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Magnetism-induced band-edge shift as mechanism for magnetoconductance in CrPS$_4$ transistors

Authors :
Wu, Fan
Gibertini, Marco
Watanabe, Kenji
Taniguchi, Takashi
GutiƩrrez-Lezama, Ignacio
Ubrig, Nicolas
Morpurgo, Alberto F.
Publication Year :
2023

Abstract

Transistors realized on 2D antiferromagnetic semiconductor CrPS$_4$ exhibit large magnetoconductance, due to magnetic-field-induced changes in magnetic state. The microscopic mechanism coupling conductance and magnetic state is not understood. We identify it by analyzing the evolution of the parameters determining the transistor behavior -- carrier mobility and threshold voltage -- with temperature and magnetic field. For temperatures T near the N\'eel temperature $T_N$, the magnetoconductance originates from a mobility increase due to the applied magnetic field that reduces spin fluctuation induced disorder. For $T << T_N$, instead, what changes is the threshold voltage, so that increasing the field at fixed gate voltage increases the density of accumulated electrons. The phenomenon is explained by a conduction band-edge shift correctly predicted by \emph{ab-initio} calculations. Our results demonstrate that the bandstructure of CrPS$_4$ depends on its magnetic state and reveal a mechanism for magnetoconductance that had not been identified earlier.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2304.12712
Document Type :
Working Paper
Full Text :
https://doi.org/10.1021/acs.nanolett.3c02274