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Robust field-dressed spectra of diatomics in an optical lattice

Authors :
Pawlak, Mariusz
Szidarovszky, Tamás
Halász, Gábor J.
Vibók, Ágnes
Publication Year :
2019

Abstract

The absorption spectra of the cold Na2 molecule dressed by a linearly polarized standing laser wave is investigated. In the studied scenario the rotational motion of the molecules is frozen while the vibrational and translational degrees of freedom are accounted for as dynamical variables. In such a situation a light-induced conical intersection (LICI) can be formed. To measure the spectra a weak field is used whose propagation direction is perpendicular to the direction of the dressing field but has identical polarization direction. Although LICIs are present in our model, the simulations demonstrate a very robust absorption spectrum, which is insensitive to the intensity and the wavelength of the dressing field and which does not reflect clear signatures of light-induced nonadiabatic phenomena related to the strong mixing between the electronic, vibration and translational motions. However, by widening artificially the very narrow translational energy level gaps, the fingerprint of the LICI appears to some extent in the spectrum.

Subjects

Subjects :
Physics - Chemical Physics

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.1905.08573
Document Type :
Working Paper
Full Text :
https://doi.org/10.1039/C9CP06587C