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Electronic interactions in Dirac fluids visualized by nano-terahertz spacetime interference of electron-photon quasiparticles

Authors :
Xu, Suheng
Li, Yutao
Vitalone, Rocco A.
Jing, Ran
Sternbach, Aaron J.
Zhang, Shuai
Ingham, Julian
Delor, Milan
McIver, James. W.
Yankowitz, Matthew
Queiroz, Raquel
Millis, Andrew J.
Fogler, Michael M.
Dean, Cory R.
Pasupathy, Abhay N.
Hone, James
Liu, Mengkun
Basov, D. N.
Publication Year :
2023

Abstract

Ultraclean graphene at charge neutrality hosts a quantum critical Dirac fluid of interacting electrons and holes. Interactions profoundly affect the charge dynamics of graphene, which is encoded in the properties of its electron-photon collective modes: surface plasmon polaritons (SPPs). Here we show that polaritonic interference patterns are particularly well suited to unveil the interactions in Dirac fluids by tracking polaritonic interference in time at temporal scales commensurate with the electronic scattering. Spacetime SPP interference patterns recorded in tera-hertz (THz) frequency range provided unobstructed readouts of the group velocity and lifetime of polariton that can be directly mapped onto the electronic spectral weight and the relaxation rate. Our data uncovered prominent departures of the electron dynamics from the predictions of the conventional Fermi-liquid theory. The deviations are particularly strong when the densities of electrons and holes are approximately equal. The proposed spacetime imaging methodology can be broadly applied to probe the electrodynamics of quantum materials.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2311.11502
Document Type :
Working Paper