Accurate Direct Measurements of Far-Field Thermal Infrared Emission and its Dynamics

Accurate direct measurements of far-field thermal infrared emission become increasingly important because conventional methods, relying on indirect assessments, such as reflectance/transmittance, are inaccurate or even unfeasible to characterize state-of-art devices with novel spectra, directionalities, and polarizations. The direct collection of the far-field emission from these tiny devices is also challenging because of their shrinking footprints and uncontrollable radiation noises from their surroundings. Here, we demonstrate a microscopic lock-in FTIR system that realizes significant improvement in signal-to-noise ratio (SNR) by combining a microscope and a lock-in amplifier with an FTIR. The lock-in FTIR is ultrasensitive, with a specific detectivity 10^6 times higher than commercial ones, to overcome the optical loss and background noise during the emission light collection. Based on an analytical model of the signal detection process, we also explore the combination of modulated Joule heating and global heating to fulfill the potential of our system for noise reduction. Our findings show that, compared to previous studies, more than 3 times lower temperatures are sufficient to generate a measurable signal. Under a heating temperature of around 125 {\deg}C, we can achieve an SNR of about 23.7, which is far above the true-signal-threshold (SNR of about 3.0). Furthermore, the system can respond fast enough (up to 175kHz) to record spectral-resolved dynamics of microdevices in the frequency domain. The measurable frequency range can be extended up to MHz or even GHz level by a high-speed circuit model. We believe the system together with the analytical signal processing can be beneficial for next-generation thermal infrared material and device exploration, boosting the applications in lighting, sensing, imaging, and energy harvesting on a small scale.
Comment: 19 pages, 4 figures