The mutual dynamics of a resonant particle inside rectangular cavity: Collective polarizability calculation via a ladder-type alternative Green's functions approach

Light-matter interaction plays a pivotal role in pushing forward nanotechnology. A particularly important setup involves a resonating particle, say an emitting molecule or a macroscopic quasi-statically resonating ferromagnetic sphere, that is located inside a cavity. In this paper, we provide an analytic formulation for the exact calculation of the mutual dynamics between a resonant particle and a rectangular cavity in which it is located. The particle is assumed to be small on the wavelength, and thus, its excitation is dominated by a dipolar response that can be described using the discrete dipole approximation and polarizability theory. The dipolar response depends on the particle's polarizability function which encapsulates the particle's materials and geometry, and on the local field acting on the particle. In principle, the latter is nothing more than the backscattering of the particle field by the cavity walls. However, it may be challenging since it involves a three-dimensional singularity subtraction of the Green's function in the cavity and the Green's function in the free space that are differently represented. In this paper, we suggest the use of a ladder-type process involving alternative Green's function representations to calculate the local field in a computationally efficient and numerically stable manner. Using this approach, we solve several strongly coupled particle-cavity systems and calculate the collective resonance frequencies of the system with isotropic, gyrotropic, and chiral particles.
Comment: 19 pages with 8 figures