Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona

Aerosols are one of the most important pollutants in the atmosphere and have been monitored for the past few decades by remote sensing and in situ observation platforms to assess the effectiveness of government-managed reduction emission policies and assess their impact on the radiative budget of the Earth's atmosphere. In fact, aerosols can directly modulate incoming short-wave solar radiation and outgoing long-wave radiation and indirectly influence cloud formation, lifetime, and precipitation. In this study, we quantitatively evaluated long-term temporal trends and seasonal variability from a climatological point of view of the optical and microphysical properties of atmospheric particulate matter at the Universitat Politècnica de Catalunya (UPC), Barcelona, Spain, over the past 17 years, through a synergy of lidar, sun photometer, and in situ concentration measurements. Interannual temporal changes in aerosol optical and microphysical properties are evaluated through the seasonal Mann–Kendall test. Long-term trends in the optical depth of the recovered aerosol; the Ångström exponent (AE); and the concentrations of PM10, PM2.5, and PM1 reveal that emission reduction policies implemented in the past decades were effective in improving air quality, with consistent drops in PM concentrations and optical depth of aerosols. The seasonal analysis of the 17-year average vertically resolved aerosol profiles obtained from lidar observations shows that during summer the aerosol layer can be found up to an altitude of 5 km, after a sharp decay in the first kilometer. In contrast, during the other seasons, the backscatter profiles fit a pronounced exponential decay well with a well-defined scale height. Long-range transport, especially dust outbreaks from the Sahara, is likely to occur throughout the year. During winter, the dust aerosol layers are floating above the boundary layer, while during the other seasons they can penetrate the layer. The analysis also revealed that
This research has been supported by the European Union through NextgenerationEU funds and by the following projects along the years: FP5 EARLINET project (grant no. ID EVR1-CT-1999-40003), FP6 EARLINET-ASOS (ID: 25991), FP7 ACTRIS (ID: 262254), H2020 ACTRIS-2 (ID: 654109), ACTRIS-PPP (ID: 739530), ACTRIS IMP (ID: 871115) and ATMO-ACCESS (ID: 101008004), projects of the Spanish National Research programs (grant nos. TIC 431/93, AMB96-1144-C02-01, REN2000-1907-CE, REN2000-1754- C02-02/CLI, REN2003-09753-C02-C02/CLI, REN2003-09753- C02-C CGL2008-01330-E/CLI 02/CLI, REN2002-12784-E, CGL2005-5131-E, CGL2006-27108-E/CLI, CGL2006-26149- E/CLI, CGL2007-28871-/CLI, CTM2006-27154-E/TECNO, TEC2006-07850/TCM, TEC2009-09106, TEC2012-34575, TEC2015-63832-P and PID2019-103886RB-I00), the project of the Catalan Regional Government IMMPACTE, and the ESA project (grant no. 21487/08/NL/HE)
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