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Flattening conduction and valence bands for interlayer excitons in a moir\'e MoS$_2$/WSe$_2$ heterobilayer

Authors :
Conti, Sara
Chaves, Andrey
Pandey, Tribhuwan
Covaci, Lucian
Peeters, François M.
Neilson, David
Milošević, Milorad V.
Source :
Nanoscale, 2023,15, 14032-14042
Publication Year :
2023

Abstract

We explore the flatness of conduction and valence bands of interlayer excitons in MoS$_2$/WSe$_2$ van der Waals heterobilayers, tuned by interlayer twist angle, pressure, and external electric field. We employ an efficient continuum model where the moir\'e pattern from lattice mismatch and/or twisting is represented by an equivalent mesoscopic periodic potential. We demonstrate that the mismatch moir\'e potential is too weak to produce significant flattening. Moreover, we draw attention to the fact that the quasi-particle effective masses around the $\Gamma$-point and the band flattening are \textit{reduced} with twisting. As an alternative approach, we show (i) that reducing the interlayer distance by uniform vertical pressure can significantly increase the effective mass of the moir\'e hole, and (ii) that the moir\'e depth and its band flattening effects are strongly enhanced by accessible electric gating fields perpendicular to the heterobilayer, with resulting electron and hole effective masses increased by more than an order of magnitude leading to record-flat bands. These findings impose boundaries on the commonly generalized benefits of moir\'e twistronics, while also revealing alternate feasible routes to achieve truly flat electron and hole bands to carry us to strongly correlated excitonic phenomena on demand.

Details

Database :
arXiv
Journal :
Nanoscale, 2023,15, 14032-14042
Publication Type :
Report
Accession number :
edsarx.2303.07755
Document Type :
Working Paper
Full Text :
https://doi.org/10.1039/D3NR01183F