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Investigation of role of antisite disorder in the pristine cage compound FeGa$_3$

Authors :
Ribeiro, C. Kaufmann
Mello, L.
Martelli, V.
Cornejo, D.
Neto, M. B. Silva
Fogh, E.
Rønnow, H. M.
Jiménez, J. Larrea
Publication Year :
2022

Abstract

The role of controlled disorder in the strong correlated narrow gap semiconductor candidate FeGa$_3$ has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations of the occupation number of Fe and Ga sites from those expected in the pristine compound were quantified with X-ray analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa$_3$ from paramagnetic semiconducting to a magnetic metal. These findings are discussed within the framework of Anderson metal-insulator transitions and spin fluctuations.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2208.09064
Document Type :
Working Paper