal over areas of complex topography presents a challenging application for meteorological models. Here, we present results from high–resolution atmospheric modeling in order to gain insight into local processes that can affect ash transport and deposition. The nested Weather Research and Forecasting (WRF) model with the finest resolution of 50 m was used to simulate atmospheric flow over the complex topography of Sakurajima volcano, Japan, for two volcanic eruption cases. The simulated airflow results were shown to compare well against surface observations. As a preliminary application, idealized trajectory modeling for the two cases revealed that accounting for local circulations can significantly impact volcanic ash deposition leading to a total fall velocity up to 2–3 times the particle's terminal velocity depending on the size. Such a modification of the estimated particle settling velocity over areas with complex topography can be used to parametrize the impact of orographic effects in dispersal models, in order to improve fidelity. [ABSTRACT FROM AUTHOR]

Vulcanian eruptions (short-lived explosions consisting of a rising thermal) occur daily in volcanoes around the world. Such small-scale eruptions represent a challenge in numerical modeling due to local-scale effects, such as the volcano's topography impact on atmospheric circulation and near-vent plume dynamics, that need to be accounted for. In an effort to improve the applicability of Tephra2, a commonly-used advection-diffusion model, in the case of vulcanian eruptions, a number of key modifications were carried out: (i) the ability to solve the equations over bending plume, (ii) temporally-evolving three-dimensional meteorological fields, (iii) the replacement of the particle diameter distribution with observed particle terminal velocity distribution which provides a simple way to account for the settling velocity variation due to particle shape and density. We verified the advantage of our modified model (Tephra4D) in the tephra dispersion from vulcanian eruptions by comparing the calculations and disdrometer observations of tephra sedimentation from four eruptions at Sakurajima volcano, Japan. The simulations of the eruptions show that Tephra4D is useful for eruptions in which small-scale movement contributes significantly to ash transport mainly due to the consideration for orographic winds in advection. [ABSTRACT FROM AUTHOR]

Ground-based remote sensing equipment have the potential to be used for the nowcasting of the tephra hazard from volcanic eruptions. To do so raw data from the equipment first need to be accurately transformed to tephra-related physical quantities. In order to establish these relations for Sakurajima volcano, Japan, we propose a methodology based on high-resolution simulations. An eruption that occurred at Sakurajima on 16 July 2018 is used as the basis of a pilot study. The westwards dispersal of the tephra cloud was ideal for the observation network that has been installed near the volcano. In total, the plume and subsequent tephra cloud were recorded by 2 XMP radars, 1 lidar and 3 optical disdrometers, providing insight on all phases of the eruption, from plume generation to tephra transport away from the volcano. The Weather Research and Forecasting (WRF) and FALL3D models were used to reconstruct the transport and deposition patterns. Simulated airborne tephra concentration and accumulated load were linked, respectively, to lidar backscatter intensity and radar reflectivity. Overall, results highlight the possibility of using such a high-resolution modelling-based methodology as a reliable complementary strategy to common approaches for retrieving tephra-related quantities from remote sensing data. [ABSTRACT FROM AUTHOR]

No abstract is available for this article. [ABSTRACT FROM AUTHOR]