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Robust block magnetism in the spin ladder compound BaFe$_2$Se$_3$ under hydrostatic pressure

Authors :
Wu, Shan
Yin, Junjie
Smart, Thomas
Acharya, Arani
Bull, Craig L.
Funnell, Nicholas P.
Forrest, Thomas R.
Simutis, Gediminas
Khasanov, Rustem
Lewin, Sylvia K.
Wang, Meng
Frandsen, Benjamin A.
Jeanloz, Raymond
Birgeneau, Robert J.
Source :
Phys. Rev. B 100, 214511 (2019)
Publication Year :
2019

Abstract

The majority of the iron-based superconductors (FeSCs) exhibit a two-dimensional square lattice structure. Recent reports of pressure-induced superconductivity in the spin-ladder system, BaFe$_2$X$_3$ (X =S,Se), introduce a quasi-one-dimensional prototype and an insulating parent compound to the FeSCs. Here we report X-ray, neutron diffraction and muon spin relaxation experiments on BaFe$_2$Se$_3$ under hydrostatic pressure to investigate its magnetic and structural properties across the pressure-temperature phase diagram. A structural phase transition was identified at a pressure of 3.7(3) GPa. Neutron diffraction measurements at 6.8(3) GPa and 120 K show that the block magnetism persists even at these high pressures. A steady increase and then fast drop of the magnetic transition temperature $T\rm_N$ and greatly reduced moment above the pressure $P_s$ indicate potentially rich and competing phases close to the superconducting phase in this ladder system.

Details

Database :
arXiv
Journal :
Phys. Rev. B 100, 214511 (2019)
Publication Type :
Report
Accession number :
edsarx.1909.06498
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.100.214511