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Origin of oscillatory structures in the magnetothermal conductivity of the putative Kitaev magnet $\alpha$-RuCl$_3$

Authors :
Bruin, J. A. N.
Claus, R. R.
Matsumoto, Y.
Nuss, J.
Laha, S.
Lotsch, B. V.
Kurita, N.
Tanaka, H.
Takagi, H.
Publication Year :
2022

Abstract

The layered honeycomb magnet $\alpha$-RuCl$_3$ has been suggested to exhibit a field-induced quantum spin liquid state, in which the reported large thermal Hall effect close to the half-quantized value still remains a subject of debate. Recently, oscillatory structures of the magnetothermal conductivity were reported and interpreted as quantum oscillations of charge-neutral particles. To investigate the origin of these oscillatory structures, we performed a comprehensive measurement of the in-plane magnetothermal conductivity $\kappa(H)$ down to low temperature (100 mK), as well as magnetization $M$, for single crystals grown by two different techniques: Bridgman and chemical vapor transport. The results show a series of dips in $\kappa(H)$ and peaks in the field derivative of $M$ located at the same fields independent of the growth method. We argue that these structures originate from field-induced phase transitions rather than quantum oscillations. The positions of several of these features are temperature-dependent and connected to the magnetic phase transitions in zero field: the main transition at 7 K and weaker additional transitions which likely arise from secondary phases at 10 K and 13 K. In contrast to what is expected for quantum oscillations, the magnitude of the structure in $\kappa(H)$ is smaller for the higher conductivity crystal and decreases rapidly upon cooling below 1 K.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2205.15839
Document Type :
Working Paper
Full Text :
https://doi.org/10.1063/5.0101377