Back to Search Start Over

Classical Spin Liquid State in the $S=\frac{5}{2}$ Heisenberg Kagom\'e Antiferromagnet Li$_9$Fe$_3$(P$_2$O$_7$)$_3$(PO$_4$)$_2$

Authors :
Kermarrec, E.
Kumar, R.
Bernard, G.
Hénaff, R.
Mendels, P.
Bert, F.
Paulose, P. L.
Hazra, B. K.
Koteswararao, B.
Source :
Phys. Rev. Lett. 127, 157202 (2021)
Publication Year :
2021

Abstract

We investigate the low temperature magnetic properties of a $S=\frac{5}{2}$ Heisenberg kagom\'e antiferromagnet, the layered monodiphosphate Li$_9$Fe$_3$(P$_2$O$_7$)$_3$(PO$_4$)$_2$, using magnetization measurements and $^{31}$P nuclear magnetic resonance. An antiferromagnetic-type order sets in at $T_{\rm N}=1.3$ K and a characteristic magnetization plateau is observed at 1/3 of the saturation magnetization below $T^* \sim 5$ K. A moderate $^{31}$P NMR line broadening reveals the development of anisotropic short-range correlations within the plateau phase concomitantly with a gapless spin-lattice relaxation time $T_1 \sim k_B T / \hbar S$, which both point to the presence of a semiclassical nematic spin liquid state predicted for the Heisenberg kagom\'e antiferromagnetic model or to the persistence of the zero-energy modes of the kagome lattice under large magnetic fields.<br />Comment: 6 pages, 5 figures

Details

Database :
arXiv
Journal :
Phys. Rev. Lett. 127, 157202 (2021)
Publication Type :
Report
Accession number :
edsarx.2102.02882
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevLett.127.157202