Energy Dissipation and Asymmetric Excitation in Hybrid Waveguides for Routing and Coloring

The delivery of optical signals from an external light source to a nanoscale waveguide is highly important for the development of nanophotonic circuits. However, the efficient coupling of external light energy into nanophotonic components is difficult and still remains a challenge. Herein, we use an external silica nanofiber to light up an organic-inorganic hybrid nano-waveguide, namely a system composed of a polymer filament doped with MoS$_{2}$ quantum dots. Nanofiber-excited nano-waveguides in a crossed geometry are found to asymmetrically couple excitation signals along two opposite directions, with different energy dissipation resulting in different colors of the light emitted by MoS$_{2}$ quantum dots and collected from the waveguide terminals. Interestingly, rainbow-like light in the hybrid waveguide is achieved by three-in-one mixing of red, green, and blue components. This hetero-dimensional system of dots-in-waveguide represents a significant advance towards all-optical routing and full-color display in integrated nanophotonic devices.
Comment: 26 pages, 11 Figures, Journal of Physical Chemistry Letters, 2021