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UV-induced catalyst-free intramolecular formal Heck reaction

Authors :
Wangsheng Liu
Dongmei Ma
Hao Guo
Guangxin Gu
Source :
Journal of Saudi Chemical Society, Vol 23, Iss 6, Pp 718-724 (2019)
Publication Year :
2019
Publisher :
Elsevier, 2019.

Abstract

A catalyst-free intramolecular formal Heck reaction has been developed, affording 9-benzylidene-9H-fluorene derivatives under UV irradiation. This reaction probably proceeds via UV-induced homolytic cleavage of CI bond, addition of the aryl radical to the alkene moiety, single electron oxidation of alkyl radical intermediate into carbocation species, and deprotonation. Keywords: Photochemistry, Cyclization, Radical, Fluorene

Subjects

Subjects :
Chemistry
QD1-999

Details

Language :
English
ISSN :
13196103
Volume :
23
Issue :
6
Database :
Directory of Open Access Journals
Journal :
Journal of Saudi Chemical Society
Publication Type :
Academic Journal
Accession number :
edsdoj.7941938b9054489a36d4b000b421d92
Document Type :
article
Full Text :
https://doi.org/10.1016/j.jscs.2018.12.001