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Interplay of the Jahn--Teller Effect and Spin-Orbit Coupling: The Case of Trigonal Vibronic Modes

Authors :
Streltsov, S. V.
Temnikov, F. V.
Kugel, K. I.
Khomskii, D. I.
Source :
Phys. Rev. B, 105(20), 205142 (2022)
Publication Year :
2022

Abstract

We study an interplay between the orbital degeneracy and spin-orbit coupling giving rise to spin-orbital entangled states. As a specific example, we analyze the interaction of electrons occupying triply degenerate single-ion $t_{2g}$ levels with trigonal vibronic modes (the $t\otimes T$ problem). A more general problem of the electron-lattice interaction involving both tetragonal and trigonal vibrations is also considered. It is shown that the result of such interaction crucially depends on the occupation of $t_{2g}$ levels leading to either the suppression or enhancement of the Jahn-Teller effect by the spin-orbit coupling.<br />Comment: 11 pages, 10 figures

Details

Database :
arXiv
Journal :
Phys. Rev. B, 105(20), 205142 (2022)
Publication Type :
Report
Accession number :
edsarx.2203.02243
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.105.205142