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Polariton condensation in an organic microcavity utilising a hybrid metal-DBR mirror

Authors :
Kirsty E. McGhee
Anton Putintsev
Rahul Jayaprakash
Kyriacos Georgiou
Mary E. O’Kane
Rachel C. Kilbride
Elena J. Cassella
Marco Cavazzini
Denis A. Sannikov
Pavlos G. Lagoudakis
David G. Lidzey
Source :
Scientific Reports, Vol 11, Iss 1, Pp 1-12 (2021)
Publication Year :
2021
Publisher :
Nature Portfolio, 2021.

Abstract

Abstract We have developed a simplified approach to fabricate high-reflectivity mirrors suitable for applications in a strongly-coupled organic-semiconductor microcavity. Such mirrors are based on a small number of quarter-wave dielectric pairs deposited on top of a thick silver film that combine high reflectivity and broad reflectivity bandwidth. Using this approach, we construct a microcavity containing the molecular dye BODIPY-Br in which the bottom cavity mirror is composed of a silver layer coated by a SiO2 and a Nb2O5 film, and show that this cavity undergoes polariton condensation at a similar threshold to that of a control cavity whose bottom mirror consists of ten quarter-wave dielectric pairs. We observe, however, that the roughness of the hybrid mirror—caused by limited adhesion between the silver and the dielectric pair—apparently prevents complete collapse of the population to the ground polariton state above the condensation threshold.

Subjects

Subjects :
Medicine
Science

Details

Language :
English
ISSN :
20452322
Volume :
11
Issue :
1
Database :
Directory of Open Access Journals
Journal :
Scientific Reports
Publication Type :
Academic Journal
Accession number :
edsdoj.167aebf98fbd43f2aadb3bcaeb9209b6
Document Type :
article
Full Text :
https://doi.org/10.1038/s41598-021-00203-y