Back to Search Start Over

High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Authors :
Lee, Changmin
Rohwer, Timm
Sie, Edbert J.
Zong, Alfred
Baldini, Edoardo
Straquadine, Joshua
Walmsley, Philip
Gardner, Dillon
Lee, Young S.
Fisher, Ian R.
Gedik, Nuh
Source :
Rev.Sci.Instrum.91.043102 (2020)
Publication Year :
2019

Abstract

Performing time and angle resolved photoemission spectroscopy (tr-ARPES) at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite recent advances, HHG-based setups still require large pulse energies (hundreds of $\mu$J to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of $5\times10^{10}$ photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 $\mu$J. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe$_3$. This novel setup offers opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.

Details

Database :
arXiv
Journal :
Rev.Sci.Instrum.91.043102 (2020)
Publication Type :
Report
Accession number :
edsarx.1910.14068
Document Type :
Working Paper
Full Text :
https://doi.org/10.1063/1.5139556