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Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water

Authors :
Yiou Wang
Xu Liu
Xiaoyu Han
Robert Godin
Jialu Chen
Wuzong Zhou
Chaoran Jiang
Jamie F. Thompson
K. Bayazit Mustafa
Stephen A. Shevlin
James R. Durrant
Zhengxiao Guo
Junwang Tang
Source :
Nature Communications, Vol 11, Iss 1, Pp 1-9 (2020)
Publication Year :
2020
Publisher :
Nature Portfolio, 2020.

Abstract

Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol.

Subjects

Subjects :
Science

Details

Language :
English
ISSN :
20411723
Volume :
11
Issue :
1
Database :
Directory of Open Access Journals
Journal :
Nature Communications
Publication Type :
Academic Journal
Accession number :
edsdoj.455d9001207c44ddbeb635584c223a1c
Document Type :
article
Full Text :
https://doi.org/10.1038/s41467-020-16227-3