Field-dependent magnetic relaxation times of magnetic nanoparticle systems: analytic approximations supported by numerical simulations

Many estimates for the magnetic relaxation time of magnetic nanoparticle systems neglect the effect of the applied field strength. This is despite many applications of magnetic nanoparticles involving relaxation dynamics under the influence of applied fields. Here, an analytic approximation for the field-dependent Brownian relaxation time of single-domain, spherical magnetic nanoparticles in an external applied field is developed mathematically. This expression is validated by comparison with existing empirically-derived expressions and by comparison to particle-level simulations that allow particle rotations. Our approximation works particularly well for larger particles. We then use the developed expression to analytically calculate the total magnetic relaxation time when both Brownian and N\'eel relaxation mechanisms are at play. Again, we show that the results match those found using particle-level simulations, this time with both particle rotations and internal magnetization dynamics allowed. However, for some particle parameters and for large field strengths, our simulations reveal that the Brownian and N\'eel relaxation mechanisms are decoupled and it is not appropriate to combine these to calculate a total relaxation time.
Comment: 10 pages, 5 figures, submitted to Physical Review B