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Continuous tunable lateral magnetic anisotropy in La0.67Ca0.33MnO3/SrRuO3 superlattices by stacking period-modulation

Authors :
Lili Qu
Da Lan
Kexuan Zhang
Enda Hua
Binghui Ge
Liqiang Xu
Feng Jin
Guanyin Gao
Lingfei Wang
Wenbin Wu
Source :
AIP Advances, Vol 11, Iss 7, Pp 075001-075001-7 (2021)
Publication Year :
2021
Publisher :
AIP Publishing LLC, 2021.

Abstract

Effective control of magnetic anisotropy is important for developing spintronic devices. In this work, we performed a case study of stacking periods (N)-mediated reorientation of lateral magnetic anisotropy in ultrathin La0.67Ca0.33MnO3/SrRuO3 superlattices. As N increases from 1 to 15, the magnetic easy-axis switches from the orthorhombic [010] to [100]-axis. The maximum anisotropy constant of the superlattice (SL) (N = 15) reaches −1.83 × 105 erg/cm3. X-ray absorption spectroscopy and x-ray linear dichroism further suggest that the observed changes in lateral magnetic anisotropy are driven by in-plane orbital polarization. For SLs with small N, anisotropic strain-induced orbital polarization along the b-axis can result in the [010]-oriented magnetic easy axis. For SLs with large N, the dimension crossover from 2-dimension to 3-dimension could enhance the hybridization of Ru t2g and Mn dx2−y2 orbitals, which can compete with the strain effect and switch the magnetic easy axis to [100]. Our results suggest a potential strategy for engineering magnetic anisotropy through the cooperation of strain engineering and interfacial orbital engineering.

Subjects

Subjects :
Physics
QC1-999

Details

Language :
English
ISSN :
21583226
Volume :
11
Issue :
7
Database :
Directory of Open Access Journals
Journal :
AIP Advances
Publication Type :
Academic Journal
Accession number :
edsdoj.93a43356b4dd40d6a93f635154c37863
Document Type :
article
Full Text :
https://doi.org/10.1063/5.0052109