Back to Search Start Over

Modified Curie-Weiss Law for $j_{\rm eff}$ Magnets

Authors :
Li, Ying
Winter, Stephen M.
Kaib, David A. S.
Riedl, Kira
Valenti, Roser
Source :
Phys. Rev. B 103, 220408 (2021)
Publication Year :
2021

Abstract

In spin-orbit-coupled magnetic materials, the usually applied Curie-Weiss law can break down. This is due to potentially sharp temperature-dependence of the local magnetic moments. We therefore propose a modified Curie-Weiss formula suitable for analysis of experimental susceptibility. We show for octahedrally coordinated materials of $d^5$ filling that the Weiss constant obtained from the improved formula is in excellent agreement with the calculated Weiss constant from microscopic exchange interactions. Reanalyzing the measured susceptibility of several Kitaev candidate materials with the modified formula resolves apparent discrepancies between various experiments regarding the magnitude and anisotropies of the underlying magnetic couplings.

Details

Database :
arXiv
Journal :
Phys. Rev. B 103, 220408 (2021)
Publication Type :
Report
Accession number :
edsarx.2102.08964
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.103.L220408