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A generalized reduced fluid dynamic model for flow fields and electrodes in redox flow batteries

Authors :
Cheng, Ziqiang
Tenny, Kevin M.
Pizzolato, Alberto
Forner-Cuenca, Antoni
Verda, Vittorio
Chiang, Yet-Ming
Brushett, Fikile R.
Behrou, Reza
Cheng, Ziqiang
Tenny, Kevin M.
Pizzolato, Alberto
Forner-Cuenca, Antoni
Verda, Vittorio
Chiang, Yet-Ming
Brushett, Fikile R.
Behrou, Reza
Source :
AIChE Journal vol.68 (2022) nr.4 [ISSN 0001-1541]
Publication Year :
2022

Abstract

High-dimensional models typically require a large computational overhead for multiphysics applications, which hamper their use for broad-sweeping domain interrogation. Herein, we develop a modeling framework to capture the through-plane fluid dynamic response of electrodes and flow fields in a redox flow cell, generating a computationally inexpensive two-dimensional (2D) model. We leverage a depth-averaging approach that also accounts for variations in out-of-plane fluid motion and departures from Darcy's law that arise from averaging across three-dimensions (3D). Our resulting depth-averaged 2D model successfully predicts the fluid dynamic response of arbitrary in-plane flow field geometries, with discrepancies of <5% for both maximum velocity and pressure drop. This corresponds to reduced computational expense, as compared to 3D representations (<1% of duration and 10% of RAM usage), providing a platform to screen and optimize a diverse set of cell geometries.

Details

Database :
OAIster
Journal :
AIChE Journal vol.68 (2022) nr.4 [ISSN 0001-1541]
Notes :
Cheng, Ziqiang
Publication Type :
Electronic Resource
Accession number :
edsoai.on1359189641
Document Type :
Electronic Resource