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Moir\'e Imaging in Twisted Bilayer Graphene Aligned on Hexagonal Boron Nitride

Authors :
Huang, Xiong
Chen, Lingxiu
Tang, Shujie
Jiang, Chengxin
Chen, Chen
Wang, Huishan
Shen, Zhi-Xun
Wang, Haomin
Cui, Yong-Tao
Publication Year :
2021

Abstract

Moir\'e superlattices (MSL) formed in angle-aligned bilayers of van der Waals materials have become a promising platform to realize novel two-dimensional electronic states. Angle-aligned trilayer structures can form two sets of MSLs which could potentially interfere with each other. In this work, we directly image the moir\'e patterns in both monolayer graphene aligned on hBN and twisted bilayer graphene aligned on hBN, using combined scanning microwave impedance microscopy and conductive atomic force microscopy. Correlation of the two techniques reveals the contrast mechanism for the achieved ultrahigh spatial resolution (<2 nm). We observe two sets of MSLs with different periodicities in the trilayer stack. The smaller MSL breaks the 6-fold rotational symmetry and exhibits abrupt discontinuities at the boundaries of the larger MSL. Using a rigid atomic-stacking model, we demonstrate that the hBN layer considerably modifies the MSL of twisted bilayer graphene. We further analyze its effect on the reciprocal space spectrum of the dual-moir\'e system.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2102.08594
Document Type :
Working Paper