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Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering : Dynamics at Core Ionization Thresholds
- Publication Year :
- 2015
-
Abstract
- Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.
Details
- Database :
- OAIster
- Notes :
- English
- Publication Type :
- Electronic Resource
- Accession number :
- edsoai.on1235009835
- Document Type :
- Electronic Resource
- Full Text :
- https://doi.org/10.1103.PhysRevLett.114.133001