Signatures of a two-dimensional ferromagnetic electron gas at the La0.7Sr0.3MnO3/SrTiO3 interface arising from orbital reconstruction

The magnetoresistance of La0.7Sr0.3MnO3/SrTiO3 superlattices with magnetic field rotating out‐of‐plane shows unexpected peaks for in‐plane fields. Resistivity calculations with spin–orbit coupling reveal that orbital reconstruction at the manganite interface leads to a 2D ferromagnetic electron gas coupled antiparallel to the manganite “bulk”. These orbital and magnetic reconstructions are supported by X‐ray linear dichroism and ab initio calculations.