Towards Accurate and Efficient Sorting of Retired Lithium-ion Batteries: A Data Driven Based Electrode Aging Assessment Approach

Retired batteries (RBs) for second-life applications offer promising economic and environmental benefits. However, accurate and efficient sorting of RBs with discrepant characteristics persists as a pressing challenge. In this study, we introduce a data driven based electrode aging assessment approach to address this concern. To this end, a number of 15 feature points are extracted from battery open circuit voltage (OCV) curves to capture their characteristics at different levels of aging, and a convolutional neural network with an optimized structure and minimized input size is established to relocate the relative positions of these OCV feature points. Next, a rapid estimation algorithm is proposed to identify the three electrode aging parameters (EAPs) which best reconstruct the 15 OCV feature points over the entire usable capacity range. Utilizing the three EAPs as sorting indices, we employ an adaptive affinity propagation algorithm to cluster RBs without the need for pre-determining the clustering number. Unlike conventional sorting methods based solely on battery capacity, the proposed method provides profound insights into electrode aging behaviors, minimizes the need for constant-current charging data, and supports module/pack-level tests for the simultaneous processing of high volumes of RBs.
Comment: 40 pages, 25 figures