Removal of microplastics and nanoplastics from urban waters: Separation and degradation.

The omnipresent micro/nanoplastics (MPs/NPs) in urban waters arouse great public concern. To build a MP/NP-free urban water system, enormous efforts have been made to meet this goal via separating and degrading MPs/NPs in urban waters. Herein, we comprehensively review the recent developments in the separation and degradation of MPs/NPs in urban waters. Efficient MP/NP separation techniques, such as adsorption, coagulation/flocculation, flotation, filtration, and magnetic separation are first summarized. The influence of functional materials/reagents, properties of MPs/NPs, and aquatic chemistry on the separation efficiency is analyzed. Then, MP/NP degradation methods, including electrochemical degradation, advanced oxidation processes (AOPs), photodegradation, photocatalytic degradation, and biological degradation are detailed. Also, the effects of critical functional materials/organisms and operational parameters on degradation performance are discussed. At last, the current challenges and prospects in the separation, degradation, and further upcycling of MPs/NPs in urban waters are outlined. This review will potentially guide the development of next-generation technologies for MP/NP pollution control in urban waters.