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High-temperature self-energy corrections to x-ray absorption spectra

Authors :
Tan, Tun S.
Kas, J. J.
Trickey, S. B.
Rehr, J. J.
Publication Year :
2022

Abstract

Effects of finite-temperature quasiparticle self-energy corrections to x-ray absorption spectra are investigated within the finite-temperature quasiparticle local density GW approximation up to temperatures $T$ of order the Fermi temperature. To facilitate the calculations, we parametrize the quasiparticle self-energy using low-order polynomial fits. We show that temperature-driven decrease in the electron lifetime substantially broadens the spectra in the near-edge region with increasing $T$. However, the quasiparticle shift is most strongly modified near the onset of plasmon excitations.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2208.02390
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.107.115122