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Unidirectional ultracompact DNA-templated optical antennas
- Publication Year :
- 2022
-
Abstract
- Optical nanoantennas are structures designed to manipulate light-matter interactions at the nanoscale by interfacing propagating light with localized optical fields. In recent years, a plethora of devices have been realized that are able to efficiently tailor the absorption and/or emission rates of fluorophores. By contrast, modifying the spatial characteristics of their radiation fields remains a challenge. Up to date, the designs providing directionality to fluorescence emission have required compound, complex geometries with overall dimensions comparable to the operating wavelength. Here, we present the fabrication and characterization of DNA-templated ultracompact optical antennas, with sub-wavelength sizes and capable of directing single-molecule fluorescence into predefined directions. Using the DNA origami methodology, two gold nanorods are assembled side-to-side with a separation gap of 5 nm. We show that a single fluorescent molecule placed at the tip of one of the nanorods drives the dimer antenna in anti-phase, leading to unidirectional emission.
- Subjects :
- Physics - Optics
Physics - Applied Physics
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.2204.03604
- Document Type :
- Working Paper
- Full Text :
- https://doi.org/10.1021/acs.nanolett.2c02424